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Xin-Yi Tian

Publications and source records attributed to Xin-Yi Tian.

3 recordsLinked to original sources

Ultrafast Fluence-Reversal Fingerprint of Fragile Kondo Hybridization in CePt$_2$In$_7$

The emergence of heavy quasiparticles in a Kondo lattice is usually viewed as the formation of a low-energy hybridization gap. Whether this gap represents a rigid electronic structure or a fragile many-body state that can be dynamically reconfigured remains a central question for heavy-fermion systems near magnetic order, quantum criticality, and unconventional superconductivity. Here we use femtosecond pump-probe reflectivity to interrogate this problem in the weakly hybridized Kondo-lattice compound CePt$_2$In$_7$. At low fluence, a slow quasiparticle relaxation channel emerges below $T^* \sim$ 40 K and follows a Rothwarf-Taylor bottleneck response with a low-energy recombination scale 2$Δ\approx$ 7.4 meV. Coherent optical phonons, independently identified by Raman spectroscopy, act as an internal lattice thermometer and rule out large quasi-equilibrium lattice heating as the origin of the nonlinear electronic response. The phonon-free electronic amplitude $A_{\rm elec}$ reveals a fluence-reversal fingerprint: with cooling from the hybridization-crossover regime, the response evolves from weak-linear behavior to Rothwarf-Taylor-like bottleneck suppression and finally to anomalous high-fluence enhancement at the lowest temperatures. This reversal cannot be accounted for by a rigid fixed-gap bottleneck alone and instead identifies an ultrafast optical signature of photoinduced redistribution of a fragile Kondo-hybridized electronic response.

cond-mat.str-el↗

Anisotropic Hybridization Dynamics in the Quasi-One-Dimensional Kondo Lattice CeCo$_2$Ga$_8$ Revealed by Ultrafast Optical Spectroscopy

We investigate the ultrafast dynamics of the quasi-one-dimensional Kondo lattice CeCo$_2$Ga$_8$ using optical pump-probe spectroscopy. Time-resolved pump-probe reflectivity measurements reveal a strong anisotropy in the photoinduced response, which is a direct consequence of the material's unique electronic structure. The temperature dependence of the relaxation dynamics provides evidence for the formation of two distinct hybridization gaps that appear at different temperatures in the heavy fermion state. A direct gap of 2$Δ_{dir}$ $\approx$ 50 meV that persists up to $T^†$ $\approx$ 90 K, well above the coherence temperature $T^*$ $\approx$ 20 K. We attribute this higher-temperature gap to the hybridization fluctuations. An indirect gap of 2$Δ_{ind}$ $\approx$ 10 meV opens closer to $T^*$, signifying the development of long-range coherence in the heavy fermion state. Furthermore, we find that the hybridization gap can be suppressed with increasing pump fluence, indicating a delicate interplay between photoexcitation and the coherent heavy fermion state. Our results provide insights into the interplay of Kondo physics and low dimensionality in CeCo$_2$Ga$_8$, and establish ultrafast optical spectroscopy as a sensitive probe of anisotropic hybridization in heavy fermion materials.

cond-mat.str-el↗

Exploring Fermi Surface Nesting and the Nature of Heavy Quasiparticles in the Spin-Triplet Superconductor Candidate CeRh$_2$As$_2$

In this study, we investigate the electronic structure of a spin-triplet superconductor candidate CeRh$_2$As$_2$ using high-resolution angle-resolved photoemission spectroscopy and density functional theory calculations. Notably, Fermi surface nesting hints at connections to magnetic excitation or quadrupole density wave phenomena, elucidating the superconducting mechanisms. Measured band structures reveal primarily localized 4f electrons, with minor itinerant contributions. Additionally, a transition from localized to itinerant behavior and significant c-f hybridization anisotropy underscore the role of f-electrons in shaping electronic properties. These findings deepen our understanding of CeRh$_2$As$_2$'s unconventional superconductivity and magnetism. Further exploration promises advances in superconductivity research.

cond-mat.supr-con↗