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Y. S. Lee

Publications and source records attributed to Y. S. Lee.

At least 55 records · Page 3Linked to original sources

Local Spin Susceptibility of the S=1/2 Kagome Lattice in ZnCu3(OD)6Cl2

We report single-crystal 2-D NMR investigation of the nearly ideal spin S=1/2 kagome lattice ZnCu3(OD)6Cl2. We successfully identify 2-D NMR signals originating from the nearest-neighbors of Cu2+ defects occupying Zn sites. From the 2-D Knight shift measurements, we demonstrate that weakly interacting Cu2+ spins at these defects cause the large Curie-Weiss enhancement toward T=0 commonly observed in the bulk susceptibility data. We estimate the intrinsic spin susceptibility of the kagome planes by subtracting defect contributions, and explore several scenarios.

cond-mat.str-el↗

The Southern Proper Motion Program IV. The SPM4 Catalog

We present the fourth installment of the Yale/San Juan Southern Proper Motion Catalog, SPM4. The SPM4 contains absolute proper motions, celestial coordinates, and (B,V) photometry for over 103 million stars and galaxies between the south celestial pole and -20 deg declination. The catalog is roughly complete to V=17.5 and is based on photographic and CCD observations taken with the Yale Southern Observatory's double-astrograph at Cesco Observatory in El Leoncito, Argentina. The proper-motion precision, for well-measured stars, is estimated to be 2 to 3 mas/yr, depending on the type of second-epoch material. At the bright end, proper motions are on the International Celestial Reference System by way of Hipparcos Catalog stars, while the faint end is anchored to the inertial system using external galaxies. Systematic uncertainties in the absolute proper motions are on the order of 1 mas/yr.

astro-ph.GA↗

Charge states and magnetic ordering in LaMnO3/SrTiO3 superlattices

We investigated the magnetic and optical properties of [(LaMnO3)n/(SrTiO3)8]20 (n = 1, 2, and 8) superlattices grown by pulsed laser deposition. We found a weak ferromagnetic and semiconducting state developed in all superlattices. An analysis of the optical conductivity showed that the LaMnO3 layers in the superlattices were slightly doped. The amount of doping was almost identical regardless of the LaMnO3 layer thickness up to eight unit cells, suggesting that the effect is not limited to the interface. On the other hand, the magnetic ordering became less stable as the LaMnO3 layer thickness decreased, probably due to a dimensional effect.

cond-mat.str-el↗

Dzyaloshinskii-Moriya interaction and spin re-orientation transition in the frustrated kagome lattice antiferromagnet

Magnetization, specific heat, and neutron scattering measurements were performed to study a magnetic transition in jarosite, a spin-5/2 kagome lattice antiferromagnet. When a magnetic field is applied perpendicular to the kagome plane, magnetizations in the ordered state show a sudden increase at a critical field H_c, indicative of the transition from antiferromagnetic to ferromagnetic states. This sudden increase arises as the spins on alternate kagome planes rotate 180 degrees to ferromagnetically align the canted moments along the field direction. The canted moment on a single kagome plane is a result of the Dzyaloshinskii-Moriya interaction. For H < H_c, the weak ferromagnetic interlayer coupling forces the spins to align in such an arrangement that the canted components on any two adjacent layers are equal and opposite, yielding a zero net magnetic moment. For H > H_c, the Zeeman energy overcomes the interlayer coupling causing the spins on the alternate layers to rotate, aligning the canted moments along the field direction. Neutron scattering measurements provide the first direct evidence of this 180-degree spin rotation at the transition.

cond-mat.str-el↗

Nonlinear optical probe of tunable surface electrons on a topological insulator

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping dependence measurements as a function of photon polarization and sample orientation we show that second harmonic generation can simultaneously probe both the surface crystalline structure and the surface charge of Bi$_2$Se$_3$. Furthermore, we find that second harmonic generation using circularly polarized photons reveals the time-reversal symmetry properties of the system and is surprisingly robust against surface charging, which makes it a promising tool for spectroscopic studies of topological surfaces and buried interfaces.

cond-mat.mtrl-sci↗

Soft phonons and structural phase transition in superconducting Ba0.59K0.41BiO3

We have observed a softening of phonons and a structural phase transition in a superconducting Ba0.59K0.41BiO3 (Tc = 31 K) single crystal using elastic and inelastic neutron scattering measurements. The soft phonon occurs for the [111] transverse acoustic mode at the zone boundary. The phonon energies in this vicinity are found to continuously decrease with decreasing temperature from above room temperature to 200 K, where a structural phase transition from cubic to tetragonal symmetry occurs. The overall results are consistent with previous data that reported phonon softening and a (0.5, 0.5, 0.5) type superstructure in several Ba1-xKxBiO3 systems. However, we also find weak (0.5, 0.5, 0) type superstructure peaks that reveal an additional component to the modulation. No significant change related to the superconductivity was observed for the soft phonon energies or linewidths.

cond-mat.supr-con↗

The stellar content of the Hamburg/ESO survey VI. The metallicity distribution of main-sequence turnoff stars in the Galactic halo

