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Yantao Cao

Publications and source records attributed to Yantao Cao.

12 recordsLinked to original sources

$^{139}$La nuclear quadrupole resonance studies of pressurized La$_4$Ni$_3$O$_{10}$

Density-wave (DW) orders are considered as competing orders to unconventional superconductivity and are commonly seen in a variety of superconductors including but not limited to the recently discovered Ruddlesden-Popper-phase nickelates. By utilizing $^{139}$La nuclear quadrupole resonance, we systematically investigate into the nature of DW orders and their evolution under pressure in La$_4$Ni$_3$O$_{10}$. Spin and charge DW orders are found to be intertwined in this material, which is in stark contrast to those in La$_3$Ni$_2$O$_7$. Short-range DW orders are observed near 150 K, well above the development of long-range DW orders at around 139 K. Upon applying a hydrostatic pressure of 2.3 GPa, the transition temperatures of the short-range and long-range orders decrease at rates of 1 K/GPa and 10 K/GPa, respectively. Our results thus affirm that both spin density wave and charge density wave as competing orders with the superconducting state in La$_4$Ni$_3$O$_{10}$, and provide new insights into the interplay between DW orders and unconventional superconductivity.

cond-mat.supr-con

Giant magnetocaloric effect at low fields in triangular-lattice NdMgAl$_{11}$O$_{19}$

Magnetic refrigeration in the sub-Kelvin regime requires refrigerant materials to retain a large magnetic entropy at low temperatures by suppressing magnetic ordering. Quantum spin liquids (QSLs), which evade long-range magnetic ordering while retaining strong quantum fluctuations to the lowest temperatures, therefore provide a promising platform for realizing high-performance magnetic refrigerants. Here, we investigate the magnetic ground state and the magnetocaloric effect of the hexaaluminate, NdMgAl$_{11}$O$_{19}$, in which the Nd$^{3+}$ ions form a network of triangular lattices. Magnetic susceptibility and specific heat measurements indicate a magnetically dynamic state down to 50~mK, consistent with a QSL state. Specific heat measurements further reveal substantial magnetic entropy retained below 50~mK. Quasi-adiabatic demagnetization measurements demonstrate a superior cooling performance of NdMgAl$_{11}$O$_{19}$, which can be cooled to 113~mK from 1.9~K by only a small magnetic field change of 2~T. The outstanding refrigeration performance is attributed to the persistent spin fluctuations associated with the QSL-like ground state, together with a large effective \textit{g} factor and the smallness of the exchange interactions along the easy-axis direction. This study demonstrates that frustration, combined with strong spin-orbit coupling and crystal-electric-field effect in the rare earth magnets provides a promising design principle for next-generation cryogenic magnetic refrigerants.

cond-mat.str-el

Directional selection of field-induced phases by weak anisotropy in triangular-lattice K$_2$Mn(SeO$_3$)$_2$

Triangular-lattice systems host a variety of ground states, ranging from quantum spin liquids to magnetically ordered phases, the latter of which can exhibit a sequence of magnetic phase transitions under applied magnetic fields. Here, we report magnetic and thermodynamic measurements, combined with powder and single-crystal neutron diffraction, on a high-spin, nearly isotropic Mn$^{2+}$ triangular-lattice system K$_2$Mn(SeO$_3$)$_2$. The compound undergoes long-range magnetic ordering below $T_\mathrm{N} \sim 4$~K in zero field. Contrary to expectations for an ideal Heisenberg system, the compound adopts an up-down-zero (UD0) magnetic structure down to the lowest temperature (0.05 K), rather than the commonly expected Y-type structure. This UD0 state is, however, highly sensitive to external magnetic fields. For fields applied along the $c$ axis, it is readily destabilized and replaced by the Y-type structure, followed by an up-up-down (UUD) phase corresponding to the 1/3 magnetization plateau. In contrast, when the field is applied within the triangular plane, the system evolves into a canted Y state at a higher critical field. These results reveal that weak anisotropy, though small in magnitude, exerts a strongly orientation-dependent influence, playing a key role in selecting the field-induced phases in this frustrated magnet.

cond-mat.str-el

Orbital-selective Mottness Driven by Geometric Frustration of Interorbital Hybridization in Pr4Ni3O10

