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Yang Qu

Publications and source records attributed to Yang Qu.

26 records · Page 2Linked to original sources

High performance integrated polarizers achieved by incorporating 2D layered graphene oxide films

Polarizers and polarization selective resonant cavities (e.g., ring resonators, gratings), are key components for applications to photography, coherent optical detection, polarization-division-multiplexing, optical sensing and liquid crystal displays. We demonstrate waveguide polarizers and polarization discriminating micro-ring resonators (MRRs) by integrating them with 2D graphene oxide (GO) layered thin films. We achieve precise control of the thickness, placement, and size of the films integrated onto photonic devices with a solution based, layer-by-layer transfer-free coating method combined with photolithography and lift-off. This overcomes limitations of layer transfer methods for 2D materials and is a significant advance to manufacturing integrated photonic devices incorporated with 2D materials. We measure the waveguide polarizer for different film thicknesses and lengths versus wavelength, polarization, and power, measuring a high polarization dependent loss (PDL) of ~ 53.8 dB. For GO-coated MRRs, we achieve an extinction ratio difference for TE/TM polarizations of 8.3-dB. We also present measurements of the linear optical properties of 2D layered GO films that yield the material loss anisotropy of the GO films and relative contribution of film loss anisotropy versus polarization-dependent mode overlap. Our results offer interesting physical insights into the transition of the layered GO films from 2D behaviour to quasi bulk like behavior and confirm the high performance of GO based integrated polarization selective devices.

physics.optics↗

Enhanced four-wave-mixing and 3rd order optical nonlinearity in SiN nanowires integrated with graphene oxide films

Layered 2D graphene oxide (GO) films are integrated with silicon nitride (SiN) waveguides to experimentally demonstrate an enhanced Kerr nonlinearity via four wave mixing (FWM). Owing to the strong light matter interaction between the SiN waveguides and the highly nonlinear GO films, the FWM performance of the hybrid waveguides is significantly improved. SiN waveguides with both uniformly coated and patterned GO films are fabricated based on a transfer free, layer by layer GO coating method together with standard photolithography and lift off processes, yielding precise control of the film thickness, placement and coating length. Detailed FWM measurements are carried out for the fabricated devices with different numbers of GO layers and at different pump powers. By optimizing the trade off between the nonlinearity and loss, we obtain a significant improvement in the FWM conversion efficiency of 7.3 dB for a uniformly coated device with 1 layer of GO and 9.1 dB for a patterned device with 5 layers of GO. We also obtain a significant increase in FWM bandwidth for the patterned devices. A detailed analysis of the influence of pattern length and position on the FWM performance is performed. Based on the FWM measurements, the dependence of GOs third-order nonlinearity on layer number and pump power is also extracted, revealing interesting physical insights about the 2D layered GO films. Finally, we obtain an enhancement in the effective nonlinear parameter of the hybrid waveguides by over a factor of 100. These results verify the enhanced nonlinear optical performance of SiN waveguides achievable by incorporating 2D layered GO films.

physics.optics↗

Enhanced nonlinear optical figure-of-merit at 1550nm for silicon nanowires integrated with graphene oxide layered films

Layered 2D GO films are integrated with silicon on insulator (SOI) nanowire waveguides to experimentally demonstrate an enhanced Kerr nonlinearity, observed through selfphase modulation (SPM). The GO films are integrated with SOI nanowires using a large area, transfer free, layer by layer coating method that yields precise control of the film thickness. The film placement and coating length are controlled by opening windows in the silica cladding of the SOI nanowires. Owing to the strong mode overlap between the SOI nanowires and the highly nonlinear GO films, the Kerr nonlinearity of the hybrid waveguides is significantly enhanced. Detailed SPM measurements using picosecond optical pulses show significant spectral broadening enhancement for SOI nanowires coated with 2.2 mm long films of 1 to 3 layers of GO, and 0.4 mm long films with 5 to 20 layers of GO. By fitting the experimental results with theory, the dependence of the n2 for GO on layer number and pulse energy is obtained, showing interesting physical insights and trends of the layered GO films from 2D monolayers to quasi bulk like behavior. Finally, we show that by coating SOI nanowires with GO films the effective nonlinear parameter of SOI nanowires is increased 16 times, with the effective nonlinear figure of merit (FOM) increasing by about 20 times to greater than 5. These results reveal the strong potential of using layered GO films to improve the Kerr nonlinear optical performance of silicon photonic devices.

physics.optics↗

Enhanced four-wave-mixing with 2D layered graphene oxide films integrated with CMOS compatible micro-ring resonators