We determine the metallicity distribution function (MDF) of the Galactic halo based on metal-poor main-sequence turnoff-stars (MSTO) which were selected from the Hamburg/ESO objective-prism survey (HES) database. Corresponding follow-up moderateresolution observations (R ~ 2000) of some 682 stars (among which 617 were accepted program stars) were carried out with the 2.3m telescope at the Siding Spring Observatory (SSO). Corrections for the survey volume covered by the sample stars were quantitatively estimated and applied to the observed MDF. The corrections are quite small, when compared with those for a previously studied sample of metal-poor giants. The corrected observational MDF of the turnoff sample was then compared with that of the giants, as well as with a number of theoretical predictions of Galactic chemical evolution, including the mass-loss modified Simple Model. Although the survey-volume corrected MDFs of the metal-poor turnoff and the halo giants notably differ in the region of [Fe/H] > -2.0, below [Fe/H] ~ -2.0, (the region we scientifically focus on most) both MDFs show a sharp drop at [Fe/H] ~ -3.6 and present rather similar distributions in the low-metallicity tail. Theoretical models can fit some parts of the observed MDF, but none is found to simultaneously reproduce the peak as well as the features in the metal-poor region with [Fe/H] between -2.0 to -3.6. Among the tested models only the GAMETE model, when normalized to the tail of the observed MDF below [Fe/H] ~ -3.0, and with Z_{cr} = 10^{-3.4}Z_{\odot}, is able to predict the sharp drop at [Fe/H] ~ -3.6.

astro-ph.GA↗

Electronic structure and anomalous band-edge absorption feature in multiferroic MnWO4: An optical spectroscopic study

We investigated the electronic structure and lattice dynamics of multiferroic MnWO4 by optical spectroscopy. With variation of polarization, temperature, and magnetic field, we obtained optical responses over a wide range of photon energies. The electronic structure of MnWO4 near to the Fermi level was examined, with inter-band transitions identified in optical conductivity spectra above a band-gap of 2.5 eV. As for the lattice dynamics, we identified all the infrared transverse optical phonon modes available according to the group-theory analysis. Although we did not observe much change in global electronic structure across the phase transition temperatures, an optical absorption at around 2.2 eV showed an evident change depending upon the spin configuration and magnetic field. The behavior of this band-edge absorption indicates that spin-orbit coupling plays an important role in multiferroic MnWO4.

cond-mat.str-el↗

A Cu2+ (S = 1/2) Kagomé Antiferromagnet: MgxCu4-x(OH)6Cl2

Spin-frustrated systems are one avenue for inducing macroscopic quantum states in materials. However, experimental realization of this goal has been difficult because of the lack of simple materials and, if available, the separation of the unusual magnetic properties arising from exotic magnetic states from behavior associated with chemical disorder, such as site mixing. Here we report the synthesis and magnetic properties of a new series of magnetically frustrated materials, MgxCu4-x(OH)6Cl2. Because of the substantially different ligand-field chemistry of Mg2+ and Cu2+, site disorder within the kagomé layers is minimized, as directly measured by X-ray diffraction. Our results reveal that many of the properties of these materials and related systems are not due to disorder of the magnetic lattice but rather reflect an unusual ground state.

cond-mat.str-el↗

Dynamic Scaling in the Susceptibility of the Spin-1\2 Kagome Lattice Antiferromagnet Herbertsmithite

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling relation in both the bulk ac susceptibility and the low energy dynamic susceptibility as measured by inelastic neutron scattering. The quantity $χT^α$ with $α\simeq 0.66$ can be expressed as a universal function of $H/T$ or $ω/T$. This scaling is discussed in relation to similar behavior seen in systems influenced by disorder or by the proximity to a quantum critical point.

cond-mat.str-el↗

Two-Dimensional Confinement of 3d1 Electrons in LaTiO3/LaAlO3 Multilayers

We report spectroscopic ellipsometry measurements of the anisotropy of the interband transitions parallel and perpendicular to the planes of (LaTiO3)n(LaAlO3)5 multilayers with n = 1-3. These provide direct information about the electronic structure of the two-dimensional (2D) 3d^1 state of the Ti ions. In combination with LDA+U calculations, we suggest that 2D confinement in the TiO2 slabs lifts the degeneracy of the t_{2g} states leaving only the planar d_xy orbitals occupied. We outline that these multilayers can serve as a model system for the study of the t_{2g} 2D Hubbard model.

cond-mat.str-el↗

Optical spectroscopic investigation on the temperature-dependent electronic structure evolution of the Jeff,1/2 Mott insulator Sr2IrO4

We investigated the temperature-dependent evolution of the electronic structure of the Jeff,1/2 Mott insulator Sr2IrO4 using optical spectroscopy. The optical conductivity spectra $σ(ω)$ of this compound has recently been found to exhibit two d-d transitions associated with the transition between the Jeff,1/2 and Jeff,3/2 bands due to the cooperation of the electron correlation and spin-orbit coupling. As the temperature increases, the two peaks show significant changes resulting in a decrease in the Mott gap. The experimental observations are compared with the results of first-principles calculation in consideration of increasing bandwidth. We discuss the effect of the temperature change on the electronic structure of Sr2IrO4 in terms of local lattice distortion, excitonic effect, electron-phonon coupling, and magnetic ordering.

