arXiv subjects

Xiulai Xu

Publications and source records attributed to Xiulai Xu.

At least 19 recordsLinked to original sources

arXiv2026

Non-Hermitian Interaction between Light and Photonic Time Crystal Beyond the Floquet Quasinormal Mode Approximation

We report non-Hermitian mode couplings in a photonic time crystal induced by the light within its momentum bandgap. When the relative phase between the light and the photonic time crystal compensates for the detuning, we observe a periodic suppression of exponentially growing Floquet modes. In contrast, the optical response in this regime cannot be reproduced by the conventional Floquet expansion of the Green's function, revealing that the light induces effective mode couplings beyond the quasinormal mode approximation. We further investigate the parity-time phase transition through the exceptional point and quantitatively explain the suppression dynamics based on the phase, detuning, and modulation amplitude. The nontrivial interaction with light and the controllable non-Hermiticity indicate the great potential of photonic time crystals in temporally modulated nanophotonics.

physics.optics↗

arXiv2025

Room-temperature magnetoelectric coupling in strontium titanate

Magnetoelectric (ME) multiferroics enable efficient interconversion of electrical and magnetic signals, offering pathways toward substantial reduction of power consumption in next-generation computing and information technologies. However, despite decades of research, the persistence of ME coupling at room-temperature, an indispensable feature for practical applications, remains exceedingly rare in single-phase materials, due to symmetry constraints imposed by magnetic point groups and competing electronic requirements for ferroelectricity and magnetism. Here we report the coexistence of ferroelectricity and ferromagnetism at 780 K and a strong ME coupling with a converse ME coupling coefficient up to 498 ps/m at room-temperature in strontium titanate by dedicated vacancy engineering. The asymmetric distribution of oxygen vacancies surrounding titanium vacancies enables atomic displacement of titanium and charge injection, providing joint origin for ferroelectricity and ferromagnetism, as confirmed by atomic-scale structural analysis and first-principles calculations. The mechanism of ME coupling is offered as the hopping of oxygen vacancies under electric fields, which leads to the rearrangement of electronic configuration. Our work opens an avenue for designing multiferroics, overcoming the long-standing scarcity of room-temperature single-phase multiferroics.

cond-mat.mtrl-sci↗

arXiv2025

Full Polarization Control of Photons with Evanescent Wave Coupling in the Ultra Subwavelength Gap of Photonic Molecules

Polarization of photons plays a key role in quantum optics and light-matter interactions, however, it is difficult to control in nanosystems since the eigenstate of a nanophotonic cavity is usually fixed and linearly polarized. Here we reveal polarization control of photons using photonic molecules (PMs) that host supermodes of two coupled nanobeam cavities. In contrast to conventional PMs in a 2D photonic crystal slab, for the two 1D photonic crystal nanobeam cavities the shift and gap between them can be tuned continuously. With an ultra subwavelength gap, the coupling between the two cavities is dominated by the evanescent wave coupling in the surrounding environment, rather not the emission wave coupling for conventional PMs. As such, non-Hermiticity of the system becomes pronounced, and the supermodes consist of a non-trivial phase difference between bare eigenstates that supports elliptical polarization. We observe that both the polarization degree and polarization angle of the antisymmetric mode strongly depend on the shift and gap between the two cavities, exhibiting polarization states from linear to circular. This full polarization control indicates great potential of PMs in quantum optical devices and spin-resolved cavity quantum electrodynamics.

physics.optics↗

arXiv2025

Twisted heterobilayer photonic crystal based on stacking and selective etching of 2D materials

