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Yakov Bloch

Publications and source records attributed to Yakov Bloch.

8 recordsLinked to original sources

Chiral, Electronically Decoupled Layers of 1T'-WS2 Topological Insulator via Neutral-Molecule Intercalation

Monolayer 1T'-WS2 is predicted to be a two-dimensional topological insulator, but its intrinsic electronic properties are masked by strong interlayer coupling in its metallic and superconducting bulk parent phase, 2M-WS2. Isolating monolayers by mechanical exfoliation is also hindered by this coupling, preventing experimental examination of monolayer properties. Here we show that 2M-WS2 undergoes amine intercalation through a simple wet-chemical reaction, yielding superlattices in which the 1T' layers are structurally preserved but electronically decoupled by neutral molecular spacers. Intercalation expands the interlayer spacing from 0.5 to 1-4 nm and reconstructs the stacking while preserving the intralayer 1T' framework. Controlled (de)intercalation reversibly switches the system between a superconducting metal and an insulator with an activation gap matching that of the isolated monolayer. Density functional theory indicates that the electronically decoupled layers retain the nontrivial Z2 topology of the monolayer. Chiral amine intercalation further induces chiroptical activity in WS2 electronic transitions. Overall, the successful intercalation challenges the long-held view that group VIB dichalcogenides are inert toward neutral-molecule intercalation and demonstrates molecular intercalation as a general chemical route for realizing monolayer-like topological-insulator physics and enabling chiral van der Waals superlattices in bulk single crystals.

cond-mat.mtrl-sci

A Sliding Ferroelectric Resonant Tunnel Junction

Ferroelectric tunnel junctions (FTJs) leverage polarization-dependent tunneling through ultrathin barriers to enable two-terminal, non-volatile memory and logic. Although conceptually appealing, the practical implementation of conventional FTJs has been hindered by high coercive voltages, low readout currents, limited cycling endurance, and significant device-to-device variability. Here, we overcome these bottlenecks by introducing the sliding ferroelectric resonant tunnel (SFeRT) junction, integrating three cooperative mechanisms: (i) spontaneous interfacial polarization of atomically thin, depolarization-resilient barriers; (ii) superlubric sliding of shear-solitons, enabling ultra-low-friction, wear-free switching; and (iii) momentum-conserving, elastic resonant tunneling between lattice-aligned graphitic electrodes, providing sensitive readouts at both positive and negative biases. We demonstrate nanometer-scale SFeRT junctions using polar polytypes of hexagonal boron nitride (hBN) or transition metal dichalcogenides (TMDs) as barriers, achieving configurable writing voltages below $0.5$ V and tunable reading biases under $0.1$ V. These devices yield current densities exceeding $50$ nA $\mu$m$^{-2}$, with a robust room-temperature ON/OFF ratio $> 7$. The crystalline and polarization integrity of sliding van der Waals (vdW) polytypes, down to the atomically thin limit, ensures exceptional device uniformity and performance that remains scalable down to sub-$0.1$ $\mu$m$^{2}$ footprints. Furthermore, we provide a predictive model for SFeRT performance across diverse doping levels, temperatures, electrodes, and polytype configurations. Integrated within a Superlubric Array of Polytypes (SLAP) architecture, SFeRT junctions enable switching energies below $1$ fJ, establishing a scalable and durable foundation for low-energy ``slidetronic'' logic and memory.

cond-mat.other

Survival acceleration

Relativistic time dilation implies that an accelerating excited atom would have its lifetime prolonged in the lab frame. In this paper, we demonstrate a complementary effect: Longer-lived excited atoms turn out to have been accelerated. We propose the following experiment. An excited atom is prepared in a superposition of momenta. Due to relativistic time dilation, in the lab frame, the decay rate of components with higher momentum is diminished. As time passes without the atom emitting a photon, higher-momentum components become more probable. This results in a time-dependent shift of the expectation value of momentum. Taking into account first-order relativistic corrections, we calculate the force and acceleration undergone by the atom due to the fact that it did not emit a photon.