cond-mat.str-el↗

Dual Character of Magnetism in Ferropnictides: Insights from Optical Measurements

We investigate the electronic structure of EuFe$_{2}$As$_{2}$ using optical spectroscopy and first-principles calculations. At low temperature we observe the evolution of \textit{two} gap-like features, one having a BCS mean-field behavior and another with strongly non-BCS behavior. Using band structure calculations, we identify the former with a spin-Peierls-like partial gap in $d_{yz}$ bands, and the latter with the transition across the large exchange gap in $d_{xz}/d_{xy}$ bands. Our results demonstrate that the antiferromagnetism in the ferropnictides is neither fully local nor fully itinerant, but contains elements of both.

cond-mat.supr-con↗

Polarized neutron scattering studies of the kagome lattice antiferromagnet KFe3(OH)6(SO4)2

We report polarized neutron scattering studies of spin-wave excitations and spin fluctuations in the S=5/2 kagome lattice antiferromagnet KFe3(OH)6(SO4)2 (jarosite). Inelastic polarized neutron scattering measurements at 10 K on a single crystal sample reveal two spin gaps, associated with in-plane and out-of-plane excitations. The polarization analysis of quasi-elastic scattering at 67 K shows in-plane spin fluctuations with XY symmetry, consistent with the disappearance of the in-plane gap above the Neel temperature T_N = 65 K. Our results suggest that jarosite is a promising candidate for studying the 2D XY universality class in magnetic systems.

cond-mat.str-el↗

Pressure-induced Spin-Peierls to Incommensurate Charge-Density-Wave Transition in the Ground State of TiOCl

The ground state of the spin-Peierls system TiOCl was probed using synchrotron x-ray diffraction on a single-crystal sample at T = 6 K. We tracked the evolution of the structural superlattice peaks associated with the dimerized ground state as a function of pressure. The dimerization along the b axis is rapidly suppressed in the vicinity of a first-order structural phase transition at Pc = 13.1(1) GPa. The high-pressure phase is characterized by an incommensurate charge density wave perpendicular to the original spin chain direction. These results show that the electronic ground state undergoes a fundamental change in symmetry, indicating a significant change in the principal interactions.

cond-mat.str-el↗

Halo streams in the 7th SDSS data release

We have detected stellar halo streams in the solar neighborhood using data from the 7th public data release of the Sloan Digital Sky Survey (SDSS), which includes the directed stellar program SEGUE: Sloan Extension For Galactic Understanding and Exploration. In order to derive distances to each star, we used the metallicity-dependent photometric parallax relation from Ivezic et al. (2008) for which we examine and quantify the accuracy. Our final sample consists of 22,321 nearby (d < 2 kpc), metal-poor ([Fe/H] < -0.5) main-sequence stars with 6D estimates of position and space velocity. We characterize the orbits of these stars through suitable kinematic proxies for their "effective" integrals of motion, angular momentum, eccentricity, and orbital polar angle and compare the observed distribution to expectations from a smooth distribution in four [Fe/H] bins. On this basis we identify at least five significant "phase-space overdensities" of stars on very similar orbits in the solar neighborhood to which we can assign unambiguously peaked [Fe/H] distributions. Three of them have been identified previously, including the halo stream discovered by Helmi et al. (1999) at a significance level of 12.0. In addition, we find at least two new genuine halo streams, judged by their kinematics and [Fe/H], at significance levels of 2.9 and 4.8, respectively. For one stream the stars even show coherence in configuration space, matching a spatial overdensity of stars found by Juric et al. (2008) at (R,z) \approx (9.5,0.8) kpc. Our results demonstrate the practical power of our search method to detect substructure in the phase-space distribution of nearby stars without making a-priori assumptions about the detailed form of the gravitational potential.

astro-ph.GA↗

Toward constraints on galaxy formation scenarios: stellar properties from Galactic surveys

We present some of the strategies being developed to classify and parameterize objects obtained with spectra from the Sloan Digital Sky Survey (SDSS) and the RAdial Velocity Experiment (RAVE) and present some results. We estimate stellar atmospheric parameters (effective temperature, gravity, and metallicity) from spectral and photometric data and use these to analyse Galactic populations. We demonstrate this through the selection of a sample of candidate Blue Horizontal-Branch and RR Lyrae stars selected from SDSS/SEGUE.

astro-ph↗

Spin Correlations in the Geometrically Frustrated Pyrochlore Tb2Mo2O7

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has little apparent chemical disorder. Diffuse elastic peaks are observed at low temperatures, indicating short-range ordering of the Tb moments in an arrangement where the Tb moments are slightly rotated from the preferred directions of the spin ice structure. In addition, a Q-independent signal is observed which likely originates from frozen, but completely uncorrelated, Tb moments. Inelastic measurements show the absence of sharp peaks due to crystal field excitations. These data show how the physics of the Tb sublattice responds to the glassy behavior of the Mo sublattice with the associated effects of lattice disorder.

cond-mat.str-el↗