Photonic-chip-based generation of sub-100-femtosecond optical frequency combs
Sub-100-fs optical pulses and frequency comb sources have been revolutionizing a wide range of applications, from ultrafast optical science to optical frequency standard and measurement. To date, the leading techniques for generating such pulses in practical systems rely on tabletop mode-locked lasers, which inherently suffer from high system complexity, limited long-term reliability, and pronounced environmental sensitivity. Meanwhile, driven by advances in photonic integration, chip-scale approaches have sought to realize miniaturized pulse sources. However, simultaneously achieving sub-100-fs duration, ideal pulse shape, and a broadband flat-topped spectrum remains a significant challenge. Here, we address these challenges by combining two key photonic chip technologies: TFLN EO modulators for picosecond seed pulse generation, and highly nonlinear optical loop mirrors (NOLM) based on AlGaAsOI nanowaveguides for efficient temporal pulse cleaning and spectral broadening. In theoretical simulation and experiment, we show that for an input seed pulse centred at ~1550nm, a single-stage AlGaAs NOLM with a loop length of 1cm can produce flat-topped, nearly tenfold spectral broadening and over tenfold compression of pulse width, and more than 10dB suppression of pulse pedestals. Using initial EO comb pulses with ps-level durations at repetition rates of 10-20GHz, we demonstrate photonic-chip-enabled pulses with an unprecedented duration of 55fs and a flat-topped comb spectrum whose 10dB optical bandwidth exceeds 90nm. Our results highlight the remarkable potential of photonic chip technologies to realize high-repetition-rate, miniaturized sub-100-fs optical pulse generators with the prospect of superior stability and operability. The demonstrated photonic-chip-based sub-100-fs optical frequency comb sources may establish a new paradigm for both scientific research and practical applications.