arXiv subjects

Xiyuan Lu

Publications and source records attributed to Xiyuan Lu.

At least 19 recordsLinked to original sources

arXiv2026

Photogalvanic second harmonic generation in Si3N4 for 1 Hz level on-chip metrology and spectroscopy

The coherent photogalvanic (PG) effect induces an effective $χ^{(2)}$ nonlinearity in natively $χ^{(3)}$ silicon nitride integrated photonics, unlocking pathways toward chip-scale precision spectroscopy and optical clockworks via second harmonic generation (SHG). While quasi-phase-matched PG-SHG using spatially varying internal electric fields offers tuning flexibility, it is often accompanied by pump-power- and detuning-dependent frequency offsets. Here, we investigate whether direct phase-matching---utilizing an intermodal scheme that generates a spatially uniform electric field---can support metrologically compatible SHG. By comparing the fundamental and doubled optical frequencies in a silicon nitride microresonator, we test the preservation of the (2:1) frequency ratio in directly phase-matched PG-SHG. We observe a frequency offset of $< 1\mathrm{~Hz}$, contrasting with previous limitations in quasi-phase-matched configurations. Furthermore, we measure a residual fractional frequency instability of $2\times 10^{-15}$ at $1\mathrm{~s}$, averaging down to the $10^{-16}$ level at $1000\mathrm{~s}$, with multi-hour deviations remaining below $1\mathrm{~Hz}$. These results establish directly phase-matched PG-SHG as a robust, metrologically compatible route to effective $χ^{(2)}$ functionality, combining sub-Hz frequency-ratio fidelity and high coherence on a mature integrated platform for optical clockworks, self-referencing, and precision spectroscopy.

physics.optics↗

arXiv2026

Thermally accessible broadband soliton microcombs in silicon carbide enabled by dynamic polarization control

Optical microcombs generated in high-Q microresonators are promising chip-scale light sources for applications ranging from optical communications to spectroscopy and metrology. However, thermo-optic instabilities remain a major obstacle to reliable soliton access. Self-cooling using auxiliary modes can stabilize the intracavity power, yet part of the power is continuously allocated to thermal compensation rather than comb generation, thereby limiting comb power and bandwidth. Here we propose a thermal compensation scheme based on dynamic polarization control. During soliton initiation, a fraction of the pump is coupled to an orthogonally polarized mode to provide self-cooling and ensure reliable soliton access. After soliton formation, polarization rotation and pump tuning transfer this cooling power to the comb-generating mode, enabling efficient single-soliton operation. Using this approach, we experimentally demonstrate a broadband 108-GHz-FSR single-soliton microcomb spanning over 450 nm, together with approximately 39% improvement in the 20-dB bandwidth and 60% increase in comb power relative to the static self-cooling configuration. This dynamic polarization-based thermal compensation enables efficient use of available laser power and provides a practical route to high-performance soliton microcombs in platforms with strong thermo-optic effects.

physics.optics↗

arXiv2025

Scalable low-latency entanglement distribution for distributed quantum computing

Practical distributed quantum computing and error correction require quantum networks with high-qubit-rate, high-fidelity, and low-reconfiguration-latency. Unfortunately, current approaches are limited by fundamental constraints: single-channel entanglement rates remain at the MHz level with millisecond-level reconfiguration, which is insufficient for fault-tolerant distributed quantum computing. Here, we propose a quantum network architecture that leverages reconfigurable quantum interfaces and wavelength-selective switches to overcome bandwidth and latency constraints. By tuning the frequency and temporal modes of photonic qubits across dense wavelength division multiplexing (DWDM) channels, our protocol achieves an entanglement generation rate of up to 183.4 MHz based on our comprehensive modeling of the networked cold atom computing systems. Our architecture enables nanosecond-scale network reconfiguration with low loss, low infidelity, and high dimensionality. Our modeling and simulation are designed for deployable distributed quantum computing and error correction, integrating the quantum interface, network switching, circuit compilation, and execution into a unified framework. The proposed architecture is fully compatible with industry-standard DWDM infrastructure, providing a scalable and cost-effective foundation for distributed quantum computing.

