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Xiuzhen Yu

Publications and source records attributed to Xiuzhen Yu.

At least 19 recordsLinked to original sources

Density-wave phases, anisotropic transport, and Planckian dissipation in single crystals of the superconductor La3Ni2O7

Pressure-induced superconductivity in bilayer nickelates provides a platform for investigating intertwined roles of charge/spin orders and electric transport in unconventional superconductivity. However, important quantitative information on the transport, such as the absolute value of the resistivity, the anisotropy, and the scattering rate of carriers, remains insufficient due to the lack of accurate measurements using large single crystals. Here we establish a high-precision pressure-temperature phase diagram of high-quality La3Ni2O7 single crystals, by measuring the in-plane and out-of-plane resistivities. We resolve two distinct anomalies associated with density-wave formation with contrasting pressure dependences. The pressure-induced structural transition enhances not only the resistivity values for both directions, but also its anisotropy at low temperatures, demonstrating a pronounced effect of density-wave order on the charge dynamics. Superconductivity with zero-resistance emerges near the boundary where the density-wave phases are fully suppressed, and above Tc, the resistivity exhibits a temperature-linear dependence over a wide temperature range while the scattering rate falls within a regime of the Planckian limit. Our results show that pressure dramatically changes the anisotropic charge transport via modifying density-wave orders, and eventually produces a pronounced strange-metal state with strong scatterings, from which superconductivity develops. This establishes robust density-wave correlations and Planckian dissipation as remarkable features of La3Ni2O7.

cond-mat.supr-con

Visualizing Microwave-Driven Dynamics of Antiskyrmions and Surface Skyrmions

Microwaves provide coherent access to low-energy excitations and serve as effective probes of high-frequency spin dynamics in quantum and magnetic systems. For topological spin textures, microwave excitation is expected to generate rich collective responses, yet direct real-space observation of ultrafast dynamics remains limited. Here we use time-resolved Lorentz transmission electron microscopy to visualize microwave-driven dynamics in a hybrid antiskyrmion structure composed of a central antiskyrmion and surface skyrmions. We resolve the picosecond evolution of antiskyrmion area and second-harmonic signals, evidencing nonlinear responses of spin textures under microwave excitations. We track the core motions of the antiskyrmion and surface skyrmions, which follow distinct trajectories while sharing the same rotational sense. Micromagnetic simulations reproduce the key observations and associate the dynamic modes with the spatial modulation of the core profile along the thickness. These achievements establish ultrafast electron microscopy as a powerful real-space approach for probing high-frequency microwave-driven dynamics of topological magnetic solitons.

cond-mat.mtrl-sci

Bond-density-wave orders induced by geometric frustration in the kagome metal CeRu3Si2

Geometric frustration gives rise to vast manifolds of degenerate ground states and competing orders in spin and charge systems. Typically, classical ground states are governed by a local ``zero-sum constraint" that relieves frustrated antiferromagnetic interactions or Coulomb repulsion. To date, the paradigm of geometric frustration has yielded a rich landscape of emergent phases, from spin ices and quantum spin liquids to charge glasses. However, an analogous phase rooted in chemical bonding has yet to be firmly demonstrated. Here we report the discovery of bond-density-wave orders induced by geometric frustration in the kagome metal CeRu$_3$Si$_2$ above room temperature. Through synchrotron X-ray diffraction, real-space transmission electron microscopy, and model calculations, we observe two distinct long-period superlattices with harmonic and anharmonic structural modulations. Crucially, interlayer bonds between kagome planes modulate in a sublattice-selective manner to fulfill the zero-sum constraint on the kagome lattice. We demonstrate the potential of kagome metals to host complex bond-ordered states constrained by geometric frustration and establish chemical bonding as a distinct pathway to frustration physics in quantum materials even above room temperature.

cond-mat.str-el

The 2026 Skyrmionics Roadmap

Magnetic skyrmions and related topological spin textures have emerged as a central topic in condensed-matter physics, combining fundamental significance with potential for transformative applications in spintronics, magnonics, and beyond. Over the past decade, advances in material platforms, imaging techniques, theoretical modeling, and device concepts have established skyrmionics as a rapidly expanding field. At the same time, challenges remain in stabilizing, controlling, and integrating such textures into functional architectures, while novel phenomena such as antiskyrmions, higher-order skyrmions, hopfions, and antiferromagnetic textures arise. The 2026 Skyrmionics Roadmap represents a collective effort of many authors, providing a comprehensive perspective on the current state-of-the-art and the outlook for the coming years. In 33 focused sections, each co-authored by two researchers, we chart progress in theory and modeling, material systems, skyrmion dynamics, and skyrmion technologies. By offering a consolidated vision, this Roadmap aims to guide both fundamental research and application-driven efforts, accelerating the transition of skyrmionics from conceptual breakthroughs toward practical technologies.

