arXiv subjects

Yang Qi

Publications and source records attributed to Yang Qi.

At least 91 records · Page 5Linked to original sources

arXiv2021

Evidences for the random singlet phase in a new honeycomb iridate SrIr$_2$O$_{6-δ}$

Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real materials$-$disorders$-$has been much less studied in Kitaev systems. Here we synthesized a trigonal SrIr$_2$O$_{6-δ}$ with $δ\approx 0.25$, which consists of two-dimensional honeycomb Ir planes with edge-sharing IrO$_6$ octahedra. First-principles computation and experimental measurements suggest that the electronic system is gapped, and there should be no magnetic moment as the Ir$^{5+}$ ion has no unpaired electrons. However, significant magnetism has been observed in the material, and it can be attributed to disorders that are most likely from oxygen vacancies. No magnetic order is found down to 0.05 K, and the low-temperature magnetic properties exhibit power-law behaviors in magnetic susceptibility and zero-field specific heat, and a single-parameter scaling of the specific heat under magnetic fields. These results provide strong evidence for the existence of the random singlet phase in SrIr$_2$O$_{6-δ}$, which offers a different member to the family of spin-orbital entangled iridates and Kitaev materials.

cond-mat.str-el↗

arXiv2021

Generalized Lieb-Schultz-Mattis theorem on bosonic symmetry protected topological phases

We propose and prove a family of generalized Lieb-Schultz-Mattis (LSM) theorems for symmetry protected topological (SPT) phases on boson/spin models in any dimensions. The "conventional" LSM theorem, applicable to e.g. any translation invariant system with an odd number of spin-1/2 particles per unit cell, forbids a symmetric short-range-entangled ground state in such a system. Here we focus on systems with no LSM anomaly, where global/crystalline symmetries and fractional spins within the unit cell ensure that any symmetric SRE ground state must be a nontrivial SPT phase with anomalous boundary excitations. Depending on models, they can be either strong or "higher-order" crystalline SPT phases, characterized by nontrivial surface/hinge/corner states. Furthermore, given the symmetry group and the spatial assignment of fractional spins, we are able to determine all possible SPT phases for a symmetric ground state, using the real space construction for SPT phases based on the spectral sequence of cohomology theory. We provide examples in one, two and three spatial dimensions, and discuss possible physical realization of these SPT phases based on condensation of topological excitations in fractionalized phases.

cond-mat.str-el↗

arXiv2021

Fermi arcs and pseudogap in a lattice model of a doped orthogonal metal

Since the discovery of the pseudogap and Fermi arc states in underdoped cuprates, the understanding of such non-Fermi-liquid states and the associated violation of Luttinger's theorem have been the central theme in correlated electron systems. However, still lacking is a well-accepted theoretical framework to unambiguously explain these metallic states that are clearly beyond Landau's Fermi liquid and Luttinger's theorem of a Fermi surface and electron filling. Here, we design a lattice model of orthogonal metals with fermion and Ising matter fields coupled to topological order and, by solving the model via unbiased quantum Monte Carlo simulation at generic electron fillings, find that the system gives birth to phenomena of the Fermi arc and pseudogap in the single-particle spectrum that go beyond the Luttinger sum rule with broken Fermi surface but no symmetry breaking. The pseudogap and Fermi arcs coexist with a background of a deconfined Z2 gauge field, and we further find that the confinement transition of the gauge field triggers a superconductivity instability and that the hopping of the gauge-neutral fermions brings the "large" Fermi surface back from the Fermi arc state. Our unbiased numerical results provide a concrete model realization and theoretical framework for the coupling between gauge field and fermions and, in the process, generate the rich phenomena of the pseudogap, the Fermi arc, and superconductivity in generic correlated electron systems.

