arXiv subjects

Xinfeng Liu

Publications and source records attributed to Xinfeng Liu.

At least 19 recordsLinked to original sources

arXiv2026

Reconfigurable ultrafast perovskite polariton logic gates via nonlinear dynamics

Exciton-polaritons provide a great platform for developing ultrafast all-optical logic gates for quantum and optical chips. However, progress toward practical polariton logic remains limited due to incomplete logical functionality on a single device. Herein, we present a single-device perovskite polariton platform enabling reconfigurable, ultrafast logic gates with functional completeness. The device consists of an optically trapped perovskite microwire, generating well-controlled non-equilibrium polariton condensation states for multiple logic operation channels. By tailoring the power of signal and gate beams, the same device is programmed to execute three basic Boolean functions (AND,OR,and NOT) and a high-order XOR function with a high on/off ratio of 21 dB, and a fast response time 6.7 ps. The reconfigurability arises from the selective activation of different nonlinear responses of polariton condensates, including amplification, seeding state transitions, and nonlinear interaction. These results provide valuable insights for advancing exciton-polariton logic gates.

physics.optics↗

arXiv2025

Ultrafast Exciton-Polariton Transport and Relaxation in Halide Perovskite

Halide perovskites offer a great platform for room-temperature exciton-polaritons (EPs) due to their strong oscillator strength and large exciton binding energy, promising applications in next-generation photonic and polaritonic devices. Efficient manipulation of EP transport and relaxation is critical for device performance, yet their spatiotemporal dynamics across different in-plane momenta (k//) remain poorly understood due to limitations in experimental access. In this work, we employ energy-resolved transient reflectance microscopy (TRM) combined with the dispersion relation of EPs to achieve high-resolution imaging of EP transport at specific k//. This approach directly reveals the quasi-ballistic transport and ultrafast relaxation of EPs in different k// regions, showcasing diffusion as fast as ~490 cm2/s and a relaxation time of ~95.1 fs. Furthermore, by tuning the detuning parameter, we manipulate the ballistic transport group velocity and relaxation time of EPs across varying k//. Our results reveal key insights into the dynamics of EP transport and relaxation, providing valuable guidance for the design and optimization of polaritonic devices.

cond-mat.mtrl-sci↗

arXiv2025

All-optical and ultrafast control of high-order exciton-polariton orbital modes

Exciton-polaritons flows within closed quantum circuits can spontaneously form phase-locked modes that carry orbital angular momentum (OAM). With its infinite set of angular momentum quantum numbers, high-order OAM represents a transformative solution to the bandwidth bottleneck in multiplexed optical communication. However, its practical application is hindered by the limited choice of materials which in general requires cryogenic temperatures and the reliance on mechanical switching. In this work, we achieve stable and high-order (up to order of 33) OAM modes by constructing a closed quantum circuit using the halide perovskite microcavities at room temperature. By controlling the spatial and temporal symmetry of the closed quantum circuits using another laser pulse, we achieve significant tuning OAM of EP flows from 8 to 12. Our work demonstrate all-optical and ultrafast control of high-order OAM using exciton-polariton condensates in perovskite microcavities that would have important applications in high-throughput optical communications.

physics.optics↗

arXiv2024

Strongly Magnetically Tuned Coupling Strength and Nonlinearity in CrSBr Exciton-Polaritons

Two-dimensional van der Waals (vdW) magnetic semiconductors CrSBr offer an ideal platform to achieve exciton-polaritons correlated with magnetic orders for developing solid-state quantum, spintronic, and photonic devices. However, for the exciton-polaritons formed by lower-energy excitons (XL = 1.37 eV), the coupling strength and nonlinear optical response are almost inert to the external magnetic field. Here, we demonstrate robust strong coupling between higher-energy excitons (XH = 1.8 eV) and photons that persists up to room temperature, along with giant magnetic-field tunability. The Rabi splitting energy is tuned up to 100 meV within a moderate 0.45 T in-plane magnetic field due to changes in excitonic states during the spin transitions. Besides, we observe significantly enhanced polariton nonlinearity in the intermediate magnetic phase, which exhibits a distinct mode-number dependence and originates from magnon-assisted long-range attractive interactions and coupling strength reduction. These results advance the development of on-demand polariton platforms for spin-correlated quantum optoelectronics.

