arXiv subjects

Xinhua Peng

Publications and source records attributed to Xinhua Peng.

At least 19 recordsLinked to original sources

arXiv2026

Correlation-enhanced metrology from scrambling dynamics in a solid-state spin system

Quantum information scrambling, the dispersal of local information into many-body degrees of freedom, provides a powerful mechanism for generating large-scale correlations and entanglement essential for quantum-enhanced metrology. However, experimentally verifying such quantum-enhanced metrology remains a demanding task. Here, we correlate thousands of spins by engineering chaotic scrambling dynamics in a solid-state nuclear spin system. By leveraging the newly developed scramblon theory, we reveal exponential scaling in both the quantum Fisher information and the signal response to a phase shift. The signal response achieves a correlation-enabled enhancement of $33(2)$ dB over uncorrelated spins. After accounting for signal loss due to imperfect time reversal in the readout stage, we obtain a total metrological gain of 18(1) dB with a phase sensitivity of 40(3) ${\mathrm{μrad}}$. Our results bridge quantum chaos with practical quantum metrology, establishing reversible scrambling dynamics as a powerful resource for precision measurements.

quant-ph↗

arXiv2026

Quantum Simulation of Spin-Dependent Electron Transfer in a Synthetic Chiral Lattice with a Trapped Ion

Electron transfer through chiral structures can exhibit spin asymmetry, known as the chiral-induced spin selectivity effect, whose microscopic origin remains an open question. While path-interference within the chiral moiety has been proposed as a key mechanism, its experimental validation requires precise and versatile tunability of system parameters. Here we implement a programmable quantum simulation of spin-dependent electron transfer in a donor--chiral-bridge--acceptor model using a trapped ion. The bridge is encoded in internal states of the ion with tunable nearest- and next-nearest-neighbor couplings, while donor and acceptor states are coupled via a spectator bosonic motional mode. We observe spin-dependent interference within the bridge, and further reveal spin-dependence in donor-to-acceptor transfer dynamics, controlled by amplitude and phase of the coupling parameter. Our results identify interference among spin-dependent pathways as a microscopic origin of spin-dependent transfer, and open a route toward quantum simulations of complex chiral lattices with multi-level and bosonic degrees of freedom.

quant-ph↗

arXiv2026

High-Accuracy Temporal Prediction via Experimental Quantum Reservoir Computing in Correlated Spins

Physical reservoir computing provides a powerful machine learning paradigm that exploits nonlinear physical dynamics for efficient information processing. By incorporating quantum effects, quantum reservoir computing offers superior potential for machine learning applications, as quantum dynamics are exponentially costly to simulate classically. Here, we present a novel quantum reservoir computing approach based on correlated quantum spin systems, exploiting natural quantum many-body interactions to generate reservoir dynamics, thereby circumventing the practical challenges of deep quantum circuits. Our experimental implementation supports nontrivial quantum entanglement and exhibits sufficient dynamical complexity for high-performance machine learning. We achieve state-of-the-art performance in experiments on standard time-series benchmarks, reducing prediction error by 1 to 2 orders of magnitude compared to previous quantum reservoir experiments. In long-term weather forecasting, our 9-spin quantum reservoir delivers greater prediction accuracy than classical reservoirs with thousands of nodes. This represents the first experimental demonstration of quantum machine learning outperforming large-scale classical models on real-world tasks.

quant-ph↗

arXiv2026

Error-resilient Reversal of Quantum Chaotic Dynamics Enabled by Scramblons

The emergence of the arrow of time in quantum many-body systems stems from the inherent tendency of Hamiltonian evolution to scramble quantum information and increase entanglement. While, in principle, one might counteract this temporal directionality by engineering a perfectly inverted Hamiltonian to reverse entanglement growth, such a scenario is fundamentally unstable because even minor imperfections in the backward evolution can be exponentially amplified, a hallmark of quantum many-body chaos. Therefore, successfully reversing quantum many-body dynamics demands a deep understanding of the underlying structure of quantum information scrambling and chaotic dynamics. In this letter, by using solid-state nuclear magnetic resonance on a macroscopic ensemble of randomly interacting spins, we measure the out-of-time-ordered correlator (OTOC) and validate key predictions of scramblon theory, a universal theoretical framework for information scrambling. Crucially, this theory enables us to isolate and mitigate errors in the OTOC caused by imperfections in the backward evolution. As a result, this protocol uncovers the anticipated exponential behavior of quantum many-body chaos and extracts the quantum Lyapunov exponent in a many-body experimental system for the first time. Our results push the fundamental limits of dynamical reversibility of complex quantum systems, with implications for quantum simulation and metrology.

