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Xin Liang Tan

Publications and source records attributed to Xin Liang Tan.

7 recordsLinked to original sources

Disentangling bulk and surface states in the electronic structure of PtBi$_2$(0001)

Recent reports of surface-localized topological superconductivity in trigonal PtBi$_2$ highlight the importance of understanding its surface electronic structure. We investigate the bulk and surface band structure of PtBi$_2$ using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations. Through photon-energy- and polarization-dependent measurements, we disentangle bulk dispersions from surface states on the two distinct surface terminations of PtBi$_2$(0001). For both terminations, we assign several different surface states and find good agreement between experiment and calculations. Based on our calculations, we analyze the orbital composition in the surface and bulk bands and compare the results to polarization-dependent ARPES measurements. Together, our results provide a coherent picture of the surface electronic structure of PtBi$_2$ across both surface terminations.

cond-mat.str-el

Fermiology and spin polarization of topological surface states in PtBi$_2$

Layered PtBi$_2$ is a candidate for topological superconductivity arising in Fermi-arc surface states. Using spin- and angle-resolved photoemission spectroscopy, we demonstrate that the Fermi arcs in PtBi$_2$ are singly degenerate and spin-polarized, which establishes their nontrivial topology and constitutes a necessary condition for topological superconductivity. We further uncover a pronounced surface-termination dependence of the Fermi-arc dispersion, yielding either nearly flat or approximately linear bands in agreement with first-principles calculations. Together, the observed spin polarization and termination-dependent bandwidth of the Fermi-arc surface states identify key ingredients underlying the potential emergence of topological superconductivity in PtBi$_2$.

cond-mat.supr-con

Electronic Structure and Resonant Circular Dichroism of La$_{0.7}$Sr$_{0.3}$MnO$_3$ from Soft X-ray Angle-Resolved Photoemission

Coupling between spin, orbital, charge, and lattice degrees of freedom in transition-metal oxides produces a variety of electronic and magnetic phenomena of importance for future technologies. Here, we explore the electronic band structure of a (111)-oriented La0.7Sr0.3MnO3 thin film through soft X-ray angle-resolved photoemission spectroscopy (ARPES). The measurements agree with the electronic band structure calculated with density functional theory using Hubbard U correction. Furthermore, we probe the circular dichroism in ARPES, and observe a pronounced momentum- resolved magnetic circular dichroism in resonant photoemission from the Mn L-edge. The approach combines the momentum- and spin-selectivity of ARPES and X-ray magnetic circular dichroism, respectively, which could provide a useful approach for the study of unconventional magnetism.

cond-mat.str-el

Orbital Topology of Chiral Crystals for Orbitronics

Chirality is ubiquitous in nature and manifests in a wide range of phenomena including chemical reactions, biological processes, and quantum transport of electrons. In quantum materials, the chirality of fermions, given by the relative directions between the electron spin and momentum, is connected to the band topology of electronic states. Here, we show that in structurally chiral materials like CoSi, the orbital angular momentum (OAM) serves as the main driver of a nontrivial band topology in this new class of unconventional topological semimetals, even when spin-orbit coupling is negligible. A nontrivial orbital-momentum locking of multifold chiral fermions in the bulk leads to a pronounced OAM texture of the helicoid Fermi arcs at the surface. Our findings highlight the pivotal role of the orbital degree of freedom for the chirality and topology of electron states, in general, and pave the way towards the application of topological chiral semimetals in orbitronic devices.

cond-mat.mes-hall

Giant Rashba-Splitting of One-Dimensional Metallic States in Bi Dimer Lines on InAs(100)

Bismuth produces different types of ordered superstructures on the InAs(100) surface, depending on the growth procedure and coverage. The (2x1) phase forms at completion of a Bi monolayer and consists of a uniformly oriented array of parallel lines of Bi dimers. Scanning tunneling and core level spectroscopies demonstrate its metallic character, in contrast with the semiconducting properties expected on the basis of the electron counting principle. The weak electronic coupling among neighboring lines gives rise to quasi one-dimensional Bi-derived bands with open contours at the Fermi level. Spin- and angle-resolved photoelectron spectroscopy reveals a giant Rashba splitting of these bands, in good agreement with ab-initio electronic structure calculations. The very high density of the dimer lines, the metallic and quasi one-dimensional band dispersion and the Rashba-like spin texture make the Bi/InAs(100)-(2x1) phase an intriguing system, where novel transport regimes can be studied.

cond-mat.mtrl-sci

Chirality-Driven Orbital Angular Momentum and Circular Dichroism in CoSi

Chiral crystals and molecules were recently predicted to form an intriguing platform for unconventional orbital physics. Here, we report the observation of chirality-driven orbital textures in the bulk electronic structure of CoSi, a prototype member of the cubic B20 family of chiral crystals. Using circular dichroism in soft X-ray angle-resolved photoemission, we demonstrate the formation of a bulk orbital-angular-momentum texture and monopole-like orbital-momentum locking that depends on crystal handedness. We introduce the intrinsic chiral circular dichroism, icCD, as a differential photoemission observable and a natural probe of chiral electron states. Our findings render chiral crystals promising for spin-orbitronics applications.

cond-mat.mtrl-sci

Link between Weyl-fermion chirality and spin texture

Topological semimetals have recently attracted great attention due to prospective applications governed by their peculiar Fermi surfaces. Weyl semimetals host chiral fermions that manifest as pairs of non-degenerate massless Weyl points in their electronic structure, giving rise to novel macroscopic quantum phenomena such as the chiral anomaly, an unusual magnetoresistance, and various kinds of Hall effects These properties enable the engineering of non-local electric transport devices, magnetic sensors and memories, and spintronics devices. Nevertheless, little is known about the underlying spin- and orbital-degrees of freedom of the electron wave functions in Weyl semimetals, that govern the electric transport. Here, we give evidence that the chirality of the Weyl points in the Type-II Weyl semimetal MoTe$_2$ is directly linked to the spin texture and orbital angular momentum of the electron wave functions. By means of state-of-the-art spin- and momentum-resolved photoemission spectroscopy the spin- and orbital texture in the Fermi surface is directly resolved. Supported by first-principles calculations, we examined the relationship between the topological chiral charge and spin texture, which significantly contributes to the understanding of the electronic structure in topological quantum materials.

cond-mat.mtrl-sci