arXiv subjects

Y. Shen

Publications and source records attributed to Y. Shen.

At least 19 recordsLinked to original sources

arXiv2026

The evolution of pairing correlation with $3d_{z^{2}}$ electron filling in a bilayer two-orbital model for La$_3$Ni$_2$O$_7$

The discovery of high-${T_c}$ superconductivity in pressurized bilayer nickelate La$_3$Ni$_2$O$_7$ presents a new arena for exploring unconventional pairing mechanisms. A pivotal yet unresolved issue is the specific role of the $3d_{z^{2}}$ orbital of Ni. While its inter-layer super-exchange antiferromagnetic coupling is widely considered crucial for superconductivity, the role of its itinerancy remains undetermined. Early studies showed that the superconductivity is accompanied by the emergence of a small Fermi pocket of the $3d_{z^{2}}$ orbitals. However, recent experiments show controversial results on the role of the $3d_{z^{2}}$ Fermi pocket on superconductivity. Motivated by these experimental results, we investigate an effective bilayer two-orbital model for La$_3$Ni$_2$O$_7$ using density-matrix renormalization group (DMRG) on a minimal one-dimensional geometry. By systematically varying the $3d_{z^{2}}$ orbital filling from $1/12$ doping to half-filling, we observe a pronounced suppression of superconducting correlations near half-filling. Our results demonstrate the itinerancy of $3d_{z^{2}}$ orbital is favorable for the pairing in the bilayer two-orbital model for La$_3$Ni$_2$O$_7$. Moreover, we observe that the pairing correlation is enhanced in regions where charge fluctuations are large, suggesting a competition between charge order and superconductivity in the model.

cond-mat.str-el↗

arXiv2026

Entangling gate performance and fidelity limits with neutral atom F\"orster resonances

Neutral-atom entangling gates are commonly analyzed with a single effective Rydberg-pair state, but near F\"orster resonances the pair manifold contains resonantly coupled interaction channels that change both the control landscape and the achievable fidelity. We develop a two-eigenstate model for this regime and show that when allowing for coupling to both pair states in the resonance, the gate fidelity is bounded by $\mathcal{F}\leq 1-(\pi/2)/(V\tau_R)$, for interaction strength $V$ and Rydberg lifetime $\tau_R$. We construct a gate protocol that saturates this bound in the large-Rabi-frequency limit, improving the existing fidelity limit by approximately $40\%$. We also evaluate common gate protocols near F\"orster resonances and find that retaining the exchange dynamics increases predicted fidelities by up to two orders of magnitude over earlier treatments.

quant-ph↗

arXiv2026

Robust AGN and host-galaxy decomposition in optical spectral fitting

Unraveling the growth of supermassive black holes and their connection to host galaxies requires disentangling the Active Galactic Nuclei (AGN) emission from that of the stellar populations. When an AGN spectrum is observed at different activity phases, if the spectral decomposition properly recognizes the nuclear and stellar components, key physical properties - such as black-hole mass, stellar mass, and stellar velocity dispersion - should remain consistent. We present a novel optical spectral-fitting approach that combines pPXF and PyQSOFit to robustly decompose spectra into stellar and AGN components. We apply this technique to three SDSS samples with repeated optical spectra of the same objects at z<0.55: 32 changing-look AGN in bright and dim states, and 15 quasars and 15 galaxies with three single-epoch and one stacked spectrum each. To compare with the literature, we use SDSS spectra and photometric data from AGN in the eFEDS field, as well as Gemini and VLT observations of some of our changing-look AGN. We evaluate the reliability of stellar mass, velocity dispersion, and black-hole mass measurements, especially in relation to the AGN-to-total continuum contribution (fAGN). For host-derived properties, especially when fAGN<0.8, our method yields consistent results. For single-epoch black-hole mass estimates from Ha and Hb, 3-sigma confidence in the broad-line flux and FWHM provides effective criteria for selecting reliable measurements. After applying these quality cuts, measurements across different epochs agree within uncertainties, and their reliability is confirmed by the alignment with previously established scaling relations. Many changing-look AGN in our sample exhibit "breathing" broad-line regions, as determined from Ha analysis, while some deviate significantly, suggesting non-virialized systems across the spectral transition.

astro-ph.GA↗

arXiv2026

Simultaneous TRACERS and THEMIS Observations of Reversed Cusp Ion Dispersions and Dual-Lobe Reconnection

