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Y. Sun

Publications and source records attributed to Y. Sun.

At least 163 records · Page 9Linked to original sources

Nature of $γ$-deformation in Ge and Se nuclei and the triaxial projected shell model description

Recent experimental data have demonstrated that $^{76}$Ge may be a rare example of a nucleus exhibiting rigid $γ$-deformation in the low-spin regime. In the present work, the experimental analysis is supported by microscopic calculations using the multi-quasiparticle triaxial projected shell model (TPSM) approach. It is shown that to best describe the data of both yrast and $γ$-vibrational bands in $^{76}$Ge, a rigid-triaxial deformation parameter $γ\approx 30^\circ$ is required. TPSM calculations are discussed in conjunction with the experimental observations and also with the published results from the spherical shell model. The occurrence of a $γγ$-band in $^{76}$Ge is predicted with the bandhead at an excitation energy of $ \sim$ 2.5 MeV. We have also performed TPSM study for the neighboring Ge- and Se-isotopes and the distinct $γ$-soft feature in these nuclei is shown to result from configuration mixing of the ground-state with multi-quasiparticle states.

nucl-th↗

Towards a unified realistic shell-model Hamiltonian with the monopole-based universal force

We propose a unified realistic shell-model Hamiltonian employing the pairing plus multipole Hamiltonian combined with the monopole interaction constructed starting from the monopole-based universal force by Otsuka it et al. (Phys. Rev. Lett. 104, 012501 (2010)). It is demonstrated that the proposed PMMU model can consistently describe a large amount of spectroscopic data as well as binding energies in the pf and pf5/2g9/2 shell spaces, and could serve as a practical shell model for even heavier mass regions.

nucl-th↗

Coexistence of two superconducting phases in Ca1-xLaxFe2As2

Single crystals of Ca1-xLaxFe2As2 for x ranging from 0 to 0.25 have been grown and characterized by structural, transport and magnetic measurements. Coexistence of two superconducting phases is observed, in which the low superconducting transition temperature (Tc) phase has Tc ~ 20 K, and the high Tc phase has Tc higher than 40 K. These data also delineate an x - T phase diagram in which the single magnetic/structural phase transition in undoped CaFe2As2 appears to split into two distinct phase transitions, both of which are suppressed with increasing La substitution. Superconductivity emerges when x is about 0.06 and coexists with the structural/magnetic transition until x is ~ 0.13. With increasing concentration of La, the structural/magnetic transition is totally suppressed, and Tc reaches its maximum value of about 45 K for 0.15 < x < 0.19. A domelike superconducting region is not observed in the phase diagram, however, because no obvious over-doping region can be found. Two superconducting phases coexist in the x - T phase diagram of Ca1-xLaxFe2As2. The formation of the two separate phases, as well as the origin of the high Tc in Ca1-xLaxFe2As2 is studied and discussed in detail.

cond-mat.supr-con↗

Upper Critical Fields and Anisotropy of Ca1-xLaxFe2As2 Single Crystals

Superconductivity of Ca1-xLaxFe2As2 single crystals with various doping level were investigated via electromagnetic measurements for out-plane (H//c) and in-plane (H//ab) directions. Obvious double superconducting transitions, which can survive in magnetic fields up to several Tesla, were observed in the medium-doped (x = 0.13) sample. Two kinds of distinct Hc2 phase diagrams were established for the low superconducting phase with Tc lower than 15 K and the high superconducting phase with Tc of over 40 K, respectively. Both the two kinds of phase diagrams exist in the medium-doped sample. Unusual upward curvature near Tc was observed in Hc2 phase diagrams and analyzed in detail. Temperature dependences of anisotropy for different doping concentrations were obtained and compared. Both superconducting phases manifest extremely large anisotropies, which may originate from the interface or intercalation superconductivity.

cond-mat.supr-con↗

Collectivity evolution in the neutron-rich Pd isotopes towards the N=82 shell closure

The neutron-rich, even-even 122,124,126Pd isotopes has been studied via in-beam gamma-ray spectroscopy at the RIKEN Radioactive Isotope Beam Factory. Excited states at 499(9), 590(11), and 686(17) keV were found in the three isotopes, which we assign to the respective 2+ -> 0+ decays. In addition, a candidate for the 4+ state at 1164(20) keV was observed in 122Pd. The resulting Ex(2+) systematics are essentially similar to those of the Xe (Z=54) isotopic chain and theoretical prediction by IBM-2, suggesting no serious shell quenching in the Pd isotopes in the vicinity of N=82.

