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Y. De Wilde

Publications and source records attributed to Y. De Wilde.

8 recordsLinked to original sources
arXiv2024

Electroluminescence and Energy Transfer Mediated by Hyperbolic Polaritons

Under high electrical current, some materials can emit electromagnetic radiation beyond incandescence. This phenomenon, referred to as electroluminescence, leads to the efficient emission of visible photons and is the basis of domestic lighting devices (e.g., light-emitting diodes). In principle, electroluminescence can lead to mid-infrared (mid-IR) emission of confined light-matter excitations called phonon-polaritons, resulting from the coupling of photons with crystal lattice vibrations (optical phonons). In particular, phonon-polaritons arising in the van der Waals crystal hexagonal boron nitride (hBN) exhibit hyperbolic dispersion, which enhances light-matter coupling. For this reason, electroluminescence of hyperbolic phonon-polaritons (HPhPs) has been proposed as an explanation for the peculiar radiative energy transfer within hBN-encapsulated graphene transistors. However, since HPhPs are confined, they are inaccessible in the far-field, so that any hint of electroluminescence is only based on indirect electronic signatures and needs to be confirmed by direct observation. Here, we demonstrate far-field mid-IR (λ = 6.5 μm) electroluminescence of HPhPs excited by strongly biased high-mobility graphene within a van der Waals heterostructure, and we quantify the associated radiative energy transfer through the material. The presence of HPhPs is revealed via far-field mid-IR spectroscopy due to their elastic scattering at discontinuities in the heterostructure. The associated radiative flux is quantified by mid-IR pyrometry of the substrate receiving the energy. This radiative energy transfer is shown to be reduced in hBN with nanoscale inhomogeneities, demonstrating the central role of the electromagnetic environment in this process.

cond-mat.mes-hall↗
arXiv2023

Electroluminescence of the graphene 2D semi-metal

Electroluminescence, a non-thermal radiative process, is ubiquitous in semi-conductors and insulators but fundamentally precluded in metals. We show here that this restriction can be circumvented in high-quality graphene. By investigating the radiative emission of semi-metallic graphene field-effect transistors over a broad spectral range, spanning the near- and mid-infrared, we demonstrate direct far-field electroluminescence from hBN-encapsulated graphene in the mid-infrared under large bias in ambient conditions. Through a series of test experiments ruling out its incandescence origin, we determine that the electroluminescent signal results from the electrical pumping produced by interband tunneling. We show that the mid-infrared electroluminescence is spectrally shaped by a natural quarter-wave resonance of the heterostructure. This work invites a reassessment of the use of metals and semi-metals as non-equilibrium light emitters, and the exploration of their intriguing specificities in terms of carrier injection and relaxation, as well as emission tunability and switching speed.

cond-mat.mes-hall↗
arXiv2016

Long-Range Plasmon Assisted Energy Transfer Between Fluorescent Emitters

We demonstrate plasmon assisted energy transfer between fluorophores located at distances up to $7 \, μ$m on the top of a thin silver film. Thanks to the strong confinement and large propagation length of surface plasmon polaritons, the range of the energy transfer is almost two orders of magnitude larger than the values reported in the literature so far. The parameters driving the energy transfer range are thoroughly characterized and are in very good agreement with theoretically expected values.

physics.optics↗
arXiv2014

Mapping the radiative and the apparent non-radiative local density of states in the near field of a metallic nanoantenna

We present a novel method to extract the various contributions to the photonic local density of states from near-field fluorescence maps. The approach is based on the simultaneous mapping of the fluorescence intensity and decay rate, and on the rigorous application of the reciprocity theorem. It allows us to separate the contributions of the radiative and the apparent non-radiative local density of states to the change in the decay rate. The apparent non-radiative contribution accounts for losses due to radiation out of the detection solid angle and to absorption in the environment. Data analysis relies on a new analytical calculation, and does not require the use of numerical simulations. One of the most relevant applications of the method is the characterization of nanostructures aimed at maximizing the number of photons emitted in the detection solid angle, which is a crucial issue in modern nanophotonics.

physics.optics↗
arXiv2012

Distance dependence of the local density of states in the near field of a disordered plasmonic film

We measure the statistical distribution of the photonic local density of states in the near field of a semi-continuous gold film. By varying the distance between the measurement plane and the film, we show that near-field confined modes play a major role in the width of the distribution. Numerical simulations in good agreement with experiments allow us to point out the influence of non-radiative decay channels at short distance.

physics.optics↗
arXiv2000

Microwave Induced Instability Observed in BSCCO 2212 in a Static Magnetic Field

We have measured the microwave dissipation at 10 GHz through the imaginary part of the susceptibility, $χ^"$, in a BSCCO 2212 single crystal in an external static magnetic field $H$ parallel to the c-axis at various fixed temperatures. The characteristics of $χ^"(H)$ exhibit a sharp step at a field $H_{step}$ which strongly depends on the amplitude of the microwave excitation $h_{ac}$. The characteristics of $h_{ac}$ vs. $H_{step}$, qualitatively reveal the behavior expected for the magnetic field dependence of Josephson coupling.

cond-mat.supr-con↗
arXiv1998

Onset of decoupling at the melting field of the vortex lattice in Bi2Sr2CaCu2O8 from microwave dissipation

We have measured the microwave dissipation at 10 GHz in a Bi2Sr2CaCu2O8 single crystal, between 75 and 50 K, as a function of the static magnetic field applied parallel to the c axis. We observe a clear-cut onset in the dissipation precisely at the melting field Hm(T), that we identify in the same sample by a step in the static magnetization. We show that this onset can be assigned to the c-axis resistivity becoming finite in our whole temperature range, whereas the in-plane resistivity displays a thermally activated behavior. This suggests that pinning is efficient even at 10 GHz. The normal state dissipation is recovered at field much higher than the melting field, implying that decoupling develops mostly gradually over a large field range.

cond-mat.supr-con↗