cond-mat.str-el↗

arXiv2021

Phase Diagram of Triangular Lattice Quantum Ising Model under External Field

Quantum Ising model on a triangular lattice hosts a finite temperature Berezinskii-Kosterlitz-Thouless (BKT) phase with emergent U(1) symmetry, and it will transit into an up-up-down (UUD) phase with $C_3$ symmetry breaking upon an infinitesimal external field along the longitudinal direction, but the overall phase diagram spanned by the axes of external field and temperature remains opaque due to the lack of systematic invesitgations with controlled methodologies. By means of quantum Monte Carlo at finite temperature and ground state density matrix renormalization group simulations, we map out the phase diagram of triangular quantum Ising model. Stemming from the upper BKT temperature at zero field, we obtain the phase boundary between the UUD and paramagnetic phases with its 2D $q=3$ Potts universality at weak field and weakly first order transition at strong field. Originated from the lower BKT temperature at zero field, we analyze the low temperature phase boundary between the clock phase and the UUD phase with Ising symmetry breaking at weak fields and the quantum phase transition between the UUD and fully polarized phases at strong fields. The accurate many-body numerical results are consistent with our field theoretical analysis. The experimental relevance towards the BKT magnet TmMgGaO$_4$ and programmable quantum simulators are also discussed.

cond-mat.str-el↗

arXiv2021

Topological phase transition and single/multi anyon dynamics of $Z_2$ spin liquid

Among the quantum many-body models that host anyon excitation and topological orders, quantum dimer models (QDM) provide a unique playground for studying the relation between single-anyon and multi-anyon continuum spectra. However, as the prototypical correlated system with local constraints, the generic solution of QDM at different lattice geometry and parameter regimes is still missing due to the lack of controlled methodologies. Here we obtain, via the newly developed sweeping cluster quantum Monte Carlo algorithm, the excitation spectra in different phases of the triangular lattice QDM. Our results reveal the single vison excitations inside the $Z_2$ quantum spin liquid (QSL) and its condensation towards the $\sqrt{12}\times\sqrt{12}$ valence bond solid (VBS), and demonstrate the translational symmetry fractionalization and emergent O(4) symmetry at the QSL-VBS transition. We find the single vison excitations, whose convolution qualitatively reproduces the dimer spectra, are not free but subject to interaction effects throughout the transition. The nature of the VBS with its O(4) order parameters are unearthed in full scope. Our approach opens the avenue for generic solution of the static and dynamic properties of QDMs and has relevance towards the realization and detection of fractional excitations in programmable quantum simulators.

cond-mat.str-el↗

arXiv2021

Vestigial anyon condensation in kagome quantum spin liquids

We construct a lattice model of topological order (kagome quantum spin liquids) and solve it with unbiased quantum Monte Carlo simulations. A three-stage anyon condensation with two transitions from a $\mathbb Z_2\boxtimes\mathbb Z_2$ topological order to a $\mathbb Z_2$ topological order and eventually to a trivial symmetric phase is revealed. These results provide concrete examples of phase transitions between topological orders in quantum magnets. The designed quantum spin liquid model and its numerical solution offer a playground for further investigations on vestigial anyon condensation.

cond-mat.str-el↗

arXiv2020

Coexistence of antiferromagnetism and topological superconductivity on the honeycomb lattice Hubbard model

Motivated by the recent numerical simulations for doped $t$-$J$ model on the honeycomb lattice, we study superconductivity of singlet and triplet pairing on the honeycomb lattice Hubbard model. We show that a superconducting state with coexisting spin-singlet and spin-triplet pairings is induced by the antiferromagnetic order near half filling. The superconducting state we obtain has a topological phase transition that separates a topologically trivial state and a nontrivial state with Chern number two. Possible experimental realization of such a topological superconductivity is also discussed.

cond-mat.str-el↗

arXiv2020

Evidence of the Berezinskii-Kosterlitz-Thouless Phase in a Frustrated Magnet

The Berezinskii-Kosterlitz-Thouless (BKT) mechanism, building upon proliferation of topological defects in 2D systems, is the first example of phase transition beyond the Landau-Ginzburg paradigm of symmetry breaking. Such a topological phase transition has long been sought yet undiscovered directly in magnetic materials. Here, we pin down two transitions that bound a BKT phase in an ideal 2D frustrated magnet TmMgGaO$_4$, via nuclear magnetic resonance under in-plane magnetic fields, which do not disturb the low-energy electronic states and allow BKT fluctuations to be detected sensitively. Moreover, by applying out-of-plane fields, we find a critical scaling behaviour of the magnetic susceptibility expected for the BKT transition. The experimental findings can be explained by quantum Monte Carlo simulations applied on an accurate triangular-lattice Ising model of the compound which hosts a BKT phase. These results provide a concrete example for the BKT phase and offer an ideal platform for future investigations on the BKT physics in magnetic materials.

