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Xudong Tian

Publications and source records attributed to Xudong Tian.

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Tunable spin-phonon polarons in a chiral molecular qubit framework

Chiral structures that produce asymmetric spin-phonon coupling can theoretically generate spin-phonon polarons -- quasiparticles exhibiting non-degenerate spin states with phonon displacements. These quasiparticles are speculated to be the origin of chirality-induced spin selectivity and presumably can display exotic dynamic behaviors. However, direct experimental evidence of spin-phonon polarons has been lacking. Using a chiral molecular qubit framework embedding stable semiquinone-like radicals, we report spin dynamic signatures that indicate the formation of spin-phonon polarons for the first time. Our non-adiabatic model reveals that these quasiparticles introduce an active spin relaxation channel when polaron reorganization energy approaches Zeeman splitting. This new channel manifests itself as anomalous, temperature-independent spin relaxation, which can be suppressed by high magnetic fields or pore-filling solvents (e.g. CH2Cl2, CS2). Such field- and guest-tunable relaxation is unattainable in conventional spin systems. Harnessing this mechanism could boost repetition rates in spin-based quantum information technologies without compromising coherence or quantum sensing performance.

cond-mat.mes-hall

PHYBench: Holistic Evaluation of Physical Perception and Reasoning in Large Language Models

Current benchmarks for evaluating the reasoning capabilities of Large Language Models (LLMs) face significant limitations: task oversimplification, data contamination, and flawed evaluation items. These deficiencies necessitate more rigorous assessment methods. To address these limitations, we introduce PHYBench, a benchmark of 500 original physics problems ranging from high school to Physics Olympiad difficulty. PHYBench addresses data contamination through original content and employs a systematic curation pipeline to eliminate flawed items. Evaluations show that PHYBench activates more tokens and provides stronger differentiation between reasoning models compared to other baselines like AIME 2024, OlympiadBench and GPQA. Even the best-performing model, Gemini 2.5 Pro, achieves only 36.9% accuracy compared to human experts' 61.9%. To further enhance evaluation precision, we introduce the Expression Edit Distance (EED) Score for mathematical expression assessment, which improves sample efficiency by 204% over binary scoring. Moreover, PHYBench effectively elicits multi-step and multi-condition reasoning, providing a platform for examining models' reasoning robustness, preferences, and deficiencies. The benchmark results and dataset are publicly available at https://www.phybench.cn/.

cs.CL

Farewell to Mutual Information: Variational Distillation for Cross-Modal Person Re-Identification

The Information Bottleneck (IB) provides an information theoretic principle for representation learning, by retaining all information relevant for predicting label while minimizing the redundancy. Though IB principle has been applied to a wide range of applications, its optimization remains a challenging problem which heavily relies on the accurate estimation of mutual information. In this paper, we present a new strategy, Variational Self-Distillation (VSD), which provides a scalable, flexible and analytic solution to essentially fitting the mutual information but without explicitly estimating it. Under rigorously theoretical guarantee, VSD enables the IB to grasp the intrinsic correlation between representation and label for supervised training. Furthermore, by extending VSD to multi-view learning, we introduce two other strategies, Variational Cross-Distillation (VCD) and Variational Mutual-Learning (VML), which significantly improve the robustness of representation to view-changes by eliminating view-specific and task-irrelevant information. To verify our theoretically grounded strategies, we apply our approaches to cross-modal person Re-ID, and conduct extensive experiments, where the superior performance against state-of-the-art methods are demonstrated. Our intriguing findings highlight the need to rethink the way to estimate mutual

cs.CV

Variational Distillation for Multi-View Learning

Information Bottleneck (IB) based multi-view learning provides an information theoretic principle for seeking shared information contained in heterogeneous data descriptions. However, its great success is generally attributed to estimate the multivariate mutual information which is intractable when the network becomes complicated. Moreover, the representation learning tradeoff, {\it i.e.}, prediction-compression and sufficiency-consistency tradeoff, makes the IB hard to satisfy both requirements simultaneously. In this paper, we design several variational information bottlenecks to exploit two key characteristics ({\it i.e.}, sufficiency and consistency) for multi-view representation learning. Specifically, we propose a Multi-View Variational Distillation (MV$^2$D) strategy to provide a scalable, flexible and analytical solution to fitting MI by giving arbitrary input of viewpoints but without explicitly estimating it. Under rigorously theoretical guarantee, our approach enables IB to grasp the intrinsic correlation between observations and semantic labels, producing predictive and compact representations naturally. Also, our information-theoretic constraint can effectively neutralize the sensitivity to heterogeneous data by eliminating both task-irrelevant and view-specific information, preventing both tradeoffs in multiple view cases. To verify our theoretically grounded strategies, we apply our approaches to various benchmarks under three different applications. Extensive experiments to quantitatively and qualitatively demonstrate the effectiveness of our approach against state-of-the-art methods.

cs.CV