arXiv subjects

Y. J. Yu

Publications and source records attributed to Y. J. Yu.

15 recordsLinked to original sources

arXiv2021

Fluctuating magnetic droplets immersed in a sea of quantum spin liquid

The search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature, is a main theme in current condensed matter physics. However, there is no smoking-gun evidence for deconfined spinons in any QSL candidate so far. The disorders and competing exchange interactions may prevent the formation of an ideal QSL state on frustrated spin lattices. Here we report comprehensive and systematic measurements of the magnetic susceptibility, ultra-low temperature specific heat, muon spin relaxation (muSR), nuclear magnetic resonance (NMR), and thermal conductivity for NaYbSe2 single crystals, in which Yb3+ ions with effective spin-1/2 form a perfect triangular lattice. All these complementary techniques find no evidence of long-range magnetic order down to their respective base temperatures. Instead, specific heat, muSR and NMR measurements suggest the coexistence of quasi-static and dynamic spins in NaYbSe2. The scattering from these quasi-static spins may cause the absence of magnetic thermal conductivity. Thus, we propose a scenario of fluctuating ferrimagnetic droplets immersed in a sea of QSL. This may be quite common on the way pursuing an ideal QSL, and provides a brand-new platform to study how a QSL state survives impurities and coexists with other magnetically ordered states.

cond-mat.str-el↗

arXiv2019

Absence of magnetic thermal conductivity in the quantum spin liquid candidate EtMe3Sb[Pd(dmit)2]2 -- revisited

We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice organic compound EtMe$_3$Sb[Pd(dmit)$_2$]$_2$, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita $et$ $al.$, Nat. Commun. {\bf 2}, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 Tesla. These results are in sharp contrast to previous thermal conductivity measurements on EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ [M. Yamashita $et$ $al.$ Science {\bf 328}, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ has to be reconsidered.

cond-mat.str-el↗

arXiv2018

Multigap nodeless superconductivity in CsCa2Fe4As4F2 probed by heat transport

Recently, a new family of iron-based superconductors called 12442 was discovered and the muon spin relaxation ($μ$SR) measurements on KCa$_2$Fe$_4$As$_4$F$_2$ and CsCa$_2$Fe$_4$As$_4$F$_2$ polycrystals, two members of the family, indicated that both have a nodal superconducting gap structure with $s+d$ pairing symmetry. Here we report the ultralow-temperature thermal conductivity measurements on CsCa$_2$Fe$_4$As$_4$F$_2$ single crystals ($T_c$ = 29.3 K). A negligible residual linear term $κ_0/T$ in zero field and the field dependence of $κ_0/T$ suggest multiple nodeless superconducting gaps in CsCa$_2$Fe$_4$As$_4$F$_2$. This gap structure is similar to CaKFe$_4$As$_4$ and moderately doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$, but contrasts to the nodal gap structure indicated by the $μ$SR measurements on CsCa$_2$Fe$_4$As$_4$F$_2$ polycrystals.

cond-mat.supr-con↗

arXiv2018

Ultralow-temperature thermal conductivity of Pr2Ir2O7: a metallic spin-liquid candidate with quantum criticality

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the Pr$_2$Ir$_2$O$_7$ single crystals to detect possible exotic excitations. In zero field, the thermal conductivity shows a dramatic suppression above a characteristic temperature $T_s \approx$ 0.12 K. With increasing field, $T_s$ increases and the thermal conductivity tends to saturate above $H$ = 5 T. The Wiedemann-Franz law is verified at high fields and inferred at zero field. It suggests the normal behavior of electrons at the quantum critical point, and the absence of mobile fermionic magnetic excitations. The strong suppression of thermal conductivity is attributed to the scattering of phonons by the spin system, likely the fluctuating spins. These results shed new light on the microscopic description on this novel compound.

cond-mat.str-el↗

arXiv2018

T0 Fan-out for Back-n White Neutron Facility at CSNS

the main physics goal for Back-n white neutron facility at China Spallation Neutron Source (CSNS) is to measure nuclear data. The energy of neutrons is one of the most important parameters for measuring nuclear data. Method of time of flight (TOF) is used to obtain the energy of neutrons. The time when proton bunches hit the thick tungsten target is considered as the start point of TOF. T0 signal, generated from the CSNS accelerator, represents this start time. Besides, the T0 signal is also used as the gate control signal that triggers the readout electronics. Obviously, the timing precision of T0 directly affects the measurement precision of TOF and controls the running or readout electronics. In this paper, the T0 fan-out for Back-n white neutron facility at CSNS is proposed. The T0 signal travelling from the CSNS accelerator is fanned out to the two underground experiment stations respectively over long cables. To guarantee the timing precision, T0 signal is conditioned with good signal edge. Furthermore, techniques of signal pre-emphasizing and equalizing are used to improve signal quality after T0 being transmitted over long cables with about 100 m length. Experiments show that the T0 fan-out works well, the T0 signal transmitted over 100 m remains a good time resolution with a standard deviation of 25 ps. It absolutely meets the required accuracy of the measurement of TOF.