cond-mat.str-el↗

arXiv2020

Evidence for the topological order in a kagome antiferromagnet

A Z2 quantum spin liquid hosts one of the simplest topological orders and exhibits many exotic properties due to long-range quantum entanglements. Its elementary excitations are anyons such as spinons carrying fractionalized spin quantum number and visons carrying emergent Z2 gauge flux. However, experimental detection of these anyons remains elusive. The difficulties lie not only in the fact that there exists few candidates for Z2 quantum spin liquids but also in that visons are magnetically inert hence immune to available experimental techniques. Here we have studied the spin excitations and specific heats of kagome-lattice antiferromagnet Cu$_4$(OH)$_6$FBr and Cu$_3$Zn(OH)$_6$FBr, which consists of two-dimensional Cu$^{2+}$ kagome layers with either Cu$^{2+}$ or Zn$^{2+}$ ions in between. By combining the first principle calculations and inelastic neutron scattering data in the former, we show that the dominate couplings in Cu$_4$(OH)$_6$FBr are between the nearest neighbor spins within the kagome planes, and the kagome and interlayer spin systems are essentially decoupled above the antiferromagnetic transition temperature. The intrinsic spin excitations and specific heats of the kagome layers for Cu$_3$Zn(OH)$_6$FBr are thus derived by removing the contributions from the residual interlayer Cu$^{2+}$ magnetic impurities. Accordingly, the kagome spin system exhibits spin continuum with momentum-dependent spin gap and a large magnetic entropy at low temperature that is insensitive to magnetic field, which can be understood as the evidences of spinons and visons in this kagome quantum spin liquid candidate. Our results suggest the existence of the Z2 anyons in the material, and therefore provide a comprehensive set of evidences for the Z2 topological order in kagome quantum spin liquid and bring their choreographed entanglement dances to the stage of real materials.

cond-mat.str-el↗

arXiv2020

Real-space recipes for general topological crystalline states

Topological crystalline states are short-range entangled states jointly protected by onsite and crystalline symmetries. While the non-interacting limit of these states, e.g., the topological crystalline insulators, have been intensively studied in band theory and have been experimentally discovered, the classification and diagnosis of their strongly interacting counterparts are relatively less well understood. Here we present a unified scheme for constructing all topological crystalline states, bosonic and fermionic, free and interacting, from real-space "building blocks" and "connectors". Building blocks are finite-size pieces of lower dimensional topological states protected by onsite symmetries alone, and connectors are "glue" that complete the open edges shared by two or multiple pieces of building blocks. The resulted assemblies are selected against two physical criteria we call the "no-open-edge condition" and the "bubble equivalence", which, respectively, ensure that each selected assembly is gapped in the bulk and cannot be deformed to a product state. The scheme is then applied to obtaining the full classification of bosonic topological crystalline states protected by several onsite symmetry groups and each of the 17 wallpaper groups in two dimensions and 230 space groups in three dimensions. We claim that our real-space recipes give the complete set of topological crystalline states for bosons and fermions, and prove the boson case analytically using a spectral sequence expansion of group cohomology.

cond-mat.str-el↗

arXiv2020

Universal Thermodynamics in the Kitaev Fractional Liquid

In the Kitaev honeycomb model, the quantum spin fractionalizes into itinerant Majorana and gauge flux spontaneously upon cooling, leading to rich experimental ramifications at finite temperature and an upsurge of research interest. In this work, we employ the exponential tensor renormalization group approach to explore the Kitaev model under various perturbations, including the external fields, Heisenberg, and the off-diagonal couplings that are common in the Kitaev materials. Through large-scale manybody calculations, we find a Kitaev fractional liquid at intermediate temperature that is robust against perturbations. The fractional liquid exhibits universal thermodynamic behaviors, including the fractional thermal entropy, metallic specific heat, and an intermediate-temperature Curie law of magnetic susceptibility. The emergent universal susceptibility behavior, with a modified Curie constant, can be ascribed to the strongly fluctuating $\mathbb{Z}_2$ fluxes as well as the extremely short-ranged and bond-directional spin correlations. With this insight, we revisit the susceptibility measurements of Na$_2$IrO$_3$ and $α$-RuCl$_3$, and find evident signatures of finite-temperature fractionalization and ferromagnetic Kitaev couplings. Moreover, the peculiar spin correlation in the fractional liquid corresponds to a stripy structure factor which rotates in the extended Brillouin zone as the spin component changes. Therefore, our findings encourage future experimental exploration of fractional liquid in the Kitaev materials by thermodynamic measurements and spin-resolved structure factor probes.

