arXiv subjects

Y. J. Wang

Publications and source records attributed to Y. J. Wang.

At least 55 records · Page 3Linked to original sources

arXiv2006

Heavy fermion fluid in high magnetic fields: an infrared study of CeRu$_4$Sb$_{12}$

We report a comprehensive infrared magneto-spectroscopy study of CeRu$_4$Sb$_{12}$ compound revealing quasiparticles with heavy effective mass m$^*$, with a detailed analysis of optical constants in fields up to 17 T. We find that the applied magnetic field strongly affects the low energy excitations in the system. In particular, the magnitude of m$^*$ $\simeq$ 70 m$_b$ (m$_b$ is the quasiparticle band mass) at 10 K is suppressed by as much as 25 % at 17 T. This effect is in quantitative agreement with the mean-field solution of the periodic Anderson model augmented with a Zeeman term.

cond-mat.str-el↗

arXiv2005

Spinodal Surface Fluctuations on Polymer Films

We study the temporal growth pattern of surface fluctuations on a series of spinodally unstable polymer films where the degree of instability is controlled by the film thickness. For films in the deep spinodal region, the growth rate function of the surface modes as a function of the wavevector,, fits well to the mean-field theory. As the film thickness is increased and the film instability decreases, the mean-field theory demonstrates marked disagreement with experiment, notwithstanding provision of the known corrections for random thermal noise. We show that the deviations arise from large-amplitude fluctuations induced by homogeneous nucleation, which has not been considered in conventional treatment of thermal noise.

cond-mat.mtrl-sci↗

arXiv2003

Electron Scattering in AlGaN/GaN Structures

We present data on mobility lifetime, $τ_t$, quantum lifetime, $τ_q$, and cyclotron resonance lifetime, $τ_{CR}$, of a sequence of high-mobility two-dimensional electron gases in the AlGaN/GaN system, covering a density range of $\sim1-4.5\times10^{12}$cm$^{-2}$. We observe a large discrepancy between $τ_q$ and $τ_{CR}$ ($τ_q\simτ_{CR}$/6) and explain it as the result of density fluctuations of only a few percent. Therefore, only $τ_{CR}$ --and not $τ_q$ -- is a reliable measure of the time between electron scattering events in these specimens. The ratio $τ_t / τ_{CR}$ increases with increasing density in this series of samples, but scattering over this density range remains predominantly in the large-angle scattering regime.

cond-mat.mes-hall↗

arXiv2003

Non-parabolicity of the conduction band of wurtzite GaN

Using cyclotron resonance, we measure the effective mass, $m$*, of electrons in AlGaN/GaN heterostructures with densities, $n_{2D}\sim 1-6\times10^{12}$cm$^{-2}$. From our extensive data, we extrapolate a band edge mass of $(0.208\pm0.002) m_e$. By comparing our $m$* data with the results of a multi-band \textbf{k.p} calculation we infer that the effect of remote bands is essential in explaining the observed conduction band non-parabolicity (NP). Our calculation of polaron mass corrections -- including finite width and screening - suggests those to be negligible. It implies that the behavior of $m*(n_{2D})$ can be understood solely in terms of NP. Finally, using our NP and polaron corrections, we are able to reduce the large scatter in the published band edge mass values.

cond-mat↗

arXiv2003

Large Splitting of the Cyclotron Resonance Line in AlGaN/GaN Heterostructures

Cyclotron-resonance (CR) measurements on two-dimensional (2D) electrons in AlGaN/GaN heterojunctions reveal large splittings (up to 2 meV) of the CR line for all investigated densities, $n_{2D}$, from 1 to $4\times 10^{12}cm^{-2}$ over wide ranges of magnetic field. The features resemble a level anti-crossing and imply a strong interaction with an unknown excitation of the solid. The critical energy of the splitting varies from 5 to 12 meV and as $\sqrt{n_{2D}}$. The phenomenon resembles data from AlGaAs/GaAs whose origin remains unresolved. It highlights a lack of basic understanding of a very elementary resonance in solids.

cond-mat.mes-hall↗

arXiv2002

X-ray Scattering and Magnetic Susceptibility Study of doped CuGeO_3

We report comprehensive synchrotron x-ray scattering and magnetic susceptibility studies of the doped spin-Peierls materials Cu_{1-x}Zn_xGeO_3 and CuGe_{1-y}Si_yO_3. Temperature versus dopant concentration phase diagrams are mapped out for both Zn and Si dopants. The phase diagrams of both Cu_{1-x}Zn_xGeO_3 and CuGe_{1-y}Si_yO_3 closely resemble that of Cu_{1-x}Mg_xGeO_3, including the observation that the spin gap is established at a much higher temperature than the temperature at which the spin-Peierls dimerization attains long-range order. The spin-Peierls transitions in doped samples exhibit unusual phase transition behavior, characterized by highly rounded phase transitions, Lorentzian squared lineshapes, and very long relaxation times. Phenomenological explanations for these observations are given by considering the effects of competing random bond interactions as well as random fields generated by the dopants. We have also confirmed the reentrance of the spin-Peierls phase when the temperature is lowered through the antiferromagnetic ordering transition. The low temperature re-entrance of the spin-Peierls phase has been explained speculatively using a local phase separation scheme between the spin-Peierls phase and the Neel phase.