cond-mat.mtrl-sci↗

arXiv2024

Giant Magneto-Exciton Coupling in 2D van der Waals CrSBr

Controlling magnetic order via external fields or heterostructures enables precise manipulation and tracking of spin and exciton information, facilitating the development of high-performance optical spin valves. However, the weak magneto-optical signals and instability of two dimensional (2D) antiferromagnetic (AFM) materials have hindered comprehensive studies on the complex coupling between magnetic order and excitons in bulk-like systems. Here, we leverage magneto-optical spectroscopy to reveal the impact of magnetic order on exciton-phonon coupling and exciton-magnetic order coupling which remains robust even under non-extreme temperature conditions (80 K) in thick layered CrSBr. A 0.425T in-plane magnetic field is sufficient to induce spin flipping and transition from AFM to ferromagnetic (FM) magnetic order in CrSBr, while magnetic circular dichroism (MCD) spectroscopy under an out-of-plane magnetic field provides direct insight into the complex spin canting behavior in thicker layers. Theoretical calculations reveal that the strong coupling between excitons and magnetic order, especially the 32 meV exciton energy shift during magnetic transitions, stems from the hybridization of Cr and S orbitals and the larger exciton wavefunction radius of higher-energy B excitons. These findings offer new opportunities and a solid foundation for future exploration of 2D AFM materials in magneto-optical sensors and quantum communication using excitons as spin carriers.

cond-mat.mtrl-sci↗

arXiv2024

Ultrafast carriers' separation imaging in WS2-WSe2 in plane heterojunction by transient reflectivity microscopy

Carrier transport in nanodevices plays a crucial role in determining their functionality. In the post-Moore era, the behavior of carriers near surface or interface domains the function of the whole devices. However, the femtosecond dynamics and nanometer-scale movement of carriers pose challenges for imaging their behavior. Techniques with high spatial-temporal resolution become imperative for tracking their intricate dynamics. In this study, we employed transient reflectivity microscopy to directly visualize the charge separation in the atomic interface of WS2-WSe2 in-plane heterojunctions. The carriers' drifting behavior was carefully tracked, enabling the extraction of drift velocities of 30 nm/ps and 10.6 nm/ps for electrons and holes. Additionally, the width of the depletion layer was determined to be 300 nm based on the carriers' moving trajectory. This work provides essential parameters for the potential effective utilization of these covalent in-plane heterojunctions,and demonstrates the success of transient optical imaging in unraveling the electrical behavior of nano devices, paving the way for a new avenue of electro-optical analysis.

cond-mat.mes-hall↗

arXiv2024

Room-temperature continuous-wave pumped exciton polariton condensation in a perovskite microcavity

Microcavity exciton polaritons (polaritons) as part-light part-matter quasiparticles, garner significant attention for non-equilibrium Bose-Einstein condensation at elevated temperatures. Recently, halide perovskites have emerged as promising room-temperature polaritonic platforms thanks to their large exciton binding energies and superior optical properties. However, currently, inducing room-temperature non-equilibrium polariton condensation in perovskite microcavities requires optical pulsed excitations with high excitation densities. Herein, we demonstrate continuous-wave optically pumped polariton condensation with an exceptionally low threshold of ~0.6 W cm-2 and a narrow linewidth of ~1 meV. Polariton condensation is unambiguously demonstrated by characterizing the nonlinear behavior and coherence properties. We also identify a microscopic mechanism involving the potential landscape in the perovskite microcavity, where numerous discretized energy levels arising from the hybridization of adjacent potential minima enhance the polariton relaxation, facilitating polariton condensate formation. Our findings lay the foundation for the next-generation energy-efficient polaritonic devices operating at room temperature.

physics.optics↗

arXiv2023

Idealizing Tauc Plot for Accurate Bandgap Determination of Semiconductor with UV-Vis: A Case Study for Cubic Boron Arsenide