Nanophotonic devices with moir\'e superlattice is currently attracting broad interest due to the unique periodicity and high efficiency control of photons. Till now, experimental investigations mainly focus on the single layer device, i.e., two or more layers of photonic crystal patterns are merged and etched in a single layer of material. By comparison, twisted photonic crystal with multilayer materials raises challenges in the nanofabrication technology, because the growth of upper layer material usually requires a smooth bottom layer without nanostructures. Hereby, we fabricate twisted heterobilayer photonic crystal in the graphite/Si$_3$N$_4$ heterostructure. We use dry transfer method to stack the graphite on top of bottom Si$_3$N$_4$ with pre-etched photonic crystal patterns. Selective dry etching recipes are used to etch two photonic crystal layers individually, which improves the quality and accuracy in alignment. The cavity photonic mode at the visible wavelength $\sim 700$ nm arsing from the moir\'e site is clearly observed in experiment. These results reveal the experimental diagram of heterobilayer nanophotonic devices and open the way to design flexibility and control of photons in new degrees of freedom.

physics.optics↗

arXiv2024

Local high chirality near exceptional points based on asymmetric backscattering

We investigate local high chirality inside a microcavity near exceptional points (EPs) achieved via asymmetric backscattering by two internal weak scatterers. At EPs, coalescent eigenmodes exhibit position-dependent and symmetric high chirality characteristics for a large azimuthal angle between the two scatterers. However, asymmetric mode field features appear near EPs. Two azimuthal regions in the microcavity classified by the scatterers exhibit different wave types and chirality. Such local mode field features are attributed to the symmetries of backscattering in direction and spatial distribution. The connections between the wave types, the symmetry of mode field distribution and different symmetries of backscattering near EPs are also analyzed and discussed. Benefiting from the small size of weak scatterers, such microcavities with a high Q/V near EPs can be used to achieve circularly polarized quantum light sources and explore EP modified quantum optical effects in cavity quantum electrodynamics systems.

physics.optics↗

arXiv2024

Non-orthogonal cavity modes near exceptional points in the far field

Non-orthogonal eigenstates are a fundamental feature of non-Hermitian systems and are accompanied by the emergence of nontrivial features. However, the platforms to explore non-Hermitian mode couplings mainly measure near-field effects, and the far-field behaviour remain mostly unexplored. Here, we study how a microcavity with non-Hermitian mode coupling exhibits eigenstate non-orthogonality by investigating the spatial field and the far-field polarization of cavity modes. The non-Hermiticity arises from asymmetric backscattering, which is controlled by integrating two scatterers of different size and location into a microdisk. We observe that the spatial field overlaps of two modes increases abruptly to its maximum value, whilst different far-field elliptical polarizations of two modes coalesce when approaching an exceptional point. We demonstrate such features experimentally by measuring the far-field polarization from the fabricated microdisks. Our work reveals the non-orthogonality in the far-field degree of freedom, and the integrability of the microdisks paves a way to integrate more non-Hermitian optical properties into nanophotonic systems.

physics.optics↗

arXiv2023

Asymmetric Chiral Coupling in a Topological Resonator

Chiral light-matter interactions supported by topological edge modes at the interface of valley photonic crystals provide a robust method to implement the unidirectional spin transfer. The valley topological photonic crystals possess a pair of counterpropagating edge modes. The edge modes are robust against the sharp bend of $60^{\circ}$ and $120^{\circ}$, which can form a resonator with whispering gallery modes. Here, we demonstrate the asymmetric emission of chiral coupling from single quantum dots in a topological resonator by tuning the coupling between a quantum emitter and a resonator mode. Under a magnetic field in Faraday configuration, the exciton state from a single quantum dot splits into two exciton spin states with opposite circularly polarized emissions due to Zeeman effect. Two branches of the quantum dot emissions couple to a resonator mode in different degrees, resulting in an asymmetric chiral emission. Without the demanding of site-control of quantum emitters for chiral quantum optics, an extra degree of freedom to tune the chiral contrast with a topological resonator could be useful for the development of on-chip integrated photonic circuits.

