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Y. J. Chen

Publications and source records attributed to Y. J. Chen.

At least 37 records · Page 2Linked to original sources

Bayesian Data Fusion of Imperfect Fission Yields for Augmented Evaluations

We demonstrate that Bayesian machine learning can be used to treat the vast amount of experimental fission data which are noisy, incomplete, discrepant, and correlated. As an example, the two-dimensional cumulative fission yields (CFY) of neutron-induced fission of $^{238}$U are evaluated with energy dependencies and uncertainty qualifications. For independent fission yields (IFY) with very few experimental data, the heterogeneous data fusion of CFY and IFY is employed to interpolate the energy dependence. This work shows that Bayesian data fusion can facilitate the further utilization of imperfect raw nuclear data.

nucl-th↗

Band-selective Holstein polaron in Luttinger liquid material A0.3MoO3 (A = K, Rb)

(Quasi-)one-dimensional systems exhibit various fascinating properties such as Luttinger liquid behavior, Peierls transition, novel topological phases, and the accommodation of unique quasiparticles (e.g., spinon, holon, and soliton, etc.). Here we study molybdenum blue bronze A0.3MoO3 (A = K, Rb), a canonical quasi-one-dimensional charge-density-wave material, using laser-based angle-resolved photoemission spectroscopy. Our experiment suggests that the normal phase of A0.3MoO3 is a prototypical Luttinger liquid, from which the charge-density-wave emerges with decreasing temperature. Prominently, we observe strong renormalizations of band dispersions, which is recognized as the spectral function of Holstein polaron derived from band-selective electron-phonon coupling in the system. We argue that the strong electron-phonon coupling plays a dominant role in electronic properties and the charge-density-wave transition in blue bronzes. Our results not only reconcile the long-standing heavy debates on the electronic properties of blue bronzes but also provide a rare platform to study novel composite quasiparticles in Luttinger liquid materials.

cond-mat.str-el↗

Potential energy surfaces and fission fragment mass yields of even-even superheavy nuclei

Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in the macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential. A standard flooding technique has been used to determine the barrier heights. It was shown the Fourier shape parametrization containing only three deformation parameters reproduces well the nuclear shapes of nuclei on their way to fission. In addition, the non-axial degree of freedom is taken into account to describe better the form of nuclei around the ground state and in the saddles region. Apart from the symmetric fission valley, a new very asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of considered nuclei are obtained by solving the 3D Langevin equations.

nucl-th↗

Coulomb Effects on time-trajectory-resolved high-order harmonic generation

We study the effect of Coulomb potential on high-order harmonic generation (HHG) numerically and analytically. We focus on the influence of Coulomb potential on emission times of HHG associated with specific electron trajectories. By using a numerical procedure based on numerical solution of time-dependent Schrödinger equation (TDSE) in three dimensions, we extract the HHG emission times both for long and short electron trajectories. We compare TDSE predictions with those of a Coulomb-modified model arising from strong-field approximation (SFA). We show that the Coulomb effect induces earlier HHG emission times than those predicted by the general SFA model without considering the Coulomb potential. In particular, this effect influences differently on long and short electron trajectories and is more remarkable for low-energy harmonics than high ones. It also changes the HHG amplitudes for long and short electron trajectories. We validate our discussions with diverse laser parameters and forms of Coulomb potential. Our results strongly support a four-step model of HHG.

physics.atom-ph↗

Local most-probable routes and classic-quantum correspondence in strong-field two-dimensional tunneling ionization

We study ionization of atoms in strong two-dimensional (2D) laser fields with various forms, numerically and analytically. We focus on the local most-probable tunneling routes (some specific electron trajectories) which are corresponding to the local maxima of photoelectron momentum distributions (PMDs). By making classic-quantum correspondence, we obtain a condition for these routes characterized by the electron position at the tunnel exit. With comparing the identified routes with the classical limit and the partial-decoupling approximation where it is assumed that tunneling is dominated by the main component of the 2D field, some semiclassical properties of 2D tunneling are addressed. The local maxima of PMD related to the local most-probable routes can be used as one of the preferred observables in ultrafast measurements.