physics.ins-det↗

arXiv2018

Electronics of Time-of-flight Measurement for Back-n at CSNS

Back-n is a white neutron experimental facility at China Spallation Neutron Source (CSNS). The time structure of the primary proton beam make it fully applicable to use TOF (time-of-flight) method for neutron energy measuring. We implement the electronics of TOF measurement on the general-purpose readout electronics designed for all of the seven detectors in Back-n. The electronics is based on PXIe (Peripheral Component Interconnect Express eXtensions for Instrumentation) platform, which is composed of FDM (Field Digitizer Modules), TCM (Trigger and Clock Module), and SCM (Signal Conditioning Module). T0 signal synchronous to the CSNS accelerator represents the neutron emission from the target. It is the start of time stamp. The trigger and clock module (TCM) receives, synchronizes and distributes the T0 signal to each FDM based on the PXIe backplane bus. Meantime, detector signals after being conditioned are fed into FDMs for waveform digitizing. First sample point of the signal is the stop of time stamp. According to the start, stop time stamp and the time of signal over threshold, the total TOF can be obtained. FPGA-based (Field Programmable Gate Array) TDC is implemented on TCM to accurately acquire the time interval between the asynchronous T0 signal and the global synchronous clock phase. There is also an FPGA-based TDC on FDM to accurately acquire the time interval between T0 arriving at FDM and the first sample point of the detector signal, the over threshold time of signal is obtained offline. This method for TOF measurement is efficient and not needed for additional modules. Test result shows the accuracy of TOF is sub-nanosecond and can meet the requirement for Back-n at CSNS.

physics.ins-det↗

arXiv2018

Ultralow-temperature heat transport in the quantum spin liquid candidate Ca10Cr7O28 with bilayer kagome lattice

Recently, a novel material with bilayer kagome lattice Ca$_{10}$Cr$_7$O$_{28}$ was proposed to be a gapless quantum spin liquid, due to the lack of long-range magnetic order and the observation of broad diffuse excitations. Here, we present the ultralow-temperature thermal conductivity measurements on single crystals of Ca$_{10}$Cr$_7$O$_{28}$ to detect its low-lying magnetic excitations. At finite temperatures, with increasing the magnetic fields, the thermal conductivity exhibits a clear dip around 6 T, which may correspond to a crossover in the magnetic ground state. At the zero-temperature limit, no residual linear term is found at any fields, indicating the absence of gapless itinerant fermionic excitations. Therefore, if the spinons do exist, they are either localized or gapped. In the gapped case, the fitting of our data gives a small gap $Δ\sim$ 0.27(2) K. These results put strong constraints on the theoretical description of the ground state in this quantum spin liquid candidate.

cond-mat.str-el↗

arXiv2017

Design of back-streaming white neutron beam line at CSNS

A white neutron beam line using the back-streaming neutrons from the spallation target at China Spallation Neutron Source (CSNS) is under construction. Different spectrometers mainly for nuclear data measurements to be installed in the so-called Back-n beam line are also under development in phases. The physics design of the beam line includes the overview of the characteristics of the neutron beam including energy spectrum, flux and time structure, and the optimizations of neutron beam spots and in-hall background with the help of a complicated collimation system and a sophisticated neutron dump. The wide neutron energy range of 1 eV~100 MeV is very good to support different applications, especially for nuclear data measurements. At Endstation#2 where is about 80 m from the target, the main properties include neutron flux of 106 n/cm2/s, time resolution of a few per mille over almost the whole energy range, in-hall background about 0.01 /cm2/s for both neutron and gamma. With its completion in late 2017, Back-n will be not only the first high-performance white neutron source in China, but also among the best white neutron sources in the world.

physics.ins-det↗

arXiv2017

Ultralow-temperature thermal conductivity of the Kitaev honeycomb magnet $α$-RuCl$_3$ across the field-induced phase transition

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $α$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal conductivity measurements on the single crystals of $α$-RuCl$_3$ down to 80 mK and up to 9 T. Our experiments clearly show a field-induced phase transition occurring at $H_c$ $\approx$ 7.5 T, above which the zigzag magnetic order is completely suppressed. The minimum of thermal conductivity at 7.5 T is attributed to the strong scattering of phonons by the magnetic fluctuations. Most importantly, above 7.5 T, we do not observe any significant contribution of thermal conductivity from gapless magnetic excitations, which puts a strong constraint on the nature of the high-field phase of $α$-RuCl$_3$.