The Tauc plot method is widely used to determine the bandgap of semiconductors via UV-visible optical spectroscopy due to its simplicity and perceived accuracy. However, the actual Tauc plot often exhibits significant baseline absorption below the expected bandgap, leading to discrepancies in the calculated bandgap depending on whether the linear fit is extrapolated to zero or non-zero baseline. In this study, we show that both extrapolation methods can produce significant errors by simulating Tauc plots with varying levels of baseline absorption. To address this issue, we propose a new method that involves idealizing the absorption spectrum by removing its baseline before constructing the Tauc plot. Experimental verification of this method using a gallium phosphide (GaP) wafer with intentionally introduced baseline absorptions shows promising results. Furthermore, we apply this new method to cubic boron arsenide (c-BAs) and resolve discrepancies in c-BAs bandgap values reported by different groups, obtaining a converging bandgap of 1.835 eV based on both previous and new transmission spectra. The method is applicable to both indirect and direct bandgap semiconductors, regardless of whether the absorption spectrum is measured via transmission or diffuse reflectance, will become essential to obtain accurate values of their bandgaps.

cond-mat.mtrl-sci↗

arXiv2023

Dual-modality Smart Shoes for Quantitative Assessment of Hemiplegic Patients' Lower Limbs' Muscle Strength

Stroke can lead to the impaired motor ability of the patient's lower limbs and hemiplegia. Accurate assessment of the lower limbs' motor ability is important for diagnosis and rehabilitation. To digitalize such assessment so that each test can be traced back any time and subjectivity can be avoided, we test how dual-modality smart shoes equipped with pressure-sensitive insoles and inertial measurement units can be used for this purpose. A 5m walking test protocol, including the left and right turns, is designed. Data are collected from 23 patients and 17 healthy subjects. For the lower limbs' motor ability, the tests are observed by two physicians and assessed using the five graded Medical Research Council scale for muscle examination. The average of two physicians' scores for the same patient is used as the ground truth. Using the feature set we developed, 100\% accuracy is achieved in classifying the patients and healthy subjects. For patients' muscle strength, a mean absolute error of 0.143 and a maximum error of 0.395 is achieved using our feature set and the regression method, closer to the ground truth than the scores from each physician (mean absolute error: 0.217, maximum error: 0.5). We thus validate the possibility of using such smart shoes to objectively and accurately evaluate the lower limbs' muscle strength of the stroke patients.

cs.HC↗

arXiv2023

Room-Temperature Bound States in the Continuum Polariton Condensation

Exciton-polaritons resulting from the strong exciton-photon interaction stimulate the development of novel coherent light sources with low threshold, long range spatial, and temporal coherence to circumvent the ever increasing energy demands of optical communications. Polaritons from bound states in the continuum (BICs) are promising for Bose-Einstein condensation owing to their infinite quality factors that enlarge photon lifetimes and benefit polariton accumulations. However, BIC polariton condensation remains limited to cryogenic temperatures ascribed to the small exciton binding energies of conventional material platforms. Herein, we demonstrated a room-temperature BIC polaritonic platform based on halide perovskite air-hole photonic crystals, profiting from the non-radiative BIC states and stable excitons of cesium lead bromide. BIC polariton condensation was achieved near the dispersion minimum that generates directional vortex beam emission with long-range coherence. Our work provides a significant basis for the applications of polariton condensates for integrated photonic and topological circuits.

cond-mat.mes-hall↗

arXiv2022

Lateral quantum confinement regulates charge carrier transfer and biexciton interaction in CdSe/CdSeS core/crown nanoplatelets

Charge carrier dynamics essentially determine the performance of various optoelectronic applications of colloidal semiconductor nanocrystals. Among them, two-dimensional nanoplatelets provide new adjustment freedom for their unique core/crown heterostructure. Herein, we demonstrate that by fine-tuning the core size and the lateral quantum confinement, the charge carrier transfer rate from the crown to the core can be varied by one order of magnitude in CdSe/CdSeS core/alloy-crown nanoplatelets. In addition, the transfer can be affected by a carrier blocking mechanism, i.e., the filled carriers hinder further possible transfer. Furthermore, we found that the biexciton interaction is oppositely affected by quantum confinement and electron delocalization, resulting in a non-monotonic variation of the biexciton binding energy with the emission wavelength. This work provides new observations and insights into the charge carrier transfer dynamics and exciton interactions in colloidal nanoplatelets and will promote their further applications in lasing, display, sensing, etc.