physics.atom-ph↗

Measurement of Electronic Structure and Surface Reconstruction in the Superionic Cu2-xTe

Recently, layered copper chalcogenides Cu2X family (X=S, Se, Te) has attracted tremendous research interests due to their high thermoelectric (TE) performance, which is partly due to the superionic behavior of mobile Cu ions, making these compounds phonon liquids. Here, we systematically investigate the electronic structure and its temperature evolution of the less studied single crystal Cu2-xTe by the combination of angle resolved photoemission spectroscopy (ARPES) and scanning tunneling microscope/spectroscopy (STM/STS) experiments. While the band structure of the Cu2-xTe shows agreement with the calculations, we clearly observe a 2 * 2 surface reconstruction from both our low temperature ARPES and STM/STS experiments which survives up to room temperature. Interestingly, our low temperature STM experiments further reveal multiple types of reconstruction patterns, which suggests the origin of the surface reconstruction being the distributed deficiency of liquid-like Cu ions. Our findings reveal the electronic structure and impurity level of Cu2Te, which provides knowledge about its thermoelectric properties from the electronic degree of freedom.

cond-mat.mtrl-sci↗

Evidence of topological edge states in a superconducting nonsymmorphic nodal-line semimetal

Topological materials host fascinating low dimensional gapless states at the boundary. As a prominent example, helical topological edge states (TESs) of two-dimensional topological insulators (2DTIs) and their stacked three-dimensional (3D) equivalent, weak topological insulators (WTIs), have sparked research enthusiasm due to their potential application in the next generation of electronics/spintronics with low dissipation. Here, we propose layered superconducting material CaSn as a WTI with nontrivial Z2 as well as nodal line semimetal protected by crystalline non-symmorphic symmetry. Our systematic angle-resolved photoemission spectroscopy (ARPES) investigation on the electronic structure exhibits excellent agreement with the calculation. Furthermore, scanning tunnelling microscopy/spectroscopy (STM/STS) at the surface step edge shows signatures of the expected TES. These integrated evidences from ARPES, STM/STS measurement and corresponding ab initio calculation strongly support the existence of TES in the non-symmorphic nodal line semimetal CaSn, which may become a versatile material platform to realize multiple exotic electronic states as well as topological superconductivity.

cond-mat.mtrl-sci↗

Observation of Topological Superconductivity in a Stoichiometric Transition Metal Dichalcogenide 2M-WS2

Topological superconductors (TSCs) are unconventional superconductors with bulk superconducting gap and in-gap Majorana states on the boundary that may be used as topological qubits for quantum computation. Despite their importance in both fundamental research and applications, natural TSCs are very rare. Here, combining state of the art synchrotron and laser-based angle-resolved photoemission spectroscopy, we investigated a stoichiometric transition metal dichalcogenide (TMD), 2M-WS2 with a superconducting transition temperature of 8.8 K (the highest among all TMDs in the natural form up to date) and observed distinctive topological surface states (TSSs). Furthermore, in the superconducting state, we found that the TSSs acquired a nodeless superconducting gap with similar magnitude as that of the bulk states. These discoveries not only evidence 2M-WS2 as an intrinsic TSC without the need of sensitive composition tuning or sophisticated heterostructures fabrication, but also provide an ideal platform for device applications thanks to its van der Waals layered structure.

cond-mat.mtrl-sci↗

Measuring Coulomb-Induced Ionization Time Lag with a Calibrated Attoclock

Electrons in atoms and molecules can not react immediately to the action of intense laser field. A time lag (about 100 attoseconds) between instants of the field maximum and the ionization-rate maximum emerges. This lag characterizes the response time of the electronic wave function to the strong-field ionization event and has important effects on subsequent ultrafast dynamics of the ionized electron. The absolute time lag is not accessible in experiments. Here, a calibrated attoclock procedure, which is related to a simple Coulomb-induced temporal correction to electron trajectories, is proposed to measure the relative lag of two different ionization events. Using this procedure,the difference (i.e., the relative lag) between the ionization time lags of polar molecules in two consecutive half laser cycles can be probed with a high accuracy.

physics.atom-ph↗

Characterization and suppression of background light shifts in an optical lattice clock

