arXiv subjects

Xiaoping Ouyang

Publications and source records attributed to Xiaoping Ouyang.

18 recordsLinked to original sources

arXiv2026

Sub-50 Picosecond exceptionally Bright Perovskite Scintillation by Unlocking Giant Oscillator Strength

Ultrafast scintillators are indispensable for precise timing in high-energy physics and medical diagnostics. Fundamentally constrained by the trade-off between emission rate and light yield, conventional scintillators remain kinetically trapped in the sub-nanosecond regime, failing to break 50-picosecond limit. Here, we demonstrate a strategy to bypass this limitation by harnessing the coherent radiative acceleration in weakly confined CsPbCl3 perovskite nanocrystals to generate an ultrafast photon burst. This effect originates from the giant oscillator strength, which we unlock by suppressing exciton-phonon scattering at mild cryogenic temperatures. Consequently, our scintillator achieves an unprecedented dominant lifetime of 13.11 ps alongside a high light yield of 21,851 ph/MeV. The resulting prompt photon emission rate more than 100 times higher than that of state-of-the-art ultrafast scintillators. We validate this breakthrough in realistic detection scenarios, achieving a coincidence time resolution of 30.8 ps and accurately resolving 13.5 ps electron bunches and 16.6 ps single-shot gamma-ray pulses. Our findings establish a robust coherent framework for next-generation ultrafast scintillators, pushing extreme radiation diagnostics into the picosecond frontier.

cond-mat.mes-hall↗

arXiv2025

Machine learning bridging battery field data and laboratory data

Aiming at the dilemma that most laboratory data-driven diagnostic and prognostic methods cannot be applied to field batteries in passenger cars and energy storage systems, this paper proposes a method to bridge field data and laboratory data using machine learning. Only two field real impedances corresponding to a medium frequency and a high frequency are needed to predict laboratory real impedance curve, laboratory charge/discharge curve, and laboratory relaxation curve. Based on the predicted laboratory data, laboratory data-driven methods can be used for field battery diagnosis and prognosis. Compared with the field data-driven methods based on massive historical field data, the proposed method has the advantages of higher accuracy, lower cost, faster speed, readily available, and no use of private data. The proposed method is tested using two open-source datasets containing 249 NMC cells. For a test set containing 76 cells, the mean absolute percentage errors of laboratory real impedance curve, charge curve, and discharge curve prediction results are 0.85%, 4.72%, and 2.69%, respectively. This work fills the gap between laboratory data-driven diagnostic and prognostic methods and field battery applications, making all laboratory data-driven methods applicable to field battery diagnosis and prognosis. Furthermore, this work overturns the fixed path of developing field battery diagnostic and prognostic methods based on massive field historical data, opening up new research and breakthrough directions for field battery diagnosis and prognosis.

stat.AP↗

arXiv2025

Machine learning accelerates fuel cell life testing

Accelerated life testing (ALT) can significantly reduce the economic, time, and labor costs of life testing in the process of equipment, device, and material research and development (R&D), and improve R&D efficiency. This paper proposes a performance characterization data prediction (PCDP) method and a life prediction-driven ALT (LP-ALT) method to accelerate the life test of polymer electrolyte membrane fuel cells (PEMFCs). The PCDP method can accurately predict different PCD using only four impedances (real and imaginary) corresponding to a high frequency and a medium frequency, greatly shortening the measurement time of offline PCD and reducing the difficulty of life testing. The test results on an open source life test dataset containing 42 PEMFCs show that compared with the determination coefficient (R^2) results of predicted aging indicators, including limiting current, total mass transport resistance, electrochemically active surface area, and crossover current, obtained based on the measured PCD, the R^2 results of predicted aging indicators based on the predicted PCD is only reduced by 0.04, 0.01, 0.05, and 0.06, respectively. The LP-ALT method can shorten the life test time through early life prediction. Test results on the same open-source life test dataset of PEMFCs show that the acceleration ratio of the LP-ALT method can reach 30 times under the premise of ensuring that the minimum R^2 of the prediction results of different aging indicators, including limiting current, total mass transport resistance, and electrochemically active surface area, is not less than 0.89. Combining the different performance characterization data predicted by the PCDP method and the life prediction of the LP-ALT method, the diagnosis and prognosis of PEMFCs and their components can be achieved.