cond-mat.mes-hall↗

arXiv2022

Integration factor combined with level set method for reaction-diffusion systems with free boundary in high spatial dimensions

For reaction-diffusion equations in irregular domain with moving boundaries, the numerical stability constraints from the reaction and diffusion terms often require very restricted time step size, while complex geometries may lead to difficulties in accuracy when discretizing the high-order derivatives on grid points near the boundary. It is very challenging to design numerical methods that can efficiently and accurately handle both difficulties. Applying an implicit scheme may be able to remove the stability constraints on the time step, however, it usually requires solving a large global system of nonlinear equations for each time step, and the computational cost could be significant. Integration factor (IF) or exponential differencing time (ETD) methods are one of the popular methods for temporal partial differential equations (PDEs) among many other methods. In our paper, we couple ETD methods with an embedded boundary method to solve a system of reaction-diffusion equations with complex geometries. In particular, we rewrite all ETD schemes into a linear combination of specific ϕ-functions and apply one start-of-the-art algorithm to compute the matrix-vector multiplications, which offers significant computational advantages with adaptive Krylov subspaces. In addition, we extend this method by incorporating the level set method to solve the free boundary problem. The accuracy, stability, and efficiency of the developed method are demonstrated by numerical examples.

math.NA↗

arXiv2021

Annotation-efficient deep learning for automatic medical image segmentation

Automatic medical image segmentation plays a critical role in scientific research and medical care. Existing high-performance deep learning methods typically rely on large training datasets with high-quality manual annotations, which are difficult to obtain in many clinical applications. Here, we introduce Annotation-effIcient Deep lEarning (AIDE), an open-source framework to handle imperfect training datasets. Methodological analyses and empirical evaluations are conducted, and we demonstrate that AIDE surpasses conventional fully-supervised models by presenting better performance on open datasets possessing scarce or noisy annotations. We further test AIDE in a real-life case study for breast tumor segmentation. Three datasets containing 11,852 breast images from three medical centers are employed, and AIDE, utilizing 10% training annotations, consistently produces segmentation maps comparable to those generated by fully-supervised counterparts or provided by independent radiologists. The 10-fold enhanced efficiency in utilizing expert labels has the potential to promote a wide range of biomedical applications.

eess.IV↗

arXiv2021

A coarse-to-fine framework for unsupervised multi-contrast MR image deformable registration with dual consistency constraint

Multi-contrast magnetic resonance (MR) image registration is useful in the clinic to achieve fast and accurate imaging-based disease diagnosis and treatment planning. Nevertheless, the efficiency and performance of the existing registration algorithms can still be improved. In this paper, we propose a novel unsupervised learning-based framework to achieve accurate and efficient multi-contrast MR image registrations. Specifically, an end-to-end coarse-to-fine network architecture consisting of affine and deformable transformations is designed to improve the robustness and achieve end-to-end registration. Furthermore, a dual consistency constraint and a new prior knowledge-based loss function are developed to enhance the registration performances. The proposed method has been evaluated on a clinical dataset containing 555 cases, and encouraging performances have been achieved. Compared to the commonly utilized registration methods, including VoxelMorph, SyN, and LT-Net, the proposed method achieves better registration performance with a Dice score of 0.8397 in identifying stroke lesions. With regards to the registration speed, our method is about 10 times faster than the most competitive method of SyN (Affine) when testing on a CPU. Moreover, we prove that our method can still perform well on more challenging tasks with lacking scanning information data, showing high robustness for the clinical application.

eess.IV↗

arXiv2020

Multi-task MR Imaging with Iterative Teacher Forcing and Re-weighted Deep Learning