quant-ph↗

arXiv2025

Full spectral response of grating-induced loss in photonic crystal microrings

Photonic crystal microrings (PhCRs) have emerged as powerful and versatile platforms for integrated nonlinear photonics, offering precise control over frequency and phase matching while maintaining high optical quality factors. Through grating-mediated mode coupling, PhCRs enable advanced dispersion engineering, which is critical for wideband nonlinear processes such as optical parametric oscillation, Kerr frequency comb generation, and dual-pump spontaneous and Bragg scattering four-wave mixing. Beyond dispersion control, PhCRs also facilitate the manipulation of orbital angular momentum (OAM) emission, a key functionality for encoding high-dimensional quantum states in emerging quantum photonic platforms. Despite these advances, the broadband spectral behavior of grating-induced losses in PhCRs remains largely unexplored, with most studies focusing on grating periods near the modal wavelength or its half. Such losses can significantly impact broadband nonlinear processes, where excess loss at unintended wavelengths can degrade device performance. In this work, we experimentally characterize grating-induced losses in PhCRs and reveal their full spectral response as a function of the ratio between modal wavelength and grating period. We identify distinct loss channels arising from either radiation or mode conversion, including a broad excess-loss region attributed to vertical out-coupling into OAM-carrying states. These observations are supported by three-dimensional finite-difference time-domain simulations and further analyzed through OAM radiation angle and phase-mismatch analysis. The resulting broadband loss spectrum highlights critical design trade-offs and provides practical guidelines for optimizing PhCR-based devices for nonlinear photonic applications involving widely separated frequencies.

physics.optics↗

arXiv2025

Parasitic loss in microring-waveguide coupling and its impact on wideband nonlinear photonics

Microring resonators enable the enhancement of nonlinear frequency mixing processes, generating output fields at frequencies that widely differ from the inputs, in some cases by more than an octave. The efficiency of such devices depends on effective in- and out-coupling between access waveguides and the microrings at these widely separated frequencies. One successful approach is to separate the coupling task across multiple waveguides, with a cutoff waveguide (a waveguide that does not support guided modes above a certain wavelength) being judiciously used to prevent unwanted excessive overcoupling at low frequencies. Here, we examine how such a cutoff waveguide can still induce parasitic loss in the coupling region of a microring resonator, thereby impacting nonlinear device performance. We verified this parasitic loss channel through both experiment and simulation, showing that a waveguide optimized for 532 nm (visible) and 780 nm (near-infrared), while nominally cut off at 1550 nm, can still introduce significant parasitic loss at telecom wavelengths. This is studied in the context of visible-telecom optical parametric oscillation, where the excess parasitic loss can be strong enough to prevent threshold from being reached. Our finding elucidates a major challenge for wideband integrated nonlinear photonics processes when efficient coupling of widely-separated frequencies is needed.

physics.optics↗

arXiv2025

Laser injection locking and nanophotonic spectral translation of electro-optic frequency combs

High-resolution electro-optic frequency combs (EO combs) consisting of thousands to millions of comb teeth across a bandwidth between 1 GHz to 500 GHz are powerful tools for atomic, molecular, and cavity-based spectroscopy, including in the context of deployable quantum sensors. However, achieving sufficiently high signal-to-noise ratio (SNR) EO combs for use across the broad range of wavelengths required in the aforementioned applications is hindered by the corresponding unavailability of relevant components such as narrow-linewidth lasers, electro-optic phase modulators with adequate optical power handling, and low-noise optical amplifiers. Here, we address the latter two points by showing that optical injection locking of commercial Fabry-Perot (FP) laser diodes can help enable high SNR EO combs. We injection lock the FP laser diode to more than 10^6 comb teeth at injected comb powers as low as 1 nW and produce a high SNR replica of the EO comb. In comparison to a commercial semiconductor optical amplifier, injection locking achieves approximately 100x greater SNR for the same input power (when <1 microwatt) and equal SNR for > 35x lower input power. Such low-power injection locking is of particular relevance in conjunction with nanophotonic spectral translation, which extends the range of wavelengths available for EO combs. We show that the usable wavelength range of an EO comb produced by photo-induced second harmonic generation of an EO comb in a silicon nitride resonator is significantly increased when combined with optical injection locking. Our results demonstrate that optical injection locking provides a versatile and high-performance approach to addressing many different scenarios in which EO comb SNR would be otherwise limited.