cond-mat.str-el↗

arXiv2020

DMFT reveals the non-Hermitian topology in heavy-fermion systems

We find that heavy fermion systems can have bulk "Fermi arcs", with the use of the non-Hermitian topological theory. In an interacting electron system, the microscopic many-body Hamiltonian is Hermitian, but the one-body quasiparticle Hamiltonian is non-Hermitian due to the finite quasiparticle lifetime. We focus on heavy electron systems as a stage of finite lifetime quasiparticles with two lifetimes, since quasiparticle lifetimes for f-electrons and c-electrons should be different. Two lifetimes induce exceptional points (EPs) of the non-Hermitian quasiparticle Hamiltonian matrix in momentum space. The line connecting between two EPs characterizes the bulk Fermi arcs. With the use of the dynamical mean field theory (DMFT) calculation, we confirm our statement in Kondo insulators with a momentum-dependent hybridization in two-dimensions. We show that the concept of the EPs in the non-Hermitian quasiparticle Hamiltonian is one of powerful tools to predict new phenomena in strongly correlated electron systems.

cond-mat.str-el↗

arXiv2020

Metal to Orthogonal Metal Transition

Orthogonal metal is a new quantum metallic state that conducts electricity but acquires no Fermi surface (FS) or quasiparticles, and hence orthogonal to the established paradigm of Landau's Fermi-liquid (FL). Such a state may hold the key of understanding the perplexing experimental observations of quantum metals that are beyond FL, i.e., dubbed non-Fermi-liquid (nFL), ranging from the Cu- and Fe-based oxides, heavy fermion compounds to the recently discovered twisted graphene heterostructures. However, to fully understand such an exotic state of matter, at least theoretically, one would like to construct a lattice model and to solve it with unbiased quantum many-body machinery. Here we achieve this goal by designing a 2D lattice model comprised of fermionic and bosonic matter fields coupled with dynamic $\mathbb Z_2$ gauge fields, and obtain its exact properties with sign-free quantum Monte Carlo simulations. We find that as the bosonic matter fields become disordered, with the help of deconfinement of the $\mathbb Z_2$ gauge fields, the system reacts with changing its nature from the conventional normal metal with an FS to an orthogonal metal of nFL without FS and quasiparticles and yet still responds to magnetic probe like an FL. Such a quantum phase transition from a normal metal to an orthogonal metal, with its electronic and magnetic spectral properties revealed, is calling for the establishment of new paradigm of quantum metals and their transition with conventional ones.

cond-mat.str-el↗

arXiv2020

Construction and classification of point group symmetry protected topological phases in 2D interacting fermionic systems

The construction and classification of symmetry-protected topological (SPT) phases in interacting bosonic and fermionic systems have been intensively studied in the past few years. Very recently, a complete classification and construction of space group SPT phases were also proposed for interacting bosonic systems. In this paper, we attempt to generalize this classification and construction scheme systematically into interacting fermion systems. In particular, we construct and classify point group SPT phases for 2D interacting fermion systems via lower-dimensional block-state decorations. We discover several intriguing fermionic SPT states that can only be realized in interacting fermion systems (i.e., not in free-fermion or bosonic SPT systems). Moreover, we also verify the recently conjectured crystalline equivalence principle for 2D interacting fermion systems. Finally, the potential experimental realization of these new classes of point group SPT phases in 2D correlated superconductors is addressed.

cond-mat.str-el↗

arXiv2020

Kosterlitz-Thouless Melting of Magnetic Order in the Triangular Quantum Ising Material TmMgGaO$_4$

