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Xintong Xu

Publications and source records attributed to Xintong Xu.

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Bringing Multimodal Large Language Models to Infrared-Visible Image Fusion Quality Assessment

Infrared-Visible image fusion (IVIF) aims to integrate thermal information and detailed spatial structures into a single fused image to enhance perception. However, existing evaluation approaches tend to over-optimize both hand-crafted no-reference statistics and full-reference metrics that treat the source images as pseudo ground truths. Recent IVIF reward-modelling efforts learn from human ratings but use scalar regression on aggregated scores, neither leveraging the reasoning of Multimodal Large Language Models (MLLMs) nor encoding per-image perceptual ambiguity in their supervision, but naively introducing MLLMs with discrete one-hot supervision likewise collapses fused images of similar quality into different rating levels. To address this, we introduce FuScore, which utilizes an MLLM to mimic human visual perception by producing continuous quality score, rather than discrete level predictions, enabling fine-grained discrimination among fused images of similar quality. We exploit the agreement among four IVIF-specific sub-dimensions to construct a per-image soft label whose sharpness reflects how consensual the overall judgment is. We further introduce a tripartite objective combining per-image distributional supervision, within-source-pair Thurstone fidelity for method-level ordering, and cross-source-pair Thurstone fidelity for scene-level ordering across scenes. Extensive experiments demonstrate that FuScore achieves state-of-the-art correlation with human visual preferences.

cs.CV

Hydrogen bonding in water under extreme confinement

Fluids under extreme confinement exhibit unique structures and intermolecular bonding, distinct from their bulk analogs, driving innovative applications at the water-energy nexus. Probing confined water experimentally at the length scale of intermolecular and surface forces has, however, remained a challenge. Here, we report direct molecular-level observations of hydrogen bonding in water confined inside individual carbon nanotubes, enabled by in-situ vibrational electron energy-loss spectroscopy with nanoscale resolution. Hydrogen bonding is probed via the intramolecular O-H stretching frequency, which serves as a sensitive spectral signature of the local intermolecular bonding environment. Water in larger carbon nanotubes exhibit the bonded O-H vibrations of bulk water, but at smaller diameters, the frequency blueshifts to near the free O-H stretch found in water vapor and hydrophobic surfaces, indicating a highly dispersed, non-H-bonded environment. Theoretical analysis based on quantum vibrational oscillators indicates that enhanced damping rates, corresponding to rapid hydrogen-bond fluctuations, leads the bimodal spectral peaks to merge into a single broad feature, matching the experimental observation. Furthermore, cryogenic experiments provide insights into complex structural phase transitions of confined water. This research reveals the quantum and dynamic nature of hydrogen bonds under confinement and the potential impact of unveiling molecular-level structure and bonding in confined fluids.

physics.chem-ph

Imaging the electron charge density in monolayer MoS2 at the Ångstrom scale

Four-dimensional scanning transmission electron microscopy (4D-STEM) has recently gained widespread attention for its ability to image atomic electric fields with sub-Ångstrom spatial resolution. These electric field maps represent the integrated effect of the nucleus, core electrons and valence electrons, and separating their contributions is non-trivial. In this paper, we utilized simultaneously acquired 4D-STEM center of mass (CoM) images and annular dark field (ADF) images to determine the electron charge density in monolayer MoS2. We find that both the core electrons and the valence electrons contribute to the derived electron charge density. However, due to blurring by the probe shape, the valence electron contribution forms a nearly featureless background while most of the spatial modulation comes from the core electrons. Our findings highlight the importance of probe shape in interpreting charge densities derived from 4D STEM.

cond-mat.mtrl-sci

Native point defects of semiconducting layered Bi2O2Se

Bi2O2Se is an emerging semiconducting, air-stable layered material (Nat. Nanotechnol. 2017, 12, 530; Nano Lett. 2017, 17, 3021), potentially exceeding MoS2 and phosphorene in electron mobility and rivalling typical Van der Waals stacked layered materials in the next-generation high-speed and low-power electronics. Holding the promise of functional versatility, it is arousing rapidly growing interest from various disciplines, including optoelectronics, thermoelectronics and piezoelectronics. In this work, we comprehensively study the electrical properties of the native point defects in Bi2O2Se, as an essential step toward understanding the fundamentals of this material. The defect landscapes dependent on both Fermi energy and the chemical potentials of atomic constituents are investigated. Along with the bulk defect analysis, a complementary inspection of the surface properties, within the simple context of charge neutrality level model, elucidates the observed n-type characteristics of Bi2O2Se based FETs. This work provides important guide to engineer the defects of Bi2O2Se for desired properties, which is key to the successful application of this emerging layered material.

cond-mat.mtrl-sci

Truly concomitant and independently expressed short- and long-term plasticity in Bi2O2Se-based three-terminal memristor

Orchestration of diverse synaptic plasticity mechanisms across different timescales produces complex cognitive processes. To achieve comparable cognitive complexity in memristive neuromorphic systems, devices that are capable to emulate short- and long-term plasticity (STP and LTP, respectively) concomitantly are essential. However, this fundamental bionic trait has not been reported in any existing memristors where STP and LTP can only be induced selectively because of the inability to be decoupled using different loci and mechanisms. In this work, we report the first demonstration of truly concomitant STP and LTP in a three-terminal memristor that uses independent physical phenomena to represent each form of plasticity. The emerging layered material Bi2O2Se is used in memristor for the first time, opening up the prospects for ultra-thin, high-speed and low-power neuromorphic devices. The concerted action of STP and LTP in our memristor allows full-range modulation of the transient synaptic efficacy, from depression to facilitation, by stimulus frequency or intensity, providing a versatile device platform for neuromorphic function implementation. A recurrent neural circuitry model is developed to simulate the intricate "sleep-wake cycle autoregulation" process, in which the concomitance of STP and LTP is posited as a key factor in enabling this neural homeostasis. This work sheds new light on the highly sophisticated computational capabilities of memristors and their prospects for realization of advanced neuromorphic functions.

physics.app-ph