cond-mat.mes-hall

Ultralow-Temperature Cryogenic Transmission Electron Microscopy Using a New Helium Flow Cryostat Stage

Advances in cryogenic electron microscopy have opened new avenues for probing quantum phenomena in correlated materials. This study reports the installation and performance of a new side-entry condenZero cryogenic cooling system for JEOL (Scanning) Transmission Electron Microscopes (S/TEM), utilizing compressed liquid helium (LHe) and designed for imaging and spectroscopy at ultra-low temperatures. The system includes an external dewar mounted on a vibration-damping stage and a pressurized, low-noise helium transfer line with a remotely controllable needle valve, ensuring stable and efficient LHe flow with minimal thermal and mechanical noise. Performance evaluation demonstrates a stable base temperature of 6.58 K measured using a Cernox bare chip sensor on the holder with temperature fluctuations within 0.04 K. Complementary in-situ electron energy-loss spectroscopy (EELS) via aluminum bulk plasmon analysis was used to measure the local specimen temperature and validate cryogenic operation during experiments. The integration of cryogenic cooling with other microscopy techniques, including electron diffraction and Lorentz TEM, was demonstrated by resolving charge density wave (CDW) transitions in NbSe2 using electron diffraction, and imaging nanometric magnetic skyrmions in MnSi via Lorentz TEM. This platform provides reliable cryogenic operation below 7 K, establishing a low-drift route for direct visualization of electronic and magnetic phase transformations in quantum materials.

cond-mat.str-el

High-temperature helical edge states in BiSbTeSe$_2$/graphene van der Waals heterostructure

Van der Waals heterostructures have been used to tailor atomic layers into various artificial materials through interactions at heterointerfaces. The interplay between the band gap created by the band folding of the interfacial potential and the band inversion driven by enhanced spin-orbit interaction (SOI) through band hybridization enables us to realize a two-dimensional topological insulator (2D-TI). Here we report the realization of graphene 2D-TIs by epitaxial growth of three-dimensional topological insulator (3D-TI) BiSbTeSe$_2$ ultrathin films on graphene. By increasing the BiSbTeSe$_2$ thickness from 2 nm to 9 nm to enhance SOI on graphene, the electronic state is altered from the trivial Kekul${\'e}$ insulator to the 2D-TI. The nonlocal transport reveals the helical edge conduction which survives up to 200 K at maximum. Our graphene 2D-TI is stable, easy to make electrical contacts, and of high quality. It offers various applications including spin-current conversion and platforms for Majorana fermions in junctions to superconductors.

cond-mat.mes-hall

Nanosculpted 3D helices of a magnetic Weyl semimetal with switchable nonreciprocity

The emergent properties of materials are defined by the symmetries of their underlying atomic, spin and charge order. The explorations of symmetry breaking effects are therefore usually limited by the intrinsic properties of known, stable materials. In recent years, advances in focused ion beam (FIB) fabrication have enabled the nanostructuring of bulk crystals into ultraprecise transport devices [1-4], facilitating the investigation of geometrical effects on mesoscopic length scales. In this work, we expand such explorations into three-dimensional (3D), curvilinear shapes, by sculpting helical nanostructure devices from single crystals of the high-mobility, centrosymmetric magnetic Weyl semimetal Co$_3$Sn$_2$S$_2$ [5,6]. The combination of the imposed chiral geometry and intrinsic ferromagnetism yields nonreciprocal electron transport [7-9]. The high coercivity results in an anomalous, reversable diode effect remnant under zero applied magnetic field, which is orders of magnitude larger than can be explained by a classical self-field mechanism. We argue the enhancement originates from the high carrier mobility and the resulting quasi-ballistic transport: the conduction electron mean free path approaches the length scale of the curvature, resulting in increased asymmetrical scattering at the boundaries. We further demonstrate the inverse effect of the nonreciprocal transport: the field-free, current-induced switching of the magnetisation. The results establish the vast potential of 3D nanosculpting to explore and enrich the functionality of quantum materials.