The interplay among orbital-selective Mott physics, Hund's coupling, tunable structural motifs, and Kondo-like scattering establishes a compelling paradigm for understanding and engineering correlated multi-orbital systems, as vividly exemplified by nickelate superconductors. Here, using high-resolution angle-resolved photoemission spectroscopy combined with theoretical calculations, we systematically investigate the electronic properties of trilayer nickelates. In La4Ni3O10, we observe pronounced interorbital hybridization, whereas in Pr4Ni3O10, the flat d_(z^2 ) band becomes markedly incoherent and diminishes in spectral weight. By contrast, the dispersive d_(x^2-y^2 ) bands retain coherence in both compounds. This striking incoherence/coherence dichotomy identifies an orbital-selective Mott phase modulated by the interlayer Ni-O-Ni bonding angle. The depletion of the d_(z^2 ) orbitals further frustrates the interorbital hybridization and influences the density-wave transition in Pr4Ni3O10. Moreover, the density-wave gap is substantially reduced in Pr4Ni3O10, likely due to extra scattering channels provided by the local moments of Pr3+ cations. Our findings elucidate the intricate interplay among lattice, orbital, spin, and electronic degrees of freedom and reveal a feasible structural control parameter for the multi-orbital correlated state in trilayer nickelates, which provide a concrete framework for understanding the emergence of superconductivity under high pressure.

cond-mat.str-el

Large longitudinal and anomalous transverse Magneto-thermoelectric effect in kagome antiferromagnet FeGe

Topological Kagome magnets, characterized by nontrivial electronic band structures featuring flat band, Dirac cone and van Hove singularities, provide a new avenue for the realization of thermoelectric devices. Unlike the conventional longitudinal Seebeck effect, transverse thermoelectric (TE) effects like the Nernst effect have attracted growing interest due to their unique transverse geometry and potential advantages. Here, we report the observation of a significant transverse thermoelectric conductivity alpha A_zx of 15 A K-1m-1 at low temperatures, together with a pronounced anomalous Nernst effect in the Kagome antiferromagnet FeGe, which exhibits a charge density wave inside the antiferromagnetic (AFM) state. This value is the highest record among known AFM materials. Furthermore, the thermopower at 14 T increases by 102-104% around the canted-AFM (CAFM) transition temperature, Tcant, comparable to that of the well-known AFM thermoelectric materials. These effects are attributed to large Berry curvature arising from the non-collinear spin texture in FeGe, highlighting its potential for enhancing thermoelectric performance and its candidacy for magneto-TE applications in Kagome antiferromagnetic materials.

cond-mat.mtrl-sci

Magnetic ground state and persistent spin fluctuations in triangular-lattice antiferromagnet NdZnAl$_{11}$O$_{19}$

Rare-earth triangular-lattice magnets serve as an excellent platform for investigating exotic quantum magnetic phenomena. Recently, the hexaaluminate \cmao\ has been proposed to host a $U(1)$ Dirac quantum spin liquid state with dominant Ising anisotropy. Here, we report a systematic study of its analogue, \nzao, employing ac susceptibility, inelastic neutron scattering, and muon spin relaxation measurements. Inelastic neutron scattering measurements establish a well-defined $J_\mathrm{eff}$ = 1/2 ground state with moderate Ising anisotropy ($g_c$ = 4.54, $g_\mathrm{ab}$ = 1.42). Muon spin relaxation measurements reveal persistent fluctuations emerging below $\sim$15\,K, and extending down to at least 0.28 K. AC susceptibility data further indicate an absence of magnetic ordering or spin freezing down to 50\,mK, despite an overall antiferromagnetic interaction with the Curie-Weiss temprature of $-0.42$\,K. These results suggest that \nzao\ is a good candidate material for realizing a quantum spin liquid state.

cond-mat.str-el

Complex spin-density-wave ordering in La$_4$Ni$_{3}$O$_{10}$

The discovery of high-temperature superconductivity in layered nickelates under pressure has recently triggered enormous interest. Studies of these compounds have revealed a density-wave-like transition at ambient pressure, though its connection with superconductivity is still not well understood. Here, we report a detailed \msr\ study on single crystals of trilayer nickelate \LNO\ at ambient pressure. We have identified a spin-density-wave (SDW) transition at the temperature of $T_\mathrm{N} \sim$130 K, as well as a broad crossover around 70 - 100 K. Based on the temperature dependence of the muon precession amplitudes and magnetic susceptibility, we attribute this additional crossover either to a spin reorientation, or to an inhomogeneous SDW ordering.

cond-mat.supr-con

U(1) Dirac quantum spin liquid candidate in triangular-lattice antiferromagnet CeMgAl$_{11}$O$_{19}$

Quantum spin liquid represents an intriguing state where electron spins are highly entangled yet spin fluctuation persists even at 0 K. Recently, the hexaaluminates \textit{R}MgAl$_{11}$O$_{19}$ (\textit{R} = rare earth) have been proposed to be a platform for realizing the quantum spin liquid state with dominant Ising anisotropic correlations. Here, we report detailed low-temperature magnetic susceptibility, muon spin relaxation, and thermodynamic studies on the CeMgAl$_{11}$O$_{19}$ single crystal. Ising anisotropy is revealed by magnetic susceptibility measurements. Muon spin relaxation and ac susceptibility measurements rule out any long-range magnetic ordering or spin freezing down to 50 mK despite the onset of spin correlations below $\sim$0.8 K. Instead, the spins keep fluctuating at a rate of 1.0(2) MHz at 50 mK. Specific heat results indicate a gapless excitation with a power-law dependence on temperature, $C_m(T) \propto T^{\alpha}$. The quasi-quadratic temperature dependence with $\alpha$ = 2.28(4) in zero field and linear temperature dependence in 0.25 T support the possible realization of the U(1) Dirac quantum spin liquid state.

