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Yannic Behovits

Publications and source records attributed to Yannic Behovits.

5 recordsLinked to original sources

Terahertz switching of antiferromagnetic order by N\'eel spin-orbit torques

Ultrafast electric manipulation of magnetic order in solids is critical for the development of future terahertz data processing. A fascinating concept for such high-speed operation is offered in metallic antiferromagnets by N\'eel spin-orbit torque. It should allow one to coherently rotate the ordered spins by simply applying an electric current of suitable amplitude and polarity. However, such switching has been severely hampered by competing heat-induced effects, and it has not yet been achieved on the intrinsically ultrafast time scales of antiferromagnets. Here, we report robust, direction-controlled and non-thermal rotation of the N\'eel vector $\mathbf{L}$ by $\pm$90{\deg} at room temperature in the antiferromagnet Mn$_2$Au driven by phase-locked terahertz current pulses. All observed features are consistent with ultrafast N\'eel spin-orbit torque: First, nonlinear optical imaging reveals that the terahertz current direction sets the final orientation of $\mathbf{L}$ in the absence of any bias field for at least two months. Second, transient optical birefringence shows that the switching proceeds ultrafast in less than 15 picoseconds. Finally, atomistic spin-dynamics simulations reproduce the observed dynamics and confirm the minor role of thermal effects. While the switching is already one order of magnitude faster than in ferromagnets at comparable dissipated energy, our simulations predict routes toward switching times and energies which are another order of magnitude lower. Our approach can be transferred to electric-field-driven switching in many more antiferromagnets, including magnetoelectric insulators. The engineering of spin torques, resonance frequencies and read-out mechanisms provides an exciting pathway toward on-chip applications of terahertz antiferromagnetic spin-orbitronics.

cond-mat.mes-hall

All-optical magnetometric characterization of the antiferromagnetic exchange-spring system Mn$_2$Au|Py by terahertz spin-torques

Antiferromagnetic materials have great potential for spintronic applications at terahertz (THz) frequencies. However, in contrast to ferromagnets, experimental studies of antiferromagnets are often challenging due to a lack of straightforward external control of the Néel vector $\mathbf{L}$. Here, we study an AFM|FM stack consisting of an antiferromagnetic metal layer (AFM) of the novel material Mn2Au and a ferromagnetic metal layer (FM) of NiFe. In this exchange-spring system, $\mathbf{L}$ of AFM Mn2Au can be controlled by the application of an external magnetic field B_ext. To characterize the AFM|FM stack as a function of the quasi-static $\mathbf{B}_{\mathrm{ext}}$, we perform THz-pump magneto-optic probe experiments. We identify signal components that can consistently be explained by the in-plane antiferromagnetic magnon mode excited by field-like Néel spin-orbit torques (NSOTs). Remarkably, we find that the $\mathbf{B}_{\mathrm{ext}}$- and THz-pump-induced changes in the optical response of the sample are dominated exclusively by the spin degrees of freedom of AFM. We fully calibrate the magnetic circular and magnetic linear optical birefringence of AFM and extract the efficiency of the NSOTs. Finally, by selective excitation of domains with different orientation of $\mathbf{L}$, we are able to determine the relative volume fraction of 0°, 90°, 180° and 270° domains distribution during the quasi-static reversal of $\mathbf{L}$ by $\mathbf{B}_{\mathrm{ext}}$. Our insights are an important prerequisite for future studies of ultrafast coherent switching of spins by THz NSOTs and show that THz-pump magneto-optic-probe experiments are a powerful tool to characterize magnetic properties of antiferromagnets.

cond-mat.mes-hall

Rotating spintronic terahertz emitter optimized for microjoule pump-pulse energies and megahertz repetition rates

Spintronic terahertz emitters (STEs) are powerful sources of ultra-broadband single-cycle terahertz (THz) field transients. They work with any pump wavelength, and their polarity and polarization direction are easily adjustable. However, at high pump powers and high repetition rates, STE operation is hampered by a significant increase in the local temperature. Here, we resolve this issue by rotating the STE at a few 100 Hz, thereby distributing the absorbed pump power over a larger area. Our approach permits stable STE operation at a fluence of ~1 mJ/cm$^2$ with up to 18 W pump power at megahertz repetition rates, corresponding to pump-pulse energies of a few 10 $μ$J and a power density far above the melting threshold of metallic films. The rotating STE is of interest for all ultra-broadband high-power THz applications requiring high repetition rates. As an example, we show that THz pulses with peak fields of 10 kV/cm can be coupled to a THz-lightwave-driven scanning tunneling microscope at 1 MHz repetition rate, demonstrating that the rotating STE can compete with standard THz sources such as LiNbO$_3$.

physics.optics

Nonlinear terahertz Néel spin-orbit torques in antiferromagnetic Mn$_2$Au

Antiferromagnets have large potential for ultrafast coherent switching of magnetic order with minimum heat dissipation. In novel materials such as Mn$_2$Au and CuMnAs, electric rather than magnetic fields may control antiferromagnetic order by Néel spin-orbit torques (NSOTs), which have, however, not been observed on ultrafast time scales yet. Here, we excite Mn$_2$Au thin films with phase-locked single-cycle terahertz electromagnetic pulses and monitor the spin response with femtosecond magneto-optic probes. We observe signals whose symmetry, dynamics, terahertz-field scaling and dependence on sample structure are fully consistent with a uniform in-plane antiferromagnetic magnon driven by field-like terahertz NSOTs with a torkance of (150$\pm$50) cm$^2$/A s. At incident terahertz electric fields above 500 kV/cm, we find pronounced nonlinear dynamics with massive Néel-vector deflections by as much as 30°. Our data are in excellent agreement with a micromagnetic model which indicates that fully coherent Néel-vector switching by 90° within 1 ps is within close reach.

cond-mat.mes-hall

Spin-voltage-driven efficient terahertz spin currents from the magnetic Weyl semimetals Co$_2$MnGa and Co$_2$MnAl

Magnetic Weyl semimetals are an emerging material class that combines magnetic order and a topologically non-trivial band structure. Here, we study ultrafast optically driven spin injection from thin films of the magnetic Weyl semimetals Co$_2$MnGa and Co$_2$MnAl into an adjacent Pt layer by means of terahertz emission spectroscopy. We find that (i) Co$_2$MnGa and Co$_2$MnAl are efficient terahertz spin-current generators reaching efficiencies of typical 3d-transition-metal ferromagnets such as Fe. (ii) The relaxation of the spin current provides an estimate of the electron-spin relaxation time of Co$_2$MnGa (165 fs) and Co$_2$MnAl (102 fs), which is comparable to Fe (92 fs). Both observations are consistent with a simple analytical model and highlight the large potential of magnetic Weyl semimetals as spin-current sources in terahertz spintronic devices. Finally, our results provide a strategy to identify magnetic materials that provide maximum spin current amplitudes for a given deposited optical energy density.

cond-mat.mes-hall