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Xuehua Wang

Publications and source records attributed to Xuehua Wang.

11 recordsLinked to original sources

Structured Cavity Quantum Electrodynamics

A cavity quantum electrodynamics (cQED) system consisting of a confined single photon and a single quantum emitter serves as a fundamental block for quantum optics and photonic quantum technologies. The canonical optical mode employed in the conventional cavity quantum electrodynamics features a uniform polarization distribution, leading to the scalar light-matter interaction in most existing experiments. Despite the rapid progress in the generation of structured light with spatially varied polarizations, the structured light-matter interaction, especially at the single quanta level, is highly intriguing yet largely unexplored. Here, we present the structured light-matter interaction at the single-photon level in a semiconductor cavity quantum electrodynamics system. Four distinct structured cavity modes that are spectrally close to each other are constructed in a micropillar cavity. By spatially locating a single epitaxial quantum dot (QD) at the periphery of a semiconductor micropillar cavity and spectrally tuning the QD emission wavelength into the resonances of the structured cavity modes, cavity-enhanced single-photon emissions with spin-locked chiral orbital angular momentum (OAM) and engineerable spin-orbit entanglements are achieved within a single wavelength-scale device. Our work opens an unexplored paradigm of structured quantum light-matter interactions and may further advance chiral quantum optics and high-dimensional photonic quantum technology.

physics.optics

High-performance Sources of Multidimensionally Engineered Quantum Light Based on Monolithic Microcavity-metalens Interfaces

The ultimate non-classic light sources for modern photonic quantum technology require on-demand generation of indistinguishable quantum light with high brightness and flexible engineering of quantum emission in multiple degrees of freedom. In this work, we present monolithic microcavity-metalens interfaces consisting of quantum-dot-micropillar single-photon sources and ultra-thin metalenses accurately aligned on opposite sides of an III-V compound semiconductor chip. The pronounced cavity quantum electrodynamics effect enabled by the micropillar cavity facilitates single-photon emission from quantum dots with simultaneous high degrees of single-photon purity, source brightness and photon indistinguishability while the multi-functional metalenses concurrently tailor quantum emission in multiple physical degrees of freedom including radiation divergence, emission directionality, polarization state and orbital angular momentum (OAM). Furthermore, high-fidelity polarization-OAM entanglement and single photons with local spin topologies are successfully generated in our integrated device. In particular, we demonstrate stable propagations of single-photon skrymions in atmospheric turbulence and reveal their topological advantages over the conventional structured quantum light. Our work advances the research fields of integrated quantum photonics and meta-optics, providing integrated high-dimensional quantum light sources for advanced photonic quantum science and technology.

physics.optics

Nonlinear Nanophotonic Chip-space Interfaces: On-chip Generation of Structured, Topological and Spatiotemporal Lights Via Nonlinear Čerenkov Radiation

Miniaturized and reconfigurable interfaces between confined optical modes within integrated photonic chips and structured light propagating in free space would serve as a cornerstone for fundamental optical science and modern photonic technology. In this work, we exploit the anisotropic nonlinear susceptibility tensors associated with thin-film lithium niobate to construct nanophotonic chip-space interfaces capable of flexibly generating and multi-dimensionally engineering structured light via injections of photons to on-chip waveguides. By harnessing the nonlinear Čerenkov radiation in integrated nonlinear microring resonators, we successfully tailor the spatial profile, polarization state, emission wavelength, topological charge and temporal wave packet of structured optical vortices, exhibiting reconfigurabilities and tuning ranges far beyond the state-of-the-art. To further showcase the capabilities of our platform, we use a single pump to generate tunable optical skyrmions via the spin-orbit coupling and multi-state integrated vortex microcombs in the visible range via synergistic $χ^{(2)}$ and $χ^{(3)}$ nonlinear optical processes. Our work bridges the research fields of structured light and integrated nonlinear optics, providing unprecedented opportunities for spatiotemporal light generation and on-chip multidimensional nonlinear optics.