cond-mat.str-el

Anisotropic transport properties and topological Hall effect in the annealed kagome antiferromagnet FeGe

Electron correlation often gives birth to various orders in quantum materials. Recently, a strongly correlated kagome antiferromagnet FeGe is discovered to undergo a charge density wave transition inside the A-type antiferromagnetic state, providing an opportunity to explore the interplay between charge order and magnetism. Here, we reported the observation of anisotropic resistivity and Hall effect, along with a topological Hall effect, in the annealed FeGe crystals. As the current flows along the \emph{ab}-plane, the temperature dependence of $\rho_{ab}$ exhibits a distinct resistivity loop related to a first-order transition at $T_{cdw}$. The applied magnetic fields do not alter $T_{cdw}$ but can induce a spin-flop transition at $H_{sf}$. Consequently, a field-induced large topological Hall effect is observed in the canting antiferromagnetic (CAFM) state below $T_{cant}$, which is possibly attributed to the non-trivial spin texture during the spin-flop process. Whereas, as current is parallel to \emph{c}-axis, both the field-induced transitions in $\rho_{c}$ and $\chi_{c}$ disappear. Instead, the Hall resistivity in the annealed FeGe significantly exhibits a deviation from the linear field-dependent. These findings provide valuable insight into revealing the interplay among magnetism, charge order and topology in the kagome magnets.

cond-mat.str-el

Electronic Correlation and Pseudogap-like Behavior of High-Temperature Superconductor La3Ni2O7

High-temperature superconductivity (HTSC) remains one of the most challenging and fascinating mysteries in condensed matter physics. Recently, superconductivity with transition temperature exceeding liquid-nitrogen temperature is discovered in La3Ni2O7 at high pressure, which provides a new platform to explore the unconventional HTSC. In this work, using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation, we systematically investigate the electronic structures of La3Ni2O7 at ambient pressure. Our experiments are in nice agreement with ab-initio calculations after considering an orbital-dependent band renormalization effect. The strong electron correlation effect pushes a flat band of d_(z^2 ) orbital component below the Fermi level (EF), which is predicted to locate right at EF under high pressure. Moreover, the d_(x^2-y^2 ) band shows a pseudogap-like behavior with suppressed spectral weight and diminished quasiparticle peak near EF. Our findings provide important insights into the electronic structure of La3Ni2O7, which will shed light on the understanding of the unconventional superconductivity in nickelates.

cond-mat.supr-con

Synthesis, disorder and Ising anisotropy in a new spin liquid candidate PrMgAl$_{11}$O$_{19}$

Here we report the successful synthesis of large single crystals of triangular frustrated PrMgAl$_{11}$O$_{19}$ using the optical floating zone technique. Single crystal X-ray diffraction measurements unveiled the presence of quenched disorder within the mirror plane, specifically $\sim$7\% of Pr ions deviating from the ideal 2\textit{d} site towards the 6\textit{h} site. Magnetic susceptibility measurements revealed an Ising anisotropy with the \textit{c}-axis being the easy axis. Despite a large spin-spin interaction that develops below $\sim$10~K and considerable site disorder, the spins do not order or freeze down to at least 50 mK. The availability of large single crystals offers a distinct opportunity to investigate the exotic magnetic state on a triangular lattice with an easy axis out of the plane.

cond-mat.str-el

Superconductivity in trilayer nickelate La4Ni3O10 under pressure

Nickelate superconductors have attracted a great deal of attention over the past few decades due to their similar crystal and electronic structures with high-temperature cuprate superconductors. Here, we report the superconductivity in a pressurized Ruddlesden-Popper phase single crystal, La4Ni3O10 (n = 3), and its interplay with the density wave order in the phase diagram. With increasing pressure, the density wave order as indicated by the anomaly in the resistivity is progressively suppressed, followed by the emergence of the superconductivity around 25 K under I4/mmm space group. The susceptibility measurements confirm bulk superconductivity with a volume fraction exceeding 80%. Moreover, theoretical analysis unveils that antiferromagnetic (AFM) super-exchange interactions can serve as the effective pairing interaction for the emergence of superconductivity (SC) in pressurized La4Ni3O10. Our research provides a new platform for the investigation of the unconventional superconductivity mechanism in Ruddlesden-Popper trilayer perovskite nickelates.

cond-mat.supr-con