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Xiaokun Zhai

Publications and source records attributed to Xiaokun Zhai.

8 recordsLinked to original sources

Observation of anomalous exciton polariton bands in PEPI perovskite based microcavity at room temperature

Recently anomalous energy bands with negative mass attract intensive attention where non Hermiticity plays an important role. In this work we observe anomalous exciton polariton bands in PEPI perovskite based microcavity at room temperature. We simulate the anomalous band structure using a non-Hermitian coupled oscillator model which agree with experiments very well. Our results offer to study non-Hermitian polariton wave dynamics at room temperature.

physics.optics↗

Electrically tunable nonrigid moire exciton polariton supersolids at room temperature

A supersolid is a macroscopic quantum state which sustains superfluid and crystallizing structure together after breaking the U(1) symmetry and translational symmetry. On the other hand, a moire pattern can form by superimposing two periodic structures along a particular direction. Up to now, supersolids and moire states are disconnected from each other. In this work we show that exciton polariton supersolids can form moire states in a double degenerate parametric scattering process which creates two constituted supersolids with different periods in a liquid crystal microcavity. In addition, we demonstrate the nonrigidity of the moire exciton polariton supersolids by electrically tuning the wavevector and period of one supersolid component with another one being fixed. Our work finds a simple way to link moire states and supersolids, which offers to study nontrivial physics emerging from the combination of moire lattices and supersolids which can be electrically tuned at room temperature.

physics.optics↗

Splitting spin-orbit coupled polariton vortex pairs in the non-Hermitian Rashba-Dresselhaus band at room temperature

Spin orbit coupling gives rise to intriguing physical phenomena in bosonic condensates, such as formation of stripe phases and domains with vortex arrays. However, how the non-Hermiticity affects the spatial distribution of spin orbit coupled topological defects such as vortex pair is still challenging to study. In the present work, we realize a non-equilibrium room-temperature exciton polariton condensate within a microdisk potential in a liquid crystal (LC) microcavity with the perovskite CsPbBr3 as optically active material. We use the interplay of TE-TM mode splitting and Rashba-Dresselhaus spin-orbit coupling (RDSOC) to realize electrically tunable polariton vortex pairs with locked spin and orbital angular momentum. Importantly, the non-Hermiticity of RDSOC bands leads to nonreciprocal transportation of the vortex pair such that they move to the opposite edges of the microdisk depending on their spin. Our results are robust against sample imperfections and pave the way to investigate the coupling of vortex orbital and spin degrees of freedom in a quantum fluid of light at room temperature, offering potential for generation of complex states of light for non-Hermitian quantum optical information processing within optoelectronic chips.

physics.optics↗

Observation of condensed moire exciton polaritons in twisted photonic lattices at room temperature

Moire lattices attract significant attention in double-layer graphene and TMD layer heterostructures as well as in photonic crystals due to the interesting exotic physics that emerges within these structures. However, direct measurement of the moiré ground, excited states and Bloch bands in twisted photonic lattices is still illusive. In this work we report strong coupling between excitons in CsPbBr3 microplates and moire photonic modes at room temperature. Depending on the coupling strength between the nearest potential sites, we observe staggered moire polariton ground states, excited states and moire polariton bands. Phase locked moire zero (in-phase) states and moire pi (antiphase) states with different spatial distributions are measured. The moire polariton distribution can be tuned into the shape of a parallelogram by controlling the depth and width of the potential in one photonic lattice with another superimposed one fixed. In addition, moire polaritons in twisted 2D honeycomb lattices are also observed. Increasing the pumping density, we realize exciton polariton condensation in the moire potential sites of the 1D/2D twisted lattices with the coherence time of around 1.4 ps. Our work lays the foundation to study coherent moire polariton condensation in twisted photonic lattices at room temperature.

physics.optics↗

Manipulating polariton condensates by Rashba-Dresselhaus coupling at room temperature

The spin-orbit coupling plays an important role in the spin Hall effect and the topological insulators. In addition, the spin-orbit coupled Bose-Einstein condensates show remarkable quantum many-body phase transition. In this work we tune the exciton polariton condensate by virtue of the Rashba-Dresselhaus (RD) spin-orbit coupling in a liquid-crystal filled microcavity where perovskite CsPbBr3 microplates act as the gain material at room temperature. We realize an artificial gauge field on the CsPbBr3 exciton polariton condensate, which splits the condensates with opposite spins in both momentum and real spaces. Our work paves the way to manipulate the exciton polariton condensate with a synthetic gauge field based on the RD spin-orbit coupling at room temperature.

cond-mat.quant-gas↗

Electrically controlling vortices in a neutral exciton polariton condensate at room temperature

Manipulating bosonic condensates with electric fields is very challenging as the electric fields do not directly interact with the neutral particles of the condensate. Here we demonstrate a simple electric method to tune the vorticity of exciton polariton condensates in a strong coupling liquid crystal (LC) microcavity with CsPbBr$_3$ microplates as active material at room temperature. In such a microcavity, the LC molecular director can be electrically modulated giving control over the polariton condensation in different modes. For isotropic non-resonant optical pumping we demonstrate the spontaneous formation of vortices with topological charges of +1, +2, -2, and -1. The topological vortex charge is controlled by a voltage in the range of 1 to 10 V applied to the microcavity sample. This control is achieved by the interplay of a built-in potential gradient, the anisotropy of the optically active perovskite microplates, and the electrically controllable LC molecular director in our system with intentionally broken rotational symmetry. Besides the fundamental interest in the achieved electric polariton vortex control at room temperature, our work paves the way to micron-sized emitters with electric control over the emitted light's phase profile and quantized orbital angular momentum for information processing and integration into photonic circuits.

physics.optics↗

Single-shot spatial instability and electric control of polariton condensates at room temperature

In planar microcavities, the transverse-electric and transverse-magnetic (TE-TM) mode splitting of cavity photons arises due to their different penetration into the Bragg mirrors and can result in optical spin-orbit coupling (SOC). In this work, we find that in a liquid crystal (LC) microcavity filled with perovskite microplates, the pronounced TE-TM splitting gives rise to a strong SOC that leads to the spatial instability of microcavity polariton condensates under single-shot excitation. Spatially varying hole burning and mode competition occurs between polarization components leading to different condensate profiles from shot to shot. The single-shot polariton condensates become stable when the SOC vanishes as the TE and TM modes are spectrally well separated from each other, which can be achieved by application of an electric field to our LC microcavity with electrically tunable anisotropy. Our findings are well reproduced and traced back to their physical origin by our detailed numerical simulations. With the electrical manipulation our work reveals how the shot-to-shot spatial instability of spatial polariton profiles can be engineered in anisotropic microcavities at room temperature, which will benefit the development of stable polariton-based optoeletronic and light-emitting devices.

physics.optics↗

Exciton interaction induced spin splitting in MoS$_2$ monolayer

By pumping nonresonantly a MoS$_2$ monolayer at $13$ K under a circularly polarized cw laser, we observe exciton energy redshifts that break the degeneracy between B excitons with opposite spin. The energy splitting increases monotonically with the laser power reaching as much as $18$ meV, while it diminishes with the temperature. The phenomenon can be explained theoretically by considering simultaneously the bandgap renormalization which gives rise to the redshift and exciton-exciton Coulomb exchange interaction which is responsible for the spin-dependent splitting. Our results offer a simple scheme to control the valley degree of freedom in MoS$_2$ monolayer and provide an accessible method in investigating many-body exciton exciton interaction in such materials.

cond-mat.mes-hall↗