arXiv subjects

Yanfeng Zhang

Publications and source records attributed to Yanfeng Zhang.

At least 91 records · Page 5Linked to original sources

arXiv2017

Spin-orbit interaction of light induced by transverse spin angular momentum engineering

We report the first demonstration of a direct interaction between the extraordinary transverse spin angular momentum in evanescent waves and the intrinsic orbital angular momentum in optical vortex beams. By tapping the evanescent wave of whispering gallery modes in a micro-ring-based optical vortex emitter and engineering the transverse spin state carried therein, a transverse-spin-to-orbital conversion of angular momentum is predicted in the emitted vortex beams. Numerical and experimental investigations are presented for the proof-of-principle demonstration of this unconventional interplay between the spin and orbital angular momenta, which could provide new possibilities and restrictions on the optical angular momentum manipulation techniques on the sub-wavelength scale. This phenomenon further gives rise to an enhanced spin-direction coupling effect in which waveguide or surface modes are unidirectional excited by incident optical vortex, with the directionality jointly controlled by spin-orbit states. Our results enrich the spin-orbit interaction phenomena by identifying a previously unknown pathway between the polarization and spatial degrees of freedom of light, and can enable a variety of functionalities employing spin and orbital angular momenta of light in applications such as communications and quantum information processing.

physics.optics↗

arXiv2017

Anomalous Hall effect and magnetic orderings in nanothick V$_5$S$_8$

The rise of graphene marks the advent of two-dimensional atomic crystals, which have exhibited a cornucopia of intriguing properties, such as the integer and fractional quantum Hall effects, valley Hall effect, charge density waves and superconductivity, to name a few. Yet, magnetism, a property of extreme importance in both science and technology, remains elusive. There is a paramount need for magnetic two-dimensional crystals. With the availability of many magnetic materials consisting of van der Waals coupled two-dimensional layers, it thus boils down to the question of how the magnetic order will evolve with reducing thickness. Here we investigate the effect of thickness on the magnetic ordering in nanothick V$_5$S$_8$. We uncover an anomalous Hall effect, by which the magnetic ordering in V$_5$S$_8$ down to 3.2 nm is probed. With decreasing thickness, a breakdown of antiferromagnetism is evident, followed by a spin-glass-like state. For thinnest samples, a weak ferromagnetic ordering emerges. The results not only show an interesting effect of reducing thickness on the magnetic ordering in a potential candidate for magnetic two-dimensional crystals, but demonstrate the anomalous Hall effect as a useful characterization tool for magnetic orderings in two-dimensional systems.

cond-mat.mes-hall↗

arXiv2017

Electron-Hole Symmetry Breaking in Charge Transport in Nitrogen-Doped Graphene

Graphitic nitrogen-doped graphene is an excellent platform to study scattering processes of massless Dirac fermions by charged impurities, in which high mobility can be preserved due to the absence of lattice defects through direct substitution of carbon atoms in the graphene lattice by nitrogen atoms. In this work, we report on electrical and magnetotransport measurements of high-quality graphitic nitrogen-doped graphene. We show that the substitutional nitrogen dopants in graphene introduce atomically sharp scatters for electrons but long-range Coulomb scatters for holes and, thus, graphitic nitrogen-doped graphene exhibits clear electron-hole asymmetry in transport properties. Dominant scattering processes of charge carriers in graphitic nitrogen-doped graphene are analyzed. It is shown that the electron-hole asymmetry originates from a distinct difference in intervalley scattering of electrons and holes. We have also carried out the magnetotransport measurements of graphitic nitrogen-doped graphene at different temperatures and the temperature dependences of intervalley scattering, intravalley scattering and phase coherent scattering rates are extracted and discussed. Our results provide an evidence for the electron-hole asymmetry in the intervalley scattering induced by substitutional nitrogen dopants in graphene and shine a light on versatile and potential applications of graphitic nitrogen-doped graphene in electronic and valleytronic devices.

cond-mat.mes-hall↗

arXiv2017

Metallic vanadium disulfide nanosheets as a platform material for multifunctional electrode applications