Layered 2D graphene oxide (GO) films are integrated with microring resonators (MRRs) to experimentally demonstrate enhanced nonlinear optics in the form of four wave mixing (FWM). Both uniformly coated and patterned GO films are integrated on CMOS compatible doped silica MRRs using a large area, transfer free, layer by layer GO coating method together with photolithography and lift off processes, yielding precise control of the film thickness, placement, and coating length. The high Kerr nonlinearity and low loss of the GO films combined with the strong light matter interaction within the MRRs results in a significant improvement in the FWM efficiency in the hybrid MRRs. Detailed FWM measurements are performed at different pump powers and resonant wavelengths for the uniformly coated MRRs with 1 to 5 layers of GO as well as the patterned devices with 10 to 50 layers of GO. The experimental results show good agreement with theory, achieving up to 7.6 dB enhancement in the FWM conversion efficiency (CE) for an MRR uniformly coated with 1 layer of GO and 10.3 dB for a patterned device with 50 layers of GO. By fitting the measured CE as a function of pump power for devices with different numbers of GO layers, we also extract the dependence of the third-order nonlinearity on layer number and pump power, revealing interesting physical insights about the evolution of the layered GO films from 2D monolayers to quasi bulk like behavior. These results confirm the high nonlinear optical performance of integrated photonic resonators incorporated with 2D layered GO films.

physics.optics↗

High third-order Kerr optical nonlinearity in BiOBr 2D films measured by the Z-scan method

We investigate the nonlinear optical properties of BiOBr nanoflakes, a novel two-dimensional (2D) layered material from the Bismuth oxyhalide family. We measure the nonlinear absorption and Kerr nonlinearity of BiOBr nanoflakes at both 800 nm and 1550 nm via the Z scan technique. We observe a large nonlinear absorption coefficient beta = 10^-7 m/W as well as a large Kerr coefficient n2 = 10^-14 m^2/W. We also observe strong dispersion in n2, with it reversing sign from negative to positive as the wavelength varies from 800 nm to 1550 nm. In addition, we characterize the thickness-dependence of the nonlinear optical properties of BiOBr nanoflakes, observing that both the magnitudes of beta and n2 increase for very thin flakes. Finally, we integrate BiOBr nanoflakes onto silicon integrated waveguides and characterize the linear optical properties of the resulting hybrid integrated devices, with the measurements agreeing with calculated parameters using independent ellipsometry measurements. These results verify the strong potential of BiOBr as an advanced nonlinear optical material for high-performance hybrid integrated photonic devices.

physics.optics↗

Integrated polarizers based on graphene oxide in waveguides and ring resonators

Integrated waveguide polarizers and polarization-selective micro-ring resonators (MRRs) incorporated with graphene oxide (GO) films are experimentally demonstrated. CMOS-compatible doped silica waveguides and MRRs with both uniformly coated and patterned GO films are fabricated based on a large-area, transfer-free, layer-by-layer GO coating method that yields precise control of the film thickness. Photolithography and lift-off processes are used to achieve photolithographic patterning of GO films with precise control of the placement and coating length. Detailed measurements are performed to characterize the performance of the devices versus GO film thickness and coating length as a function of polarization, wavelength and power. A high polarization dependent loss of ~53.8 dB is achieved for the waveguide coated with 2-mm-long patterned GO films. It is found that intrinsic film material loss anisotropy dominates the performance for less than 20 layers whereas polarization dependent mode overlap dominates for thicker layers. For the MRRs, the GO coating length is reduced to 50 microns, yielding a ~ 8.3-dB polarization extinction ratio between TE and TM resonances. These results offer interesting physical insights and trends of the layered GO films and demonstrate the effectiveness of introducing GO films into photonic integrated devices to realize high-performance polarization selective components.

physics.optics↗

Transition of defect patterns from 2D to 3D in liquid crystals

Defects arise when nematic liquid crystals are under topological constraints at the boundary. Recently the study of defects has drawn a lot of attention. In this paper, we investigate the relationship between two-dimensional defects and three-dimensional defects within nematic liquid crystals confined in a shell under the Landau-de Gennes model. We use a highly accurate spectral method to numerically solve the Landau- de Gennes model to get the detailed static structures of defects. Interestingly, the solution is radial-invariant when the thickness of the shell is sufficiently small. As the shell thickness increase, the solution undergo symmetry break to reconfigure the disclination lines. We study this three-dimensional reconfiguration of disclination lines in detail under different boundary conditions. We also discuss the topological charge of defects in two- and three-dimensional spaces within the tensor model.

cond-mat.soft↗

On the Disclination Lines of Nematic Liquid Crystals

Defects in liquid crystals are of great practical importance and theoretical interest. Despite tremendous efforts, predicting the location and transition of defects under various topological constraint and external field remains to be a challenge. We investigate defect patterns of nematic liquid crystals confined in three-dimensional spherical droplet and two-dimensional disk under different boundary conditions, within the Landau-de Gennes model. We implement a spectral method that numerically solves the Landau-de Gennes model with high accuracy, which allows us to study the detailed static structure of defects. We observe five types of defect structures. Among them the 1/2-disclination lines are the most stable structure at low temperature. Inspired by numerical results, we obtain the profile of disclination lines analytically. Moreover, the connection and difference between defect patterns under the Landau-de Gennes model and the Oseen-Frank model are discussed. Finally, four conjectures are made to summarize some important characteristics of defects in the Landau-de Gennes theory. This work is a continuing effort to deepen our understanding on defect patterns in nematic liquid crystals.

cond-mat.soft↗