cond-mat.str-el↗

arXiv2025

Hyperpolarized Molecular Nuclear Spins Achieve Magnetic Amplification

The use of nuclear spins as physical sensing systems is disadvantaged by their low signal responsivity, particularly when compared to sensing techniques based on electron spins. This primarily results from the small nuclear gyromagnetic ratio and the difficulties in achieving high spin polarization. Here we develop a new approach to investigating the response of hyperpolarized molecular nuclear spins to magnetic fields and demonstrate orders-of-magnitude enhanced magnetic responsivity over state-of-the-art proton and Overhauser magnetometers. Using hyperpolarized molecules with proton spins, we report the realization of magnetic amplification in linear and nonlinear types. We further extend this amplification to hyperpolarized scalar-coupled multi-spin molecules and observe substantial magnetic amplification exceeding 10%. Moreover, we observe an anomalous amplification with dispersive frequency dependence that originates from magnetic interference effects. Our work highlights the potential of hyperpolarized molecular nuclear spins for use in a new class of quantum sensors, with promising applications in both applied and fundamental physics, including highly accurate absolute magnetometry and the exploration of axion-nucleon exotic interactions.

quant-ph↗

arXiv2025

Search for New Particles with Flying Quantum Sensors in Space

Recent advancements in space science and technologies offer exciting prospects for investigating novel research that is unattainable within terrestrial laboratories. Here we propose the implementation of space-based quantum sensing to explore ultralight new particles beyond the standard model. The central idea involves probing long-range interactions between spin ensembles of space quantum sensors and the particles residing within Earth, mediated by ultralight particles. We show that such interactions can be substantially enhanced in space platforms and thus increase the search sensitivity. In contrast to their terrestrial counterparts, space-based quantum searches exhibit remarkable velocity enhancements, approaching the first cosmic speed, and thus enables the exploration of unexplored parameter space concerning ultralight new particles. Furthermore, the substantial abundance of electrons and nucleons within Earth plays a crucial role in extending the scope of our mission. Our projected search sensitivity can surpass the sensitivities of both terrestrial experiments and proposals by up to approximately 7 orders of magnitude. We also briefly discuss other space mission, including ``space-ground integrated" network of quantum sensors for dark matter searches.

quant-ph↗

arXiv2025

Experimental realization and synchronization of a quantum van der Pol oscillator

Classical self-sustained oscillators, that generate periodic motion without periodic external forcing, are ubiquitous in science and technology. The realization of nonclassical self-oscillators is an important goal of quantum physics. We here present the experimental implementation of a quantum van der Pol oscillator, a paradigmatic autonomous quantum driven-dissipative system with nonlinear damping, using a single trapped atom. We demonstrate the existence of a quantum limit cycle in phase space in the absence of a drive and the occurrence of quantum synchronization when the nonlinear oscillator is externally driven. We additionally show that synchronization can be enhanced with the help of squeezing perpendicular to the direction of the drive and, counterintuitively, linear dissipation. We also observe the bifurcation to a bistable phase-space distribution for large squeezing. Our results pave the way for the exploration of self-sustained quantum oscillators and their application to quantum technology.