Nano-thick metallic transition metal dichalcogenides such as VS$_{2}$ are essential building blocks for constructing next-generation electronic and energy-storage applications, as well as for exploring unique physical issues associated with the dimensionality effect. However, such 2D layered materials have yet to be achieved through either mechanical exfoliation or bottom-up synthesis. Herein, we report a facile chemical vapor deposition route for direct production of crystalline VS$_{2}$ nanosheets with sub-10 nm thicknesses and domain sizes of tens of micrometers. The obtained nanosheets feature spontaneous superlattice periodicities and excellent electrical conductivities (~3$\times$10$^{3}$ S cm$^{-1}$), which has enabled a variety of applications such as contact electrodes for monolayer MoS$_{2}$ with contact resistances of ~1/4 to that of Ni/Au metals, and as supercapacitor electrodes in aqueous electrolytes showing specific capacitances as high as 8.6$\times$10$^{2}$ F g$^{-1}$. This work provides fresh insights into the delicate structure-property relationship and the broad application prospects of such metallic 2D materials.

cond-mat.mtrl-sci↗

arXiv2016

Design and optimization of optical modulators based on graphene-on-silicon nitride microring resonators

In order to overcome the challenge of obtaining high modulation depth due to weak graphene-light interaction, a graphene-on-silicon nitride (SiNx) microring resonator based on graphene's gate-tunable optical conductivity is proposed and studied. Geometrical parameters of graphene-on-SiNx waveguide are systematically analyzed and optimized, yielding a loss tunability of 0.04 dB/μm and an effective index variation of 0.0022. We explicitly study the interaction between graphene and a 40-μm-radius microring resonator, where electro-absorptive and electro-refractive modulation are both taken into account. By choosing appropriate graphene coverage and coupling coefficient, a high modulation depth of over 40 dB with large fabrication tolerance is obtained.

physics.optics↗

arXiv2016

Tailoring Accelerating Beams in Phase Space

An appropriate design of wavefront will enable light fields propagating along arbitrary trajectories thus forming accelerating beams in free space. Previous ways of designing such accelerating beams mainly rely on caustic methods, which start from diffraction integrals and only deal with two-dimensional fields. Here we introduce a new perspective to construct accelerating beams in phase space by designing the corresponding Wigner distribution function (WDF). We find such a WDF-based method is capable of providing both the initial field distribution and the angular spectrum in need by projecting the WDF into the real space and the Fourier space respectively. Moreover, this approach applies to the construction of both two- and three-dimensional fields, greatly generalizing previous caustic methods. It may therefore open up a new route to construct highly-tailored accelerating beams and facilitate applications ranging from particle manipulation and trapping to optical routing as well as material processing.

physics.optics↗

arXiv2016

Transport properties of photonic topological insulators based on microring resonator array

An array of ring resonators specifically designed can perform as a topological insulator. We conduct simulations using both Tight-Binding Model (TBM) and Transfer Matrix Method (TMM) to analyze the transport properties of such optical structure, verifying the presence of robust topological edge states which is immune to disorder and defect. We have also made a comparison between these two methods, of which results suggesting that TBM is only applicable under weakly-coupling condition while TMM is more rigorous. Finally we compared the structure with common microring array and coupled resonator optical waveguide (CROW) to demonstrate that it has desired transmission properties with wide and flat spectral response.

physics.optics↗

arXiv2016

Generalised Hermite-Gaussian beams and mode transformations

Generalised Hermite-Gaussian modes (gHG modes), an extended notion of Hermite-Gaussian modes (HG modes), are formed by the summation of normal HG modes with a characteristic function $α$, which can be used to unite conventional HG modes and Laguerre-Gaussian modes (LG modes). An infinite number of normalised orthogonal modes can thus be obtained by modulation of the function $α$. The gHG mode notion provides a useful tool in analysis of the deformation and transformation phenomena occurring in propagation of HG and LG modes with astigmatic perturbation.

physics.optics↗

arXiv2016

Winding light beams along elliptical helical trajectories

Conventional caustic methods in real or Fourier space produced accelerating optical beams only with convex trajectories. We develop a superposition caustic method capable of winding light beams along non-convex trajectories. We ascertain this method by constructing a one-dimensional (1D) accelerating beam moving along a sinusoidal trajectory, and subsequently extending to two-dimensional (2D) accelerating beams along arbitrarily elliptical helical trajectories. We experimentally implement the method with a compact and robust integrated optics approach by fabricating micro-optical structures on quartz glass plates to perform the spatial phase and amplitude modulation to the incident light, generating beam trajectories highly consistent with prediction. The theoretical and implementation methods can in principle be extended to the construction of accelerating beams with a wide variety of non-convex trajectories, thereby opening up a new route of manipulating light beams for fundamental research and practical applications.