physics.optics

Integrated Optical Vortex Microcomb

The explorations of physical degrees of freedom with infinite dimensionalities, such as orbital angular momentum and frequency of light, have profoundly reshaped the landscape of modern optics with representative photonic functional devices including optical vortex emitters and frequency combs. In nanophotonics, whispering gallery mode microresonators naturally support orbital angular momentum of light and have been demonstrated as on-chip emitters of monochromatic optical vortices. On the other hand, whispering gallery mode microresonators serve as a highly efficient nonlinear optical platform for producing light at different frequencies - i.e., microcombs. Here, we interlace the optical vortices and microcombs by demonstrating an optical vortex comb on an III-V integrated nonlinear microresonator. The angular-grating-dressed nonlinear microring simultaneously emits spatiotemporal light springs consisting of 50 orbital angular momentum modes that are each spectrally addressed to the frequency components (longitudinal whispering gallery modes) of the generated microcomb. We further experimentally generate optical pulses with time-varying orbital angular momenta by carefully introducing a specific intermodal phase relation to spatiotemporal light springs. This work may immediately boost the development of integrated nonlinear/quantum photonics for exploring fundamental optical physics and advancing photonic quantum technology.

physics.optics

Super-resolved snapshot hyperspectral imaging of solid-state quantum emitters for high-throughput integrated quantum technologies

Solid-state quantum emitters coupled to integrated photonic nanostructures are quintessential for exploring fundamental phenomena in cavity quantum electrodynamics and widely employed in photonic quantum technologies such as non-classical light sources, quantum repeaters, and quantum transducers, etc. One of the most exciting promises from integrated quantum photonics is the potential of scalability that enables massive productions of miniaturized devices on a single chip. In reality, the yield of efficient and reproducible light-matter couplings is greatly hindered by the spectral and spatial mismatches between the single solid-state quantum emitters and confined or propagating optical modes supported by the photonic nanostructures, preventing the high-throughput realization of large-scale integrated quantum photonic circuits for more advanced quantum information processing tasks. In this work, we introduce the concept of hyperspectral imaging in quantum optics, for the first time, to address such a long-standing issue. By exploiting the extended mode with a unique dispersion in a 1D planar cavity, the spectral and spatial information of each individual quantum dot in an ensemble can be accurately and reliably extracted from a single wide-field photoluminescence image with super-resolutions. With the extracted quantum dot positions and emission wavelengths, surface-emitting quantum light sources and in-plane photonic circuits can be deterministically fabricated with a high-throughput by etching the 1D confined planar cavity into 3D confined micropillars and 2D confined waveguides. Further extension of this technique by employing an open planar cavity could be exploited for pursuing a variety of compact quantum photonic devices with expanded functionalities for large-scale integration. Our work is expected to change the landscape of integrated quantum photonic technology.

physics.optics

Dynamic resonance fluorescence in solid-state cavity quantum electrodynamics

The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.

quant-ph

Tailoring solid-state single-photon sources with stimulated emissions

The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on three-level systems is limited mainly due to a lack of high photon indistinguishability. Here, we tailor the cavity-enhanced spontaneous emission from a ladder-type three-level system in a single epitaxial quantum dot (QD) through stimulated emission. After populating the biexciton (XX) of the QD through two-photon resonant excitation (TPE), we use another laser pulse to selectively depopulate the XX state into an exciton (X) state with a predefined polarization. The stimulated XX-X emission modifies the X decay dynamics and yields improved polarized single-photon source characteristics such as a source brightness of 0.030(2), a single-photon purity of 0.998(1), and an indistinguishability of 0.926(4). Our method can be readily applied to existing QD single-photon sources and expands the capabilities of three-level systems for advanced quantum photonic functionalities.

physics.optics

Dual-Resonance Enhanced Quantum Light-Matter Interactions In Deterministically Coupled Quantum-Dot-Micopillars