cond-mat.mes-hall↗

arXiv2023

Transport of topologically protected photonic waveguide on chip

We propose a new design on integrated optical devices on-chip with an extra width degree of freedom by using a photonic crystal waveguide with Dirac points between two photonic crystals with opposite valley Chern numbers. With such an extra waveguide, we demonstrate numerically that the topologically protected photonic waveguide keeps properties of valley-locking and immunity to defects. Due to the design flexibility of the width-tunable topologically protected photonic waveguide, many unique on-chip integrated devices have been proposed, such as energy concentrators with a concentration efficiency improvement by more than one order of magnitude, topological photonic power splitter with arbitrary power splitting ratio. The topologically protected photonic waveguide with the width degree of freedom could be beneficial for scaling up photonic devices, which provides a new flexible platform to implement integrated photonic networks on chip.

physics.optics↗

arXiv2023

Controllable Spin-Resolved Photon Emission Enhanced by Slow-Light Mode in Photonic Crystal Waveguides on Chip

We report the slow-light enhanced spin-resolved in-plane emission from a single quantum dot (QD) in a photonic crystal waveguide (PCW). The slow light dispersions in PCWs are designed to match the emission wavelengths of single QDs. The resonance between two spin states emitted from a single QD and a slow light mode of a waveguide is investigated under a magnetic field with Faraday configuration. Two spin states of a single QD experience different degrees of enhancement as their emission wavelengths are shifted by combining diamagnetic and Zeeman effects with an optical excitation power control. A circular polarization degree up to 0.81 is achieved by changing the off-resonant excitation power. Strongly polarized photon emission enhanced by a slow light mode shows great potential to attain controllable spin-resolved photon sources for integrated optical quantum networks on chip.

cond-mat.mes-hall↗

arXiv2022

Micropascal-sensitivity ultrasound sensors based on optical microcavities

Whispering gallery mode (WGM) microcavities have been widely used for high-sensitivity ultrasound detection, due to their optical and mechanical resonances enhanced sensitivity. The ultrasound sensitivity of the cavity optomechanical system is fundamentally limited by the thermal noise. In this work, we theoretically and experimentally investigate the thermal-noise-limited sensitivity of a WGM microdisk ultrasound sensor, and optimize the sensitivity by varying the radius and thickness of the microdisk, as well as using a trench structure around the disk. Using a microdisk with a radius of 300 um and thickness of 2 um, a peak sensitivity of 1.18 uPa Hz^{-1/2} is achieved at 82.6 kHz, which is to our knowledge the record sensitivity among the cavity optomechanical ultrasound sensors. Such high sensitivity can improve the detection range of air-coupled ultrasound sensing technology.

physics.optics↗

arXiv2022

Single charge control of localized excitons in heterostructures with ferroelectric thin films and two-dimensional transition metal dichalcogenides

Single charge control of localized excitons (LXs) in two-dimensional transition metal dichalcogenides (TMDCs) is crucial for potential applications in quantum information processing and storage. However, traditional electrostatic doping method with applying metallic gates onto TMDCs may cause the inhomogeneous charge distribution, optical quench, and energy loss. Here, by locally controlling the ferroelectric polarization of the ferroelectric thin film BiFeO3 (BFO) with a scanning probe, we can deterministically manipulate the doping type of monolayer WSe2 to achieve the p-type and n-type doping. This nonvolatile approach can maintain the doping type and hold the localized excitonic charges for a long time without applied voltage. Our work demonstrated that ferroelectric polarization of BFO can control the charges of LXs effectively. Neutral and charged LXs have been observed in different ferroelectric polarization regions, confirmed by magnetic optical measurement. Highly circular polarization degree about 90 % of the photon emission from these quantum emitters have been achieved in high magnetic fields. Controlling single charge of LXs in a non-volatile way shows a great potential for deterministic photon emission with desired charge states for photonic long-term memory.

cond-mat.mes-hall↗

arXiv2022

High sensitivity air-coupled MHz frequency ultrasound detection using on-chip microcavities

