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Y. Tokura

Publications and source records attributed to Y. Tokura.

At least 343 records · Page 19Linked to original sources
arXiv2000

Fermi surface of Sr2RuO4 from angle resolved photoemission

We investigated the low-energy electronic structure of Sr2RuO4 by angle-resolved photoemission spectroscopy (ARPES) focusing, in particular, on the controversial issues of the Fermi surface (FS) topology and of the extended van Hove singularity (evHs). A detailed study of temperature and photon energy dependence demonstrates the surface-state nature of the electronic band responsible for the evHs, and may suggest the presence of ferromagnetic correlations at the surface. In addition, we detected a replica of the primary FS that indicates a (sqrt2 x sqrt2) surface reconstruction, as confirmed by LEED. In light of these findings, the FS determined by ARPES is consistent with LDA and de Haas-van Alphen (dHvA) results, and it provides additional information on the detailed shape of the alpha, beta and gamma sheets. Also, at this stage, because of the strong sensitivity of the cleaved surface, we could not find any robust signature of the crossover from 2D to 3D Fermi liquid behavior in our ARPES measurements for T<130 K.

cond-mat.str-el↗
arXiv2000

Superconducting Gap Anisotropy in Nd$_{1.85}$Ce$_{0.15}$CuO$_4$: Results from Photoemission

We have performed angle resolved photoelectron spectroscopy on the electron doped cuprate superconductor Nd$_{1.85}$Ce$_{0.15}$CuO$_4$. A comparison of the leading edge midpoints between the superconducting and normal states reveals a small, but finite shift of 1.5-2 meV near the ($π$,0) position, but no observable shift along the zone diagonal near ($π$/2,$π$/2). This is interpreted as evidence for an anisotropic superconducting gap in the electron doped materials, which is consistent with the presence of d-wave superconducting order in this cuprate superconductor.

cond-mat.supr-con↗
arXiv2000

Correlated Polarons in Dissimilar Perovskite Manganites

We report x-ray scattering studies of broad peaks located at a (0.5 0 0)/(0 0.5 0)-type wavevector in the paramagnetic insulating phases of La_{0.7}Ca_{0.3}MnO_{3} and Pr_{0.7}Ca_{0.3}MnO_{3}. We interpret the scattering in terms of correlated polarons and measure isotropic correlation lengths of 1-2 lattice constants in both samples. Based on the wavevector and correlation lengths, the correlated polarons are found to be consistent with CE-type bipolarons. Differences in behavior between the samples arise as they are cooled through their respective transition temperatures and become ferromagnetic metallic (La_{0.7}Ca_{0.3}MnO_{3}) or charge and orbitally ordered insulating (Pr_{0.7}Ca_{0.3}MnO_{3}). Since the primary difference between the two samples is the trivalent cation size, these results illustrate the robust nature of the correlated polarons to variations in the relative strength of the electron-phonon coupling, and the sensitivity of the low-temperature ground state to such variations.

cond-mat.str-el↗
arXiv2000

Spin Dynamics and Orbital State in LaTiO_3

A neutron scattering study of the Mott-Hubbard insulator LaTiO$_{3}$ (T$_{\rm N}=132$ K) reveals a spin wave spectrum that is well described by a nearest-neighbor superexchange constant $J=15.5$ meV and a small Dzyaloshinskii-Moriya interaction ($D=1.1$ meV). The nearly isotropic spin wave spectrum is surprising in view of the absence of a static Jahn-Teller distortion that could quench the orbital angular momentum, and it may indicate strong orbital fluctuations. A resonant x-ray scattering study has uncovered no evidence of orbital order in LaTiO$_{3}$.

cond-mat.str-el↗
arXiv2000

Fermi Surface, Surface States, and Surface Reconstruction in Sr2RuO4

The electronic structure of Sr2RuO4 is investigated by high angular resolution ARPES at several incident photon energies. We address the controversial issues of the Fermi surface (FS) topology and of the van Hove singularity at the M point, showing that a surface state and the replica of the primary FS due to (sqrt2 x sqrt2) surface reconstruction are responsible for previous conflicting interpretations. The FS thus determined by ARPES is consistent with the de Haas-van Alphen results, and it provides additional information on the detailed shape of the alpha, beta and gamma sheets.

cond-mat.str-el↗
arXiv2000

Short-range polaron correlations in the ferromagnetic La(1-x)Ca(x)MnO(3)

We use neutron scattering to demonstrate the presence of lattice polarons and their short-range correlations for several samples of La$_{1-x}$Ca$_x$MnO$_3$ in the Ca doping range $0.15\leq x\leq 0.3$. We establish the doping dependence of the orientation, commensuration, and coherence length of the polaron correlations and show that the populations of correlated and uncorrelated polarons are intimately related to the transport properties of the materials.

