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Yaroslav M. Blanter

Publications and source records attributed to Yaroslav M. Blanter.

At least 19 recordsLinked to original sources

Strain-controlled magnetism and magnetoelasticity in monolayer NiPS$_3$ and CrPS$_4$

We develop a first-principles framework for magnetoelastic coupling in two-dimensional magnets based on a strain-dependent Heisenberg model. In this approach, strain derivatives of the exchange interactions provide direct access to magnetostriction and to the magnetic renormalization of the elastic tensor, establishing a microscopic link between spin interactions and elastic response. We apply the method to monolayer NiPS$_3$ and CrPS$_4$, which exhibit contrasting magnetoelastic behavior. NiPS$_3$ shows weak and nearly isotropic spin-lattice coupling, consistent with a robust zigzag antiferromagnetic ground state. In contrast, CrPS$_4$ displays strong anisotropic coupling, leading to strain-driven transitions between spin-spiral and ferromagnetic phases and significant changes in the critical temperature and elastic response. Our results demonstrate a general route to quantify magnetoelastic effects in low-dimensional magnets and highlight CrPS$_4$ as a promising platform for strain engineering of magnetic order.

cond-mat.mtrl-sci↗

Magnetic ground states of CrPS$_4$ and NiPS$_3$ monolayers from long-range exchange interactions

We investigate the magnetic properties of monolayer CrPS$_4$ and NiPS$_3$ by combining first-principles calculations, second-principles spin models, and Monte Carlo simulations. Unlike conventional approaches that truncate exchange interactions after only a few shells and determine them by fitting total energies, we extract the magnetic exchange tensors directly from density functional theory using the LKAG formalism and include interactions until numerical convergence is achieved. We show that long-range exchange interactions qualitatively modify the magnetic behavior of both materials. In CrPS$_4$, they destabilize the previously predicted ferromagnetic ground state and stabilize a spin-spiral phase, reducing the critical temperature to about 21\,K, in agreement with available experiments. The resulting magnetic phase diagram contains multiple collinear and non-collinear phases that can be tuned by temperature and external magnetic fields. In NiPS$_3$, the experimentally observed zigzag antiferromagnetic order only emerges when exchange interactions up to the fifth shell are included. These results demonstrate that quantitatively predictive spin models for thiophosphate monolayers require long-range exchange interactions and provide a predictive framework for accurately describing two-dimensional van der Waals magnets.

cond-mat.mtrl-sci↗

Pseudo-superconducting-diode effect in ferroelectric Josephson junctions

The superconducting diode effect (SDE), characterized by unequal critical supercurrents in opposite current directions, enables supercurrent rectification. We propose a magnetic-field-free pseudo-superconducting-diode effect in ferroelectric Josephson junctions with broken inversion symmetry. Using a coupled dynamical model that combines a polarization-dependent RCSJ description with Landau-Khalatnikov-Tani ferroelectric dynamics, we show that ferroelectric polarization switching induces asymmetric critical and retrapping currents under current sweeps. The resulting nonreciprocity is highly tunable via ferroelectric parameters and the sweep protocol and remains robust at finite temperatures. Our work identifies ferroelectric Josephson junctions as a promising platform for magnetic-field-free nonreciprocal superconducting devices.

cond-mat.supr-con↗

Magnon-polaron mediated spin Seebeck effect in altermagnets

Altermagnets, distinguished by compensated antiparallel spins yet nondegenerate magnon spectra, bridge the gap between ferromagnets and antiferromagnets. Although several probes such as anisotropic transport and spectroscopic measurements have been proposed to identify altermagnetic order, experimentally accessible transport signatures remain highly desirable. Here, we show that in altermagnets subject to an external magnetic field, the spin Seebeck effect exhibits pronounced directional anisotropy. Specifically, the spin Seebeck coefficient differs significantly along in-plane directions, and this anisotropy increases with field strength. Magnetoelastic interactions further produce resonant peaks whose positions with respect to an applied magnetic field reflect the intrinsic magnon band anisotropy, and provide localized features that enhance the distinguishability of the altermagnetic response. The peaks provide a robust experimental signature of altermagnetic order. Our findings serve as signatures of altermagnetic order while laying the groundwork for their application in spintronic devices.

cond-mat.mes-hall↗

Spin-caloritronic signatures of soft magnons in bilayer CrSBr

Spin transport in magnetic insulators is often treated by assuming that magnons carry a fixed spin angular momentum of $\hbar$, which does not hold in general, however. Here we calculate the magnon spin angular momentum of a layered antiferromagnet as a function of applied magnetic field and wave vector. We show that the triaxial anisotropy and intralayer dipolar interactions in bilayer CrSBr renormalize the magnon spin angular momentum, which diverges upon field-induced magnon softening. This divergence gives rise to a pronounced peak in the thermal spin Seebeck response and provides a clear spin-caloritronic signature of soft magnons.

