arXiv subjects

Yali Tian

Publications and source records attributed to Yali Tian.

6 recordsLinked to original sources

arXiv2026

Radiative Association of Ag and H: Formation of AgH from Ab Initio Calculations

Radiative association processes leading to the formation of AgH in cold astrophysical environments are investigated for the first time using full quantum scattering theory. High accuracy potential energy curves and transition dipole moments for the low-lying electronic states (X$^1\Sigma^+$, A$^1\Sigma^+$, $1^1\Pi$, $3^1\Sigma^+$, $2^1\Pi$) are computed employing the internally contracted multireference configuration interaction method with Davidson correction. Vibrationally and rotationally resolved radiative association cross sections are calculated for transitions from these initial states to the ground X$^1\Sigma^+$ state. Prominent shape resonances arising from quasi-bound rovibrational levels behind centrifugal barriers are identified, with the $2^1\Pi \to$ X$^1\Sigma^+$ channel exhibiting the strongest contribution at low collision energies. Stimulated radiative association under blackbody radiation fields (up to $T = 20\,000$ K) produces modest enhancements, predominantly in the ground-state channel. Thermal rate coefficients computed over 10$^{-1}$--$10^4$~K reveal a general decreasing trend with temperature for all channels. The results provide essential kinetic data for astrochemical models of transition-metal hydride formation in low-temperature interstellar and circumstellar environments.

physics.atom-ph↗

arXiv2022

A multi-band atomic candle with microwave-dressed Rydberg atoms

Stabilizing important physical quantities to atom-based standards lies at the heart of modern atomic, molecular and optical physics, and is widely applied to the field of precision metrology. Of particular importance is the atom-based microwave field amplitude stabilizer, the so-called atomic candle. Previous atomic candles are realized with atoms in their ground state, and hence suffer from the lack of frequency band tunability and small stabilization bandwidth, severely limiting their development and potential applications. To tackle these limitations, we employ microwave-dressed Rydberg atoms to realize a novel atomic candle that features multi-band frequency tunability and large stabilization bandwidth. We demonstrate amplitude stabilization of microwave field from C-band to Ka-band, which could be extended to quasi-DC and terahertz fields by exploring abundant Rydberg levels. Our atomic candle achieves stabilization bandwidth of 100 Hz, outperforming previous ones by more than two orders of magnitude. Our simulation indicates the stabilization bandwidth can be further increased up to 100 kHz. Our work paves a route to develop novel electric field control and applications with a noise-resilient, miniaturized, sensitive and broadband atomic candle.

physics.atom-ph↗

arXiv2020

Triply magic conditions for microwave transitions of optically trapped alkali-metal atoms

We report the finding of "triply magic" conditions (the doubly magic frequency-intensity conditions of an optical dipole trap plus the magic magnetic field) for the microwave transitions of optically trapped alkali-metal atoms. The differential light shift (DLS) induced by a degenerate two-photon process is adopted to compensate a DLS associated with the one-photon process. Thus, doubly magic conditions for the intensity and frequency of the optical trap beam can be found. Moreover, the DLS decouples from the magnetic field in a linearly polarized optical dipole trap, so that the magic condition of the magnetic field can be applied independently. Therefore, the "triply magic" conditions can be realized simultaneously. We also experimentally demonstrate the doubly magic frequency-intensity conditions as well as the independence of the magnetic field. When the triply magic conditions are fulfilled, the inhomogeneous and homogeneous decoherences for the optically trapped atom will be dramatically suppressed, and the coherence time can be extended significantly.

quant-ph↗

arXiv2019

High-numerical-aperture and long-working-distance objectives for single-atom experiments

We present two long-working-distance objective lenses with numerical apertures (NA) of 0.29 and 0.4 for single-atom experiments. The objective lenses are assembled entirely by the commercial on-catalog $Φ$1'' singlets. Both the objectives are capable to correct the spherical aberrations due to the standard flat vacuum glass windows with various thickness. The working distances of NA$=0.29$ and NA$=0.4$ objectives are 34.6 mm and 18.2 mm, respectively, at the design wavelength of 852 nm with 5-mm thick silica window. In addition, the objectives can also be optimized to work at diffraction limit at single wavelength in the entire visible and near infrared regions by slightly tuning the distance between the first two lenses. The diffraction limited fields of view for NA$=0.29$ and NA$=0.4$ objectives are 0.62 mm and 0.61 mm, and the spatial resolutions are 1.8 $μ$m and 1.3 $μ$m at the design wavelength. The performances are simulated by the commercial ray-tracing software and confirmed by imaging the resolution chart and a 1.18 $μ$m pinhole. The two objectives can be used for trapping and manipulating single atoms of various species.

physics.optics↗

arXiv2018

Measurement of complete and continuous Wigner functions for discrete atomic systems

We measure complete and continuous Wigner functions of a two-level cesium atom in both a nearly pure state and highly mixed states. We apply the method [T. Tilma et al., Phys. Rev. Lett. 117, 180401 (2016)] of strictly constructing continuous Wigner functions for qubit or spin systems. We find that the Wigner function of all pure states of a qubit has negative regions and the negativity completely vanishes when the purity of an arbitrary mixed state is less than $\frac{2}{3}$. We experimentally demonstrate these findings using a single cesium atom confined in an optical dipole trap, which undergoes a nearly pure dephasing process. Our method can be applied straightforwardly to multi-atom systems for measuring the Wigner function of their collective spin state.

quant-ph↗

arXiv2016

Loss-based Experimental Test of Bohr's Complementarity Principle with Single Neutral Atom

An experimental test of quantum complementarity principle based on single neutral atom trapped in a blue detuned bottle trap was here performed. A Ramsey interferometer was used to assess the wavelike behavior or particle-like behavior with second $π/2$-rotation on or off. The wavelike behavior or particle-like behavior is characterized by the visibility $V$ of the interference or the predictability $P$ of which-path information, respectively. The measured results fulfill the complementarity relation $P^2+V^2\leq1$. Imbalance losses were deliberately introduced to the stem and find the complementarity relation is then formally "violated." All the experimental results can be completely explained theoretically by quantum mechanics without considering the interference between wave and particle behaviors. This observation complements existing information concerning the BCP based on wave-particle duality of massive quantum.

quant-ph↗