Frustrated magnets host the promises of material realizations of new paradigm of quantum matter, while direct comparison of unbiased model calculations with experimental measurements is still very challenging. Here, we design and implement a protocol of employing many-body computation methodologies for accurate model calculation -- both equilibrium and dynamical properties -- of a frustrated rare-earth magnet TmMgGaO$_4$ (TMGO), which perfectly explains the corresponding experimental findings. Our results confirm TMGO is an ideal realization of triangular-lattice Ising model with an intrinsic transverse field. The magnetic order of TMGO is predicted to melt through two successive Kosterlitz-Thouless (KT) phase transitions, with a floating KT phase in between. The dynamical spectra calculated suggest remnant images of a vanishing magnetic stripe order that represent vortex-antivortex pairs, resembling rotons in a superfluid helium film. TMGO therefore constitutes a rare quantum magnet for realizing KT physics and we further propose experimental detections of its intriguing properties.

cond-mat.str-el↗

arXiv2020

Possible Kitaev Quantum Spin Liquid State in 2D Materials with S=3/2

Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static long-range-ordered magnetism. Such intriguing phenomena are not only of great fundamental relevance in themselves, but also hold the promise for quantum computing and quantum information. Among different types of QSLs, the exactly solvable Kitaev model is attracting much attention, with most proposed candidate materials, e.g., RuCl$_3$ and Na$_2$IrO$_3$, having an effective $S$=1/2 spin value. Here, via extensive first-principle-based simulations, we report the investigation of the Kitaev physics and possible Kitaev QSL state in epitaxially strained Cr-based monolayers, such as CrSiTe$_3$, that rather possess a $S$=3/2 spin value. Our study thus extends the playground of Kitaev physics and QSLs to 3$d$ transition metal compounds.

cond-mat.mtrl-sci↗

arXiv2020

Anomalous symmetry protected topological states in interacting fermion systems

The classification and construction of symmetry protected topological (SPT) phases have been intensively studied in interacting systems recently. To our surprise, in interacting fermion systems, there exists a new class of the so-called anomalous SPT (ASPT) states which are only well defined on the boundary of a trivial fermionic bulk system. We first demonstrate the essential idea by considering an anomalous topological superconductor with time reversal symmetry $T^2=1$ in 2D. The physical reason is that the fermion parity might be changed locally by certain symmetry action, but is conserved if we introduce a bulk. Then we discuss the layer structure and systematical construction of ASPT states in interacting fermion systems in 2D with a total symmetry $G_f=G_b\times\mathbb{Z}_2^f$. Finally, potential experimental realizations of ASPT states are also addressed.

cond-mat.str-el↗

arXiv2019

Best k-layer neural network approximations

We show that the empirical risk minimization (ERM) problem for neural networks has no solution in general. Given a training set $s_1, \dots, s_n \in \mathbb{R}^p$ with corresponding responses $t_1,\dots,t_n \in \mathbb{R}^q$, fitting a $k$-layer neural network $ν_θ: \mathbb{R}^p \to \mathbb{R}^q$ involves estimation of the weights $θ\in \mathbb{R}^m$ via an ERM: \[ \inf_{θ\in \mathbb{R}^m} \; \sum_{i=1}^n \lVert t_i - ν_θ(s_i) \rVert_2^2. \] We show that even for $k = 2$, this infimum is not attainable in general for common activations like ReLU, hyperbolic tangent, and sigmoid functions. A high-level explanation is like that for the nonexistence of best rank-$r$ approximations of higher-order tensors --- the set of parameters is not a closed set --- but the geometry involved for best $k$-layer neural networks approximations is more subtle. In addition, we show that for smooth activations $σ(x)= 1/\bigl(1 + \exp(-x)\bigr)$ and $σ(x)=\tanh(x)$, such failure to attain an infimum can happen on a positive-measured subset of responses. For the ReLU activation $σ(x)=\max(0,x)$, we completely classifying cases where the ERM for a best two-layer neural network approximation attains its infimum. As an aside, we obtain a precise description of the geometry of the space of two-layer neural networks with $d$ neurons in the hidden layer: it is the join locus of a line and the $d$-secant locus of a cone.

cs.LG↗