arXiv subjects

Y. Chiashi

Publications and source records attributed to Y. Chiashi.

3 recordsLinked to original sources

arXiv2026

Photo- and thermally-induced huge layer decoupling in twisted bilayer WSe$_2$

Twisted bilayer systems host a wealth of emergent phenomena, such as flat-band superconductivity, ferromagnetism, and ferroelectricity, arising from moir\'e superlattices and unconventional interlayer coupling. Despite their central role, direct and quantitative access to the three-dimensional atomic arrangement in these systems has remained elusive due to their nanoscale dimensions. Here, we introduce an automated dark-field electron tomography technique that enables quantitative three-dimensional structural analysis of atomically thin materials with sub-\r{A} precision. By applying this method to twisted bilayer WSe$_2$, we precisely visualize the twist-angle-dependent structural relaxation appearing as the AB/BA stacking domains separated by 10-20 nm domain walls.In the marginally twisted region ($\theta \leq 0.1^\circ$), we uncover a significant expansion of the interlayer spacing compared to the bulk configuration, exceeding 0.1 \r{A}, along with a remarkable temperature-driven interlayer decoupling. Ultrafast measurements further reveal optically induced interlayer separation of ~0.2 \r{A} on the picosecond timescale, attributed to transient exciton formation. These findings not only establish a powerful approach for visualizing hidden out-of-plane structures in atomically thin micro-flake materials, but also uncover the intrinsic fragility and dynamical tunability of interlayer coupling in moir\'e-engineered 2-dimensional materials.

cond-mat.mes-hall↗

arXiv2024

Unusual photoinduced crystal structure dynamics in TaTe$_2$ with double zigzag chain superstructure

Transition metal dichalcogenides with superperiodic lattice distortions have been widely investigated as the platform of ultrafast structural phase manipulations. Here we performed ultrafast electron diffraction on room-temperature TaTe$_2$, which exhibits peculiar double zigzag chain pattern of Ta atoms. From the time-dependent electron diffraction pattern, we revealed a photoinduced change in the crystal structure occurring within <0.5 ps, though there is no corresponding high-temperature equilibrium phase. We further clarified the slower response (~1.5 ps) reflecting the lattice thermalization. Our result suggests the unusual ultrafast crystal structure dynamics specific to the non-equilibrium transient process in TaTe$_2$.

cond-mat.mtrl-sci↗

arXiv2020

Nanoscale imaging of unusual photo-acoustic waves in thin flake VTe$_2$

Controlling acoustic phonons, the carriers of sound and heat, has been attracting great attention toward the manipulation of sonic and thermal properties in nanometric devices. In particular, the photo-acoustic effect using ultrafast optical pulses has a promising potential to optically manipulate phonons in picoseconds time regime. However, its mechanism has been so far mostly based on the commonplace thermoelastic expansion in isotropic media, limiting the spectrum of potential applications. We investigate a conceptually new mechanism of photo-acoustic effect involving the structural instability, by utilizing a transition-metal dichalcogenide VTe$_2$ with the ribbon-type charge-density-wave (CDW). Ultrafast electron microscope imaging and diffraction measurements reveal the generation and propagation of unusual acoustic waves in the nanometric thin plate associated with the optically induced instantaneous charge-density-wave dissolution. Our results highlight the capability of photo-induced structural instability as a source of coherent acoustic waves.

cond-mat.mtrl-sci↗