physics.optics↗

arXiv2024

Strong interactions between integrated microresonators and alkali atomic vapors: towards single-atom, single-photon operation

Cavity quantum electrodynamics (cQED), the interaction of a two-level system with a high quality factor (Q) cavity, is a foundational building block in different architectures for quantum computation, communication, and metrology. The strong interaction between the atom and the cavity enables single photon operation which is required for quantum gates and sources. Cold atoms, quantum dots, and color centers in crystals are amongst the systems that have shown single photon operations, but they require significant physical infrastructure. Atomic vapors, on the other hand, require limited experimental infrastructure and are hence much easier to deploy outside a laboratory, but they produce an ensemble of moving atoms that results in short interaction times involving multiple atoms, which can hamper quantum operations. A solution to this issue can be found in nanophotonic cavities, where light-matter interaction is enhanced and the volume of operation is small, so that fast single-atom, single-photon operations are enabled. In this work, we study the interaction of an atomically-clad microring resonator (ACMRR) with different-sized ensembles of Rb atoms. We demonstrate strong coupling between an ensemble of ~50 atoms interacting with a high-quality factor (Q > 4 x 10^5) ACMRR, yielding a many-atom cooperativity C ~ 5.5. We continue to observe signatures of atom-photon interaction for a few (< 3) atoms, for which we observe saturation at the level of one intracavity photon. Further development of our platform, which includes integrated thermo-optic heaters to enable cavity tuning and stabilization, should enable the observation of interactions between single photons and single atoms.

quant-ph↗

arXiv2024

Advancing on-chip Kerr optical parametric oscillation towards coherent applications covering the green gap

Optical parametric oscillation (OPO) in Kerr microresonators can efficiently transfer near-infrared laser light into the visible spectrum. To date, however, chromatic dispersion has mostly limited output wavelengths to >560 nm, and robust access to the whole green light spectrum has not been demonstrated. In fact, wavelengths between 532 nm and 633 nm, commonly referred to as the "green gap", are especially challenging to produce with conventional laser gain. Hence, there is motivation to extend the Kerr OPO wavelength range and develop reliable device designs. Here, we experimentally show how to robustly access the entire green gap with Kerr OPO in silicon nitride microrings pumped near 780 nm. Our microring geometries are optimized for green-gap emission; in particular, we introduce a dispersion engineering technique, based on partially undercutting the microring, which not only expands wavelength access but also proves robust to variations in resonator dimensions, in particular, the microring width. Using just two devices, we generate >100 wavelengths evenly distributed throughout the green gap, as predicted by our dispersion simulations. Moreover, we establish the usefulness of Kerr OPO to coherent applications by demonstrating continuous frequency tuning (>50 GHz) and narrow optical linewidths (<1 MHz). Our work represents an important step in the quest to bring nonlinear nanophotonics and its advantages to the visible spectrum.

physics.optics↗

arXiv2023

Band flipping and bandgap closing in a photonic crystal ring and its applications

The size of the bandgap in a photonic crystal ring is typically intuitively considered to monotonically grow as the modulation amplitude of the grating increases, causing increasingly large frequency splittings between the 'dielectric' and 'air' bands. In contrast, here we report that as the modulation amplitude in a photonic crystal ring increases, the bandgap does not simply increase monotonically. Instead, after the initial increase, the bandgap closes and then reopens again with the dielectric band and the air bands flipped in energy. The air and dielectric band edges are degenerate at the bandgap closing point. We demonstrate this behavior experimentally in silicon nitride photonic crystal microrings, where we show that the bandgap is closed to within the linewidth of the optical cavity mode, whose quality factor remains unperturbed with a value $\approx$ 1$\times$10$^6$ (i.e., linewidth of 2 pm). Moreover, through finite-element simulations, we show that such bandgap closing and band flipping phenomena exist in a variety of photonic crystal rings with varying units cell geometries and cladding layers. At the bandgap closing point, the two standing wave modes with a degenerate frequency are particularly promising for single-frequency lasing applications. Along this line, we propose a compact self-injection locking scheme that integrates many core functionalities in one photonic crystal ring. Additionally, the single-frequency lasing might be applicable to DFB lasers to increase their manufacturing yield.

