arXiv subjects

Yaozhang Zhou

Publications and source records attributed to Yaozhang Zhou.

5 recordsLinked to original sources

arXiv2026

Thermodynamic evidence for interaction-driven first-order topological quantum phase transitions

Topological quantum phase transitions in non interacting systems occur through continuous gap closing and reopening. In strongly interacting systems, however, competing ordered states have long been predicted to drive first order transitions, although this possibility has remained experimentally unresolved. Recent transport studies of correlated phases in charge neutral rhombohedral graphene were interpreted as evidence for continuous topological transitions. Here, using nanoSQUID on tip magnetometry, we directly image the local orbital magnetization of a spin orbit proximitized rhombohedral graphene quantum anomalous Hall (QAH) state. We provide the first real space visualization of a QAH phase with a record Chern number, reconstruct its local thermodynamic gap, and track the evolution of its magnetization across competing correlated states. Combined with self consistent Hartree Fock calculations, these measurements show that the sequential transitions between the layer antiferromagnetic, QAH, and layer polarized insulating states are first order, accompanied by discontinuous changes in orbital magnetization. Near the phase boundaries, we observe fluctuating magnetic domains, providing direct microscopic evidence of phase coexistence between nearly degenerate competing ordered states. Together, these observations provide the first direct thermodynamic evidence for first order topological quantum phase transitions and establish a microscopic framework for understanding interaction driven topological quantum phase transitions through phase competition and coexistence.

cond-mat.mes-hall↗

arXiv2026

Reconfigurable chiral superconductivity

Rhombohedral multilayer graphene at high displacement fields hosts superconductivity emerging from a spin valley polarized quarter metal, with transport signatures suggestive of time reversal symmetry (TRS) breaking and chiral superconductivity (CSC). These observations have motivated proposals of topological superconductivity and non-Abelian quasiparticles, yet direct magnetic evidence and microscopic insight into the superconducting state remain lacking, limiting understanding of this unique state. Here we use nanoscale SQUID on tip magnetometry to image isospin-polarized domains in rhombohedral pentalayer graphene and establish CSC via spatially resolved thermodynamic detection of TRS breaking. We find that the density at which domain walls proliferate at elevated temperatures coincides with the onset of CSC, indicating an underlying transition in the parent state that both induces superconductivity and reduces domain wall energy. We further show that the chiral domain structure in the superconducting phase is inherited from the isospin-polarized parent state. Strikingly, the CSC phase exhibits multiple transport regimes governed by configurations of chiral domains separated by highly resistive domain walls. We demonstrate deterministic, ultra low current control of these domains, enabling reversible switching between states of opposite chirality a defining CSC property absent in other superconductors. These results establish rhombohedral graphene as a unique platform for reconfigurable CSC and ultra low power electronic functionality based on controllable isospin textures.

cond-mat.mes-hall↗

arXiv2025

Visualizing isospin magnetic texture and intervalley exchange interaction in rhombohedral tetralayer graphene

The tunable band structure and nontrivial topology of multilayer rhombohedral graphene lead to a variety of correlated electronic states with isospin orders-meaning ordered states in the combined spin and valley degrees of freedom-dictated by the interplay of spin-orbit coupling and Hunds exchange interactions. However, methods for mapping local isospin textures and determining the exchange energies are currently lacking. Here, we image the magnetization textures in tetralayer rhombohedral graphene using a nanoscale superconducting quantum interference device. We observe sharp magnetic phase transitions that indicate spontaneous time-reversal symmetry breaking. In the quarter-metal phase, the spin and orbital moments align closely, providing a bound on the spin-orbit coupling energy. We also show that the half-metal phase has a very small magnetic anisotropy, which provides an experimental lower bound on the intervalley Hunds exchange interaction energy. This is found to be close to its theoretical upper bound. The ability to resolve the local isospin texture and the different interaction energies will allow a better understanding of the phase transition hierarchy and the numerous correlated electronic states arising from spontaneous and induced isospin symmetry breaking in graphene heterostructures.

cond-mat.mes-hall↗

arXiv2024

Imaging Coulomb interactions and migrating Dirac cones in twisted graphene by local quantum oscillations

Flat band moiré graphene systems have emerged as a quintessential platform to investigate correlated phases of matter. A plethora of interaction-driven ground states have been proposed, and yet despite extensive experimental effort, there has been little direct evidence that distinguishes between the various phases, in particular near charge neutrality point. Here, we use a nanoscale scanning superconducting quantum interference device to image the local thermodynamic quantum oscillations in alternating-twist trilayer graphene at magnetic fields as low as 56 mT, which reveal ultrafine details of the density of states and of the renormalization of the single-particle band structure by Coulomb interactions. We find that the charging self-energy due to occupied electronic states, is critical in explaining the high carrier density physics. At half-filling of the conduction flat band, we observe a Stoner-like symmetry breaking, suggesting that it is the most robust mechanism in the hierarchy of phase transitions. On approaching charge neutrality, where the charging energy is negligible and exchange energy is dominant, we find the ground state to be a nematic semimetal which is favored over gapped states in the presence of heterostrain. In the revealed semimetallic phase, the flat-band Dirac cones migrate towards the mini-Brillouin zone center, spontaneously breaking the C_3 rotational symmetry. Our low-field local quantum oscillations technique presents an alluring avenue to explore the ground states of diverse strongly interacting van der Waals systems.

cond-mat.mes-hall↗

arXiv2023

Imaging de Haas-van Alphen quantum oscillations and milli-Tesla pseudomagnetic fields

A unique attribute of atomically thin quantum materials is the in-situ tunability of their electronic band structure by externally controllable parameters like electrostatic doping, electric field, strain, electron interactions, and displacement or twisting of atomic layers. This unparalleled control of the electronic bands has led to the discovery of a plethora of exotic emergent phenomena. But despite its key role, there is currently no versatile method for mapping the local band structure in advanced 2D materials devices in which the active layer is commonly embedded in various insulating layers and metallic gates. Utilizing a scanning superconducting quantum interference device, we image the de Haas-van Alphen quantum oscillations in a model system, the Bernal-stacked trilayer graphene with dual gates, which displays multiple highly-tunable bands. By resolving thermodynamic quantum oscillations spanning over 100 Landau levels in low magnetic fields, we reconstruct the band structure and its controllable evolution with the displacement field with unprecedented precision and spatial resolution of 150 nm. Moreover, by developing Landau level interferometry, we reveal shear-strain-induced pseudomagnetic fields and map their spatial dependence. In contrast to artificially-induced large strain, which leads to pseudomagnetic fields of hundreds of Tesla, we detect naturally occurring pseudomagnetic fields as low as 1 mT corresponding to graphene twisting by just 1 millidegree over one μm distance, two orders of magnitude lower than the typical angle disorder in high-quality twisted bilayer graphene devices. This ability to resolve the local band structure and strain on the nanoscale opens the door to the characterization and utilization of tunable band engineering in practical van der Waals devices.

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