SearcharxivSearch

arXiv subjects

Yaakov Kleeorin

Publications and source records attributed to Yaakov Kleeorin.

9 recordsLinked to original sources

Entropic signatures of the single-impurity Kondo state

The Kondo singlet---a many-body state formed by entanglement between a localized spin and the Fermi sea---has been studied extensively through its transport signatures in quantum dots. Here we report a thermodynamic measurement of the entropy suppression associated with the formation of the Kondo singlet, using temperature-dependent charge sensing and a Maxwell relation to track the suppression of spin entropy as the first electron is added to a strongly-coupled GaAs quantum dot. Plotting $dN/dT$ against the simultaneously measured occupation $N$ reveals an asymmetric lineshape with its peak shifted to $N>1/2$---a hallmark of Kondo screening---that weakens with increasing temperature and is qualitatively reproduced by numerical renormalization group (NRG) calculations, with a small but persistent offset to lower occupation relative to the theory. An independent measurement of conductance versus occupation on the same device provides a test of these quantities through the mixed-valence crossover and matches NRG within experimental uncertainty.

cond-mat.mes-hall

Remote entropy measurement in coupled quantum dots

Recent experiments have demonstrated that measurements of the entropy change associated with the addition of electrons to semiconductor- and graphene-based quantum dots accurately quantify the spin and orbital degeneracy of the states into which they are added. However, measuring more exotic entropies requires probing the entropy change of an entire system in response to an added particle. Here, we demonstrate that Maxwell relation-based measurements probe not only the entropy change associated with the added electron but also that of the surrounding system as it responds to that electron. Using a pair of capacitively coupled GaAs quantum dots, we show that charge measurements on one dot reveal entropy changes associated with the entire two-dot system, both at weak dot--reservoir coupling where microstate counting applies and at stronger coupling where numerical renormalization group calculations are required.

cond-mat.mes-hall

Fractional entropy of multichannel Kondo systems from conductance-charge relations

Fractional entropy is a signature of nonlocal degrees of freedom, such as Majorana zero modes or more exotic non-Abelian anyons. Although direct experimental measurements remain challenging, Maxwell relations provide an indirect route to the entropy through charge measurements. Here we consider multichannel charge-Kondo systems, which are predicted to host exotic quasiparticles due to a frustration of Kondo screening at low temperatures. In the absence of experimental data for the charge occupation, we derive relations connecting the latter to the conductance, for which experimental results have recently been obtained. Our analysis indicates that Majorana and Fibonacci anyon quasiparticles are well-developed in existing two- and three-channel charge-Kondo devices, and that their characteristic $k_{\rm{B}}\log\sqrt{2}$ and $k_{\rm{B}}\log\frac{1+\sqrt{5}}{2}$ entropies are experimentally measurable.

cond-mat.mes-hall

Entropy measurement of a strongly coupled quantum dot

The spin 1/2 entropy of electrons trapped in a quantum dot has previously been measured with great accuracy, but the protocol used for that measurement is valid only within a restrictive set of conditions. Here, we demonstrate a novel entropy measurement protocol that is universal for arbitrary mesoscopic circuits and apply this new approach to measure the entropy of a quantum dot hybridized with a reservoir, where Kondo correlations dominate spin physics. The experimental results match closely to numerical renormalization group (NRG) calculations for small and intermediate coupling. For the largest couplings investigated in this work, NRG predicts a suppression of spin entropy at the charge transition due to the formation of a Kondo singlet, but that suppression is not observed in the experiment.

