arXiv subjects

Xiaofu Zhang

Publications and source records attributed to Xiaofu Zhang.

At least 19 recordsLinked to original sources

arXiv2024

Drone based superconducting single photon detection system with detection efficiency more than 90%

Bounded by the size, weight, and power consumption (SWaP) of conventional superconducting single photon detectors (SSPD), applications of SSPDs were commonly confined in the laboratory. However, booming demands for high efficiency single photon detector incorporated with avionic platforms arise with the development of remote imaging and sensing or long-haul quantum communication without topographical constraints. We herein designed and manufactured the first drone based SSPD system with a SDE as high as 91.8%. This drone based SSPD system is established with high performance NbTiN SSPDs, self-developed miniature liquid helium dewar, and homemade integrated electric setups, which is able to be launched in complex topographical conditions. Such a drone based SSPD system may open the use of SSPDs for applications that demand high-SDE in complex environments.

cond-mat.supr-con↗

arXiv2023

Superconducting nanowire diode

Semiconducting diode with nonreciprocal transport effect underlies the cornerstone of contemporary integrated circuits (ICs) technology. Due to isotropic superconducting properties and the lack of breaking of inversion symmetry for conventional s-wave superconductors, such a superconducting peer is absent. Recently, a series of superconducting structures, including superconducting superlattice and quantum-material-based superconducting Josephson junction, have exhibited a superconducting diode effect in terms of polarity-dependent critical current. However, due to complex structures, these composite systems are not able to construct large-scale integrated superconducting circuits. Here, we demonstrated the minimal superconducting electric component-superconducting nanowire-based diode with a nonreciprocal transport effect under a perpendicular magnetic field, in which the superconducting to normal metallic phase transition relies on the polarity and amplitude of the bias current. Our nanowire diodes can be reliably operated nearly at all temperatures below the critical temperature, and the rectification efficiency at 2 K can be more than 24%. Moreover, the superconducting nanowire diode is able to rectify both square wave and sine wave signals without any distortion. Combining the superconducting nanowire-based diodes and transistors, superconducting nanowires hold the possibility to construct novel low-dissipation superconducting ICs.

cond-mat.supr-con↗

arXiv2023

Competing spin-glass and spin-fluctuation states in NdxPr4-xNi3O8

Neodymium nickelates have attracted research interest due to their strongly correlated behaviour and remarkable magnetic properties. More importantly, superconductivity has recently been confirmed in thin-film samples of Sr-doped NdNiO2, bringing the layered rare earth nickel oxides into the research spotlight. In this report, we present results on a series of NdNiO2 analogues, NdxPr4-xNi3O8 (x = 0.1, 0.25, 1, 2, and 4) obtained by topotactic reduction, in which we observe systematic changes in the magnetic behaviour. As the Nd3+ content increases, the initially large spin-freezing region with magnetic frustration becomes smaller and gradually shifts to low temperatures, while the magnetic response gradually increases. The muon-spin spectroscopy measurements on Nd4Ni3O8 show that this phenomenon is likely due to the enhancement of spin fluctuations in NdxPr4-xNi3O8, which weakens the spin frustration behaviour for high Nd3+ contents and at low temperatures. These spin fluctuations can be caused by both Nd and Ni ions and could be one of the factors determining the occurrence of possible superconductivity.

cond-mat.supr-con↗

arXiv2023

Superconductivity in hydrated Lix(H2O)yTaS2

We have systematically studied the structural and physical properties of the superconducting hydrated Lix(H2O)yTaS2. The powder X-ray diffraction patterns suggest that all the samples are single-phase compounds, and the crystal structure is similar to that of 2H-TaS2. The transition temperature to superconductivity shows a dome-shape dependence on the lithium content x with a maximum Tc of 4.6 K for x=0.42, which is larger than in corresponding optimally doped 2H-TaS2 superconductors without water or organic intercalants (Tc ~ 4.2 K). There are no signs for a charge-density-wave formation in hydrated Lix(H2O)yTaS2. While our magnetic data indicate a rather strongly type-II behavior, heat-capacity measurements reveal, like in other 2H-TaS2-type compounds. From the corresponding Sommerfeld constants and Debye temperatures, we can derive the parameter describing the electron-phonon coupling and the electron density of states DOS(EF) at the Fermi level as functions of x. While the variation of the DOS(EF) is consistent with that of Tc, indicating that the lithium intercalation is tuning Tc via changing the DOS(EF) in 2H-Lix(H2O)yTaS2, the simultaneous changes of electron-phonon coupling and Debye temperatures may also play a certain role.

