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Xiaoli Dong

Publications and source records attributed to Xiaoli Dong.

103 records · Page 6Linked to original sources

Growth, characterization and physical properties of high-quality large single crystals of Bi$_2$Sr$_{2-x}$La$_{x}$CuO$_6$ high-temperature superconductors

High quality large Bi$_2$Sr$_{2-x}$La$_{x}$CuO$_6$(La-Bi2201) single crystals have been successfully grown by the traveling solvent floating zone technique. The samples are characterized by compositional and structural analyzes and their physical properties are investigated by magnetic susceptibility and resistivity measurements. Superconducting samples with sharp superconducting transitions are obtained covering a wide range of doping from overdoped (x<0.40), optimally-doped (x~0.40), underdoped (0.40 0.84). Crystals as large as ~40 * 2.0 * 1 mm3 are obtained for x=0.73. Sharp superconducting transition with a width less than 2 K and nearly perfect Meissner signal of superconductivity are achieved for x=0.40. The availability of the La-Bi2201 single crystals will provide an ideal system to study the physical properties, electronic structure and mechanism of high temperature superconductivity

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Multiple Nodeless Superconducting Gaps in (Ba0.6K0.4)Fe2As2 Superconductor from Angle-Resolved Photoemission Spectroscopy

High resolution angle-resolved photoemission measurements have been carried out to study the superconducting gap in the (Ba0.6K0.4)Fe2As2 superconductor with Tc=35 K. Two hole-like Fermi surface sheets around the G(0,0) point exhibit different superconducting gaps. The inner Fermi surface sheet shows larger (10-12 meV) and slightly momentum-dependent gap while the outer one has smaller (7-8 meV) and nearly isotropic gap. The lack of gap node in both Fermi surface sheets favours s-wave superconducting gap symmetry. Superconducting gap opening is also observed at the M(pi,pi) point. The two Fermi surface spots near the M point are gapped below Tc but the gap persists above Tc. The rich and detailed superconducting gap information will provide key insights and constraints in understanding pairing mechanism in the iron-based superconductors.

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Floating-zone growth and property characterizations of high-quality La2-xSrxCuO4 single crystals

We have grown underdoped (x = 0.11, 0.12) and optimally doped (x = 0.16) La2-xSrxCuO4 (LSCO) crystals by traveling-solvent floating-zone (TSFZ) technique. In order to obtain LSCO single crystals of high quality, we have made much effort to optimize the preparation procedures. For example, we have adopted sol-gel route to prepare highly fine and homogeneous LSCO precursor powder, and used quite slow growth rate. The sizable grown crystal ingots are typically about 6.6 mm in diameter and 100 mm in length, and no impurity phases were detected. The high quality of grown crystals has been verified by double-crystal x-ray rocking curves, with full-width-at-half-maximum (FWHM) being only 113 ~ 150 arcseconds (or 0.03 deg - 0.04 deg), which are the best data reported so far for LSCO crystals. The superconducting critical temperatures (TC's) of the cuprate crystals are 30 K for x = 0.11, 31 K for x = 0.12 and 38.5 K for x = 0.16 samples according to magnetic measurements.

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High pressure study on LaFeAsO with different Tc

We report studies on pressure dependence of superconducting transition temperature (Tc) of LaFeAsO, LaFeAs(O0.5F0.5) and LaFeAs(O0.89F0.11) samples. In-situ resistance measurements under high pressure showed that the Tc of these three compounds increases with pressure initially, reaches a maximum value and then decreases with further increasing pressure, although the Tc at ambient pressure are different. The onset Tc of LaFeAsO is ~50 K at 1.5 GPa, which is the highest record in La-based oxypnicited system. The significant change in Tc induced by pressure is attributed to the orbital degeneracy and the electron density of state at the Fermi level.

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Monotonic d-wave Superconducting Gap in Optimally-Doped Bi$_2$Sr$_{1.6}$La$_{0.4}$CuO$_6$ Superconductor by Laser-Based Angle-Resolved Photoemission Spectroscopy

The momentum and temperature dependence of the superconducting gap and pseudogap in optimally-doped Bi$_2$Sr$_{1.6}$La$_{0.4}$CuO$_6$ superconductor is investigated by super-high resolution laser-based angle-resolved photoemission spectroscopy. The measured energy gap in the superconducting state exhibits a standard {\it d}-wave form. Pseudogap opens above T$_c$ over a large portion of the Fermi surface with a "Fermi arc" formed near the nodal region. In the region outside of the "Fermi arc", the pseudogap has the similar magnitude and momentum dependence as the gap in the superconducting state which changes little with temperature and shows no abrupt change across T$_c$. These observations indicate that the pseudogap and superconducting gap are closely related and favor the picture that the pseudogap is a precursor to the superconducting gap.

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Identification of Nodal Kink in Electron-Doped (Nd$_{1.85}$Ce$_{0.15}$)CuO$_4$ Superconductor from Laser-Based Angle-Resolved Photoemission Spectroscopy

High-resolution laser-based angle-resolved photoemission measurements have been carried out on the electron-doped (Nd$_{1.85}$Ce$_{0.15}$)CuO$_4$ high temperature superconductor. We have revealed a clear kink at $\sim$60 meV in the dispersion along the (0,0)-($π$,$π$) nodal direction, accompanied by a peak-dip-hump feature in the photoemission spectra. This indicates that the nodal electrons are coupled to collective excitations (bosons) in electron-doped superconductors, with the phonons as the most likely candidate of the boson. This finding has established a universality of nodal electron coupling in both hole- and electron-doped high temperature cuprate superconductors.