Noises, artifacts, and loss of information caused by the magnetic resonance (MR) reconstruction may compromise the final performance of the downstream applications. In this paper, we develop a re-weighted multi-task deep learning method to learn prior knowledge from the existing big dataset and then utilize them to assist simultaneous MR reconstruction and segmentation from the under-sampled k-space data. The multi-task deep learning framework is equipped with two network sub-modules, which are integrated and trained by our designed iterative teacher forcing scheme (ITFS) under the dynamic re-weighted loss constraint (DRLC). The ITFS is designed to avoid error accumulation by injecting the fully-sampled data into the training process. The DRLC is proposed to dynamically balance the contributions from the reconstruction and segmentation sub-modules so as to co-prompt the multi-task accuracy. The proposed method has been evaluated on two open datasets and one in vivo in-house dataset and compared to six state-of-the-art methods. Results show that the proposed method possesses encouraging capabilities for simultaneous and accurate MR reconstruction and segmentation.

cs.CV↗

arXiv2020

Zone-folded longnitude acoustic phonons driving self-trapped state emission in colloidal CdSe nanoplate superlattice

Colloidal cadmium chalcogenide nanoplates are two-dimensional semiconductors that have shown great application prospect for light-emitting technologies. Self-trapped state (STS), a special localized state originated from strong electron-phonon coupling (EPC), has great potential in one-step white light luminance owing to its broadband emission linewidth. However, achieving STS in cadmium chalcogenide nanocrystals is extremely challenging due to their intrinic weak EPC nature. By building hybrid superlattice (SL) structures via self-assembly of colloidal CdSe nanoplates (NPLs), we demonstrated an emergence of zone-folded longnitude acoustic phonons (ZFLAP) differ from monodispersed NPLs, and observed a broadband STS emission in spectra range of 450-600 nm. Through femtosecond transient absorption and impulsive vibrational spectroscopy, we revealed that STS is generated in time scale of ~500 fs and is driven by strong coupling of excitons and ZFLAPs with Huang-Rhys parameter as large as ~22.7. Our findings provide a new avenue for generating and manipulating STS emission by artificially designing and building hybrid periodic structures superior to single material optimization.

cond-mat.mtrl-sci↗

arXiv2019

CLCI-Net: Cross-Level fusion and Context Inference Networks for Lesion Segmentation of Chronic Stroke

Segmenting stroke lesions from T1-weighted MR images is of great value for large-scale stroke rehabilitation neuroimaging analyses. Nevertheless, there are great challenges with this task, such as large range of stroke lesion scales and the tissue intensity similarity. The famous encoder-decoder convolutional neural network, which although has made great achievements in medical image segmentation areas, may fail to address these challenges due to the insufficient uses of multi-scale features and context information. To address these challenges, this paper proposes a Cross-Level fusion and Context Inference Network (CLCI-Net) for the chronic stroke lesion segmentation from T1-weighted MR images. Specifically, a Cross-Level feature Fusion (CLF) strategy was developed to make full use of different scale features across different levels; Extending Atrous Spatial Pyramid Pooling (ASPP) with CLF, we have enriched multi-scale features to handle the different lesion sizes; In addition, convolutional long short-term memory (ConvLSTM) is employed to infer context information and thus capture fine structures to address the intensity similarity issue. The proposed approach was evaluated on an open-source dataset, the Anatomical Tracings of Lesions After Stroke (ATLAS) with the results showing that our network outperforms five state-of-the-art methods. We make our code and models available at https://github.com/YH0517/CLCI_Net.

eess.IV↗

arXiv2018

Room Temperature Continuous-wave Excited Biexciton Emission in CsPbBr3 Nanocrystals

Biexcitons are a manifestation of many-body excitonic interactions crucial for quantum information and quantum computation in the construction of coherent combinations of quantum states. However, due to their small binding energy and low transition efficiency, most biexcitons in conventional semiconductors exist either at cryogenic temperature or under femtosecond pulse laser excitation. Here we demonstrate room temperature, continuous wave driven biexciton states in CsPbBr3 perovskite nanocrystals through coupling with a plasmonic nanogap. The room temperature CsPbBr3 biexciton excitation fluence (~100 mW/cm2) is reduced by ~10^13 times in the Ag nanowire-film nanogaps. The giant enhancement of biexciton emission is driven by coherent biexciton-plasmon Fano interference. These results provide new pathways to develop high efficiency non-blinking single photon sources, entangled light sources and lasers based on biexciton states.

cond-mat.mes-hall↗