cond-mat.supr-con↗

arXiv2022

Single photon detection performance of highly disordered NbTiN thin films

We experimentally investigated the detection performance of highly disordered NbxTi1-xN based superconducting nanowire single photon detectors (SNSPDs). The dependence on the composition of the transition temperature Tc for NbxTi1-xN films show a dome-like behavior on the Nb content, with a maximal Tc at xNb~0.65 , and the Nb0.65Ti0.35N films also combine relatively large sheet resistance and intermediate residual resistivity ratio. Moreover, 60-nm-wide and 7-nm-thick Nb0.65Ti0.35N nanowires show a switching current as high as 14.5 uA, and saturated intrinsic detection efficiency with a plateau of more than 2 uA at 2.4 K. Finally, the corresponding SNSPDs on an alternative SiO2/Ta2O5 dielectric mirror showed a system detection efficiency of approximately 92% for 1550 nm photons, and the timing jitter is around 26 ps. Our results demonstrate that the highly disordered NbxTi1-xN films are promising for fabricating SNSPDs for near- and middle-infrared single photons with high detection efficiency and low timing jitter.

cond-mat.supr-con↗

arXiv2021

Group-9 Transition Metal Suboxides Adopting the Filled-Ti$_2$Ni Structure: A Class of Superconductors Exhibiting Exceptionally High Upper Critical Fields

The Ti$_2$Ni and the related $η$-carbide structure are known to exhibit various intriguing physical properties. The Ti$_2$Ni structure with the cubic space group $Fd\bar{3}m$ is surprisingly complex, consisting of a unit cell with 96 metal atoms. The related $η$-carbide compounds correspond to a filled version of the Ti$_2$Ni structure. Here, we report on the structure and superconductivity in the $η$-carbide type suboxides Ti$_4$M$_2$O with M = Co, Rh, Ir. We have successfully synthesized all three compounds in single phase form. We find all three compounds to be type-II bulk superconductors with transition temperatures of $T_{\rm c}$ = 2.7, 2.8, and 5.4 K, and with normalized specific heat jumps of $ΔC/γT_{\rm c}$ = 1.65, 1.28, and 1.80 for Ti$_4$Co$_2$O, Ti$_4$Rh$_2$O, and Ti$_4$Ir$_2$O, respectively. We find that all three superconductors, exhibit high upper-critical fields. Particularly noteworthy is Ti$_4$Ir$_2$O with an upper critical field of $μ_0 H_{\rm c2}{\rm (0)}$ =~16.06~T, which exceeds by far the weak-coupling Pauli limit of 9.86~T. The role of the void filling light atom X has so far been uncertain for the overall physical properties of these materials. Herein, we have successfully grown single crystals of Ti$_2$Co. In contrast to the metallic $η$-carbide type suboxides Ti$_4$M$_2$O, we find that Ti$_2$Co displays a semimetallic behavior. Hence, the octahedral void-filling oxygen plays a crucial role for the overall physical properties, even though its effect on the crystal structure is small. Our results indicate that the design of new superconductors by incorporation of electron-acceptor atoms may in the Ti$_2$Ni-type structures and other materials with crystallographic void position be a promising future approach. The remarkably high upper critical fields, in this family of compounds, may furthermore spark significant future interest.

cond-mat.supr-con↗

arXiv2021

Evidence for Isotropic s-Wave Superconductivity in High-Entropy Alloys

High-entropy alloys (HEA) form through the random arrangement of five or more chemical elements on a crystalline lattice. Despite the significant amount of resulting compositional disorder, a subset of HEAs enters a superconducting state below critical temperatures $T_c<10$ K. The superconducting properties of the known HEAs seem to suffice a Bardeen-Cooper-Schrieffer (BCS) description, but little is known about their superconducting order parameter and the microscopic role of disorder. We report on magnetic susceptibility measurements on films of the superconducting HEA (TaNb)$_{1-x}$(ZrHfTi)$_x$ for characterizing the lower and upper critical fields $H_{c1}(T)$ and $H_{c2}(T)$, respectively as a function of temperature $T$. Our resulting analysis of the Ginzburg-Landau coherence length and penetration depth demonstrates that HEAs of this type are single-band isotropic s-wave superconductors in the dirty limit. Despite a significant difference in the elemental composition between the $x=0.35$ and $x=0.71$ films, we find that the observed $T_c$ variations cannot be explained by disorder effects.