quant-ph↗

arXiv2025

Variational Quantum Metrology with Loschmidt Echo

By utilizing quantum mechanical effects, such as superposition and entanglement, quantum metrology promises higher precision than the classical strategies. It is, however, practically challenging to realize the quantum advantages. This is mainly due to the difficulties in engineering non-classical probe state and performing nontrivial measurement in practise, particularly with a large number of particles. Here we propose a scalable scheme with a symmetrical variational quantum circuit which, same as the Loschmidt echo, consists of a forward and a backward evolution. We show that in this scheme the quantum Fisher information, which quantifies the precision limit, can be efficiently obtained from a measurement signal of the Loschmidt echo. We experimentally implement the scheme on an ensemble of 10-spin quantum processor and successfully achieves a precision near the theoretical limit which outperforms the standard quantum limit with 12.4 dB. The scheme can be efficiently implemented on various noisy intermediate-scale quantum devices which provides a promising routine to demonstrate quantum advantages.

quant-ph↗

arXiv2024

Searches for exotic spin-dependent interactions with spin sensors

Numerous theories have postulated the existence of exotic spin-dependent interactions beyond the Standard Model of particle physics. Spin-based quantum sensors, which utilize the quantum properties of spins to enhance measurement precision, emerge as powerful tools for probing these exotic interactions. These sensors encompass a wide range of technologies, such as optically pumped magnetometers, atomic comagnetometers, spin masers, nuclear magnetic resonance, spin amplifiers, and nitrogen-vacancy centers. These technologies stand out for their ultrahigh sensitivity, compact tabletop design, and cost-effectiveness, offering complementary approaches to the large-scale particle colliders and astrophysical observations. This article reviews the underlying physical principles of various spin sensors and highlights the recent theoretical and experimental progress in the searches for exotic spin-dependent interactions with these quantum sensors. Investigations covered include the exotic interactions of spins with ultralight dark matter, exotic spin-dependent forces, electric dipole moment, spin-gravity interactions, and among others. Ongoing and forthcoming experiments using advanced spin-based sensors to investigate exotic spin-dependent interactions are discussed.

quant-ph↗

arXiv2024

Observation of continuous time crystals and quasi-crystals in spin gases

Continuous time crystal (CTC) and quasi-crystal (CTQC) are two novel phases of matter characterized by the spontaneous breaking of continuous time-translation symmetry. To date, realizations of CTCs with periodic oscillations have been reported in only a few physical platforms, and their complex properties still require further exploration. Additionally, CTQCs, which feature quasi-periodic oscillations at multiple incommensurate frequencies, remain elusive. Here we report the experimental observation of CTC and CTQC signatures in noble-gas nuclear spins that interact nonlinearly with each other through feedback mechanisms. The observed limit cycle and quasi-periodic phases display persistent spin oscillations with coherence times extending beyond several hours. Notably, these oscillations are robust against noise perturbations and exhibit random time phases upon repetitive realization, epitomizing the continuous time-translation symmetry-breaking intrinsic to CTCs and CTQCs. As the feedback strength increases, the system undergoes a phase transition into a new phase characterized by chaotic oscillations, indicative of the ``melting" of time crystals. Interestingly, within certain feedback regimes, we even observe an unusual reverse phase transition from a chaotic phase back to time crystal phases. This work broadens the catalog of new phases of spin gas and unlocks opportunities in precision measurements, including multimode masers and tests of fundamental symmetries.

quant-ph↗

arXiv2024

SCEP: a Cosmic Magnetic Monopole Search Experiment

Magnetic monopole is a well-motivated class of beyond-Standard-Model particles that could provide insights into the long-standing puzzle of the quantization of electric charge. These hypothetical particles are likely to be super heavy ($\sim$10$^{15}$ GeV) and be produced in the very early stages of the Universe's evolution. We propose a novel detection scenario for the search of such cosmic magnetic monopoles, utilizing a hybrid approach that combines radio-frequency atomic magnetometers and plastic scintillators. Such setup allows for the collection of both the induction and scintillation signals generated by the passage of a magnetic monopole, which provides acceptance to the magnetic monopoles with their velocities larger than about 10$^{-6}$ light speed (assuming a signal-to-noise ratio of $\sim$4) and their masses larger than approximately 10$^7$ GeV (at $β\sim10^{-3}$). The proposed detector design has the potential to scale up to large area, enabling the exploration of the parameter space of the cosmic magnetic monopole beyond the current experimental and astrophysical constraints. It is estimated that such detector can reach current most stringent limits of the flux set by previous searches, with a signal-to-noise ratio of the induction signal larger than about 4.5, assuming an effective exposure being 20000 year$\cdot$m$^2$ and coil layer of 3.

