Y. Sakakieda | Searcharxiv

arXiv2024

Development of a method to measure trace level of uranium and thorium in scintillation films

We have established a method to measure picograms-per-gram (pg g$^{-1}$) levels of $^{238}$U and $^{232}$Th in scintillation films by combining the dry ashing method and inductively coupled plasma mass spectrometry. Trace amounts of $^{238}$U and $^{232}$Th were measured in up to 2~g of the scintillation film with almost 100% collection efficiency. This paper details the experimental procedure, including the pretreatment of the samples and labware, detection limit of the method, collection efficiencies of $^{238}$U and $^{232}$Th, and measurement of $^{238}$U and $^{232}$Th in a polyethylene naphthalate film. This method is also applicable to $^{238}$U and $^{232}$Th measurements in other low-background organic materials for rare event search experiments.

physics.ins-det↗

arXiv2023

Rapid Analysis of $\mathrm{^{226}Ra}$ in Ultrapure Gadolinium Sulfate Octahydrate

Numerous particle physics experiments utilize gadolinium (Gd), a rare earth element with the most significant neutron capture cross-section among all elements, to detect anti-neutrinos via inverse beta-decays or to remove neutron-induced background events. For example, to load Gd into water Cherenkov detectors, $\mathrm{{Gd_{2}(SO_{4})_{3}\cdot 8H_{2}O}}$ is dissolved and rare event search experiments are required to screen for radioactive impurities in $\mathrm{{Gd_{2}(SO_{4})_{3}\cdot 8H_{2}O}}$ before dissolution. This study developed a new method to rapidly measure the radium-226($\mathrm{^{226}Ra}$) concentration in $\mathrm{{Gd_{2}(SO_{4})_{3}\cdot 8H_{2}O}}$. This method requires only three days to measure a batch of samples, as opposed to the usual method using high-purity germanium detectors, which takes approximately 20 days after arrival. The detection limit for the measurement of $\mathrm{^{226}Ra}$ is 0.32 mBq/kg. This method has been already used for $\mathrm{{Gd_{2}(SO_{4})_{3}\cdot 8H_{2}O}}$ screening at the Super-Kamiokande Gd(SK-Gd) project, and it can be applied to future experiments.

physics.ins-det↗