cond-mat.supr-con↗

arXiv2021

Physical properties of amorphous molybdenum silicide films for single photon detectors

We systematically investigated the physical properties of amorphous Mo$_{\rm x}$Si$_{1-x}$ films deposited by the magnetron co-sputtering technique. The critical temperature $T_C$ of Mo$_{\rm x}$ Si$_{1-x}$ films increases gradually with the stoichiometry x, and the highest $T_C$=7.9 K was found in Mo$_{\rm 0.83}$ Si$_{0.17}$. Beyond $x$=0.83, preformed Cooper pairs and superconducting domains persist in the films, despite the superconducting state with perfect zero-resistivity is absent. The thick films of Mo$_{\rm 0.83}$ Si$_{0.17}$ show surprising degradation in which the onset of zero-resistivity is suppressed below 2 K. The thin Mo$_{\rm 0.83}$ Si$_{0.17}$ films, however, reveal robust superconductivity even with thickness d$\leq$1 nm. We also characterized wide microwires based on the 2 nm thin Mo$_{\rm 0.8}$ Si$_{0.2}$ films with widths 40 and 60 $μ$m, which show single-photon sensitivity at 780 nm and 1550 nm wavelength

cond-mat.supr-con↗

arXiv2021

Size dependent nature of the magnetic-field driven superconductor-to-insulator quantum-phase transitions

The nature of the magnetic-field driven superconductor-to-insulator quantum-phase transition in two-dimensional systems at zero temperature has been under debate since the 1980s, and became even more controversial after the observation of a quantum-Griffiths singularity. Whether it is induced by quantum fluctuations of the superconducting phase and the localization of Cooper pairs, or is directly driven by depairing of these pairs, remains an open question. We herein experimentally demonstrate that in weakly-pinning systems and in the limit of infinitely wide films, a sequential superconductor-to-Bose insulator-to-Fermi insulator quantum-phase transition takes place. By limiting their size smaller than the effective penetration depth, however, the vortex interaction alters, and the superconducting state re-enters the Bose-insulating state. As a consequence, one observes a direct superconductor-to-Fermi insulator in the zero-temperature limit. In narrow films, the associated critical-exponent products diverge along the corresponding phase boundaries with increasing magnetic field, which is a hallmark of the quantum-Griffiths singularity.

cond-mat.supr-con↗

arXiv2021

Superconductivity and charge-density wave formation in lithium intercalated 2H-LixTaS2

We systematically investigated the superconducting properties and the interplay between charge-density-waves (CDW) and superconductivity in lithium-intercalated 2H-TaS2. By gradually increasing the lithium content x, the CDW formation temperature is continuously suppressed, and the onset temperature of superconductivity is increased with a maximum transition temperature Tc = 3.5 K for x = 0.096. The bulk nature of superconductivity is confirmed by a superconducting shielding fraction of the order of unity for this composition. The electronic contribution to the specific heat and Hall resistivity data demonstrate that the CDW weakens with lithium-intercalation, thereby indirectly increasing carrier density and boosting superconductivity. While the sign of the charge carriers in undoped 2H-TaS2 changes from electron-like to hole type near the CDW formation temperature around 75 K, the lithium intercalated LixTaS2 show predominantly hole-type carriers in the CDW phase even for very low lithium contents.

cond-mat.supr-con↗

arXiv2021

Two-carrier Magnetoresistance: Applications to Ca$_3$Ru$_2$O$_7$

Ambipolar transport is a commonly occurring theme in semimetals and semiconductors. Here we present an analytical formulation of the conductivity for a two-band system. Electron and hole carrier densities and their respective conductivities are mapped into a two-dimensional unit-less phase space. Provided that one of the carrier densities is known, the dimensionless phase space can be probed through magnetoresistance measurements. This formulation of the two-band model for conductivity is applied to magnetoresistance experiments on Ca$_3$Ru$_2$O$_7$. While previous such measurements focused on the low-temperature limit, we cover a broad temperature range and find negative magnetoresistance in an intermediate interval below the electronic transition at 48 K. The low-temperature magnetoresistance in Ca$_3$Ru$_2$O$_7$ is consistent with a two-band structure. However, the model fails to describe the full temperature and magnetic field dependence. Negative magnetoresistance found in an intermediate temperature range is, for example, not captured by this model. We thus conclude that the electronic and magnetic structure in this intermediate temperature range render the system beyond the most simple two-band model.