stat.AP↗

arXiv2025

Phase stabilization of In2Se3 by disordered Ni intercalation and its enhanced thermoelectrical performance

Van der Waals (vdW) layered materials have gained significant attention owing to their distinctive structure and unique properties. The weak interlayer bonding in vdW layered materials enables guest atom intercalation, allowing precise tuning of their physical and chemical properties. In this work, a ternary compound, NixIn2Se3 (x = 0-0.3), with Ni randomly occupying the interlayers of In2Se3, was synthesized via an intercalation route driven by electron injection. The intercalated Ni atoms act as anchor points within the interlayer of In2Se3, which effectively suppresses the phase transition of In2Se3 at elevated temperatures. Furthermore, the disordered Ni intercalation significantly enhanced the electrical conductivity of In2Se3 through electron injection, while reducing the thermal conductivity due to the interlayer phonon scattering, leading to an improved thermoelectric performance. For instance, the thermoelectric figure of merit (ZT) of Ni0.3In2Se3 increased by 86% (in-plane) and 222% (out-of-plane) compared to In2Se3 at 500 oC. These findings not only provide an effective strategy to enhance the performance of layered thermoelectric materials, but also demonstrate the potential of intercalation chemistry for expanding the application scope of van der Waals (vdW) layered materials.

cond-mat.mtrl-sci↗

arXiv2025

Unconventional topological edge states in one-dimensional gapless systems stemming from nonisolated hypersurface singularities

Topologically protected edge states have been extensively studied in systems characterized by the topological invariants in band gaps (also called line gaps). In this study, we unveil a whole new form of edge states that transcends the established paradigms of band-gap topology. In contrast to the traditional stable edge states in topological insulators with specific band gaps, the one-dimensional systems we investigate are inherently gapless with the Brillouin zones being mapped to the loops encircling hypersurface singularities in a higher-dimensional space with parity-time symmetry. These hypersurface singularities are nonisolated degeneracies embedded entirely on exceptional surfaces, rendering the energy gaps in our systems inevitably closed at the intersections of the Brillouin zone loop and the exceptional surfaces. Unexpectedly, such gapless systems still afford topologically protected edge states at system boundaries, challenging the conventional understanding based on band gaps. To elucidate the existence of these edge states in the absence of a band-gap-based invariant, we propose a theoretical framework based on eigen-frame rotation and deformation that incorporates non-Bloch band theory. Finally, we experimentally demonstrate this new form of topological edge states with nonreciprocal circuits for the first time. Our work constitutes a major advance that extends topological edge states from gapped phases to gapless phases, offering new insights into topological phenomena.

cond-mat.mes-hall↗

arXiv2024

Convective meta-thermal dispersion for self-adaptive cooling enhancement

Improving the heat transfer coefficient is crucial across various energy utilization processes for maintaining device safety and stability with high energy efficiency. However, in scenarios with limited heat capacity flow rates, increasing the thermal conductivity of encapsulated internal heat source (IHS) packaging can paradoxically impede heat transfer. Herein, we introduced a convective-meta thermal dispersion (CMTD) strategy applicable throughout the energy domain. By integrating low thermal conductivity materials into high thermal conductivity package structures, we disrupted tangential heat flow while preserving efficient radial heat transport. Through this approach, a notable reduction in tangential temperature within the fluid channel was achieved, effectively lowering the IHS temperature. Remarkably, this cooling mechanism does not need additional energy input, thermal property enhancements, or expanded heat transfer areas, which are often prerequisites in existing technologies. Moreover, spontaneous enhancement phenomena emerged under constrained heat transfer conditions, termed self-adaptive cooling enhancement. Our investigations revealed, under steady-state conditions, a maximum 24.5% decrease in IHS average temperature, while transient conditions exhibited a maximum 32.3% increase in heat transfer between the IHS and cooling fluid, validating the efficacy of the CMTD strategy. These findings offer a promising pathway for efficient thermal management in various thermal energy utilization fields with high power density such as nuclear fission and fusion and contributed to a deeper understanding of fundamental fluid-solid heat transfer mechanisms across the energy science.

physics.app-ph↗

arXiv2024

Chlorine and zinc co-doping effects on the electronic structure and optical properties of γ-CuI