Owing to their dual-resonance enhanced sensitivity, cavity optomechanical systems provide an ideal platform for ultrasound sensing. In this work, we realize high sensitivity air-coupled ultrasound sensing from kilohertz (kHz) to megahertz (MHz) frequency range based on whispering gallery mode microcavities. Using a 57 um-diameter microtoroid with high optical Q factor (~10^7) and mechanical Q factor (~700), we achieve sensitivities of 46 uPa Hz^{-1/2}-10 mPa Hz^{-1/2} in a frequency range of 0.25-3.2 MHz. Thermal-noise-limited sensitivity is realized around the mechanical resonance at 2.56 MHz, in a frequency range of 0.6 MHz. We also observe the second- and third-order mechanical sidebands, and quantitatively study the intensities of each mechanical sideband as a function of the mechanical displacement. Measuring the combination of signal to noise ratios at all sidebands has the potential to extend the dynamic range of ultrasound sensing. In addition, to improve the ultrasound sensitivity in the kHz frequency range, we use a microdisk with a diameter of 200 um, and achieve sensitivities of 1.83 uPa Hz^{-1/2}-10.4 mPa Hz^{-1/2} in 30 kHz-1.65 MHz range.

physics.optics↗

arXiv2022

Fully reconfigurable optomechanical add-drop filters

Fully reconfigurable add-drop filters (ADFs) have important applications in optical communication and information processing. Here we demonstrate a broadly tunable add-drop filter based on a double-disk cavity optomechanical system, side-coupled with a pair of tapered fiber waveguides. By varying the coupling rates between the cavity and the two waveguides, we investigate the dependence of the through (drop) efficiency on the coupling rates, which agrees well with the theoretical results. By optimizing the cavity-waveguide coupling rates, a drop efficiency of 89% and a transmission of 1.9% have been achieved. Benefiting from the large optomechanical coupling coefficient of the double-disk microcavity, a tuning range of 8 nm has been realized, which is more than one free spectral range (FSR) of the cavity. This is realized by changing the air gap of the double disk using a fiber tip, which is controlled by a piezoelectrical nanostage, with a required voltage of 7 V. As a result, both the through and drop signals can be resonant with any wavelength within the transparent window of the cavity material, which indicates that the ADF is fully reconfigurable.

physics.optics↗

arXiv2022

Strong light-matter interactions between gap plasmons and two-dimensional excitons at ambient condition in a deterministic way

Strong exciton-plasmon interaction between the layered two-dimensional (2D) semiconductors and gap plasmons shows a great potential to implement cavity quantum-electrodynamics in ambient condition. However, achieving a robust plasmon-exciton coupling with nanocavity is still very challenging, because the layer area is usually small with conventional approaches. Here, we report on a robust strong exciton-plasmon coupling between the gap mode of bowtie and the excitons in MoS$_2$ layers with gold-assisted mechanical exfoliation and the nondestructive wet transfer techniques for large-area layer. Benefiting from the ultrasmall mode volume and strong in-plane field, the estimated effective exciton number contributing to the coupling is largely reduced. With a corrected exciton transition dipole moment, the exciton numbers are extracted with 40 for the case of monolayer and 48 for 8 layers. Our work paves a way to realize the strong coupling with 2D materials with few excitons at room temperature.

cond-mat.mes-hall↗

arXiv2022

Strain-engineered high-temperature ferromagnetic Oxygen-substituted NaMnF3 from first principles

Using first-principles calculations, we investigated the magnetic, electronic, and structural properties of oxygen-substituted NaMnF3 (NaMnF1.5O1.5) with in-plane biaxial strain. For simplicity, a structure containing an oxygen octahedron is used to explore the underlying physical mechanism. We found that the oxygen octahedron induces a transition from an insulating antiferromagnet to a high-temperature half-metallic ferromagnet. More importantly, the Curie temperature can be significantly enhanced and even might reach room temperature by applying tensile strain. The changing trends of exchange coupling constants with the increasing biaxial tensile strain can be attributed to the cooperative effects of Jahn-Teller distortion and rotation distortion. It is expected that these findings can enrich the versatility of NaMnF3 and make it a promising candidate for spintronic applications.