physics.optics↗

arXiv2023

Multi-mode microcavity frequency engineering through a shifted grating in a photonic crystal ring

Frequency engineering of whispering-gallery resonances is essential in microcavity nonlinear optics. The key is to control the frequencies of the cavity modes involved in the underlying nonlinear optical process to satisfy its energy conservation criterion. Compared to the conventional method that tailors dispersion by the cross-sectional geometry, thereby impacting all cavity mode frequencies, grating-assisted microring cavities, often termed as photonic crystal microrings, provide more enabling capabilities through mode-selective frequency control. For example, a simple single period grating added to a microring has been used for single-frequency engineering in Kerr optical parametric oscillation (OPO) and frequency combs. Recently, this approach has been extended to multi-frequency engineering by using multi-period grating functions, but at the cost of increasingly complex grating profiles that require challenging fabrication. Here, we demonstrate a simple approach, which we term as shifted grating multiple mode splitting (SGMMS), where spatial displacement of a single period grating imprinted on the inner boundary of the microring creates a rotational asymmetry that frequency splits multiple adjacent cavity modes. This approach is easy to implement and presents no additional fabrication challenges than an un-shifted grating, and yet is very powerful in providing multi-frequency engineering functionality for nonlinear optics. We showcase an example where SGMMS enables OPO generation across a wide range of pump wavelengths in a normal-dispersion device that otherwise would not support OPO.

physics.optics↗

arXiv2023

Fourier synthesis dispersion engineering of photonic crystal microrings for broadband frequency combs

Dispersion engineering of microring resonators is crucial for optical frequency comb applications, to achieve targeted bandwidths and powers of individual comb teeth. However, conventional microrings only present two geometric degrees of freedom -- width and thickness -- which limits the degree to which dispersion can be controlled. We present a technique where we tune individual resonance frequencies for arbitrary dispersion tailoring. Using a photonic crystal microring resonator that induces coupling to both directions of propagation within the ring, we investigate an intuitive design based on Fourier synthesis. Here, the desired photonic crystal spatial profile is obtained through a Fourier relationship with the targeted modal frequency shifts, where each modal shift is determined based on the corresponding effective index modulation of the ring. Experimentally, we demonstrate several distinct dispersion profiles over dozens of modes in transverse magnetic polarization. In contrast, we find that the transverse electric polarization requires a more advanced model that accounts for the discontinuity of the field at the modulated interface. Finally, we present simulations showing arbitrary frequency comb spectral envelope tailoring using our Frequency synthesis approach.

physics.optics↗

arXiv2022

Wavelength-Accurate Nonlinear Conversion through Wavenumber Selectivity in Photonic Crystal Resonators

Integrated nonlinear wavelength converters transfer optical energy from lasers or quantum emitters to other useful colors, but chromatic dispersion limits the range of achievable wavelength shifts. Moreover, because of geometric dispersion, fabrication tolerances reduce the accuracy with which devices produce specific target wavelengths. Here, we report nonlinear wavelength converters whose operation is not contingent on dispersion engineering; yet, the output wavelengths are controlled with high accuracy. In our scheme, coherent coupling between counter-propagating waves in a photonic crystal microresonator induces a photonic bandgap that isolates (in dispersion space) specific wavenumbers for nonlinear gain. We first demonstrate the wide applicability of this strategy to parametric nonlinear processes, by simulating its use in third harmonic generation, dispersive wave formation in Kerr microcombs, and four-wave mixing Bragg scattering. In experiments, we demonstrate Kerr optical parametric oscillators in which such wavenumber-selective coherent coupling designates the signal mode. As a result, differences between the targeted and realized signal wavelengths are <0.3 percent. Moreover, leveraging the bandgap-protected wavenumber selectivity, we continuously tune the output frequencies by nearly 300 GHz without compromising efficiency. Our results will bring about a paradigm shift in how microresonators are designed for nonlinear optics, and they make headway on the larger problem of building wavelength-accurate light sources using integrated photonics.

physics.optics↗

arXiv2022

Fractional optical angular momentum and multi-defect-mediated mode re-normalization and orientation control in photonic crystal microring resonators

