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Xinlong Shi

Publications and source records attributed to Xinlong Shi.

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Anomalous magnetocaloric effects in the quasi-one-dimensional antiferromagnet BaCo$_2$V$_2$O$_8$

We investigate the transverse-field thermodynamics of the quasi-one-dimensional Ising-like antiferromagnet BaCo$_2$V$_2$O$_8$, whose tilted screw-chain geometry and anisotropic Land\'e $g$ tensor generate spatially modulated Zeeman couplings. Angle-resolved magnetocaloric-effect (MCE) measurements reveal a high-field temperature minimum near the transverse-field Ising critical field for $H\parallel[110]$ that persists and shifts only weakly upon field rotation. Tensor-network calculations show that the rotation-induced staggered transverse field rapidly lowers the Ising critical field and that the magnetic Gr\"uneisen ratio changes sign near the high-field temperature minimum, consistent with experiment. Our results establish that a dominant MCE response can persist away from the Ising critical region, suggesting a route to magnetic cooling by tailoring anisotropic Zeeman-coupling configurations in quantum magnets.

cond-mat.str-el

Realization of large magnetocaloric effect in the Kagome antiferromagnet Gd3BWO9 for Sub-Kelvin cryogenic refrigeration

Rare-earth (RE) based frustrated magnets have attracted great attention as excellent candidates for magnetic refrigeration at sub-Kelvin temperatures, while the experimental identification on systems exhibiting both large volumetric cooling capacity and reduced working temperatures far below 1 K remain to be a challenge. Here, through the ultra-low temperature magnetism and thermodynamic characterizations, we unveil the large magnetocaloric effect (MCE) realized at sub-Kelvin temperatures in the frustrated Kagome antiferromagnet Gd3BWO9 with TN~1.0 K. The isothermal magnetization curves indicate the existence of field (B) induced anisotropic magnetic phase diagrams, where four distinct magnetic phases for B // c-axis and five magnetic phases for B // ab-plane are identified at T< TN. The analysis of magnetic entropy S(B, T) data and direct adiabatic demagnetization tests reveal a remarkable cooling performance at sub-Kelvin temperatures featured by a large volumetric entropy density 502.2 mJ/K/cm3 and a low attainable minimal temperature Tmin~168 mK from the initial cooling condition of 2 K and 6 T, surpassing most of Gd-based refrigerants previously documented in temperature ranges of 0.25-4 K. The realized Tmin~168 mK far below TN ~ 1.0 K in Gd3BWO9 is related to the combined effects of magnetic frustration and criticality-enhanced MCE, which together leave a substantial magnetic entropy at reduced temperatures by enhancing spin fluctuations.

cond-mat.str-el