We present observations from two consecutive TRACERS-2 orbits through the northern low-altitude cusp. During the first crossing, TRACERS-2 observed reversed cusp ion dispersion and sunward convection, consistent with magnetopause reconnection tailward of the cusp during this northward IMF interval. Simultaneous THEMIS-D observations at the equatorial magnetopause show heated magnetosheath plasma captured on closed field lines, with similar particle spectra as in in the low-altitude cusp, indicating that reconnection indeed occurred tailward of the cusp and in both hemispheres. When TRACERS-2 traversed the northern cusp again, 95 minutes later, the IMF was dominated by a negative BX component. Despite the different IMF conditions, TRACERS-2 recorded nearly the same cusp signatures as before, i.e., reversed ion dispersion and sunward convection. The observations indicate that tailward-of-cusp reconnection can occur for both northward and BX-dominated IMF and that these distinct IMF geometries can produce remarkably similar plasma and field signatures in the low-altitude cusp.

physics.space-ph↗

arXiv2026

Observation of correlated plasmons in low-valence nickelates

The discovery of nickelate superconductors has opened a new arena for studying the behavior of correlated electron liquids that give rise to unconventional superconductivity. While critical information about a material's charge dynamics is encoded in its plasmons, collective modes of the electron gas, these excitations have not yet been observed in nickelate materials. Here, we use resonant inelastic x-ray scattering (RIXS) to detect plasmons in the metallic, low-valence nickelate Pr4Ni3O8. Although qualitatively similar to those in cuprates, the nickelate plasmons are more heavily damped and have a lower velocity than those in a cuprate at comparable doping, which we attribute to reduced electronic hopping and enhanced screening of the long-range Coulomb interactions. Furthermore, the plasmons in Pr4Ni3O8 soften with increasing temperature, in contrast to the cuprate, where plasmons remain at nearly fixed energy but become more strongly damped. Taken together, these results reveal a distinct charge-screening landscape in nickelates and place quantitative constraints on analogies to cuprates.

cond-mat.str-el↗

arXiv2025

Observation of anisotropic dispersive dark exciton dynamics in CrSBr

Many-body excitons in CrSBr are attracting intense interest in view of their highly anisotropic magneto-optical coupling and their potential for novel optical interfaces within spintronic and magnonic devices. Characterizing the orbital character and propagation of these electronic excitations is crucial for understanding and controlling their behavior; however, this information is challenging to access. Ultra-high resolution resonant inelastic x-ray scattering is a momentum-resolved technique that can address these crucial questions. We present measurements collected at the Cr $L_3$-edge which show a rich spectrum of excitations with a variety of spin-orbital characters. While most of these excitations appear to be localized, the dispersion of the lowest energy dark exciton indicates that it is able to propagate along both the $a$ and $b$ directions within the planes of the crystal. This two-dimensional character is surprising as it contrasts with electrical conductivity and the behavior of the bright exciton, both of which are strongly one-dimensional. The discovery of this propagating dark exciton highlights an unusual coexistence of one- and two-dimensional electronic behaviors in CrSBr.

cond-mat.str-el↗

arXiv2024

Estimating Masses of Supermassive Black Holes in Active Galactic Nuclei from the Halpha Emission Line

The goal of this project is to construct an estimator for the masses of supermassive black holes in active galactic nuclei (AGNs) based on the broad Halpha emission line. We make use of published reverberation mapping data. We remeasure all Halpha time lags from the original data as we find that often the reverberation measurements are improved by detrending the light curves. We produce mass estimators that require only the Halpha luminosity and the width of the Halpha emission line as characterized by either the FWHM or the line dispersion. It is possible, on the basis of a single spectrum covering the Halpha emission line, to estimate the mass of the central supermassive black hole in AGNs, taking into account all three parameters believed to affect mass measurement: luminosity, line width, and Eddington ratio. The typical formal accuracy in such estimates is of order 0.2-0.3 dex.

astro-ph.GA↗

arXiv2024

Searching for Beyond the Standard Model physics using the improved description of $^{100}$Mo $2\nu\beta\beta$ decay spectral shape with CUPID-Mo