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Lattice and Magnetic structures of PrFeAsO, PrFeAsO0.85F0.15 and PrFeAsO0.85

We use powder neutron diffraction to study the spin and lattice structures of polycrystalline samples of nonsuperconducting PrFeAsO and superconducting PrFeAsO0.85F0.15 and PrFeAsO0.85. We find that PrFeAsO exhibits an abrupt structural phase transitions at 153 K, followed by static long range antiferromagnetic order at 127 K. Both the structural distortion and magnetic order are identical to other rare-earth oxypnictides. Electron-doping the system with either Fluorine or oxygen deficiency suppresses the structural distortion and static long range antiferromagnetic order, therefore placing these materials into the same class of FeAs-based superconductors.

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Fermi Surface and Band Renormalization in (Sr,K)Fe$_2$As$_2$ Superconductor from Angle-Resolved Photoemission Spectroscopy

High resolution angle-resolved photoemission measurements have been carried out on (Sr,K)Fe$_2$As$_2$ superconductor (Tc=21 K). Three hole-like Fermi surface sheets are clearly resolved for the first time around the Gamma point. The overall electronic structure shows significant difference from the band structure calculations. Qualitative agreement between the measured and calculated band structure is realized by assuming a chemical potential shift of -0.2 eV. The obvious band renormalization suggests the importance of electron correlation in understanding the electronic structure of the Fe-based compounds.

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Common Features in Electronic Structure of the Fe-Based Layered Superconductors from Photoemission Spectroscopy

High resolution photoemission measurements have been carried out on non-superconducting LaOFeAs parent compound and various superconducting R(O1-xFx)FeAs (R=La, Ce and Pr) compounds. We found that the parent LaOFeAs compound shows a metallic character. Through extensive measurements, we have identified several common features in the electronic structure of these Fe-based compounds: (1). 0.2 eV feature in the valence band; (2). A universal 13~16 meV feature; (3). A clear Fermi cutoff showing zero leading-edge shift in the superconducting state;(4). Lack of superconducting coherence peak(s); (5). Near EF spectral weight suppression with decreasing temperature. These universal features can provide important information about band structure, superconducting gap and pseudogap in these Fe-based materials.

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Superconducting Gap and Pseudogap in Sm(O$_{1-x}$F$_x$)FeAs Layered Superconductor from Photoemission Spectroscopy

High resolution photoemission measurements have been carried out on non-superconducting SmOFeAs parent compound and superconducting Sm(O$_{1-x}$F$_x$)FeAs (x=0.12, and 0.15) compounds. The momentum-integrated spectra exhibit a clear Fermi cutoff that shows little leading-edge shift in the superconducting state which suggests the Fermi surface sheet(s) around the $Γ$ point may not be gapped in this multiband superconductors. A robust feature at 13 meV is identified in all these samples. Spectral weight suppression near E$_F$ with decreasing temperature is observed in both undoped and doped samples that points to a possible existence of a pseudogap in these Fe-based compounds.

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Identification of a New Form of Electron Coupling in Bi2Sr2CaCu2O8 Superconductor by Laser-Based Angle-Resolved Photoemission

Laser-based angle-resolved photoemission measurements with super-high resolution have been carried out on an optimally-doped Bi$_2$Sr$_2$CaCu$_2$O$_8$ high temperature superconductor. New high energy features at $\sim$115 meV and $\sim$150 meV, besides the prominent $\sim$70 meV one, are found to develop in the nodal electron self-energy in the superconducting state. These high energy features, which can not be attributed to electron coupling with single phonon or magnetic resonance mode, point to the existence of a new form of electron coupling in high temperature superconductors.

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High Energy Dispersions in Bi2Sr2CaCu2O8 High Temperature Superconductor from Laser-Based Angle-Resolved Photoemission

Super-high resolution laser-based angle-resolved photoemission (ARPES) measurements have been carried out on the high energy electron dynamics in Bi2Sr2CaCu2O8 (Bi2212) high temperature superconductor. Momentum dependent measurements provide new insights on the nature of high energy kink at 200~400 meV and high energy dispersions. The strong dichotomy between the MDC- and EDC-derived bands is revealed which raises critical issues about its origin and which one represents intrinsic band structure. The MDC-derived high energy features are affected by the high-intensity valence band at higher binding energy and may not be intrinsic.

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Development of a Vacuum Ultra-Violet Laser-Based Angle-Resolved Photoemission System with a Super-High Energy Resolution Better Than 1 meV

The design and performance of the first vacuum ultra-violet (VUV) laser-based angle-resolved photoemission (ARPES) system are described. The VUV laser with a photon energy of 6.994 eV and bandwidth of 0.26 meV is achieved from the second harmonic generation using a novel non-linear optical crystal KBe2BO3F2 (KBBF). The new VUV laser-based ARPES system exhibits superior performance, including super-high energy resolution better than 1 meV, high momentum resolution, super-high photon flux and much enhanced bulk sensitivity, which are demonstrated from measurements on a typical Bi2Sr2CaCu2O8 high temperature superconductor. Issues and further development related to the VUV laser-based photoemission technique are discussed.

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