arXiv subjects

Xueshi Li

Publications and source records attributed to Xueshi Li.

11 recordsLinked to original sources

arXiv2026

Structured Cavity Quantum Electrodynamics

A cavity quantum electrodynamics (cQED) system consisting of a confined single photon and a single quantum emitter serves as a fundamental block for quantum optics and photonic quantum technologies. The canonical optical mode employed in the conventional cavity quantum electrodynamics features a uniform polarization distribution, leading to the scalar light-matter interaction in most existing experiments. Despite the rapid progress in the generation of structured light with spatially varied polarizations, the structured light-matter interaction, especially at the single quanta level, is highly intriguing yet largely unexplored. Here, we present the structured light-matter interaction at the single-photon level in a semiconductor cavity quantum electrodynamics system. Four distinct structured cavity modes that are spectrally close to each other are constructed in a micropillar cavity. By spatially locating a single epitaxial quantum dot (QD) at the periphery of a semiconductor micropillar cavity and spectrally tuning the QD emission wavelength into the resonances of the structured cavity modes, cavity-enhanced single-photon emissions with spin-locked chiral orbital angular momentum (OAM) and engineerable spin-orbit entanglements are achieved within a single wavelength-scale device. Our work opens an unexplored paradigm of structured quantum light-matter interactions and may further advance chiral quantum optics and high-dimensional photonic quantum technology.

physics.optics↗

arXiv2026

High-performance Sources of Multidimensionally Engineered Quantum Light Based on Monolithic Microcavity-metalens Interfaces

The ultimate non-classic light sources for modern photonic quantum technology require on-demand generation of indistinguishable quantum light with high brightness and flexible engineering of quantum emission in multiple degrees of freedom. In this work, we present monolithic microcavity-metalens interfaces consisting of quantum-dot-micropillar single-photon sources and ultra-thin metalenses accurately aligned on opposite sides of an III-V compound semiconductor chip. The pronounced cavity quantum electrodynamics effect enabled by the micropillar cavity facilitates single-photon emission from quantum dots with simultaneous high degrees of single-photon purity, source brightness and photon indistinguishability while the multi-functional metalenses concurrently tailor quantum emission in multiple physical degrees of freedom including radiation divergence, emission directionality, polarization state and orbital angular momentum (OAM). Furthermore, high-fidelity polarization-OAM entanglement and single photons with local spin topologies are successfully generated in our integrated device. In particular, we demonstrate stable propagations of single-photon skrymions in atmospheric turbulence and reveal their topological advantages over the conventional structured quantum light. Our work advances the research fields of integrated quantum photonics and meta-optics, providing integrated high-dimensional quantum light sources for advanced photonic quantum science and technology.

physics.optics↗

arXiv2026

Hybrid Integration of Quantum Dot Single Photon Sources with Lithium Tantalate Photonics for On Chip Routing

A promising pathway towards scalable quantum photonic processors involves the simultaneous integration of deterministic single-photon sources, low-loss photonic circuitry, and fast reconfigurability. Thin-film lithium tantalate on insulator (LTOI) offers an exceptional electro-optic response and low optical loss at 900 nm wavelength band, yet its lack of efficient quantum emitters has hindered progress toward fully integrated quantum technologies. Here, we demonstrate heterogeneous integration of indium arsenide quantum dots (QDs) with low-loss reconfigurable LTOI waveguides using micro-transfer printing. By directly butt-coupling tapered gallium arsenide waveguides with inversely tapered LTOI waveguides, we achieve robust and alignment-tolerant inter-waveguide coupling. The hybrid chip operates at cryogenic temperatures, enabling deterministic routing of successively emitted single photons from the QDs with a halfwave voltage-length product, confirming the cryogenic stability of LTOI's electro-optic coefficient. These results establish the first demonstration of high-speed on-chip routing of single photons with hybrid QD-LTOI circuits, providing a scalable pathway toward integrated quantum photonic processors.