nucl-ex↗

Magnetoelectric coupling in the paramagnetic state of a metal-organic framework

Although the magnetoelectric effects - the mutual control of electric polarization by magnetic fields and magnetism by electric fields, have been intensively studied in a large number of inorganic compounds and heterostructures, they have been rarely observed in organic materials. Here we demonstrate magnetoelectric coupling in a metal-organic framework [(CH3)2NH2]Mn(HCOO)3 which exhibits an order-disorder type of ferroelectricity below 185 K. The magnetic susceptibility starts to deviate from the Curie-Weiss law at the paraelectric-ferroelectric transition temperature, suggesting an enhancement of short-range magnetic correlation in the ferroelectric state. Electron spin resonance study further confirms that the magnetic state indeed changes following the ferroelectric phase transition. Inversely, the ferroelectric polarization can be improved by applying high magnetic fields. We interpret the magnetoelectric coupling in the paramagnetic state in the metal-organic framework as a consequence of the magnetoelastic effect that modifies both the superexchange interaction and the hydrogen bonding.

cond-mat.mtrl-sci↗

Toroidal modeling of penetration of the resonant magnetic perturbation field

A toroidal, quasi-linear model is proposed to study the penetration dynamics of the resonant magnetic perturbation (RMP) field into the plasma. The model couples the linear, fluid plasma response to a toroidal momentum balance equation, which includes torques induced by both fluid electromagnetic force and by (kinetic) neoclassical toroidal viscous force. The numerical results for a test toroidal equilibrium quantify the effects of various physical parameters on the field penetration and on the plasma rotation braking. The neoclassical toroidal viscous torque plays a dominant role in certain region of the plasma, for the RMP penetration problem considered in this work.

physics.plasm-ph↗

Variation in displacement energies due to isospin nonconserving forces

For mirror nuclei with masses A=42-95, the effects of isospin nonconserving nuclear forces are studied with nuclear shell model using the Coulomb displacement energy and triplet displacement energy as probes. It is shown that the characteristic behavior of the displacement energies can be well reproduced if the isovector and isotensor nuclear interactions with J=0 and T=1 are introduced into the f7/2 shell. These forces, with their strengths being found consistent with the nucleon-nucleon scattering data, tend to modify nuclear binding energies near the N=Z line. At present, no evidence is found that these forces are needed for the upper fp-shell. Theoretical one- and two-proton separation energies are predicted accordingly, and locations of the proton drip-line are thereby suggested.

nucl-th↗

Large transport critical currents and magneto-optical imaging of textured Sr1-xKxFe2As2 superconducting tapes

We report the temperature dependence of the transport critical current density (Jc) in textured Sr1-xKxFe2As2/Fe (Sr122) tapes fabricated by an ex situ powder-in-tube process. Critical currents were measured in magnetic fields up to 0-15 T and/or the temperature range 4.2-30 K by using a dc four-probe method. It was found that textured Sr122 tapes heat-treated at low temperatures showed higher transport Jc performance due to much improved intergrain connections. At temperatures of 20 K, easily obtained using a cryocooler, Jc reached ~ 10^4 A/cm^2 in self field, which is the highest transport value of ferropnictide wires and tapes reported so far. Magneto-optical imaging observations further revealed significant and well distributed global Jc at 20 K in our tapes. These results demonstrate that 122 type superconducting tapes are promising for high-field applications at around 20 K.

cond-mat.supr-con↗

A Geometric Blind Source Separation Method Based on Facet Component Analysis

Given a set of mixtures, blind source separation attempts to retrieve the source signals without or with very little information of the the mixing process. We present a geometric approach for blind separation of nonnegative linear mixtures termed {\em facet component analysis} (FCA). The approach is based on facet identification of the underlying cone structure of the data. Earlier works focus on recovering the cone by locating its vertices (vertex component analysis or VCA) based on a mutual sparsity condition which requires each source signal to possess a stand-alone peak in its spectrum. We formulate alternative conditions so that enough data points fall on the facets of a cone instead of accumulating around the vertices. To find a regime of unique solvability, we make use of both geometric and density properties of the data points, and develop an efficient facet identification method by combining data classification and linear regression. For noisy data, we show that denoising methods may be employed, such as the total variation technique in imaging processing, and principle component analysis. We show computational results on nuclear magnetic resonance spectroscopic data to substantiate our method.