Experiments involving optical traps often require careful control of the ac Stark shifts induced by strong confining light fields. By carefully balancing light shifts between two atomic states of interest, optical traps at the magic wavelength have been especially effective at suppressing deleterious effects stemming from such shifts. Highlighting the power of this technique, optical clocks today exploit Lamb-Dicke confinement in magic-wavelength optical traps, in some cases realizing shift cancellation at the ten parts per billion level. Theory and empirical measurements can be used at varying levels of precision to determine the magic wavelength where shift cancellation occurs. However, lasers exhibit background spectra from amplified spontaneous emission or other lasing modes which can easily contaminate measurement of the magic wavelength and its reproducibility in other experiments or conditions. Indeed, residual light shifts from laser background have plagued optical lattice clock measurements for years. In this work, we develop a simple theoretical model allowing prediction of light shifts from measured background spectra. We demonstrate good agreement between this model and measurements of the background light shift from an amplified diode laser in an Yb optical lattice clock. Additionally, we model and experimentally characterize the filtering effect of a volume Bragg grating bandpass filter, demonstrating that application of the filter can reduce background light shifts from amplified spontaneous emission well below the $10^{-18}$ fractional clock frequency level. This demonstration is corroborated by direct clock comparisons between a filtered amplified diode laser and a filtered titanium:sapphire laser.

physics.atom-ph↗

Bayesian evaluation of charge yields of fission fragments of 239U

Recent experiments [Phys. Rev. Lett. 123, 092503(2019); Phys. Rev. Lett. 118, 222501 (2017)] have made remarkable progress in measurements of the isotopic fission-fragment yields of the compound nucleus $^{239}$U, which is of great interests for fast-neutron reactors and for benchmarks of fission models. We apply the Bayesian neural network (BNN) approach to learn existing evaluated charge yields and infer the incomplete charge yields of $^{239}$U. We found the two-layer BNN is improved compared to the single-layer BNN for the overall performance. Our results support the normal charge yields of $^{239}$U around Sn and Mo isotopes. The role of odd-even effects in charge yields has also been studied.

nucl-th↗

High ellipticity of harmonics from molecules in strong laser fields of small ellipticity

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular alignment and the laser ellipticity. In particular, for small laser ellipticity, large ellipticity of harmonics with high intensity is observed for parallel alignment, with forming a striking ellipticity hump around the threshold. We show that the interplay of the molecular structure and two-dimensional electron motion plays an important role here. This phenomenon can be used to generate bright elliptically-polarized EUV pulses.

physics.atom-ph↗

Tracing origins of asymmetric momentum distribution for polar molecules in strong linearly-polarized laser fields

We study the ionization dynamics of oriented HeH$^+$ in strong linearly-polarized laser fields by numerically solving the time-dependent Schrödinger equation. The calculated photoelectron momentum distributions for parallel orientation show a striking asymmetric structure. With a developed model pertinent to polar molecules, we trace the electron motion in real time. We show that this asymmetric structure arises from the interplay of the Coulomb effect and the permanent dipole in strong laser fields. This structure can be used to probe the degree of orientation which is important in ultrafast experiments for polar molecules. we also check our results for other polar molecules such as CO and BF.

physics.atom-ph↗

Spectroscopic Signature for Local-moment Magnetism in van der Waals Ferromagnet Fe$_3$GeTe$_2$

The van der Waals ferromagnet Fe$_3$GeTe$_2$ has recently attracted extensive research attention due to its intertwined magnetic, electronic and topological properties. Here, using high-resolution angle-resolved photoemission spectroscopy, we systematically investigate the temperature evolution of the electronic structure of bulk Fe$_3$GeTe$_2$. We observe largely dispersive energy bands that are narrowed by a factor of 1.6 compared with ab-initio calculation. Upon heating towards the ferromagnetic transition near 225 K, we observe a massive reduction of quasiparticle coherence in a large energy range, which is attributed to the enhanced magnetic fluctuation in the system. Remarkably, the electron bands barely shift with increasing temperature, which deviates from the exchange splitting picture within the itinerant Stoner model. We argue that the local magnetic moments play a crucial role in the ferromagnetism of Fe$_3$GeTe$_2$, despite its strongly itinerant nature. Our results provide important insights into the electronic and magnetic properties of Fe$_3$GeTe$_2$ and shed light on the generic understanding of itinerant magnetism in correlated materials.