physics.optics↗

arXiv2026

Meta-cavity Quantum Electrodynamics

Cavity quantum electrodynamics (cQED) harnesses light-matter interactions to produce nonclassical light states. However, a fundamental challenge lies in simultaneously achieving Purcell enhancement and tailored wavefront control within a single cavity, due to conflicting resonator requirements. Here, we overcome this limitation by demonstrating triggered single-photon emission with customizable wavefronts from semiconductor quantum dots embedded in geometric-phase metacavities. These monolithic devices - only 200 nm thick - deliver Purcell-enhanced emission alongside spin-momentum-locked radiation, vortex beams, and holographic patterns. The meta-atom lattice provides high-Q optical confinement, while spatially modulated orientations enable efficient outcoupling of photons with designed states. This work establishes a new paradigm for intrinsically multiplexing metasurface-based wavefront shaping with cQED, enabling high-performance quantum light sources from subwavelength-scale monolithic platforms.

physics.optics↗

arXiv2025

On-chip Non-Hermitian Cavity Quantum Electrodynamics

Exceptional points (EPs) promise revolutionary control over quantum light-matter interactions. Here, we experimentally demonstrate flexible and reversible engineering of quantum vacuum fluctuation in an integrated microcavity supporting chiral Eps. We develop a hybrid lithium niobate (LN)-GaAs quantum photonic platform, seamlessly combining high-quality quantum emitters, a low-loss photonic circuit, efficient electro-optic (EO) effect, and local strain actuator in a single device. Chiral EPs are implemented by dynamically tuning the coupling between the modes associated with a micro-ring resonator, resulting in anomalous spontaneous emission dynamic with a 7-fold modulation of the lifetime (120 ps to 850 ps). Meanwhile, we reshape single-photon spectra via cavity local density of states (LDOS) engineering and generate non-Lorentzian spectral profiles: squared-Lorentzian, Fano-like, and EP-induced transparency (EPIT), a suppression of emission at zero detuning. This work unveils exotic cavity quantum electrodynamics (cQED) effects unique to EPs and establishes a universal paradigm for non-Hermitian quantum photonics.

physics.optics↗

arXiv2025

In-situ three-dimensional strain engineering of solid-state quantum emitters in photonic structures towards scalable quantum networks

Solid-state quantum emitters are pivotal for modern photonic quantum technology, yet their inherent spectral inhomogeneity imposes a critical challenge in pursuing scalable quantum network. Here, we develop a cryogenic-compatible strain-engineering platform based on a polydimethylsiloxane (PDMS) stamp that is not obviously working properly at cryogenic temperature. In-situ three-dimensional (3D) strain control is achieved for quantum dots (QDs) embedded in photonic nanostructures. The compliant PDMS enables independent tuning of emission energy and elimination of fine structure splitting (FSS) of single QDs, as demonstrated by a 7 meV spectral shift with a near-vanishing FSS in circular Bragg resonators and an unprecedented 15 meV tuning range in the micropillar. The PDMS-based 3D strain-engineering platform, compatible with diverse photonic structures at cryogenic temperature, provides a powerful and versatile tool for exploring fundamental strain-related physics and advancing integrated photonic quantum technology.

physics.optics↗

arXiv2023

Super-resolved snapshot hyperspectral imaging of solid-state quantum emitters for high-throughput integrated quantum technologies

Solid-state quantum emitters coupled to integrated photonic nanostructures are quintessential for exploring fundamental phenomena in cavity quantum electrodynamics and widely employed in photonic quantum technologies such as non-classical light sources, quantum repeaters, and quantum transducers, etc. One of the most exciting promises from integrated quantum photonics is the potential of scalability that enables massive productions of miniaturized devices on a single chip. In reality, the yield of efficient and reproducible light-matter couplings is greatly hindered by the spectral and spatial mismatches between the single solid-state quantum emitters and confined or propagating optical modes supported by the photonic nanostructures, preventing the high-throughput realization of large-scale integrated quantum photonic circuits for more advanced quantum information processing tasks. In this work, we introduce the concept of hyperspectral imaging in quantum optics, for the first time, to address such a long-standing issue. By exploiting the extended mode with a unique dispersion in a 1D planar cavity, the spectral and spatial information of each individual quantum dot in an ensemble can be accurately and reliably extracted from a single wide-field photoluminescence image with super-resolutions. With the extracted quantum dot positions and emission wavelengths, surface-emitting quantum light sources and in-plane photonic circuits can be deterministically fabricated with a high-throughput by etching the 1D confined planar cavity into 3D confined micropillars and 2D confined waveguides. Further extension of this technique by employing an open planar cavity could be exploited for pursuing a variety of compact quantum photonic devices with expanded functionalities for large-scale integration. Our work is expected to change the landscape of integrated quantum photonic technology.