cond-mat.str-el↗

arXiv2017

Heat transport study of the spin liquid candidate 1T-TaS2

We present the ultra-low-temperature thermal conductivity measurements on single crystals of the prototypical charge-density-wave material 1$T$-TaS$_2$, which was recently argued to be a candidate for quantum spin liquid. Our experiments show that the residual linear term of thermal conductivity at zero field is essentially zero, within the experimental accuracy. Furthermore, the thermal conductivity is found to be insensitive to the magnetic field up to 9 T. These results clearly demonstrate the absence of itinerant magnetic excitations with fermionic statistics in bulk 1$T$-TaS$_2$ and, thus, put a strong constraint on the theories of the ground state of this material.

cond-mat.str-el↗

arXiv2016

Absence of magnetic thermal conductivity in the quantum spin liquid candidate YbMgGaO4

We present the ultra-low-temperature specific heat and thermal conductivity measurements on the single crystals of YbMgGaO$_4$, which was recently argued to be a promising candidate for quantum spin liquid (QSL). In the zero magnetic field, a large magnetic contribution of specific heat is observed, and exhibits a power-law temperature dependence ($C_m \sim T^{0.74}$). On the contrary, we do not observed any significant contribution of thermal conductivity from magnetic excitations. In magnetic fields $H \ge$ 6 T, the exponential $T$-dependence of $C_m$ and the enhanced thermal conductivity indicate a magnon gap of the fully-polarized state. The absence of magnetic thermal conductivity at the zero field in this QSL candidate puts a strong constraint on the theories of its ground state.

cond-mat.str-el↗

arXiv2016

Tuning phase transitions of FeSe thin flakes by field effect transistor with solid ion conductor as gate dielectric

We develop a novel field effect transistor (FET) device using solid ion conductor (SIC) as a gate dielectric, and we can tune the carrier density of FeSe by driving lithium ions in and out of the FeSe thin flakes, and consequently control the material properties and its phase transitions. A dome-shaped superconducting phase diagram was mapped out with increasing Li content, with $T_c$ $\sim$ 46.6 K for the optimal doping, and an insulating phase was reached at the extremely overdoped regime. Our study suggests that, using solid ion conductor as a gate dielectric, the SIC-FET device can achieve much higher carrier doping in the bulk, and suit many surface sensitive experimental probes, and can stabilize novel structural phases that are inaccessible in ordinary conditions.

cond-mat.supr-con↗

arXiv2016

Fully gapped superconducting state in Au2Pb: a natural candidate for topological superconductor

We measured the ultra-low-temperature specific heat and thermal conductivity of Au$_2$Pb single crystal, a possible three-dimensional Dirac semimetal with a superconducting transition temperature $T_c \approx$ 1.05 K. The electronic specific heat can be fitted by a two-band s-wave model, which gives the gap amplitudes $Δ_1$(0)/$k_BT_c$ = 1.38 and $Δ_2$(0)/$k_BT_c$ = 5.25. From the thermal conductivity measurements, a negligible residual linear term $κ_0/T$ in zero field and a slow field dependence of $κ_0/T$ at low field are obtained. These results suggest that Au$_2$Pb has a fully gapped superconducting state in the bulk, which is a necessary condition for topological superconductor if Au$_2$Pb is indeed one.

cond-mat.supr-con↗

arXiv2016

Nodal superconductivity in FeS: Evidence from quasiparticle heat transport

We report low-temperature heat transport measurements on superconducting iron sulfide FeS with $T_c \approx$ 5 K, which has the same crystal structure and similar electronic band structure to the superconducting iron selenide FeSe. In zero magnetic field, a significant residual linear term $κ_0/T$ is observed. At low field, $κ_0/T$ increases rapidly with the increase of field. These results provide strong evidence for nodal superconducting gap in FeS. We compare it with the sister compound FeSe, and other iron-based superconductors with nodal gap.

cond-mat.supr-con↗

arXiv2016

Observation of two distinct superconducting domes under pressure in tetragonal FeS

As the simplest iron-based superconductor, FeSe forms a tetragonal structure with transition temperature Tc ~ 8 K. With assistance of pressure, or other techniques, Tc can be greatly enhanced, even to above liquid nitrogen temperature. The newly discovered superconducting tetragonal FeS (Tc ~ 4.5 K), a sulfide counterpart of FeSe, promotes us on its high pressure investigation. The transport and structure evolution of FeS with pressure have been studied. A rapid suppression of Tc and vanishing of superconductivity at 4.0 GPa are observed, followed by a second superconducting dome with a 30% enhancement in maximum Tc. An onsite tetragonal to hexagonal phase transition occurs around 7.0 GPa, followed by a broad pressure range of phase coexistence. The residual deformed tetragonal phase is considered as the source of second superconducting dome. The observation of two superconducting domes in iron-based superconductors poses great challenges for understanding their pairing mechanism.

cond-mat.supr-con↗