cond-mat.mtrl-sci↗

arXiv2021

Ferromagnetic Enhancement in LaMnO3 Films with Release and Flexure

A variety of novel phenomena and functionalities emerge from lowering the dimensionality of materials and enriching the degrees of freedom in modulation. In this work, it is found that the saturation magnetization of LaMnO3 (LMO) films is largely enhanced by 56% after releasing from a brand-new phase of tetragonal strontium aluminate buffer layer, and is significantly increased by 92% with bending films to a curvature of 1 mm-1 using a water-assisted direct-transferring method. Meanwhile, the Curie temperature of LMO films has been improved by 13 K. High-resolution spherical aberration-corrected scanning transmission electron microscopy and first-principles calculations unambiguously demonstrate that the enhanced ferromagnetism is attributed to the strengthened Mn-O-Mn super-exchange interactions from the augmented characteristics of the unconventional P21/n structure caused by the out-of-plane lattice shrinking after strain releasing and increased flexure degree of freestanding LMO films. This work paves a way to achieve large-scale and crack-and-wrinkle-free freestanding films of oxides with largely improved functionalities.

cond-mat.mtrl-sci↗

arXiv2021

Enhanced valley polarization in WS$_2$/LaMnO$_3$ heterostructure

Monolayer transition metal dichalcogenides have attracted great attentions for potential applications in valleytronics. However, the valley polarization degree is usually not high because of the intervalley scattering. Here, we demonstrate a largely enhanced valley polarization up to 80\% in monolayer WS$_2$ under non-resonant excitation at 4.2 K using WS$_2$/LaMnO$_3$ thin film heterostructure, which is much higher than that for monolayer WS$_2$ on SiO$_2$/Si substrate with a valley polarization of 15\%. Furthermore, the greatly enhanced valley polarization can be maintained to a high temperature of about 160 K with a valley polarization of 53\%. The temperature dependence of valley polarization is strongly correlated with the thermomagnetic curve of LaMnO$_3$, indicating an exciton-magnon coupling between WS$_2$ and LaMnO$_3$. A simple model is introduced to illustrate the underlying mechanisms. The coupling of WS$_2$ and LaMnO$_3$ is further confirmed with an observation of two interlayer excitons with opposite valley polarizations in the heterostructure, resulting from the spin-orbit coupling induced splitting of the conduction bands in monolayer transition metal dichalcogenides. Our results provide a pathway to control the valleytronic properties of transition metal dichalcogenides by means of ferromagnetic van der Waals engineering, paving a way to practical valleytronic applications.

cond-mat.mtrl-sci↗

arXiv2021

Optimization and robustness of topological corner state in second-order topological photonic crystal

The second-order topological photonic crystal with 0D corner state provides a new way to investigate cavity quantum electrodynamics and develop topological nanophotonic devices with diverse functionalities. Here, we report on the optimization and robustness of topological corner state in the second-order topological photonic crystal both in theory and in experiment. The topological nanocavity is formed based on the 2D generalized Su-Schrieffer-Heeger model. The quality factor of corner state is optimized theoretically and experimentally by changing the gap between two photonic crystals or just modulating the position or size of the airholes surrounding the corner. The fabricated quality factors are further optimized by the surface passivation treatment which reduces surface absorption. A maximum quality factor of the fabricated devices is about 6000, which is the highest value ever reported for the active topological corner state. Furthermore, we demonstrate the robustness of corner state against strong disorders including the bulk defect, edge defect, and even corner defect. Our results lay a solid foundation for the further investigations and applications of the topological corner state, such as the investigation of strong coupling regime and the development of optical devices for topological nanophotonic circuitry.

physics.optics↗