Whispering gallery modes (WGMs) in circularly symmetric optical microresonators exhibit integer quantized angular momentum numbers due to the boundary condition imposed by the geometry. Here, we show that incorporating a photonic crystal pattern in an integrated microring can result in WGMs with fractional optical angular momentum. By choosing the photonic crystal periodicity to open a photonic bandgap with a band-edge momentum lying between that of two WGMs of the unperturbed ring, we observe hybridized WGMs with half-integer quantized angular momentum numbers ($m \in \mathbb{Z}$ + 1/2). Moreover, we show that these modes with fractional angular momenta exhibit high optical quality factors with good cavity-waveguide coupling and an order of magnitude reduced group velocity. Additionally, by introducing multiple artificial defects, multiple modes can be localized to small volumes within the ring, while the relative orientation of the de-localized band-edge states can be well-controlled. Our work unveils the renormalization of WGMs by the photonic crystal, demonstrating novel fractional angular momentum states and nontrivial multi-mode orientation control arising from continuous rotational symmetry breaking. The findings are expected to be useful for sensing/metrology, nonlinear optics, and cavity quantum electrodynamics.

physics.optics↗

arXiv2022

Rod and slit photonic crystal microrings for on-chip cavity quantum electrodynamics

Micro-/nanocavities that combine high quality factor ($Q$) and small mode volume ($V$) have been used to enhance light-matter interactions for cavity quantum electrodynamics (cQED). Whispering gallery mode (WGM) geometries such as microdisks and microrings support high-$Q$ and are design- and fabrication-friendly, but $V$ is often limited to tens of cubic wavelengths to avoid WGM radiation. The stronger modal confinement provided by either one-dimensional or two-dimensional photonic crystal defect geometries can yield sub-cubic-wavelength $V$, yet the requirements on precise design and dimensional control are typically much more stringent to ensure high-$Q$. Given their complementary features, there has been sustained interest in geometries that combine the advantages of WGM and photonic crystal cavities. Recently, a `microgear' photonic crystal ring (MPhCR) has shown promise in enabling additional defect localization ($>$ 10$\times$ reduction of $V$) of a WGM, while maintaining high-$Q$ ($\approx10^6$) and other WGM characteristics in ease of coupling and design. However, the unit cell geometry used is unlike traditional PhC cavities, and etched surfaces may be too close to embedded quantum nodes (quantum dots, atomic defect spins, etc.) for cQED applications. Here, we report two novel PhCR designs with `rod' and `slit' unit cells, whose geometries are more traditional and suitable for solid-state cQED. Both rod and slit PhCRs have high-$Q$ ($>10^6$) with WGM coupling properties preserved. A further $\approx$~10$\times$ reduction of $V$ by defect localization is observed in rod PhCRs. Moreover, both fundamental and 2nd-order PhC modes co-exist in slit PhCRs with high $Q$s and good coupling. Our work showcases that high-$Q/V$ PhCRs are in general straightforward to design and fabricate and are a promising platform to explore for cQED.

physics.optics↗

arXiv2022

High-performance microresonator optical parametric oscillator on a silicon chip

Optical parametric oscillation (OPO) is distinguished by its wavelength access, that is, the ability to flexibly generate coherent light at wavelengths that are dramatically different from the pump laser, and in principle bounded solely by energy conservation between the input pump field and the output signal/idler fields. As society adopts advanced tools in quantum information science, metrology, and sensing, microchip OPO may provide an important path for accessing relevant wavelengths. However, a practical source of coherent light should additionally have high conversion efficiency and high output power. Here, we demonstrate a silicon photonics OPO device with unprecedented performance. Our OPO device, based on the third-order ($χ^{(3)}$) nonlinearity in a silicon nitride microresonator, produces output signal and idler fields widely separated from each other in frequency ($>$150 THz), and exhibits a pump-to-idler conversion efficiency up to 29 $\%$ with a corresponding output idler power of $>$18 mW on-chip. This performance is achieved by suppressing competitive processes and by strongly overcoupling the output light. This methodology can be readily applied to existing silicon photonics platforms with heterogeneously-integrated pump lasers, enabling flexible coherent light generation across a broad range of wavelengths with high output power and efficiency.