hep-ex↗

arXiv2024

Long-baseline quantum sensor network as dark matter haloscope

Ultralight dark photons constitute a well-motivated candidate for dark matter. A coherent electromagnetic wave is expected to be induced by dark photons when coupled with Standard-Model photons through kinetic mixing mechanism, and should be spatially correlated within the de Broglie wavelength of dark photons. Here we report the first search for correlated dark-photon signals using a long-baseline network of 15 atomic magnetometers, which are situated in two separated meter-scale shield rooms with a distance of about 1700 km. Both the network's multiple sensors and the shields large size significantly enhance the expected dark-photon electromagnetic signals, and long-baseline measurements confidently reduce many local noise sources. Using this network, we constrain the kinetic mixing coefficient of dark photon dark matter over the mass range 4.1 feV-2.1 peV, which represents the most stringent constraints derived from any terrestrial experiments operating over the aforementioned mass range. Our prospect indicates that future data releases may go beyond the astrophysical constraints from the cosmic microwave background and the plasma heating.

quant-ph↗

arXiv2024

Enhanced quantum hypothesis testing via the interplay between coherent evolution and noises

Previous studies in quantum information have recognized that specific types of noise can encode information in certain applications. However, the role of noise in Quantum Hypothesis Testing (QHT), traditionally assumed to undermine performance and reduce success probability, has not been thoroughly explored. Our study bridges this gap by establishing sufficient conditions for noisy dynamics that can surpass the success probabilities achievable under noiseless (unitary) dynamics within certain time intervals. We then devise and experimentally implement a noise-assisted QHT protocol in the setting of ultralow-field nuclear magnetic resonance spin systems. Our experimental results demonstrate that the success probability of QHT under the noisy dynamics can indeed surpass the ceiling set by unitary evolution alone. Moreover, we have shown that in cases where noise initially hampers the performance, strategic application of coherent controls on the system can transform these previously detrimental noises into advantageous factors. This transformative approach demonstrates the potential to harness and leverage noise in QHT, which pushes the boundaries of QHT and general quantum information processing.

quant-ph↗

arXiv2024

Emergent Universal Quench Dynamics in Randomly Interacting Spin Models

Universality often emerges in low-energy equilibrium physics of quantum many-body systems, despite their microscopic complexity and variety. Recently, there has been a growing interest in studying far-from-equilibrium dynamics of quantum many-body systems. Such dynamics usually involves highly excited states beyond the traditional low-energy theory description. Whether universal behaviors can also emerge in such non-equilibrium dynamics is a central issue at the frontier of quantum dynamics. Here we report the experimental observation of universal dynamics by monitoring the spin depolarization process in a solid-state NMR system described by an ensemble of randomly interacting spins. The spin depolarization can be related to temporal spin-spin correlation functions at high temperatures. We discover a remarkable phenomenon that these correlation functions obey a universal functional form. This experimental fact helps us identify the dominant interacting processes in the spin depolarization dynamics that lead to this universality. Our observation demonstrates the existence of universality even in non-equilibrium dynamics at high temperatures, thereby complementing the well-established universality in low-energy physics.

cond-mat.str-el↗

arXiv2024

Femtotesla Atomic Magnetometer for Zero- and Ultralow-field Nuclear Magnetic Resonance