The current experiments searching for neutrinoless double-$\beta$ ($0\nu\beta\beta$) decay also collect large statistics of Standard Model allowed two-neutrino double-$\beta$ ($2\nu\beta\beta$) decay events. These can be used to search for Beyond Standard Model (BSM) physics via $2\nu\beta\beta$ decay spectral distortions. $^{100}$Mo has a natural advantage due to its relatively short half-life, allowing higher $2\nu\beta\beta$ decay statistics at equal exposures compared to the other isotopes. We demonstrate the potential of the dual read-out bolometric technique exploiting a $^{100}$Mo exposure of 1.47 kg $\times$ y, acquired in the CUPID-Mo experiment at the Modane underground laboratory (France). We set limits on $0\nu\beta\beta$ decays with the emission of one or more Majorons, on $2\nu\beta\beta$ decay with Lorentz violation, and $2\nu\beta\beta$ decay with a sterile neutrino emission. In this analysis, we investigate the systematic uncertainty induced by modeling the $2\nu\beta\beta$ decay spectral shape parameterized through an improved model, an effect never considered before. This work motivates searches for BSM processes in the upcoming CUPID experiment, which will collect the largest amount of $2\nu\beta\beta$ decay events among the next-generation experiments.

nucl-ex↗

arXiv2024

Magnetically propagating Hund's exciton in van der Waals antiferromagnet NiPS3

Magnetic van der Waals (vdW) materials have opened new frontiers for realizing novel many-body phenomena. Recently NiPS3 has received intense interest since it hosts an excitonic quasiparticle whose properties appear to be intimately linked to the magnetic state of the lattice. Despite extensive studies, the electronic character, mobility, and magnetic interactions of the exciton remain unresolved. Here we address these issues by measuring NiPS3 with ultra-high energy resolution resonant inelastic x-ray scattering (RIXS). We find that Hund's exchange interactions are primarily responsible for the energy of formation of the exciton. Measuring the dispersion of the Hund's exciton reveals that it propagates in a way that is analogous to a double-magnon. We trace this unique behavior to fundamental similarities between the NiPS3 exciton hopping and spin exchange processes, underlining the unique magnetic characteristics of this novel quasiparticle.

cond-mat.str-el↗

arXiv2024

The eROSITA Final Equatorial Depth Survey (eFEDS): the hard X-ray selected sample

During its calibration and performance verification phase, the eROSITA instrument aboard the SRG satellite performed a uniform wide--area X-ray survey of approximately 140 deg$^{2}$ in a region of the sky known as the eROSITA Final Equatorial Depth Survey (eFEDS). The primary aim of eFEDS is to demonstrate the scientific performance to be expected at the end of the 8-pass eROSITA all sky survey. This will provide the first focussed image of the whole sky in the hard X-ray ($>2$~keV) bandpass. The expected source population in this energy range is thus of great interest, particularly for AGN studies. We use the 2.3--5 keV selection presented by Brunner et al. (2022) to construct a sample of 246 point-like hard X-ray sources for further study and characterization. These are classified as either extragalactic ($\sim 90$~\%) or Galactic ($\sim 10$~\%), with the former consisting overwhelmingly of AGN and the latter active stars. We concentrate our further analysis on the extragalactic/AGN sample, describing their X-ray and multiwavelength properties and comparing them to the eFEDS main AGN sample selected in the softer 0.2-2.3 keV band. The eROSITA hard band selects a subsample of sources that is a factor $>10$ brighter than the eFEDS main sample. The AGN within the hard population reach up to $z=3.2$ but on the whole are relatively nearby, with median $z$=0.34 compared to $z$=0.94 for the main sample. The hard survey probes typical luminosities in the range $\log L_{\rm X} = 43-46$. X-ray spectral analysis shows significant intrinsic absorption (with $\log N_{\rm H}>21$) in $\sim 20$~\% of the sources, with a hard X-ray power law continuum with mean $<\Gamma>=1.83\pm0.04$, typical of AGN, but slightly harder than the soft-selected eROSITA sample. (abridged)

astro-ph.HE↗

arXiv2023

Multiple superconducting phases driven by pressure in the topological insulator GeSb4Te7