The effects of chlorine (Cl) and zinc (Zn) co-doping on the electronic structure and optical properties of the zinc blende (γ) phase of copper iodide (γ-CuI) scintillator material are investigated by using first-principles density functional theory calculations. The band structure, density of states, dielectric function, absorption coefficients, and reflectivity were analyzed before and after doping. Results show co-doping significantly modifies the band structure, reduces the band gap, and generates impurity energy levels. Cl doping enhances absorption in the high energy region while reducing visible light absorption. Zn doping induces a redshift in absorption and n-type conductivity at high concentrations. With suitable co-doping ratios, the absorption coefficient and reflectivity of γ-CuI can be optimized in the visible range to improve scintillation light yield. The calculations provide guidance for co-doping γ-CuI scintillators to achieve superior detection performance. The n-type conductivity also makes doped γ-CuI promising for optoelectronic applications.

cond-mat.mtrl-sci↗

arXiv2024

Controlling mass and energy diffusion with metamaterials

Diffusion driven by temperature or concentration gradients is a fundamental mechanism of energy and mass transport, which inherently differs from wave propagation in both physical foundations and application prospects. Compared with conventional schemes, metamaterials provide an unprecedented potential for governing diffusion processes, based on emerging theories like the transformation and the scattering cancellation theory, which enormously expanded the original concepts and suggest innovative metamaterial-based devices. We hereby use the term "diffusionics" to generalize these remarkable achievements in various energy (e.g., heat) and mass (e.g., particles and plasmas) diffusion systems. For clarity, we categorize the numerous studies appeared during the last decade by diffusion field (i.e., heat, particles, and plasmas) and discuss them from three different perspectives: the theoretical perspective, to detail how the transformation principle is applied to each diffusion field; the application perspective, to introduce various intriguing metamaterial-based devices, such as cloaks and radiative coolers; and the physics perspective, to connect with concepts of recent concern, such as non-Hermitian topology, nonreciprocal transport, and spatiotemporal modulation. We also discuss the possibility of controlling diffusion processes beyond metamaterials. Finally, we point out several future directions for diffusion metamaterial research, including the integration with artificial intelligence and topology concepts.

physics.app-ph↗

arXiv2024

Convective meta-thermal concentration for ultrahigh efficient Stirling engine with waste heat and cold utilization

The Stirling engine, which possesses external combustion characteristics, a simple structure, and high theoretical thermal efficiency, has excellent potential for utilizing finite waste heat and cold resources. However, practical applications of this technology suffered from thermal inefficiency due to the discontinuity and instability of waste resources. Despite advances in energy storage technology, temperature variations in the heat-exchanging fluids at the hot and cold ends of the Stirling engine remained significant obstacles. In this work, convective meta-thermal concentration (CMTC) was introduced between the heating (cooling) fluids and the hot (cold) end of the Stirling engine, employing alternating isotropic materials with high and low thermal conductivities. It was demonstrated that CMTC effectively enhanced the temperature difference between the hot and cold ends, leading to a remarkable improvement in Stirling engine efficiency. Particularly, when the Stirling engine efficiency tended to zero due to the limited availability of waste heat and cold resources, CMTC overcame this limitation, surpassing existing optimization technology. Further analysis under various operating conditions showed that CMTC achieved a significant thermal efficiency improvement of up to 1460%. This work expanded the application of thermal metamaterials to heat engine systems, offering an exciting avenue for sustainable energy utilization.

physics.app-ph↗

arXiv2024

Reconfigurable Three-Dimensional Thermal Dome

Thermal metamaterial represents a groundbreaking approach to control heat conduction, and, as a crucial component, thermal invisibility is of utmost importance for heat management. Despite the flourishing development of thermal invisibility schemes, they still face two limitations in practical applications. First, objects are typically completely enclosed in traditional cloaks, making them difficult to use and unsuitable for objects with heat sources. Second, although some theoretical proposals have been put forth to change the thermal conductivity of materials to achieve dynamic invisibility, their designs are complex and rigid, making them unsuitable for large-scale use in real three-dimensional spaces. Here, we propose a concept of a thermal dome to achieve three-dimensional invisibility. Our scheme includes an open functional area, greatly enhancing its usability and applicability. It features a reconfigurable structure, constructed with simple isotropic natural materials, making it suitable for dynamic requirements. The performance of our reconfigurable thermal dome has been confirmed through simulations and experiments, consistent with the theory. The introduction of this concept can greatly advance the development of thermal invisibility technology from theory to engineering and provide inspiration for other physical domains, such as direct current electric fields and magnetic fields.