physics.optics↗

arXiv2023

Dynamic resonance fluorescence in solid-state cavity quantum electrodynamics

The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.

quant-ph↗

arXiv2023

Bright Semiconductor Single-Photon Sources Pumped by Heterogeneously Integrated Micropillar lasers with Electrical Injections

The emerging hybrid integrated quantum photonics combines advantages of different functional components into a single chip to meet the stringent requirements for quantum information processing. Despite the tremendous progress in hybrid integrations of III-V quantum emitters with silicon-based photonic circuits and superconducting single-photon detectors, on-chip optical excitations of quantum emitters via miniaturized lasers towards single-photon sources (SPSs) with low power consumptions, small device footprints and excellent coherence properties is highly desirable yet illusive. In this work, we present realizations of bright semiconductor singe-photon sources heterogeneously integrated with on-chip electrically-injected microlasers. Different from previous one-by-one transfer printing technique implemented in hybrid quantum dot (QD) photonic devices, multiple deterministically coupled QD-circular Bragg Grating (CBG) SPSs were integrated with electrically-injected micropillar lasers at one time via a potentially scalable transfer printing process assisted by the wide-field photoluminescence (PL) imaging technique. Optically pumped by electrically-injected microlasers, pure single photons are generated with a high-brightness of a count rate of 3.8 M/s and an extraction efficiency of 25.44%. Such a high-brightness is due to the enhancement by the cavity mode of the CBG, which is confirmed by a Purcell factor of 2.5. Our work provides a powerful tool for advancing hybrid integrated quantum photonics in general and boosts the developments for realizing highly-compact, energy-efficient and coherent SPSs in particular.

quant-ph↗

arXiv2022

Tailoring solid-state single-photon sources with stimulated emissions

The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on three-level systems is limited mainly due to a lack of high photon indistinguishability. Here, we tailor the cavity-enhanced spontaneous emission from a ladder-type three-level system in a single epitaxial quantum dot (QD) through stimulated emission. After populating the biexciton (XX) of the QD through two-photon resonant excitation (TPE), we use another laser pulse to selectively depopulate the XX state into an exciton (X) state with a predefined polarization. The stimulated XX-X emission modifies the X decay dynamics and yields improved polarized single-photon source characteristics such as a source brightness of 0.030(2), a single-photon purity of 0.998(1), and an indistinguishability of 0.926(4). Our method can be readily applied to existing QD single-photon sources and expands the capabilities of three-level systems for advanced quantum photonic functionalities.

physics.optics↗

arXiv2021

Dual-Resonance Enhanced Quantum Light-Matter Interactions In Deterministically Coupled Quantum-Dot-Micopillars

Optical microcavities have widely been employed to enhance either the optical excitation or the photon emission processes for boosting light matter interactions at nanoscale. When both the excitation and emission processes are simultaneously facilitated by the optical resonances provided by the microcavities, as referred to the dual-resonance condition in this article, the performances of many nanophotonic devices approach to the optima. In this work, we present versatile accessing of dual-resonance conditions in deterministically coupled quantum-dot(QD)-micopillars, which enables emission from exciton (X) - charged exciton (CX) transition with improved single-photon purity. In addition, the rarely observed up-converted single-photon emission process is achieved under dual-resonance condition. We further exploit the vectorial nature of the high-order cavity modes to significantly improve the excitation efficiency under the dual-resonance condition. The dual-resonance enhanced light-matter interactions in the quantum regime provides a viable path for developing integrated quantum photonic devices based on cavity quantum electrodynamics (QED) effect e.g., highly-efficient quantum light sources and quantum logical gates.

physics.optics↗