Tuning superconductivity in topological materials by means of chemical substitution, electrostatic gating, or pressure is thought to be an effective route towards realizing topological superconductivity with their inherent Majorana fermions, the manipulation of which may form the basis for future topological quantum computing. It has recently been established that the pseudo-binary chalcogenides (ACh)m(Pn2Ch3)n (A = Ge, Mn, Pb, etc.; Pn = Sb or Bi; Ch = Te, Se) may host novel topological quantum states such as the quantum anomalous Hall effect and topological axion states. Here we map out the phase diagram of one member in this series, the topological insulator candidate GeSb4Te7 up to pressures of ~35 GPa, through a combination of electrical resistance measurements, Raman spectroscopy, as well as first-principles calculations. Three distinct superconducting phases emerge under the pressure above ~11, ~17, and ~31 GPa, which are accompanied by concomitant structural transitions, evidenced from the changes in the Raman modes. The first-principles calculations validate the existence of a topological insulating state at ambient pressure and predict two possible structural transitions at 10 and 17 GPa, in agreement with the experimental observations. Overall, our results establish the GeSb4Te7 family of materials as a fertile arena for further exploring various topological phenomena, including topological phase transitions and putative topological superconductivity.

cond-mat.supr-con↗

arXiv2023

Stacking disorder in $\alpha$-RuCl$_3$ via x-ray three-dimensional difference pair distribution function analysis

The van der Waals layered magnet $\alpha$-RuCl$_3$ offers tantalizing prospects for the realization of Majorana quasiparticles. Efforts to understand this are, however, hampered by inconsistent magnetic and thermal transport properties likely coming from the formation of structural disorder during crystal growth, postgrowth processing, or upon cooling through the first order structural transition. Here, we investigate structural disorder in $\alpha$-RuCl$_3$ using x-ray diffuse scattering and three-dimensional difference pair distribution function (3D-$\Delta$PDF) analysis. We develop a quantitative model that describes disorder in $\alpha$-RuCl$_3$ in terms of rotational twinning and intermixing of the high and low-temperature structural layer stacking. This disorder may be important to consider when investigating the detailed magnetic and electronic properties of this widely studied material.

cond-mat.str-el↗

arXiv2023

Measurement of the $2\nu\beta\beta$ decay rate and spectral shape of $^{100}$Mo from the CUPID-Mo experiment

Neutrinoless double beta decay ($0\nu\beta\beta$) is a yet unobserved nuclear process which would demonstrate Lepton Number violation, a clear evidence of beyond Standard Model physics. The process two neutrino double beta decay ($2\nu\beta\beta)$ is allowed by the Standard Model and has been measured in numerous experiments. In this letter, we report a measurement of $2\nu\beta\beta$ decay half-life of $^{100}$Mo to the ground state of $^{100}$Ru of $(7.07~\pm~0.02~\text{(stat.)}~\pm~0.11~\text{(syst.)})~\times~10^{18}$~yr by the CUPID-Mo experiment. With a relative precision of $\pm~1.6$ \% this is the most precise measurement to date of a $2\nu\beta\beta$ decay rate in $^{100}$Mo. In addition, we constrain higher-order corrections to the spectral shape which provides complementary nuclear structure information. We report a novel measurement of the shape factor $\xi_{3,1}=0.45~\pm 0.03~\text{(stat.)} \ \pm 0.05 \ \text{(syst.)}$, which is compared to theoretical predictions for different nuclear models. We also extract the first value for the effective axial vector coupling constant obtained from a spectral shape study of $2\nu\beta\beta$ decay.

nucl-ex↗

arXiv2023

The background model of the CUPID-Mo $0\nu\beta\beta$ experiment

CUPID-Mo, located in the Laboratoire Souterrain de Modane (France), was a demonstrator for the next generation $0\nu\beta\beta$ decay experiment, CUPID. It consisted of an array of 20 enriched Li$_{2}$$ ^{100}$MoO$_4$ bolometers and 20 Ge light detectors and has demonstrated that the technology of scintillating bolometers with particle identification capabilities is mature. Furthermore, CUPID-Mo can inform and validate the background prediction for CUPID. In this paper, we present a detailed model of the CUPID-Mo backgrounds. This model is able to describe well the features of the experimental data and enables studies of the $2\nu\beta\beta$ decay and other processes with high precision. We also measure the radio-purity of the Li$_{2}$$^{100}$MoO$_4$ crystals which are found to be sufficient for the CUPID goals. Finally, we also obtain a background index in the region of interest of 3.7$^{+0.9}_{-0.8}$(stat)$^{+1.5}_{-0.7}$(syst)$\times10^{-3}$counts/$\Delta$E$_{FWHM}$/mol$_{iso}$/yr, the lowest in a bolometric $0\nu\beta\beta$ decay experiment.

hep-ex↗

arXiv2023

Resonant inelastic x-ray scattering data for Ruddlesden-Popper and reduced Ruddlesden-Popper nickelates