cond-mat.str-el↗
arXiv2000

X-ray Resonant Scattering Studies of Orbital and Charge Ordering in Pr$_{1-x}$Ca$_x$MnO$_3$

We present the results of a systematic x-ray scattering study of the charge and orbital ordering in the manganite series Pr$_{1-x}$Ca$_x$MnO$_3$ with $x$=0.25, 0.4 and 0.5. The temperature dependence of the scattering at the charge and orbital wavevectors, and of the lattice constants, was characterized throughout the ordered phase of each sample. It was found that the charge and orbital order wavevectors are commensurate with the lattice, in striking contrast to the results of earlier electron diffraction studies of samples with $x$=0.5. High momentum-transfer resolution studies of the x=0.4 and 0.5 samples further revealed that while long-range charge order is present, long-range orbital order is never established. Above the charge/orbital ordering temperature T$_o$, the charge order fluctuations are more highly correlated than the orbital fluctuations. This suggests that charge order drives orbital order in these samples. In addition, a longitudinal modulation of the lattice with the same periodicity as the charge and orbital ordering was discovered in the x=0.4 and 0.5 samples. For x=0.25, only long-range orbital order was observed with no indication of charge ordering, nor of an additional lattice modulation. We also report the results of a preliminary investigation of the loss of charge and orbital ordering in the x=0.4 sample by application of a magnetic field. Finally, the polarization and azimuthal dependence of the charge and orbital ordering in these compounds is characterized both in the resonant and nonresonant limits, and compared with the predictions of current theories. The results are qualitatively consistent with both cluster and LDA+U calculations of the electronic structure.

cond-mat.str-el↗
arXiv2000

Ultrafast spin dynamics and critical behavior in half-metallic ferromagnet : Sr_2FeMoO_6

Ultrafast spin dynamics in ferromagnetic half-metallic compound Sr_2FeMoO_6 is investigated by pump-probe measurements of magneto-optical Kerr effect. Half-metallic nature of this material gives rise to anomalous thermal insulation between spins and electrons, and allows us to pursue the spin dynamics from a few to several hundred picoseconds after the optical excitation. The optically detected magnetization dynamics clearly shows the crossover from microscopic photoinduced demagnetization to macroscopic critical behavior with universal power law divergence of relaxation time for wide dynamical critical region.

cond-mat.str-el↗
arXiv2000

Ultrafast optical nonlinearity in quasi-one-dimensional Mott-insulator ${\rm Sr_2CuO_3}$

We report strong instantaneous photoinduced absorption (PA) in the quasi-one-dimensional Mott insulator ${\rm Sr_2CuO_3}$ in the IR spectral region. The observed PA is to an even-parity two-photon state that occurs immediately above the absorption edge. Theoretical calculations based on a two-band extended Hubbard model explains the experimental features and indicates that the strong two-photon absorption is due to a very large dipole-coupling between nearly degenerate one- and two-photon states. Room temperature picosecond recovery of the optical transparency suggests the strong potential of ${\rm Sr_2CuO_3}$ for all-optical switching.

cond-mat.str-el↗
arXiv2000

Breakdown of the lattice polaron picture in La0.7Ca0.3MnO3 single crystals

When heated through the magnetic transition at Tc, La0.7Ca0.3MnO3 changes from a band metal to a polaronic insulator. The Hall constant R_H, through its activated behavior and sign anomaly, provides key evidence for polaronic behavior. We use R_H and the Hall mobility to demonstrate the breakdown of the polaron phase. Above 1.4Tc, the polaron picture holds in detail, while below, the activation energies of both R_H and the mobility deviate strongly from their polaronic values. These changes reflect the presence of metallic, ferromagnetic fluctuations, in the volume of which the Hall effect develops additional contributions tied to quantal phases.

cond-mat.str-el↗
arXiv2000

Charge and spin ordering in Nd{1/3}Sr{2/3}FeO{3}

We have investigated the charge and spin ordering in Nd{1/3}Sr{2/3}FeO{3} with neutron diffraction technique. This sample undergoes a charge ordering transition accompanying charge disproportionation of 2Fe4+ -> Fe3+ + Fe5+. We measured the superlattice reflections due to the charge and spin ordering, and confirmed that charges and spins order simultaneously at Tco = 185 K. The ordering pattern of charges and spins in this sample can be viewed as three dimensional stripe order, and is compared with two dimensional stripe order observed in other transition metal oxides.