physics.app-ph↗

arXiv2023

Muon radiography experiments on the subway overburden structure detection

Muon radiography is an innovative and non-destructive technique for internal density structure imaging, based on measuring the attenuation of cosmic-ray muons after they penetrate the target. Due to the strong penetration ability of muons, the detection range of muon radiography can reach the order of hundreds of meters or even kilometers. Using a portable muon detector composed of plastic scintillators and silicon photomultipliers, we performed a short-duration(1h) flux scanning experiment of the overburden above the platform and tunnel of the Xiaoying West Road subway station under construction. With the observation direction facing up, the detector is placed on the north side of the track and moved eastward from the platform section inside the station to the tunnel section. The scanning length is 264m and a total of 21 locations are observed. By comparing the observed and predicted values of the muon survival ratio at different locations, the experiment accurately detects the jump in thickness at the interface of the platform section and tunnel section. Furthermore, unknown anomalies caused by random placed light brick piles and side passage mouth above the observation locations are detected and confirmed later. This experiment verifies the feasibility of using natural muons to quickly detect abnormal structures of the overburden of tunnel, and shows that muon radiography has broad application prospects in tunnel safety and other similar aspects.

physics.ins-det↗

arXiv2023

Tunable liquid-solid hybrid thermal metamaterials with a topology transition

Thermal metamaterials provide rich control of heat transport which is becoming the foundations of cutting-edge applications ranging from chip cooling to biomedical. However, due to the fundamental laws of physics, the manipulation of heat is much constrained in conventional thermal metamaterials where effective heat conduction with Onsager reciprocity dominates. Here, through the inclusion of thermal convection and breaking the Onsager reciprocity, we unveil a regime in thermal metamaterials and transformation thermotics that goes beyond effective heat conduction. By designing a liquid-solid hybrid thermal metamaterial, we demonstrate a continuous switch from thermal cloaking to thermal concentration in one device with external tuning. Underlying such a switch is a topology transition in the virtual space of the thermotic transformation which is achieved by tuning the liquid flow via external control. These discoveries illustrate the extraordinary heat transport in complex multi-component thermal metamaterials and pave the way toward an unprecedented regime of heat manipulation.

physics.app-ph↗

arXiv2022

Blackhole-Inspired Thermal Trapping with Graded Heat-Conduction Metadevices

Black holes are one of the most intriguing predictions of general relativity. So far, metadevices have enabled analogous black holes to trap light or sound in laboratory spacetime. However, trapping heat in a conductive ambient is still challenging because diffusive behaviors are directionless. Inspired by black holes, we construct graded heat-conduction metadevices to achieve thermal trapping, resorting to the imitated advection produced by graded thermal conductivities rather than the trivial solution of using insulation materials to confine thermal diffusion. We experimentally demonstrate thermal trapping for guiding hot spots to diffuse towards the center. Graded heat-conduction metadevices have advantages in energy-efficient thermal regulation because the imitated advection has a similar temperature field effect to the realistic advection that is usually driven by external energy sources. These results also provide insights into correlating transformation thermotics with other disciplines such as cosmology for emerging heat control schemes.

physics.app-ph↗

arXiv2021

Manipulation of polar vortex chirality in oxide superlattices

Topological polar vortices that are the electric analogues of magnetic objects, present great potential in applications of future nanoelectronics due to their nanometer size, anomalous dielectric response, and chirality. To enable the functionalities, it is prerequisite to manipulate the polar states and chirality by using external stimuli. Here, we probe the evolutions of polar state and chirality of polar vortices in PbTiO3/SrTiO3 superlattices under electric field by using atomically resolved in situ scanning transmission electron microscopy and phase-field simulations. We find that the adjacent clockwise and counterclockwise vortex usually have opposite chirality. The phase-field simulations suggest that the rotation reversal or axial polarization switching can lead to the chirality change. Guided by which, we experimentally validate that the vortex rotation direction can be changed by applying and subsequently removing of electric fields, offering a potential strategy to manipulate the vortex chirality. The revealed details of dynamic behavior for individual polar vortices at atomic scale and the proposed strategy for chirality manipulation provide fundamentals for future device applications.