Ruddlesden-Popper and reduced Ruddlesden-Popper nickelates are intriguing candidates for mimicking the properties of high-temperature superconducting cuprates. The degree of similarity between these nickelates and cuprates has been the subject of considerable debate. Resonant inelastic x-ray scattering (RIXS) has played an important role in exploring their electronic and magnetic excitations, but these efforts have been stymied by inconsistencies between different samples and the lack of publicly available data for detailed comparison. To address this issue, we present open RIXS data on La4Ni3O10 and La4Ni3O8.

cond-mat.str-el↗

arXiv2023

Orbital polarization, charge transfer, and fluorescence in reduced valence nickelates

This paper presents a simple formalism for calculating X-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) that has as input orbital-resolved density of states from a single-particle or many-body \textit{ab initio} calculation and is designed to capture itinerant-like features. We use this formalism to calculate both the XAS and RIXS with input from DFT and DFT+DMFT for the recently studied reduced valence nickelates $R_4$Ni$_3$O$_8$ and $R$NiO$_2$ ($R$ a rare earth), and these results are then contrasted with those for the cuprate CaCuO$_2$ and the unreduced nickelate $R_4$Ni$_3$O$_{10}$. In contrast to the unreduced $R_4$Ni$_3$O$_{10}$, the reduced valence nickelates as well as the cuprate show strong orbital polarization due to the dominance of $x^2-y^2$ orbitals for the unoccupied $3d$ states. We also reproduce two key aspects of a recent RIXS experiment for $R_4$Ni$_3$O$_8$: (i) a charge transfer feature between $3d$ and oxygen $2p$ states whose energy we find to decrease as one goes from $R$NiO$_2$ to $R_4$Ni$_3$O$_8$ to the cuprate, and (ii) an energy-dependent polarization reversal of the fluorescence line that arises from hybridization of the unoccupied $z^2$ states with $R$ 5d states. We end with some implications of our results for the nature of the $3d$ electrons in reduced valence nickelates.

cond-mat.str-el↗

arXiv2023

Electronic character of charge order in square planar low valence nickelates

Charge order is a central feature of the physics of cuprate superconductors and is known to arise from a modulation of holes with primarily oxygen character. Low-valence nickelate superconductors also host charge order, but the electronic character of this symmetry breaking is unsettled. Here, using resonant inelastic x-ray scattering at the Ni $L_2$-edge, we identify intertwined involvements of Ni $3d_{x^2-y^2}$, $3d_{3z^2-r^2}$, and O $2p_{\sigma}$ orbitals in the formation of diagonal charge order in an overdoped low-valence nickelate La$_{4}$Ni$_{3}$O$_{8}$. The Ni $3d_{x^2-y^2}$ orbitals, strongly hybridized with planar O $2p_{\sigma}$, largely shape the spatial charge distribution and lead to Ni site-centered charge order. The $3d_{3z^2-r^2}$ orbitals play a small, but non-negligible role in the charge order as they hybridize with the rare-earth $5d$ orbitals. Our results reveal that the low-energy physics and ground-state character of these nickelates are more complex than those in cuprates.

cond-mat.str-el↗

arXiv2022

Structure of Charge Density Waves in La$_{1.875}$Ba$_{0.125}$CuO$_4$

Although charge-density wave (CDW) correlations exist in several families of cuprate supercon-ductors, they exhibit substantial variation in CDW wavevector and correlation length, indicating a key role for CDW-lattice interactions. We investigated this interaction in La$_{1.875}$Ba$_{0.125}$CuO$_4$ using single crystal x-ray diffraction to collect a large number of CDW peak intensities, and determined the Cu and La/Ba atomic distortions induced by the formation of CDW order. Within the CuO$_2$ planes, the distortions involve a periodic modulation of the Cu-Cu spacing along the direction of the ordering wave vector. The charge ordering within the copper-oxygen layer induces an out-of-plane breathing modulation of the surrounding lanthanum layers, which leads to a related distortion on the adjacent copper-oxygen layer. Our result implies that the CDW-related structural distortions do not remain confined to a single layer but rather propagate an appreciable distance through the crystal. This leads to overlapping structural modulations, in which CuO$_2$ planes exhibit distortions arising from the orthogonal CDWs in adjacent layers as well as distortions from the CDW within the layer itself. We attribute this striking effect to the weak c-axis charge screening in cuprates and suggest this effect could help couple the CDW between adjacent planes in the crystal.

cond-mat.supr-con↗