cond-mat.str-el↗

arXiv2021

Magnetotransport of dirty-limit van Hove singularity quasiparticles

Tuning of electronic density-of-states singularities is a common route to unconventional metal physics. Conceptually, van Hove singularities are realized only in clean two-dimensional systems. Little attention has therefore been given to the disordered (dirty) limit. Here, we provide a magnetotransport study of the dirty metamagnetic system calcium-doped strontium ruthenate. Fermi liquid properties persist across the metamagnetic transition, but with an unusually strong variation of the Kadowaki-Woods ratio. This is revealed by a strong decoupling of inelastic electron scattering and electronic mass inferred from density-of-state probes. We discuss this Fermi liquid behavior in terms of a magnetic field tunable van Hove singularity in the presence of disorder. More generally, we show how dimensionality and disorder control the fate of transport properties across metamagnetic transitions.

cond-mat.str-el↗

arXiv2020

Electron energy relaxation in disordered superconducting NbN films

We report on the inelastic-scattering rate of electrons on phonons and relaxation of electron energy studied by means of magnetoconductance, and photoresponse, respectively, in a series of strongly disordered superconducting NbN films. The studied films with thicknesses in the range from 3 to 33 nm are characterized by different Ioffe-Regel parameters but an almost constant product q_Tl(q_T is the wave vector of thermal phonons and l is the elastic mean free path of electrons). In the temperature range 14-30 K, the electron-phonon scattering rates obey temperature dependencies close to the power law 1/τ_{e-ph} \sim T^n with the exponents n = 3.2-3.8. We found that in this temperature range τ_{e-ph} and n of studied films vary weakly with the thickness and square resistance. At 10 K electron-phonon scattering times are in the range 11.9-17.5 ps. The data extracted from magnetoconductance measurements were used to describe the experimental photoresponse with the two-temperature model. For thick films, the photoresponse is reasonably well described without fitting parameters, however, for thinner films, the fit requires a smaller heat capacity of phonons. We attribute this finding to the reduced density of phonon states in thin films at low temperatures. We also show that the estimated Debye temperature in the studied NbN films is noticeably smaller than in bulk material.

cond-mat.supr-con↗

arXiv2020

Correlation between the tolerance factor and phase transition in Ln4-xLnxNi3O10 (Ln and Ln' = La, Pr and Nd; x = 0, 1, 2 and 3)

We have synthesized a series of the Ruddlesden-Popper nickelate solid solution Ln4-xLn'xNi3O10 (Ln and Ln' = La, Pr and Nd; x = 0, 1, 2 and 3) via the citrate precursor method at different reacting atmospheres. Both the electronic-transport and magnetization measurements on these samples show well-defined phase transitions at temperatures between 135 K and 165 K. These transition temperatures, the room-temperature resistivities, as well as the changes of the Pauli-paramagnetic susceptibilities at the respective phase transitions, strongly correlate with the Goldschmidt tolerance factor t, irrespective of the combination of the magnetic rare-earth ions with unmagnetic La3+. We conclude that these changes of the electronic properties are mostly related to the distortion of the NiO6 octahedra at the phase transition which is strongly correlated with the tolerance factor t, but are rather insensitive to the magnetism of the rare-earth ions Ln3+ and Ln'3+.

cond-mat.supr-con↗

arXiv2020

Short-range magnetic interactions and spin-glass behavior in the quasi-2D nickelate Pr4Ni3O8

The nickelate Pr4Ni3O8 features quasi-two-dimensional layers consisting of three stacked square-planar NiO2 planes, in a similar way to the well-known cuprate superconductors. The mixed-valent nature of Ni and its metallic properties makes it a candidate for potentially unconventional superconductivity. We have synthesized Pr4Ni3O8 by topotactic reduction of Pr4Ni3O10 in 10 percent hydrogen gas, and report on measurements of powder-neutron diffraction, magnetization and muon-spin rotation (uSR). We find that Pr4Ni3O8 shows complicated spin-glass behavior with a distinct magnetic memory effect in the temperature range from 2 to 300 K and a freezing temperature T_s ~ 68 K. Moreover, the analysis of uSR spectra indicates two magnetic processes characterized by remarkably different relaxation rates: a slowly-relaxing signal, resulting from paramagnetic fluctuations of Pr/Ni ions, and a fast-relaxing signal, whose relaxation rate increases substantially below ~ 70 K which can be ascribed to the presence of short-range correlated regions. We conclude that the complex spin-freezing process in Pr4Ni3O8 is governed by these multiple magnetic interactions. It is possible that the complex magnetism in Pr4Ni3O8 is detrimental to the occurrence of superconductivity.