cond-mat.mtrl-sci↗

arXiv2021

Resolving ultrahigh-contrast ultrashort pulses with single-shot cross-correlator at the photon noise limit

In strong-field physics experiments with intense lasers, it is of paramount importance to single-shot diagnose the temporal contrast between laser pulse peak and its noise pedestal. This allows fast optimization of pulse contrast and meaningful comparison with theory for each pulse shot, and it can help new outcomes from clean laser-plasma interactions. Thus far, high contrast ratios up to ~10^10, required by present petawatt (PW) class lasers, have been accessible in both generation and single-shot characterization. However, ultrahigh contrast ~10^13, required by the planned 200-PW lasers, challenges intense laser technology and remains an open question. This paper reports on the first demonstration of such an ultrahigh-contrast measurement by adapting single-shot cross-correlator (SSCC). We introduce an ultrafast method that enables to determine the SSCC detection limit. Our strategy mimics the test laser having known ultrahigh contrast in the measurement frame of time-to-space mapping. The ultimate contrast-measurement limit of 10^13 is achieved, which corresponds to the highest pulse intensity set by SSCC damage threshold and the lowest noise pedestal set by single-photon detection. As a consequence, photon noise in the detection is observed and increases as the noise pedestal reduces. The demonstrated measurement ability at the photon noise limit is applied to a high-contrast laser system based on second-harmonic generation and optical parametric chirped-pulse amplification, suggesting accessible of ultrahigh contrast pulses.

physics.optics↗

arXiv2020

Bremsstrahlung emission and plasma characterization driven by moderately relativistic laser-plasma interactions

Relativistic electrons generated by the interaction of petawatt-class short laser pulses with solid targets can be used to generate bright X-rays via bremsstrahlung. The efficiency of laser energy transfer into these electrons depends on multiple parameters including the focused intensity and pre-plasma level. This paper reports experimental results from the interaction of a high intensity petawatt-class glass laser pulses with solid targets at a maximum intensity of $10^{19}$ W/cm$^2$. In-situ measurements of specularly reflected light are used to provide an upper bound of laser absorption and to characterize focused laser intensity, the pre-plasma level and the generation mechanism of second harmonic light. The measured spectrum of electrons and bremsstrahlung radiation provide information about the efficiency of laser energy transfer.

physics.plasm-ph↗

arXiv2019

Effects of transmutation elements in tungsten

Tungsten (W) is widely considered as the most promising plasma facing material (PFM), which will be used in nuclear fusion devices. Due to the transmutation reaction caused by the fusion neutron irradiation, transmutation elements (such as Re, Os, and Ta) are generated in the W-based PFM during the operation of nuclear fusion devices. In this paper, transmutation elements effects on mechanical properties of the W and the behavior of hydrogen/helium (H/He) atom in the W were investigated by using the first-principles calculation method. The results show that the ductility of the W is enhanced by transmutation elements if dislocation and other defects were ignored, while mechanical properties of the W incompletely depend on transmutation elements content. Compared with the pure W, the formation energy of the H/He in the W is reduced by transmutation elements, but the most favorable sites of the H/He in the W is not changed. Except for a repulsion between Ta and He in the W, the H/He in the W is attracted by transmutation elements. In addition, transmutation elements can change the best diffusion path of the H/He in the W and increase the diffusion rate of the H/He in W. This study provides a theoretical basis for the Tungsten (W) application, and further study on the effects of transmutation elements in the W will be needed.

cond-mat.mtrl-sci↗

arXiv2016

Potential reduction interior point algorithm unfolding of neutron energy spectrum measured by recoil proton method

A reconstruction algorithm for unfolding the neutron energy spectrum has been developed based on the potential reduction interior point. This algorithm can be easily applied to the neutron energy spectrum reconstruction in the recoil proton method. We transform neutron energy spectrum unfolding problem into a typical nonnegative linear complementarity problem. The recoil proton energy spectrum and response matrix at angles of 0° and 30° are generated by the Geant4 simulation toolkit. Several different neutron energy test spectrums are also employed. It is found that this unfolding algorithm is stable and provide efficiency accurate results.

physics.ins-det↗