physics.optics↗

arXiv2015

i2MapReduce: Incremental MapReduce for Mining Evolving Big Data

As new data and updates are constantly arriving, the results of data mining applications become stale and obsolete over time. Incremental processing is a promising approach to refreshing mining results. It utilizes previously saved states to avoid the expense of re-computation from scratch. In this paper, we propose i2MapReduce, a novel incremental processing extension to MapReduce, the most widely used framework for mining big data. Compared with the state-of-the-art work on Incoop, i2MapReduce (i) performs key-value pair level incremental processing rather than task level re-computation, (ii) supports not only one-step computation but also more sophisticated iterative computation, which is widely used in data mining applications, and (iii) incorporates a set of novel techniques to reduce I/O overhead for accessing preserved fine-grain computation states. We evaluate i2MapReduce using a one-step algorithm and three iterative algorithms with diverse computation characteristics. Experimental results on Amazon EC2 show significant performance improvements of i2MapReduce compared to both plain and iterative MapReduce performing re-computation.

cs.DC↗

arXiv2015

Wafer-scale CVD Growth of Monolayer Hexagonal Boron Nitride with Large Domain Size by Cu Foil Enclosure Approach

Chemical vapor deposition synthesis of large domain hexagonal boron nitride (h-BN) with uniform thickness on Cu foils is of great challenge, originating from the extremely high nucleation densities and the reverse hydrogen etching competition reaction. We report herein the successful growth of wafer-scale high-quality h-BN monolayer film with the largest single crystalline domain sizes up to 72 micrometer in edge length using a folded Cu enclosure approach. The highly-confined growth space with this facile and unique approach enables the drastic decrease of nucleation centers together with the effective suppression of hydrogen etching reaction. It is revealed, for the first time, that the orientations of as-grown h-BN monolayers are strongly correlated with the crystalline facets of growth substrates, with the Cu (111) being the best substrate for growing high-quality single crystalline h-BN monolayer, consistent with the density functional theory calculations. The present study offers a practical pathway for growing high-quality h-BN films and deepens the fundamental understanding of h-BN growth process.

cond-mat.mtrl-sci↗

arXiv2015

Etching-free transfer of wafer-scale MoS2 films

How to transfer MoS2 films from growth substrates onto target substrates is a critical issue for its practical applications. However, it remains a great challenge to avoid the sample degradation and substrate destruction, since current transfer method inevitably employs a wet chemical etching process. Herein, we develop an etching-free transfer method for transferring wafer-scale MoS2 films onto arbitrary substrates by using ultrasonication. Briefly, the collapse of ultrasonication-generated microbubbles at the interface between polymer-coated MoS2 film and substrates induce sufficient force to delaminate the MoS2 films. Using this method the MoS2 films can be transferred from all the substrates (silica, mica, strontium titanate, sapphire) and remains the original sample morphology and quality. This method guarantees a simple transfer process, allows the reuse of growth substrates, without the presence of any hazardous etchants. The etching-free transfer method may promote the broad applications of MoS2 in electronics, optoelectronics and catalysis.

cond-mat.mtrl-sci↗

arXiv2014

Ultrafast Terahertz Probe of Transient Evolution of Charged and Neutral Phase of Photoexcited Electron-hole Gas in Monolayer Semiconductor

We investigate the dynamical formation of excitons from photoexcited electron-hole plasma and its subsequent decay dynamics in monolayer MoS2 grown by chemical vapor deposition using ultrafast pump and terahertz probe spectroscopy. Different photoexcited electron-hole states are resolved based on their distinct responses to THz photon and decay lifetime. The observed transient THz transmission can be fit with two decay components: a fast component with decay lifetime of 20 ps, which is attributed to exciton life time including the exciton formation and subsequent intraexciton relaxation; a slow component with extremely long decay lifetime of several ns due to either localized exciton state or a long live dark exciton state which is uncovered for the first time. The relaxation dynamics is further verified by temperature and pump fluence dependent studies of the decay time constants.