cond-mat.supr-con↗

arXiv2020

Strong suppression of the resistivity near the transition to superconductivity in narrow micro-bridges in external magnetic fields

We have investigated a series of superconducting bridges based on homogeneous amorphous WSi and MoSi films, with bridge widths w ranging from 2 um to 1000 um and film thicknesses d ~ 4-6 nm and 100 nm. Upon decreasing the bridge widths below the respective Pearl lengths, we observe in all cases distinct changes in the characteristics of the resistive transitions to superconductivity. For each of the films, the resistivity curves R(B,T) separate at a well-defined and field-dependent temperature T*(B) with decreasing the temperature, resulting in a dramatic suppression of the resistivity and a sharpening of the transitions with decreasing bridge width w. The associated excess conductivity in all the bridges scales as 1/w, which may suggest the presence of a highly conducting region that is dominating the electric transport in narrow bridges. We argue that this effect can only be observed in materials with sufficiently weak vortex pinning.

cond-mat.supr-con↗

arXiv2020

Anisotropic character of the metal-to-metal transition in Pr4Ni$_3$O$_{10}$

As a member of the Ruddlesden-Popper Ln$_{n+1}$Ni$_n$O$_{3n+1}$ series rare-earth-nickelates, the Pr4Ni$_3$O$_{10}$ consists of infinite quasi-two-dimensional perovskite-like Ni-O based layers. Although a metal-to-metal phase transition at Tpt = 157 K has been revealed by previous studies, a comprehensive study of physical properties associated with this transition has not yet been performed. We have grown single crystals of Pr4Ni3O10 at high oxygen pressure, and report on the physical properties around that phase transition, such as heat-capacity, electric-transport and magnetization. We observe a distinctly anisotropic behavior between in-plane and out-of-plane properties: a metal-to-metal transition at Tpt within the a-b plane, and a metal-to-insulator-like transition along the c-axis with decreasing temperature. Moreover, an anisotropic and anomalous negative magneto-resistance is observed at Tpt that we attribute to a slight suppression of the first-order transition with magnetic field. The magnetic-susceptibility can be well described by a Curie-Weiss law, with different Curie-constants and Pauli-spin susceptibilities between the high-temperature and the low-temperature phases. The single crystal X-ray diffraction measurements show a shape variation of the different NiO6 octahedra from the high-temperature phase to the low-temperature phase. This subtle change of the environment of the Ni sites is likely responsible for the different physical properties at high and low temperatures.

cond-mat.mtrl-sci↗

arXiv2020

Preparation and Characterization of High-Entropy Alloy (TaNb)$_{1-x}$(ZrHfTi)$_x$ Superconducting Films

We report on the preparation and the physical properties of superconducting (TaNb)_1-x(ZrHfTi)_x high-entropy alloy films. The films were prepared by means of magnetron sputtering at room temperature, with x ranging from 0 to 1 with an average thickness of 600 - 950 nm. All films crystallize in a pseudo body-centered cubic (BCC) structure. For samples with x < 0.65, the normal-state properties are metallic, while for x > 0.65 the films are weakly insulating. The transition from metallic to weakly insulating occurs right at the near-equimolar stoichiometry. We find all films, except for x = 0 or 1, to become superconducting at low temperatures, and we interpret their superconducting properties within the Bardeen-Cooper-Schrieffer (BCS) framework. The highest transition temperature T_c = 6.9 K of the solid solution is observed for x = 0.43. The highest upper-critical field B_c2(0) = 11.05 T is found for the near-equimolar ratio x = 0.65, where the mixing entropy is the largest. The superconducting parameters derived for all the films from transport measurements are found to be close to those that are reported for amorphous superconductors. Our results indicate that these films of high-entropy alloys are promising candidates for superconducting device fabrication.

cond-mat.supr-con↗