Zero- and ultralow-field nuclear magnetic resonance (ZULF NMR) has experienced rapid development and provides an excellent tool for diverse research fields ranging from materials science, quantum information processing to fundamental physics. The detection of ZULF NMR signals in samples with natural abundance remains a challenging endeavor, due to the limited sensitivity of NMR detectors and thermal polarization. In this work, we demonstrate a femtotesla potassium spin-exchange relaxation-free (SERF) magnetometer designed for ZULF NMR detection. A potassium vapor cell with high buffer gas pressure and high atomic number density is used in the magnetometer. With absorption spectroscopy and SERF effect, the key parameters of the vapor cell are characterized and applied to optimize the magnetometer sensitivity. To combine our SERF magnetometer and ZULF NMR detection, a custom-made vacuum chamber is employed to keep NMR sample close to the magnetometer cell and protect the sample from undesired heating effects. Gradiometric measurement is performed to greatly reduce the magnetic noise. With the phase calibration applied, the gradiometric measurement achieves 7-fold enhancement in magnetic-field sensitivity compared to the single channel and has a magnetic noise floor of 1.2 fT/Hz$^{1/2}$. Our SERF magnetometer exhibits high sensitivity and is promising to realize ZULF NMR detection of samples with natural abundance.

quant-ph↗

arXiv2023

Multi-parameter quantum metrology with stabilized multi-mode squeezed state

Squeezing a quantum state along a specific direction has long been recognized as a crucial technique for enhancing the precision of quantum metrology by reducing parameter uncertainty. However, practical quantum metrology often involves the simultaneous estimation of multiple parameters, necessitating the use of high-quality squeezed states along multiple orthogonal axes to surpass the standard quantum limit for all relevant parameters. In addition, a temporally stabilized squeezed state can provide an event-ready probe for parameters, regardless of the initial state, and robust to the timing of the state preparation process once stabilized. In this work, we generate and stabilize a two-mode squeezed state along two secular motional modes in a vibrating trapped ion with reservoir engineering, despite starting from a thermal state of the motion. Leveraging this resource, we demonstrate an estimation of two simultaneous collective displacements along the squeezed axes, achieving improvements surpassing the classical limit by up to 6.9(3) and 7.0(3) decibels (dB), respectively. Our demonstration can be readily scaled to squeezed states with even more modes. The practical implications of our findings span a wide range of applications, including quantum sensing, quantum imaging, and various fields that demand precise measurements of multiple parameters.

quant-ph↗

arXiv2023

Cooperative Spin Amplification

Quantum amplification is recognized as a key resource for precision measurements. However, most conventional paradigms employ an ensemble of independent particles that usually limit the performance of quantum amplification in gain, spectral linewidth, etc. Here we demonstrate a new signal amplification using cooperative 129Xe nuclear spins embedded within a feedback circuit, where the noble-gas spin coherence time is enhanced by at least one order of magnitude. Using such a technique, magnetic field can be substantially pre-enhanced by more than three orders and is in situ readout with an embedded 87Rb magnetometer. We realize an ultrahigh magnetic sensitivity of 4.0 fT/Hz$^{1/2}$ that surpasses the photon-shot noise and even below the spin-projection noise of the embedded atomic magnetometer, allowing for exciting applications including searches for dark matter with sensitivity well beyond supernova constraints. Our findings extend the physics of quantum amplification to cooperative spin systems and can be generalized to a wide variety of existing sensors, enabling a new class of cooperative quantum sensors.

quant-ph↗

arXiv2023

Enhanced quantum sensing with amplification and deamplification

Quantum sensing is a fundamental building block of modern technology that employs quantum resources and creates new opportunities for precision measurements. However, previous methods usually have a common assumption that detection noise levels should be below the intrinsic sensitivity provided by quantum resources. Here we report the first demonstration of Fano resonance between coupled alkali-metal and noble gases through rapid spin-exchange collisions. The Fano resonance gives rise to two intriguing phenomena: spin amplification and deamplification, which serve as crucial resources for enhanced sensing. Further we develop a novel scheme of quantum sensing enhanced by amplification and deamplification, with relaxed requirements on the detection noise. The coupled systems of alkali-metal and noble gases act as amplifiers or de-amplifiers, enabling to extract small signals above the detection noise before final detection. We demonstrate magnetic-field measurement about 54 decibels below the photon-shot noise, which outperforms the state-of-the-art squeezed-light technology and realizes femtotesla-level sensitivity. Our work opens new avenues to applications in searches for ultralight dark matter with sensitivity well beyond the supernova-observation constraints.

quant-ph↗