Optical microcavities have widely been employed to enhance either the optical excitation or the photon emission processes for boosting light matter interactions at nanoscale. When both the excitation and emission processes are simultaneously facilitated by the optical resonances provided by the microcavities, as referred to the dual-resonance condition in this article, the performances of many nanophotonic devices approach to the optima. In this work, we present versatile accessing of dual-resonance conditions in deterministically coupled quantum-dot(QD)-micopillars, which enables emission from exciton (X) - charged exciton (CX) transition with improved single-photon purity. In addition, the rarely observed up-converted single-photon emission process is achieved under dual-resonance condition. We further exploit the vectorial nature of the high-order cavity modes to significantly improve the excitation efficiency under the dual-resonance condition. The dual-resonance enhanced light-matter interactions in the quantum regime provides a viable path for developing integrated quantum photonic devices based on cavity quantum electrodynamics (QED) effect e.g., highly-efficient quantum light sources and quantum logical gates.

physics.optics

A solid-state entangled photon pair source with high brightness and indistinguishability

The generation of high-quality entangled photon pairs has been being a long-sought goal in modern quantum communication and computation. To date, the most widely-used entangled photon pairs are generated from spontaneous parametric downconversion, a process that is intrinsically probabilistic and thus relegated to a regime of low pair-generation rates. In contrast, semiconductor quantum dots can generate triggered entangled photon pairs via a cascaded radiative decay process, and do not suffer from any fundamental trade-off between source brightness and multi-pair generation. However, a source featuring simultaneously high photon-extraction efficiency, high-degree of entanglement fidelity and photon indistinguishability has not yet been reported. Here, we present an entangled photon pair source with high brightness and indistinguishability by deterministically embedding GaAs quantum dots in broadband photonic nanostructures that enable Purcell-enhanced emission. Our source produces entangled photon pairs with a record pair collection probability of up to 0.65(4) (single-photon extraction efficiency of 0.85(3)), entanglement fidelity of 0.88(2), and indistinguishabilities of 0.901(3) and 0.903(3), which immediately creates opportunities for advancing quantum photonic technologies.

quant-ph

1305 nm MoTe2-on-silicon Laser

The missing piece in the jigsaw of silicon photonics is a light source that can be easily incorporated into the standard silicon fabrication process. Recent advances in the development of atomically thin layers of semiconducting transition metal dichalogenides (TMDs), with direct bandgaps in the near-infrared region, have opened up new possibilities for addressing this need. Here, we report a unique silicon laser source that employs molybdenum ditelluride (MoTe2) as a gain material in a photonic crystal nanocavity resonator, fabricated in silicon-on-insulator. We demonstrate optically pumped MoTe2-on-silicon devices lasing at 1305 nm, i.e. in the centre of the O-band used in optical communications, operating in the continuous-wave (CW) regime, at room temperature and with a threshold power density as low as 1.5 kW/cm2. This 2D-on-silicon geometry offers the promise of an integrated low-cost electrically pumped nanoscale silicon light source, thereby adding an essential building block to the silicon photonics platform.

cond-mat.mes-hall

Efficient silicon metasurfaces for visible light

Dielectric metasurfaces require high refractive index contrast materials for optimum performance. This requirement imposes a severe restraint; devices have either been demonstrated at wavelengths of 700nm and above using high-index semiconductors such as silicon, or they use lower index dielectric materials such as TiO$_{2}$ or Si$_{3}$N$_{4}$ and operate in the visible wavelength regime. Here, we show that the high refractive index of silicon can be exploited at wavelengths as short as 532 nm by demonstrating a silicon metasurface with a transmission efficiency of 47% at this wavelength. The metasurface consists of a graded array of silicon posts arranged in a square lattice on a quartz substrate. We show full 2π phase control and we experimentally demonstrate polarization-independent beam deflection at 532nm wavelength. The crystalline silicon is placed on a quartz substrate by a bespoke layer transfer technique and we note that an efficiency >70% may be achieved for a further optimized structure in the same material. Our results open a new way for realizing efficient metasurfaces based on silicon in the visible wavelength regime.

physics.optics