cond-mat.mes-hall

Kondo effect and spin-orbit coupling in graphene quantum dots

The Kondo effect is a cornerstone in the study of strongly correlated fermions. The coherent exchange coupling of conduction electrons to local magnetic moments gives rise to a Kondo cloud that screens the impurity spin. Whereas complete Kondo screening has been explored widely, realizations of the underscreened scenario - where only some of several Kondo channels participate in the screening - remain rare. Here we report the observation of fully screened and underscreened Kondo effects in quantum dots in bilayer graphene. More generally, we introduce a unique platform for studying Kondo physics. In contrast to carbon nanotubes, whose curved surfaces give rise to strong spin-orbit coupling breaking the SU(4) symmetry of the electronic states relevant for the Kondo effect, we study a nominally flat carbon material with small spin-orbit coupling. Moreover, the unusual two-electron triplet ground state in bilayer graphene dots provides a route to exploring the underscreened spin-1 Kondo effect.

cond-mat.mes-hall

How to measure the entropy of a mesoscopic system via thermoelectric transport

Entropy is a fundamental thermodynamic quantity indicative of the accessible degrees of freedom in a system. While it has been suggested that the entropy of a mesoscopic system can yield nontrivial information on emergence of exotic states, its measurement in such small electron-number system is a daunting task. Here we propose a method to extract the entropy of a Coulomb-blockaded mesoscopic system from transport measurements. We prove analytically and demonstrate numerically the applicability of the method to such a mesoscopic system of arbitrary spectrum and degeneracies. We then apply our procedure to measurements of thermoelectric response of a single quantum dot, and demonstrate how it can be used to deduce the entropy change across Coulomb-blockade valleys, resolving, along the way, a long-standing puzzle of the experimentally observed finite thermoelectric response at the apparent particle-hole symmetric point.

cond-mat.mes-hall

Quantum phase transition in a realistic double-quantum-dot system

Observing quantum phase transitions in mesoscopic systems is a daunting task, thwarted by the difficulty of experimentally varying the magnetic interactions, the typical driving force behind these phase transitions. Here we demonstrate that in realistic coupled double-dot systems, the level energy difference between the two dots, which can be easily tuned experimentally, can drive the system through a phase transition, when its value crosses the difference between the intra- and inter-dot Coulomb repulsion. Using the numerical renormalization group and the semi-analytic slave-boson mean-field theory, we study the nature of this phase transition, and demonstrate, by mapping the Hamiltonian into an even-odd basis, that indeed the competition between the dot level energy difference and the difference in repulsion energies governs the sign and magnitude of the effective magnetic interaction. The observational consequences of this transition are discussed.

cond-mat.str-el

Abrupt disappearance and reemergence of the SU(2) and SU(4) Kondo effects due to population inversion

The interplay of almost degenerate levels in quantum dots and molecular junctions with possibly different couplings to the reservoirs has lead to many observable phenomena, such as the Fano effect, transmission phase slips and the SU(4) Kondo effect. Here we predict a dramatic repeated disappearance and reemergence of the SU(4) and anomalous SU(2) Kondo effects with increasing gate voltage. This phenomenon is attributed to the level occupation switching which has been previously invoked to explain the universal transmission phase slips in the conductance through a quantum dot. We use analytical arguments and numerical renormalization group calculations to explain the observations and discuss their experimental relevance and dependence on the physical parameters.

cond-mat.str-el

Large Tunable Thermophase in Superconductor -- Quantum Dot -- Superconductor Josephson Junctions

In spite of extended efforts, detecting thermoelectric effects in superconductors have proven to be a challenging task, due to the inherent superconducting particle-hole symmetry. Here we present a theoretical study of an experimentally attainable Superconductor -- Quantum Dot -- Superconductor (SC-QD-SC) Josephson Junction with highly tunable thermoelectric properties and a thermal response that is far larger than previous suggestions. The QD energy level between the SCs breaks particle-hole symmetry in a gradual manner, allowing, in the presence of a temperature gradient, for gate controlled appearance of a superconducting thermo-phase. This thermo-phase increases up to a maximal value of $π/2$ after which thermovoltage is expected to develop. Using time-independent Keldysh countour Green's functions we derive the exact thermo-phase and thermal response on the junction. These are shown to be orders of magnitude larger than usual SC tunnel junctions with a sharp dependence on gate voltage.

cond-mat.mes-hall