physics.optics↗

arXiv2022

Highly-twisted states of light from a high quality factor photonic crystal ring

Twisted light with orbital angular momentum (OAM) has been extensively studied for applications in quantum and classical communications, microscopy, and optical micromanipulation. Ejecting the naturally high angular momentum whispering gallery modes (WGMs) of an optical microresonator through a grating-assisted mechanism, where the generated OAM number ($l$) is the difference of the angular momentum of the WGM and that of the grating, provides a scalable, chip-integrated solution for OAM generation. However, demonstrated OAM microresonators have exhibited a much lower quality factor ($Q$) than conventional WGM resonators (by $>100\times$), and an understanding of the ultimate limits on $Q$ has been lacking. This is crucial given the importance of $Q$ in enhancing light-matter interactions, such as single emitter coupling and parametric nonlinear processes, that underpin many important microresonator applications. Moreover, though high-OAM states are often desirable, the limits on what is achievable in a microresonator configuration are not well understood. Here, we provide new physical insight on these two longstanding questions, through understanding OAM from the perspective of mode coupling in a photonic crystal ring, and linking it to the commonly studied case of coherent backscattering between counter-propagating WGMs. In addition to demonstrating high-$Q$ ($10^5$ to $10^6$), high estimated OAM ejection efficiency (up to $90~\%$), and high-OAM number (up to $l$ = 60), our empirical model is supported by experiments and provides a quantitative explanation for the behavior of $Q$ and OAM ejection efficiency with $l$ for the first time. The state-of-the-art performance and new understanding of the physics of microresonator OAM generation will open new opportunities for realizing OAM applications using chip-integrated technologies.

physics.optics↗

arXiv2022

Efficient chip-based optical parametric oscillators from 590 nm to 1150 nm

Optical parametric oscillators are widely used to generate coherent light at frequencies not accessible by conventional laser gain. However, chip-based parametric oscillators operating in the visible spectrum have suffered from pump-to-signal conversion efficiencies typically less than 0.1 %. Here, we demonstrate efficient optical parametric oscillators based on silicon nitride photonics that address frequencies between 260 THz (1150 nm) and 510 THz (590 nm). Pumping silicon nitride microrings near 385 THz (780 nm) yields monochromatic signal and idler waves with unprecedented output powers in this wavelength range. We estimate on-chip output powers (separately for the signal and idler) between 1 mW and 5 mW and conversion efficiencies reaching approximately 15 %. Underlying this improved performance is our development of pulley waveguides for broadband near-critical coupling, which exploits a fundamental connection between the waveguide-resonator coupling rate and conversion efficiency. Finally, we find that mode competition reduces conversion efficiency at high pump powers, thereby constraining the maximum realizable output power. Our work proves that optical parametric oscillators built with integrated photonics can produce useful amounts of visible laser light with high efficiency.

physics.optics↗

arXiv2022

Kerr optical parametric oscillation in a photonic crystal microring for accessing the infrared

Continuous wave optical parametric oscillation (OPO) provides a flexible approach for accessing mid-infrared wavelengths between 2 $μ$m to 5 $μ$m, but has not yet been integrated into silicon nanophotonics. Typically, Kerr OPO uses a single transverse mode family for pump, signal, and idler modes, and relies on a delicate balance to achieve normal (but close-to-zero) dispersion near the pump and the requisite higher-order dispersion needed for phase- and frequency-matching. Within integrated photonics platforms, this approach results in two major problems. First, the dispersion is very sensitive to geometry, so that small fabrication errors can have a large impact. Second, the device is susceptible to competing nonlinear processes near the pump. In this letter, we propose a flexible solution to infrared OPO that addresses these two problems, by using a silicon nitride photonic crystal microring (PhCR). The frequency shifts created by the PhCR bandgap enable OPO that would otherwise be forbidden. We report an intrinsic optical quality factor up to (1.2 $\pm$ 0.1)$\times$10$^6$ in the 2 $μ$m band, and use a PhCR ring to demonstrate an OPO with threshold power of (90 $\pm$ 20) mW dropped into the cavity, with the pump wavelength at 1998~nm, and the signal and idler wavelengths at 1937 nm and 2063 nm, respectively. We further discuss how to extend OPO spectral coverage in the mid-infrared. These results establish the PhCR OPO as a promising route for integrated laser sources in the infrared.

physics.optics↗