cond-mat.str-el↗

arXiv2002

An Infrared study of the Josephson vortex state in high-Tc cuprates

We report the results of the c-axis infrared spectroscopy of La_{2-x} Sr_x CuO_4 in high magnetic field oriented parallel to the CuO_2 planes. A significant suppression of the superfluid density with magnetic field rho_s(H) is observed for both underdoped (x=0.125) and overdoped (x=0.17) samples. We show that the existing theoretical models of the Josephson vortex state fail to consistently describe the observed effects and discuss possible reasons for the discrepancies.

cond-mat.supr-con↗

arXiv2002

Complicated nature of the gap in MgB2: magnetic field-dependent optical studies

We investigated the magnetic field (H)-dependent optical conductivity spectra of MgB2 thin film in the far-infrared region. The H-dependences can be explained by the increase of normal metallic regions embedded in the superconducting background. The area fraction of the normal metallic region increases rather quickly at low field, but slowly at high field. It follows neither H- nor H^{1/2}-dependences. The results suggest the complicated nature of the superconducting gap in MgB2.

cond-mat.str-el↗

arXiv2002

Optical Evidence of Multiphase Coexistence in Single Crystalline (La,Pr,Ca)MnO3

We investigated temperature (T)- and magnetic field-dependent optical conductivity spectra (\s\w) of a La_5/8-yPr_yCa_3/8MnO_3 (y~0.35) single crystal, showing intriguing phase coexistence at low T. At T_C < T < T_CO, a dominant charge-ordered phase produces a large optical gap energy of ~0.4 eV. At T < T_C, at least two absorption bands newly emerge below 0.4 eV. Analyses of (\s\w) indicate that the new bands should be attributed to a ferromagnetic metallic and a charge-disordered phase that coexist with the charge-ordered phase. This optical study clearly shows that La_5/8-yPrCa_3/8MnO_3 (y~0.35) is composed of multiphases that might have different lattice strains.

cond-mat.str-el↗

arXiv2001

Charge dynamics and metal-insulator transition in Si$_{1-x}$Gd$_{x}$ and Si$_{1-x}$Y$_{x}$ alloys

Carrier dynamics in amorphous a-Si$_{1-x}$RE$_{x}$ (RE=Gd, Y) films has been studied in the doping regime close to the metal-insulator transition by means of infrared spectroscopy. Optical constants throughout the entire intra-gap region ($\hbar ω<$ 1 eV) have been found to be anomalously sensitive to changes of temperature and/or magnetic field. The observed behavior is consistent with the model of hopping transport where the interaction of carriers with both the lattice and large core spin of Gd ions is taken into account.

cond-mat.str-el↗

arXiv2001

Magnetic Field Effects on the Far-Infrared Absorption in Mn_12-acetate

We report the far-infrared spectra of the molecular nanomagnet Mn_12-acetate (Mn_12) as a function of temperature (5-300 K) and magnetic field (0-17 T). The large number of observed vibrational modes is related to the low symmetry of the molecule, and they are grouped together in clusters. Analysis of the mode character based on molecular dynamics simulations and model compound studies shows that all vibrations are complex; motion from a majority of atoms in the molecule contribute to most modes. Three features involving intramolecular vibrations of the Mn_12 molecule centered at 284, 306 and 409 cm-1 show changes with applied magnetic field. The structure near 284 cm$^{-1}$ displays the largest deviation with field and is mainly intensity related. A comparison between the temperature dependent absorption difference spectra, the gradual low-temperature cluster framework distortion as assessed by neutron diffraction data, and field dependent absorption difference spectra suggests that this mode may involve Mn motion in the crown.

cond-mat.str-el↗

arXiv2000

X-ray scattering study of two length scales in the critical fluctuations of CuGeO3

The critical fluctuations of CuGeO$_3$ have been measured by synchrotron x-ray scattering, and two length scales are clearly observed. The ratio between the two length scales is found to be significantly different along the $a$ axis, with the $a$ axis along the surface normal direction. We believe that such a directional preference is a clear sign that surface random strains, especially those caused by dislocations, are the origin of the long length scale fluctuations.

cond-mat.str-el↗

arXiv2000

Magnetic Field Dependent Optical Studies of a Layered Antiferromagnet Pr$%_{1/2}$Sr$_{1/2}$MnO$_3$

Magnetic field ($H$)-dependent optical conductivity spectra $σ(ω) $ and dielectric constant spectra $ε(ω)$ of a layered antiferromagnet ($A$-type) Pr$_{1/2}$Sr$_{1/2}$MnO$_3$ were presented. At 0.0 T in 4.2 K, the $σ(ω)$ showed a small Drude-like peak in the far-infrared region and a broad absorption peak in the mid-infrared region. With increasing $H$, large spectral weights were transferred from high to low energy regions with increase of the Drude-like peak. We found that a polaron picture could explain most of the $H$-dependent spectral changes. By comparing with the $H$-dependent spectral weight changes and $ε(ω)$ of Nd$_{1/2}$Sr$_{1/2}$MnO$_3$, which has the $CE$-type spin ordering, we showed that a dimensional crossover from a 2-dimensional to a 3-dimensional metal occurs in Pr$_{1/2}$Sr$_{1/2}$MnO$_3$.