math.NA↗

Annealing, acid, and alcoholic beverage effects on Fe1+yTe0.6Se0.4

We have systematically investigated and compared different methods to induce superconductivity in iron chalcogenide Fe1+yTe0.6Se0.4 including annealing in vacuum, N2, O2, I2 atmosphere, and immersing samples into acid and alcoholic beverages. Vacuum and N2 annealing are proved to be ineffective to induce superconductivity in Fe1+yTe0.6Se0.4 single crystal. O2 and I2 annealing, acid and alcoholic beverages can induce superconductivity by oxidizing the excess Fe in the sample. Superconductivity in O2 annealed sample is in bulk nature, while I2, acid and alcoholic beverages can only induce superconductivity near the surface. By comparing different effects of O2, I2, acid and alcoholic beverages, we propose a scenario to explain how the superconductivity is induced in the non-superconducting as-grown Fe1+yTe0.6Se0.4.

cond-mat.supr-con↗

Coulomb energy difference as a probe of isospin-symmetry breaking in the upper fp-shell nuclei

The anomaly in Coulomb energy differences (CED) between the isospin T=1 states in the odd-odd N=Z nucleus 70Br and the analogue states in its even-even partner 70Se has remained a puzzle. This is a direct manifestation of isospin-symmetry breaking in effective nuclear interactions. Here, we perform large-scale shell-model calculations for nuclei with A=66-78 using the new filter diagonalization method based on the Sakurai-Sugiura algorithm. The calculations reproduce well the experimental CED. The observed negative CED for A=70 are accounted for by the cross-shell neutron excitations from the fp-shell to the g9/2 intruder orbit with the enhanced electromagnetic spin-orbit contribution at this special nucleon number.

nucl-th↗

Density effect on critical current density and flux pinning properties of polycrystalline SmFeAsO1-xFx superconductor

A series of polycrystalline SmFeAs1-xOx bulks was prepared to systematically investigate the influence of sample density on flux pinning properties. Different sample densities were achieved by controlling the pelletizing pressure. The superconducting volume fraction, the critical current densities Jcm and the flux pinning force densities Fp were estimated from the magnetization measurements. Experimental results manifest that: (1) the superconducting volume fraction decreases with the decreasing of sample density. (2) The Jcm values have the similar trend except for the sample with very high density may due to different connectivity and pinning mechanism. Moreover, The Jcm(B) curve develops a peak effect at approximately the same field at which the high-density sample shows a kink. (3) The Fp(B) curve of the high-density sample shows a low-field peak and a high-field peak at several temperatures, which can be explained by improved intergranular current, while only one peak can be observed in Fp(B) of the low-density samples. Based on the scaling behaviour of flux pinning force densities, the main intragranular pinning is normal point pinning.

cond-mat.supr-con↗

A Sparse Semi-Blind Source Identification Method and Its Application to Raman Spectroscopy for Explosives Detection

Rapid and reliable detection and identification of unknown chemical substances is critical to homeland security. It is challenging to identify chemical components from a wide range of explosives. There are two key steps involved. One is a nondestructive and informative spectroscopic technique for data acquisition. The other is an associated library of reference features along with a computational method for feature matching and meaningful detection within or beyond the library. Recently several experimental techniques based on Raman scattering have been developed to perform standoff detection and identification of explosives, and they prove to be successful under certain idealized conditions. However data analysis is limited to standard least squares method assuming the complete knowledge of the chemical components. In this paper, we develop a new iterative method to identify unknown substances from mixture samples of Raman spectroscopy. In the first step, a constrained least squares method decomposes the data into a sum of linear combination of the known components and a non-negative residual. In the second step, a sparse and convex blind source separation method extracts components geometrically from the residuals. Verification based on the library templates or expert knowledge helps to confirm these components. If necessary, the confirmed meaningful components are fed back into step one to refine the residual and then step two extracts possibly more hidden components. The two steps may be iterated until no more components can be identified. We illustrate the proposed method in processing a set of the so called swept wavelength optical resonant Raman spectroscopy experimental data by a satisfactory blind extraction of a priori unknown chemical explosives from mixture samples.

math.NA↗

A Semi-Blind Source Separation Method for Differential Optical Absorption Spectroscopy of Atmospheric Gas Mixtures