cond-mat.mes-hall

Skyrmion Bubbles by Design in a Centrosymmetric Kagome Magnet

Topologically protected nanoscale spin textures, such as magnetic skyrmions, have attracted significant interest for spintronics applications. While skyrmions in noncentrosymmetric materials are known to be stabilized by Dzyaloshinskii$-$Moriya interaction (DMI), their deliberate design in centrosymmetric materials remains a challenge. This difficulty largely stems from the complexity of controlling magnetocrystalline anisotropy $-$ a critical factor in the absence of DMI. Here, we demonstrate the chemical tuning of magnetocrystalline anisotropy in the centrosymmetric Kagome magnet TmMn$_6$Sn$_6$. The resulting compound exhibits a spin reorientation transition accompanied by an emergent skyrmion bubble lattice, confirmed by Lorentz transmission electron microscopy. Our findings overcome a key materials design challenge and open possibilities for deliberate design of skyrmionic textures in centrosymmetric systems.

cond-mat.mtrl-sci

Bimerons create bimerons: proliferation and aggregation induced by currents and magnetic fields

The aggregation of topological spin textures at nano and micro scales has practical applications in spintronic technologies. Here, the authors report the in-plane current-induced proliferation and aggregation of bimerons in a bulk chiral magnet. It is found that the spin-transfer torques can induce the proliferation and aggregation of bimerons only in the presence of an appropriate out-of-plane magnetic field. It is also found that a relatively small damping and a relatively large non-adiabatic spin-transfer torque could lead to more pronounced bimeron proliferation and aggregation. Particularly, the current density should be larger than a certain threshold in order to trigger the proliferation; namely, the bimerons may only be driven into translational motion under weak current injection. Besides, the authors find that the aggregate bimerons could relax into a deformed honeycomb bimeron lattice with a few lattice structure defects after the current injection. The results are promising for the development of bio-inspired spintronic devices that use a large number of aggregate bimerons. The findings also provide a platform for studying aggregation-induced effects in spintronic systems, such as the aggregation-induced lattice phase transitions.

cond-mat.mes-hall

Discovery of a Bloch point quadrupole constituting hybrid topological strings

Topological magnetic (anti)skrymions are robust string-like objects heralded as potential components in next-generation topological spintronics devices due to their manipulability via low-energy stimuli such as magnetic fields, heat, and electric/thermal current. While these two-dimensional (2D) topological objects are widely studied, intrinsically three-dimensional (3D) electron-spin real-space topology remains less explored despite its prevalence in bulky magnets. Here, we capture the 3D structure of antiskyrmions in a single-crystal, precision-doped (Fe_{0.63}Ni_{0.3}Pd_{0.07})_{3}P lamellae using holographic vector field electron tomography at room temperature and zero field. Our measurements reveal hybrid string-like solitons composed of skyrmions with topological number W = -1 on the lamellae's surfaces and an antiskyrmion (W = +1) connecting them. High resolution images uncover a Bloch point (BP) quadrupole (four magnetic (anti)monopoles) positioned along the rectangular antiskyrmion's four corners (Bloch lines), which enable the observed lengthwise topological transitions. Furthermore, we calculate and compare the energy densities of hybrid strings with ideal (anti)skyrmion strings using micromagnetic simulations, which suggest that this composite (anti)BP structure stabilizes via the subtle interplay between the magnetostatic interaction and anisotropic Dzyaloshinskii-Moriya interaction. The discovery of these hybrid spin textures enables topological tunabilty, a tunable topological Hall effect, and the suppression of skyrmion Hall motion, disrupting existing paradigms within spintronics.

cond-mat.str-el

Signature of geometry modulation on interface magnetism emerged in isomeric IrO2-CoFe2O4 heterostructures

The interface composed of magnets and strong spin-orbit coupling (SOC) materials forms an important platform for spintronic devices and intriguing magnetic phenomena, such as the chiral spin textures and magnetic proximity effect (MPE). The interface exchange interaction and Dzyaloshinskii-Moriya interaction (DMI) have been discussed in a wide range of heterostructures, while the crystal stacking geometry modulation on these interface interactions has rarely been considered. Here, we show a pronounced geometry modulation on the interface magnetism through comparing a rutile and an anatase IrO2 capping on a ferrimagnetic CoFe2O4. The rutile heterostructure with a high-symmetry interface shows a conventional anomalous Hall effect (AHE) profile due to the MPE. In contrast, the anatase one with a low-symmetry interface exhibits a topological-like AHE even at zero-field, suggesting the emergence of non-coplanar magnetic order at the interface. Our results suggest that the influence of DMI at the interface can be more accentuated by forming a low-symmetry interface and raises a new means of designing interface magnetism via the geometry modulation.