cond-mat.str-el↗

arXiv1999

Melting of Charge/Orbital Ordered States in Nd$_{1/2}$Sr$_{1/2}$MnO$_3$: Temperature and Magnetic Field Dependent Optical Studies

We investigated the temperature ($T=$ 15 $\sim $ 290 K) and the magnetic field ($H=$ 0 $\sim $ 17 T) dependent optical conductivity spectra of a charge/orbital ordered manganite, Nd$_{1/2}$Sr$_{1/2}$MnO$_3$. With variation of $T$ and $H$, large spectral weight changes were observed up to 4.0 eV. These spectral weight changes could be explained using the polaron picture. Interestingly, our results suggested that some local ordered state might remain above the charge ordering temperature, and that the charge/orbital melted state at a high magnetic field (i.e. at $H=$ 17 T and $% T=$ 4.2 K) should be a three dimensional ferromagnetic metal. We also investigated the first order phase transition from the charge/orbital ordered state to ferromagnetic metallic state using the $T$- and $H$% -dependent dielectric constants $ε_1$. In the charge/orbital ordered insulating state, $ε_1$ was positive and $dε_1/dω\approx 0$. With increasing $T$ and $H$, $ε_1$ was increased up to the insulator-metal phase boundaries. And then, $ε_1$ abruptly changed into negative and $dε_1/dω>0$, which was consistent with typical responses of a metal. Through the analysis of $% ε_1$ using an effective medium approximation, we found that the melting of charge/orbital ordered states should occur through the percolation of ferromagnetic metal domains.

cond-mat.str-el↗

arXiv1999

The first-order phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic phases in Cu_(1-x)M_xGeO_3

We have performed detailed magnetic susceptibility measurements as well as synchrotron x-ray diffraction studies to determine the temperature vs concentration ($T$ - $x$) phase diagram of Cu${}_{1-x}$Mg${}_x$GeO${}_3$. We observe clear double peaks in the magnetic susceptibility implying two antiferromagnetic (AF) transition temperatures in samples with Mg concentrations in the range 0.0237 $\le x \le$ 0.0271. We also observe a drastic change in the inverse correlation length in this concentration range by x-ray diffraction. The drastic change of the AF transition temperature as well as the disappearance of the spin-Peierls (SP) phase have been clarified; these results are consistent with a first-order phase transition between dimerized AF (D-AF) and uniform AF (U-AF) phases as reported by T. Masuda {\it et al.} \lbrack Phys. Rev. Lett. {\bf 80}, 4566 (1998)\rbrack. The $T$ - $x$ phase diagram of Cu${}_{1-x}$Zn${}_x$GeO${}_3$ is similar to that of Cu${}_{1-x}$Mg${}_x$GeO${}_3$, which suggests that the present phase transition is universal for Cu${}_{1-x}M_{x}$GeO${}_3$.

cond-mat.str-el↗

arXiv1999

Reentrant Spin-Peierls Transition in Mg-Doped CuGeO_3

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_{1-x}Mg_xGeO_3. In a recent paper we have shown that the SP dimerization attains long-range order only for x < x_c = 0.022(0.001). Here we report that the SP transition is reentrant in the vicinity of the critical concentration x_c. This is manifested by broadening of the SP dimerization superlattice peaks below the reentrance temperature, T_r, which may mean either the complete loss of the long-range SP order or the development of a short-range ordered component within the long-range ordered SP state. Marked hysteresis and very large relaxation times are found in the samples with Mg concentrations in the vicinity of x_c. The reentrant transition is likely related to the competing Neel transition which occurs at a temperature similar to T_r. We argue that impurity-induced competing interchain interactions play an essential role in these phenomena.

cond-mat.str-el↗

arXiv1999

Structural Critical Scattering Study of Mg-Doped CuGeO3

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_(1-x)Mg_xGeO_3. We find that for x>0 the temperature T_m at which the spin gap is established is significantly higher than the temperature T_s at which the SP dimerization attains long-range order. The latter is observed only for x x_c the SP correlation length quickly decreases with increasing x. We argue that impurity-induced competing interactions play a central role in these phenomena.

cond-mat.str-el↗

arXiv1999

Spin-Peierls Transition in CuGeO_3: Critical, Tricritical, or Mean Field?

The spin-Peierls phase transition in CuGeO_3 has been extensively studied utilizing a variety of experimental techniques. Interpretations of the phase transition behavior vary from tricritical to mean field to Ising critical to XY critical. We show that the behavior in the vicinity of the phase transition of each of the order parameter, the magnetic energy gap and the heat capacity can be quantitatively fitted with few adjustable parameters with a mean field model incorporating a tricritical to mean field critical crossover in the transition region.

cond-mat.str-el↗