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Xintian Chen

Publications and source records attributed to Xintian Chen.

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T-linear specific heat in pressurized and magnetized Shastry-Sutherland Mott insulator SrCu2(BO3)2

The pressurized Shastry-Sutherland Mott insulator SrCu2(BO3)2 has been found to host a plaquette-singlet phase and an antiferromagnetic phase that break different symmetries spontaneously.The recent experiment showed that their transition is of a first order nature, which seems against the pursuit of exotic and deconfined degrees of freedom in this famous frustrated quantum magnet. We found a new direction in this study. By applying a magnetic field to the material, we discover that SrCu2(BO3)2 exhibits a universal and metallic T-linear specific heat behavior in a large magnetitic field range close to the pressure of zero-field first order transition between plaquette-singlet and antiferromagnetic phases. Such an unexpected gapless response from an electronically gapped Mott insulator could be attributed to magnetized Dirac spinons liberated by the combined effect of magnetic field and pressure, consistently seen from our quantum many-body thermal tensor network computation of the Shastry-Sutherland model under magnetic field. Such a robust and universal T-linear specific heat phase points out the richness of the phase diagram of the material expanded by the axes of pressure and magnetic field and is calling for new theoretical frameworks to its full explanation.

cond-mat.str-el

Electrothermal manipulation of current-induced phase transitions in ferrimagnetic Mn$_3$Si$_2$Te$_6$

Phase transitions driven by external stimuli are central to condensed matter physics, providing critical insights into symmetry breaking and emergent phenomena. Recently, ferrimagnetic (FiM) Mn$_3$Si$_2$Te$_6$ has attracted considerable attention for its magnetic-field-induced insulator-metal transitions (IMTs) and unconventional current-driven phase transitions, yet the role of applied currents in the magnetic phase remains poorly understood. Here, by combining local magnetization probes and time-resolved transport measurements, we uncover an electrothermal origin for the current-induced first-order-like phase transitions, characterized by abrupt voltage jumps and distinct magnetic domain evolution. Current-voltage (I-V) characteristics measured under triangular waveforms exhibit strong non-reciprocal and hysteretic behaviors, which are significantly suppressed at frequencies ~1000 Hz. Time-resolved studies using rectangular pulsed currents demonstrate that the resistance dynamics closely mirror the equilibrium resistance-temperature profile, directly implicating Joule heating as the driving mechanism. Furthermore, we reveal that the intrinsic I-V response adheres to Ohm's law, displaying linearity across various magnetic fields and temperatures. Our work advocates for a cautious approach in distinguishing between genuine current-induced nonequilibrium quantum states and thermal effects.

cond-mat.mtrl-sci

Investigations of key issues on the reproducibility of high-Tc superconductivity emerging from compressed La3Ni2O7

Recently, the signatures of superconductivity near 80 K have been discovered in the single crystal of La3Ni2O7 under pressure, which makes it a new candidate of the high-temperature superconductors dominated by 3d transition elements after the cuprate and iron-pnictide superconductors. However, there are several critical questions that have been perplexing the scientific community. These questions include (1) what factors contribute to the inconsistent reproducibility of the experimental results? (2) what is the fundamental nature of pressure-induced superconductivity: bulk or non-bulk (filamentary-like)? (3) where does the superconducting phase locate within the sample if it is filamentary-like? (4) is the oxygen content important for developing and stabilizing its superconductivity? In this study, we employ comprehensive high-pressure techniques to address these crucial issues. Through our modulated ac susceptibility measurements, we are the first to find that the superconductivity in this nickelate is filamentary-like. Our scanning transmission electron microscopy (STEM) investigations suggest that the filamentary-like superconductivity most likely emerges at the interface between the La3Ni2O7 and La4Ni3O10 phases. By tuning the oxygen content on the polycrystalline La3Ni2O7, we also find that the oxygen content plays vital role for developing and stabilizing its superconductivity. The upper and lower bounds of the oxygen content are 7.35 and 6.89, respectively. Our results provide not only new insights into understanding the puzzling issues in this material, but also significant information for achieving a better understanding on the superconductivity of this material.

cond-mat.supr-con

Deconfined quantum critical point lost in pressurized SrCu2(BO3)2

In the field of correlated electron materials, the relation between the resonating spin singlet and antiferromagnetic states has long been an attractive topic for understanding of the interesting macroscopic quantum phenomena, such as the ones emerging from magnetic frustrated materials, antiferromagnets and high-temperature superconductors. SrCu2(BO3)2 is a well-known quantum magnet, and it is theoretically expected to be the candidate of correlated electron material for clarifying the existence of a pressure-induced deconfined quantum critical point (DQCP), featured by a continuous quantum phase transition, between the plaquette-singlet (PS) valence bond solid phase and the antiferromagnetic (AF) phase. However, the real nature of the transition is yet to be identified experimentally due to the technical challenge. Here we show the experimental results for the first time, through the state-of-the-art high-pressure heat capacity measurement, that the PS-AF phase transition of the pressurized SrCu2(BO3)2 at zero field is clearly a first-order one. Our result clarifies the more than two-decade long debates about this key issue, and resonates nicely with the recent quantum entanglement understanding that the theoretically predicted DQCPs in representative lattice models are actually a first-order transition. Intriguingly, we also find that the transition temperatures of the PS and AF phase meet at the same pressure-temperature point, which signifies a bi-critical point as those observed in Fe-based superconductor and heavy-fermion compound, and constitutes the first experimental discovery of the pressure-induced bi-critical point in frustrated magnets. Our results provide fresh information for understanding the evolution among different spin states of correlated electron materials under pressure.

cond-mat.str-el