cond-mat.mtrl-sci

Doping control of magnetic anisotropy for stable antiskyrmion formation in schreibersite (Fe,Ni)$_3$P with $S_4$ symmetry

Magnetic skyrmions, vortex-like topological spin textures, have attracted much interest in a wide range of research fields from fundamental physics to spintronics applications. Recently, growing attention has also been paid to antiskyrmions emerging in opposite topological charge in non-centrosymmetric magnets with $D_{2\mathrm{d}}$ or $S_4$ symmetry. In these magnets, complex interplay among anisotropic Dzyaloshinskii-Moriya interaction, uniaxial magnetic anisotropy, and magnetic dipolar interactions generates a variety of magnetic structures. However, the relation between the stability of antiskyrmions and these magnetic interactions remains to be elucidated. In this work, we control the uniaxial magnetic anisotropy of schreibersite (Fe,Ni)$_3$P with $S_4$ symmetry by doping and investigate its impact on the stability of antiskyrmions. Our magnetometry study, supported by ferromagnetic resonance spectroscopy, shows that the variation of the Ni content and slight doping with 4$d$ transition metals considerably change the magnetic anisotropy. In particular, doping with Pd induces easy-axis anisotropy, giving rise to formation of antiskyrmions, while a temperature-induced spin reorientation is observed in a Rh-doped compound. In combination with Lorentz transmission electron microscopy and micromagnetic simulations, we quantitatively analyze the stability of antiskyrmion as functions of uniaxial anisotropy and demagnetization energy, and demonstrate that subtle balance between them is necessary to stabilize the antiskyrmions.

cond-mat.mtrl-sci

Tunable N\'eel-Bloch magnetic twists in Fe3GeTe2 with van der Waals structure

The advent of ferromagnetism in two-dimensional (2D) van der Waals (vdW) magnets has stimulated high interest in exploring topological magnetic textures, such as skyrmions for use in future skyrmion-based spintronic devices. To engineer skyrmions in vdW magnets by transforming Bloch-type magnetic bubbles into N\'eel-type skyrmions, the heterostructure of heavy metal/vdW magnetic thin film has been made to induce interfacial Dzyaloshinskii-Moriya interaction (DMI). However, the unambiguous identification of the magnetic textures inherent to vdW magnets, e.g., whether the magnetic twists (skyrmions/domain walls) are N\'eel- or Bloch-type, is unclear. Here we demonstrate that the N\'eel- or Bloch-type magnetic twists can be tuned in the vdW magnet Fe3GeTe2 (FGT) with/without interfacial DMI. We use an in-plane magnetic field to align the modulation wavevector q of the magnetizations in order to distinguish the N\'eel- or Bloch-type magnetic twists. We observe that q is perpendicular to the in-plane field in the heterostructure (Pt/oxidized-FGT/FGT/oxidized-FGT), while q aligns at a rotated angle with respect to the field direction in the thin plate by thinning bulk FGT. We find that the aligned domain wall twists hold fan-like modulations, coinciding qualitatively with our computational results.

cond-mat.mtrl-sci

Room-temperature antiskyrmions and sawtooth surface textures in a noncentrosymmetric magnet with $S_4$ symmetry

Topological spin textures have attracted much attention both for fundamental physics and spintronics applications. Among them, antiskyrmions possess a unique spin configuration with Bloch-type and N\'eel-type domain walls due to anisotropic Dzyaloshinskii-Moriya interaction (DMI) in the noncentrosymmetric crystal structure. However, antiskyrmions have thus far only been observed in a few Heusler compounds with $D_{2\mathrm{d}}$ symmetry. Here, we report a new material Fe$_{1.9}$Ni$_{0.9}$Pd$_{0.2}$P in a different symmetry class ($S_4$ symmetry), where antiskyrmions exist over a wide temperature region including room temperature, and transform to skyrmions upon changing magnetic field and lamella thickness. The periodicity of magnetic textures greatly depends on crystal thickness, and domains with anisotropic sawtooth fractals are observed at the surface of thick crystals, which are attributed to the interplay between dipolar interaction and DMI as governed by crystal symmetry. Our findings provide a new arena to study antiskyrmions, and should stimulate further research on topological spin textures and their applications.

