arXiv subjects

Xinhui Lu

Publications and source records attributed to Xinhui Lu.

4 recordsLinked to original sources

arXiv2025

Spherical Phase Metalenses: Intrinsic Suppression of Spherical Aberration via Equiphase Surface Modulation

Recent progress in large-scale metasurfaces requires phase profiles beyond traditional hyperbolic designs. We show hyperbolic phase distributions cause spherical aberration from mismatched light propagation geometry and unrealistic phase assumptions. By analyzing metalens fundamentals via isophase surfaces, we develop a spherical phase profile based on spherical wavefront theory. This method prevents spherical aberration, essential for wide-aperture metalenses. Simulations prove superior focusing: spherical phase reduces FWHM by 7.3% and increases peak intensity by 20.4% versus hyperbolic designs at 31.46 micron radius. Spherical phase maintains consistent focusing across radii, while hyperbolic phase shows strong correlation (R squared = 0.95) with aberration. We also propose a normal vector tracing metric to measure design aberrations. This work establishes a scalable framework for diffraction-limited metalenses.

physics.optics↗

arXiv2023

Understanding the Role of Triplet-triplet Annihilation in Non-fullerene Acceptor Organic Solar Cells

Non-fullerene acceptors (NFAs) have enabled power conversion efficiencies exceeding 19% in organic solar cells (OSCs). However, the open-circuit voltage of OSCs remains low relative to their optical gap due to excessive non-radiative recombination, and this now limits performance. Here, we consider an important aspect of OSC design, namely management of the triplet exciton population formed after non-geminate charge recombination. By comparing the blends PM6:Y11 and PM6:Y6, we show that the greater crystallinity of the NFA domains in PM6:Y11 leads to a higher rate of triplet-triplet annihilation (TTA). We attribute this to the four times larger ground state dipole moment of Y11 versus Y6, which improves the long range NFA out-of-plane ordering. Since TTA converts a fraction of the non-emissive triplet states into bright singlet states, it has the potential to reduce non-radiative voltage losses. Through a kinetic analysis of the recombination processes under 1-Sun illumination, we provide a framework for determining the conditions under which TTA may improve OSC performance. If these could be satisfied, TTA has the potential to reduce non-radiative voltage losses by up to several tens of mV and could thus improve OSC performance.

physics.app-ph↗

arXiv2011

X-ray Near Field Speckle: Implementation and Critical Analysis

We have implemented the newly-introduced, coherence-based technique of x-ray near-field speckle (XNFS) at 8-ID-I at the Advanced Photon Source. In the near field regime of high-brilliance synchrotron x-rays scattered from a sample of interest, it turns out, that, when the scattered radiation and the main beam both impinge upon an x-ray area detector, the measured intensity shows low-contrast speckles, resulting from interference between the incident and scattered beams. We built a micrometer-resolution XNFS detector with a high numerical aperture microscope objective and demonstrate its capability for studying static structures and dynamics at longer length scales than traditional far field x-ray scattering techniques. Specifically, we characterized the structure and dynamics of dilute silica and polystyrene colloidal samples. Our study reveals certain limitations of the XNFS technique, which we discuss.

cond-mat.soft↗

arXiv2008

How a liquid becomes a glass both on cooling and on heating

The onset of structural arrest and glass formation in a concentrated suspension of silica nanoparticles in a water-lutidine binary mixture near its consolute point is studied by exploiting the near-critical fluid degrees of freedom to control the strength of an attraction between particles and multispeckle x-ray photon correlation spectroscopy to determine the particles' collective dynamics. This model system undergoes a glass transition both on cooling and on heating, and the intermediate liquid realizes unusual logarithmic relaxations. How vitrification occurs for the two different glass transitions is characterized in detail and comparisons are drawn to recent theoretical predictions for glass formation in systems with attractive interactions.

cond-mat.soft↗