cond-mat.mtrl-sci↗

Strong-field double ionization dynamics of vibrating HeH$^+$ versus HeT$^+$

We study double ionization (DI) dynamics of vibrating HeH$^+$ versus its isotopic variant HeT$^+$ in strong laser fields numerically. Our simulations show that for both cases, these two electrons in DI prefer to release together along the H(T) side. At the same time, however, the single ionization (SI) is preferred when the first electron escapes along the He side. This potential mechanism is attributed to the interplay of the rescattering of the first electron and the Coulomb induced large ionization time lag. On the other hand, the nuclear motion increases the contributions of these two electrons releasing together along the He side. This effect differentiates DI of HeH$^+$ from HeT$^+$.

physics.atom-ph↗

Persistent gapless surface states in MnBi2Te4/Bi2Te3 superlattice antiferromagnetic topological insulator

Magnetic topological quantum materials (TQMs) provide a fertile ground for the emergence of fascinating topological magneto-electric effects. Recently, the discovery of intrinsic antiferromagnetic (AFM) topological insulator MnBi2Te4 that could realize quantized anomalous Hall effect and axion insulator phase ignited intensive study on this family of TQM compounds. Here, we investigated the AFM compound MnBi4Te7 where Bi2Te3 and MnBi2Te4 layers alternate to form a superlattice. Using spatial- and angle-resolved photoemission spectroscopy, we identified ubiquitous (albeit termination dependent) topological electronic structures from both Bi2Te3 and MnBi2Te4 terminations. Unexpectedly, while the bulk bands show strong temperature dependence correlated with the AFM transition, the topological surface states show little temperature dependence and remain gapless across the AFM transition. The detailed electronic structure of MnBi4Te7 and its temperature evolution, together with the results of its sister compound MnBi2Te4, will not only help understand the exotic properties of this family of magnetic TQMs, but also guide the design for possible applications.

cond-mat.mtrl-sci↗

Topological Electronic Structure and Its Temperature Evolution in Antiferromagnetic Topological Insulator MnBi2Te4

Topological quantum materials coupled with magnetism can provide a platform for realizing rich exotic physical phenomena, including quantum anomalous Hall effect, axion electrodynamics and Majorana fermions. However, these unusual effects typically require extreme experimental conditions such as ultralow temperature or sophisticate material growth and fabrication. Recently, new intrinsic magnetic topological insulators were proposed in MnBi2Te4-family compounds - on which rich topological effects could be realized under much relaxed experimental conditions. However, despite the exciting progresses, the detailed electronic structures observed in this family of compounds remain controversial up to date. Here, combining the use of synchrotron and laser light sources, we carried out comprehensive and high resolution angle-resolved photoemission spectroscopy studies on MnBi2Te4, and clearly identified its topological electronic structures including the characteristic gapless topological surface states. In addition, the temperature evolution of the energy bands clearly reveals their interplay with the magnetic phase transition by showing interesting differences for the bulk and surface states, respectively. The identification of the detailed electronic structures of MnBi2Te4 will not only help understand its exotic properties, but also pave the way for the design and realization of novel phenomena and applications.

cond-mat.mtrl-sci↗

Coulomb-induced ionization time lag after electrons tunnel out of a barrier

After electrons tunnel out of a laser-Coulomb-formed barrier, %formed by the strong laser field and the atomic Coulomb potential, the movement of the tunneling electron can be affected by the Coulomb tail. We show that this Coulomb effect induces a large time difference (longer than a hundred attoseconds) between the exiting time at which the electron exits the barrier and the ionization time at which the electron is free. This large time difference has important influences on strong-field processes such as above-threshold ionization and high-harmonic generation, with remarkably changing time-frequency properties of electron trajectories. Some semi-quantitative evaluations on these influences are addressed, which provide new insight into strong-field physics and give important suggestions on attosecond measurements.

physics.atom-ph↗