cond-mat.str-el

Giant anomalous Hall effect from spin-chirality scattering in a chiral magnet

The electrical Hall effect can be significantly enhanced through the interplay of the conduction electrons with magnetism, which is known as the anomalous Hall effect (AHE). Whereas the mechanism related to band topology has been intensively studied towards energy efficient electronics, those related to electron scattering have received limited attention. Here we report the observation of giant AHE of electron-scattering origin in a chiral magnet MnGe thin film. The Hall conductivity and Hall angle respectively reach 40,000 {\Omega}-1cm-1 and 18 % in the ferromagnetic region, exceeding the conventional limits of AHE of intrinsic and extrinsic origins, respectively. A possible origin of the large AHE is attributed to a new type of skew-scattering via thermally-excited spin-clusters with scalar spin chirality, which is corroborated by the temperature-magnetic-field profile of the AHE being sensitive to the film-thickness or magneto-crystalline anisotropy. Our results may open up a new platform to explore giant AHE responses in various systems, including frustrated magnets and thin-film heterostructures.

cond-mat.mtrl-sci

Combing the helical phase of chiral magnets with electric currents

The competition between the ferromagnetic exchange interaction and anti-symmetric Dzyaloshinskii-Moriya interaction can stabilize a helical phase or support the formation of skyrmions. In thin films of chiral magnets, the current density can be large enough to unpin the helical phase and reveal its nontrivial dynamics. We theoretically study the dynamics of the helical phase under spin-transfer torques that reveal distinct orientation processes, driven by topological defects in the bulk or induced by edges, limited by instabilities at higher currents. Our experiments confirm the possibility of on-demand switching the helical orientation by current pulses. This helical orientation might serve as a novel order parameter in future spintronics applications.

cond-mat.mes-hall

Quantum anomalous Hall effect driven by magnetic proximity coupling in all-telluride based heterostructure

The quantum anomalous Hall effect (QAHE) is an exotic quantum phenomenon originating from dissipation-less chiral channels at the sample edge. While the QAHE has been observed in magnetically doped topological insulators (TIs), exploiting magnetic proximity effect on the TI surface from adjacent ferromagnet layers may provide an alternative approach to the QAHE by opening an exchange gap with less disorder than that in the doped system. Nevertheless, the engineering of a favorable heterointerface that realizes the QAHE based on the magnetic proximity effect remains to be achieved. Here, we report on the observation of the QAHE in a proximity coupled system of non-magnetic TI and ferromagnetic insulator (FMI). We have designed sandwich heterostructures of (Zn,Cr)Te/(Bi,Sb)2Te3/(Zn,Cr)Te that fulfills two prerequisites for the emergence of the QAHE; the formation of a sizable exchange gap at the TI surface state and the tuning of the Fermi energy into the exchange gap. The efficient proximity coupling in the all-telluride based heterostructure as demonstrated here will enable a realistic design of versatile tailor-made topological materials coupled with ferromagnetism, ferroelectricity, superconductivity, and so on.

cond-mat.mes-hall

N\'eel-type skyrmions and their current-induced motion in van der Waals ferromagnet-based heterostructures

Since the discovery of ferromagnetic two-dimensional (2D) van der Waals (vdW) crystals, significant interest on such 2D magnets has emerged, inspired by their appealing properties and integration with other 2D family for unique heterostructures. In known 2D magnets, spin-orbit coupling (SOC) stabilizes perpendicular magnetic anisotropy (PMA). Such a strong SOC could also lift the chiral degeneracy, leading to the formation of topological magnetic textures such as skyrmions through the Dzyaloshinskii-Moriya interaction (DMI). Here, we report the experimental observation of N\'eel-type chiral magnetic skyrmions and their lattice (SkX) formation in a vdW ferromagnet Fe3GeTe2 (FGT). We demonstrate the ability to drive individual skyrmion by short current pulses along a vdW heterostructure, FGT/h-BN, as highly required for any skyrmion-based spintronic device. Using first principle calculations supported by experiments, we unveil the origin of DMI being the interfaces with oxides, which then allows us to engineer vdW heterostructures for desired chiral states. Our finding opens the door to topological spin textures in the 2D vdW magnet and their potential device application.

cond-mat.mtrl-sci