cond-mat.mtrl-sci↗

arXiv2014

Ultrafast Charge Transfer in Atomically Thin MoS2/WS2 Heterostructures

Van der Waals heterostructures have recently emerged as a new class of materials, where quantum coupling between stacked atomically thin two-dimensional (2D) layers, including graphene, hexagonal-boron nitride, and transition metal dichalcogenides (MX2), give rise to fascinating new phenomena. MX2 heterostructures are particularly exciting for novel optoelectronic and photovoltaic applications, because 2D MX2 monolayers can have an optical bandgap in the near-infrared to visible spectral range and exhibit extremely strong light-matter interactions. Theory predicts that many stacked MX2 heterostructures form type-II semiconductor heterojunctions that facilitate efficient electron-hole separation for light detection and harvesting. Here we report the first experimental observation of ultrafast charge transfer in photo-excited MoS2/WS2 heterostructures using both photoluminescence mapping and femtosecond (fs) pump-probe spectroscopy. We show that hole transfer from the MoS2 layer to the WS2 layer takes place within 50 fs after optical excitation, a remarkable rate for van der Waals coupled 2D layers. Such ultrafast charge transfer in van der Waals heterostructures can enable novel 2D devices for optoelectronics and light harvesting.

cond-mat.mes-hall↗

arXiv2014

Quasi-freestanding monolayer heterostructure of graphene and hexagonal boron nitride on Ir(111) with a chiral boundary

Monolayer lateral heterostructure of graphene and hexagonal boron nitride (h-BNC) has attracted a growing attention mainly due to its tunable band-gap character and unique physical properties at interface. Hereby, we reported the first-time synthesis of a nearly freestanding h-BNC hybrid on a weakly coupled substrate of Ir (111), where graphene and h-BN possessing different surface heights and corrugations formed a perfect monolayer hybrid. With the aid of scanning tunneling microscopy/spectroscopy (STM/STS), we demonstrated that h-BN can patch alongside the boundary of pre-deposited graphene domains and vice versa to form a seamless monolayer hybrid, with the realization of predominant zigzag type chiral boundaries at the interface. Density-functional theory calculations and STM/STS measurements aided us to reveal that this interface between graphene and h-BN were atomically sharp in aspects of the chemical bonding as well as the local electronic property from both theoretical and experimental points of view.

physics.chem-ph↗

arXiv2014

Directly grown monolayer MoS2 on Au foils as efficient hydrogen evolution catalysts

Synthesis of monolayer MoS2 is essential for fulfilling the potential of MoS2 in catalysis, optoelectronics and valleytronics, etc. Herein, we report for the first time the scalable growth of high quality, domain size tunable (edge length from ~ 200 nm to 50 μm), strictly monolayer MoS2 on commercially available Au foils, via a low pressure chemical vapor deposition method. The nanosized triangular MoS2 flakes on Au foils was proved to be an excellent electrocatalyst for hydrogen evolution reaction (HER), featured by a rather low Tafel slope (61 mV/decade) and a supreme exchange current density (38.1 μA/cm2). The abundant active edge sites and the excellent electron coupling between MoS2 and Au foils account for the extraordinary HER activity. Our work presents a sound proof that strictly monolayer MoS2 assembled on a well selected electrode can manifest comparable or even superior HER property than that of nanoparticles or few-layer MoS2 electrocatalyst.

cond-mat.mtrl-sci↗

arXiv2013

Electronic Structures of Graphene Layers on Metal Foil: Effect of Point Defects

Here we report a facile method to generate a high density of point defects in graphene on metal foil and show how the point defects affect the electronic structures of graphene layers. Our scanning tunneling microscopy (STM) measurements, complemented by first principle calculations, reveal that the point defects result in both the intervalley and intravalley scattering of graphene. The Fermi velocity is reduced in the vicinity area of the defect due to the enhanced scattering. Additionally, our analysis further points out that periodic point defects can tailor the electronic properties of graphene by introducing a significant bandgap, which opens an avenue towards all-graphene electronics.

cond-mat.mes-hall↗

arXiv2013

Strain Induced One-Dimensional Landau-Level Quantization in Corrugated Graphene

Theoretical research has predicted that ripples of graphene generates effective gauge field on its low energy electronic structure and could lead to zero-energy flat bands, which are the analog of Landau levels in real magnetic fields. Here we demonstrate, using a combination of scanning tunneling microscopy and tight-binding approximation, that the zero-energy Landau levels with vanishing Fermi velocities will form when the effective pseudomagnetic flux per ripple is larger than the flux quantum. Our analysis indicates that the effective gauge field of the ripples results in zero-energy flat bands in one direction but not in another. The Fermi velocities in the perpendicular direction of the ripples are not renormalized at all. The condition to generate the ripples is also discussed according to classical thin-film elasticity theory.

cond-mat.mes-hall↗