cond-mat.str-el↗
arXiv2000

Direct Coulomb and Exchange Interaction in Artificial Atoms

We determine the contributions from the direct Coulomb and exchange interactions to the total interaction in semiconductor artificial atoms. We tune the relative strengths of the two interactions and measure them as a function of the number of confined electrons. We find that electrons tend to have parallel spins when they occupy nearly degenerate single-particle states. We use a magnetic field to adjust the single-particle state degeneracy, and find that the spin-configurations in an arbitrary magnetic field are well explained in terms of two-electron singlet and triplet states.

cond-mat.mes-hall↗
arXiv1999

Photoemission Spectral Weight Transfer and Mass Renormalization in the Fermi-Liquid System La$_{1-x}$Sr$_x$TiO$_{3+y/2}$

We have performed a photoemission study of La$_{1-x}$Sr$_x$TiO$_{3+y/2}$ near the filling-control metal-insulator transition (MIT) as a function of hole doping. Mass renormalization deduced from the spectral weight and the width of the quasi-particle band around the chemical potential $μ$ is compared with that deduced from the electronic specific heat. The result implies that, near the MIT, band narrowing occurs strongly in the vicinity of $μ$. Spectral weight transfer occurs from the coherent to the incoherent parts upon antiferromagnetic ordering, which we associate with the partial gap opening at $μ$.

cond-mat.str-el↗
arXiv1999

Temperature-Dependent Pseudogaps in Colossal Magnetoresistive Oxides

Direct electronic structure measurements of a variety of the colossal magnetoresistive oxides show the presence of a pseudogap at the Fermi energy E_F which drastically suppresses the electron spectral function at E_F. The pseudogap is a strong function of the layer number of the samples (sample dimensionality) and is strongly temperature dependent, with the changes beginning at the ferromagnetic transition temperature T_c. These trends are consistent with the major transport trends of the CMR oxides, implying a direct relationship between the pseudogap and transport, including the "colossal" conductivity changes which occur across T_c. The k-dependence of the temperature-dependent effects indicate that the pseudogap observed in these compounds is not due to the extrinsic effects proposed by Joynt.

cond-mat.str-el↗
arXiv1999

Persistent X-Ray Photoconductivity and Percolation of Metallic Clusters in Charge-Ordered Manganites

Charge-ordered manganites of composition $\rm Pr_{1-x}(Ca_{1-y}Sr_{y})_{x}MnO_3$ exhibit persistent photoconductivity upon exposure to x-rays. This is not always accompanied by a significant increase in the {\it number} of conduction electrons as predicted by conventional models of persistent photoconductivity. An analysis of the x-ray diffraction patterns and current-voltage characteristics shows that x-ray illumination results in a microscopically phase separated state in which charge-ordered insulating regions provide barriers against charge transport between metallic clusters. The dominant effect of x-ray illumination is to enhance the electron {\it mobility} by lowering or removing these barriers. A mechanism based on magnetic degrees of freedom is proposed.

cond-mat.mtrl-sci↗
arXiv1999

Charge ordering and chemical potential shift in La$_{2-x}$Sr$_x$NiO$_4$ studied by photoemission spectroscopy

We have studied the chemical potential shift in La$_{2-x}$Sr$_x$NiO$_4$ and the charge ordering transition in La$_{1.67}$Sr$_{0.33}$NiO$_4$ by photoemission spectroscopy. The result shows a large ($\sim$ 1 eV/hole) downward shift of the chemical potential with hole doping in the high-doping regime ($δ\gtrsim$ 0.33) while the shift is suppressed in the low-doping regime ($δ\lesssim$ 0.33). This suppression is attributed to a segregation of doped holes on a microscopic scale when the hole concentration is lower than $δ\simeq 1/3$. In the $δ= 1/3$ sample, the photoemission intensity at the chemical potential vanishes below the charge ordering transition temperature $T_{\rm CO}=$ 240 K.

cond-mat.str-el↗
arXiv1999

Interplay between charge, orbital and magnetic order in Pr_{1-x}Ca_xMnO_3

We report resonant x-ray scattering studies of charge and orbital order in Pr_{1-x}Ca_{x}MnO_3 with x=0.4 and 0.5. Below the ordering temperature, T_O=245 K, the charge and orbital order intensities follow the same temperature dependence, including an increase at the antiferromagnetic ordering temperature, T_N. High resolution measurements reveal, however, that long range orbital order is never achieved. Rather, an orbital domain state is formed. Above T_O, the charge order fluctuations are more highly correlated than the orbital fluctuations. Similar phenomenology is observed in a magnetic field. We conclude that the charge order drives the orbital order at the transition.

cond-mat.str-el↗