quant-ph

The time qubit

A spin precessing in a magnetic field is often used as a quantum clock, for example in tunneling-time measurements. We show that such a clock can exist in a coherent superposition of opposite temporal orientations, treating the arrow of time as a quantum two-level system. A Mach-Zehnder interferometer with equal and opposite magnetic fields provides a simple implementation, enabling interference between forward and backward evolution and Bell-type tests of temporal coherence. Extending the framework to relativistic dynamics reveals that the Dirac Hamiltonian describes an intrinsic coupling between a spin qubit and a time qubit, with matter and antimatter corresponding to opposite poles on the temporal Bloch sphere.

quant-ph

How the result of a measurement of a photon's mass can turn out to be 100

Bohmian mechanics has garnered significant attention as an interpretation of quantum theory since the paradigmatic experiments by Kocsis et. al. [Science 332, 6034 (2011)] and Mahler et. al. [Sci. Adv. 2, 2 (2016)], which inferred the average trajectories of photons in the nonrelativistic regime. These experiments were largely motivated by Wiseman's formulation of Bohmian mechanics, which grounded these trajectories in weak measurements. Recently, Wiseman's framework was extended to the relativistic regime by expressing the velocity field of single photons in terms of weak values of the photon energy and momentum. Here, we propose an operational, weak value-based definition for the Bohmian "local mass" of relativistic single particles. For relativistic wavefunctions satisfying the scalar Klein-Gordon equation, this mass coincides with the effective mass defined by de Broglie in his relativistic pilot-wave theory, a quantity closely connected with the quantum potential that is responsible for Bohmian trajectory self-bending and the anomalous photoelectric effect. We demonstrate the relationship between the photon trajectories and the mass in an interferometric setup.

quant-ph

Multi-Agent Distributed and Decentralized Geometric Task Allocation

We consider the general problem of geometric task allocation, wherein a large, decentralised swarm of simple mobile agents must detect the locations of tasks in the plane and position themselves nearby. The tasks are represented by an a priori unknown demand profile $Φ(x,y)$ that determines how many agents are needed in each location. The agents are autonomous, oblivious and indistinguishable, and have finite sensing range. They must configure themselves according to $Φ$ using only local information about $Φ$ and about the positions of nearby agents. All agents act according to the same local sensing-based rule of motion, and cannot explicitly communicate nor share information. We propose an optimization-based approach to the problem which results in attraction-repulsion dynamics. Repulsion encourages agents to spread out and explore the region so as to find the tasks, and attraction causes them to accumulate at task locations. We derive this approach via gradient descent over an appropriate ``error'' functional, and test it extensively through numerical simulations. The figures in this work are snapshots of simulations that can be viewed online at https://youtu.be/kyUiGYSaaoQ.

cs.MA

The identification of mean quantum potential with Fisher information leads to a strong uncertainty relation

The Cramer-Rao bound, satisfied by classical Fisher information, a key quantity in information theory, has been shown in different contexts to give rise to the Heisenberg uncertainty principle of quantum mechanics. In this paper, we show that the identification of the mean quantum potential, an important notion in Bohmian mechanics, with the Fisher information, leads, through the Cramer-Rao bound, to an uncertainty principle which is stronger, in general, than both Heisenberg and Robertson-Schrodinger uncertainty relations, allowing to experimentally test the validity of such an identification.

quant-ph

Quantum Hall response to time-dependent strain gradients in graphene

Mechanical deformations of graphene induce a term in the Dirac Hamiltonian which is reminiscent of an electromagnetic vector potential. Strain gradients along particular lattice directions induce local pseudomagnetic fields and substantial energy gaps as indeed observed experimentally. Expanding this analogy, we propose to complement the pseudomagnetic field by a pseudoelectric field, generated by a time dependent oscillating stress applied to a graphene ribbon. The joint Hall-like response to these crossed fields results in a strain-induced charge current along the ribbon. We analyze in detail a particular experimental implementation in the (pseudo) quantum Hall regime with weak intervalley scattering. This allows us to predict an (approximately) quantized Hall current which is unaffected by screening due to diffusion currents.

cond-mat.mes-hall