Differential optical absorption spectroscopy (DOAS) is a powerful tool for detecting and quantifying trace gases in atmospheric chemistry \cite{Platt_Stutz08}. DOAS spectra consist of a linear combination of complex multi-peak multi-scale structures. Most DOAS analysis routines in use today are based on least squares techniques, for example, the approach developed in the 1970s uses polynomial fits to remove a slowly varying background, and known reference spectra to retrieve the identity and concentrations of reference gases. An open problem is to identify unknown gases in the fitting residuals for complex atmospheric mixtures. In this work, we develop a novel three step semi-blind source separation method. The first step uses a multi-resolution analysis to remove the slow-varying and fast-varying components in the DOAS spectral data matrix $X$. The second step decomposes the preprocessed data $\hat{X}$ in the first step into a linear combination of the reference spectra plus a remainder, or $\hat{X} = A\,S + R$, where columns of matrix $A$ are known reference spectra, and the matrix $S$ contains the unknown non-negative coefficients that are proportional to concentration. The second step is realized by a convex minimization problem $S = \mathrm{arg} \min \mathrm{norm}\,(\hat{X} - A\,S)$, where the norm is a hybrid $\ell_1/\ell_2$ norm (Huber estimator) that helps to maintain the non-negativity of $S$. The third step performs a blind independent component analysis of the remainder matrix $R$ to extract remnant gas components. We first illustrate the proposed method in processing a set of DOAS experimental data by a satisfactory blind extraction of an a-priori unknown trace gas (ozone) from the remainder matrix. Numerical results also show that the method can identify multiple trace gases from the residuals.

math.NA↗

Fluorescence Efficiency and Visible Re-emission Spectrum of Tetraphenyl Butadiene Films at Extreme Ultraviolet Wavelengths

A large number of current and future experiments in neutrino and dark matter detection use the scintillation light from noble elements as a mechanism for measuring energy deposition. The scintillation light from these elements is produced in the extreme ultraviolet (EUV) range, from 60 - 200 nm. Currently, the most practical technique for observing light at these wavelengths is to surround the scintillation volume with a thin film of Tetraphenyl Butadiene (TPB) to act as a fluor. The TPB film absorbs EUV photons and reemits visible photons, detectable with a variety of commercial photosensors. Here we present a measurement of the re-emission spectrum of TPB films when illuminated with 128, 160, 175, and 250 nm light. We also measure the fluorescence efficiency as a function of incident wavelength from 120 to 250 nm.

astro-ph.IM↗

Correlation of conductivity and angle integrated valence band photoemission characteristics in single crystal iron perovskites for 300 K < T < 800 K: Comparison of surface and bulk sensitive methods

A single crystal monolith of La0.9Sr0.1FeO3 and thin pulsed laser deposited film of La0.8Sr0.2Fe0.8Ni0.2O3 were subject to angle integrated valence band photoemission spectroscopy in ultra high vacuum and conductivity experiments in ambient air at temperatures from 300 K to 800 K. Except for several sputtering and annealing cycles, the specimen were not prepared in-situ.. Peculiar changes in the temperature dependent, bulk representative conductivity profile as a result of reversible phase transitions, and irreversible chemical changes are semi-quantitatively reflected by the intensity variation in the more surface representative valence band spectra near the Fermi energy. X-ray photoelectron diffraction images reflect the symmetry as expected from bulk iron perovskites. The correlation of spectral details in the valence band photoemission spectra (VB PES) and details of the conductivity during temperature variation suggest that valuable information on electronic structure and transport properties of complex materials may be obtained without in-situ preparation.

cond-mat.str-el↗

Correlation of high temperature X-ray photoemission spectral features and conductivity of epitaxially strained (La0.8Sr0.2)0.95Ni0.2Fe0.8O3/SrTiO3(110)

Reversible and irreversible discontinuities at around 573 K and 823 K in the electric conductivity of a strained 175 nm thin film of (La0.8Sr0.2)0.95Ni0.2Fe0.8O3-δ grown by pulsed laser deposition on SrTiO3 (110) are reflected by valence band changes as monitored in photoemission and oxygen K-edge x-ray absorption spectra. The irreversible jump at 823 K is attributed to depletion of doped electron holes and reduction of Fe4+ to Fe3+, as evidenced by oxygen and iron core level soft x-ray spectroscopy, and possibly of a chemical origin, whereas the reversible jump at 573 K possibly originates from structural changes.

cond-mat.str-el↗