cond-mat.mes-hall↗

Magnon polaritons in a van der Waals ferromagnet coupled to a superconducting resonator

Achieving magnon-photon hybridization in the microwave regime is essential for integrating magnetic excitations with superconducting circuits. While this has been extensively demonstrated in bulk magnetic systems, realizing it in two-dimensional van der Waals materials remains challenging due to their reduced magnetic volume and increased dissipation. Here, magnon-photon hybridization is observed in exfoliated flakes of the van der Waals ferromagnet Cr$_2$Ge$_2$Te$_6$, with thicknesses down to 30 nm. The resulting magnon polaritons-hybrid excitations of cavity photons and magnons-are evidenced by reproducible avoided crossings across six devices, enabled by a low-impedance superconducting resonator design. The coupling strength follows the expected square-root dependence on thickness, and extrapolation of this scaling indicates that hybridization in the monolayer limit is within reach.

cond-mat.mes-hall↗

Magnomechanical Coupling in Suspended 2D van der Waals Ferromagnets

Magnomechanical systems provide a promising route for exploring coherent hybrid magnon-phonon interactions and hybrid information processing, but their realization has so far been limited by weak magnon-phonon coupling in conventional bulk platforms. We show that a suspended membrane of a two-dimensional van der Waals ferromagnet with in-plane magnetization and out-of-plane mechanical oscillations exhibits large magnomechanical coupling dominated by magnetoelastic interactions. The parametric single magnon-phonon coupling rate scales linearly with pre-strain and can reach hundreds of Hertz to low kiloHertz in suspended membranes of van der Waals ferromagnets such as CrGeTe_3 under experimentally realistic conditions. This rate exceeds typical values reported for YIG spheres by more than three orders of magnitude. Our results demonstrate that suspended membranes of van der Waals magnets provide a robust and highly tunable platform for magnomechanics.

cond-mat.mes-hall↗

Quantum-Material Josephson Junctions: Unconventional Barriers, Emerging Functionality

Josephson junctions translate quantum phase coherence into an electrical response and underpin superconducting sensors and quantum circuits. In conventional junctions, the barrier acts primarily as a passive weak link, however, when the barrier is a quantum material with its own internal degrees of freedom like magnetism, strong correlations, or switchable polarization, the Josephson effect becomes a sensitive probe of symmetry and many-body physics in the interlayer. Here we review progress in quantum-material Josephson junctions, (QMJJ) focusing on three rapidly advancing barrier families: 1. magnetic barriers, where exchange, noncollinearity, and spin-active scattering enable 0-π-ϕ ground states, singlet-triplet conversion, and nonreciprocal transport, 2. correlated barriers, where proximity effects acquire many-body character and recent van der Waals Kagome Mott interlayers exhibit field-free Josephson diode behavior, and 3. ferroelectric and multiferroic barriers, where nonvolatile polarization provides an internal control knob and can produce superconducting memory and memristive dynamics.

cond-mat.supr-con↗

Magnetoelastic conversion in integrated YIG nanostructures

Motivated by the recent proposal of two-step transduction from microwave to optical domain using magnetic and elastic intermediate stages arXiv:2205.05088, we consider the coupling between resonant magnetic and elastic modes within a simple axially-symmetric nanodevice designed to host high-quality-factor acoustic modes: A suspended YIG ring structure supported by a central stem, fabricated from a continuous single-crystal film. We study the modes of the system with our custom finite element solvers. We identify the lowest order ``breathing'' mode of a magnetic vortex and the lowest order elastic breathing mode as having the largest mode overlap. For this pair of modes, the external out-of-plane magnetic bias field is critical for bringing them into resonance; however, we show that at the same time it also affects the strength of the coupling. To counteract this, we optimize the radius of the ring at fixed thickness. For the 100 nm-thick film the resonant coupling is maximized at $g/2π= 8\text{MHz}$ at $R\approx1.7μ\text{m}$, indicating that the overlap integral approaches the idealized limit assumed in previous order-of-magnitude estimates. Our results pave the way for the design of tunable frequency-conversion devices based on magnetoelastics.

cond-mat.mes-hall↗

Isofrequency spin-wave imaging using color center magnetometry for magnon spintronics

Magnon spintronics aims to harness spin waves in magnetic films for information technologies. Color center magnetometry is a promising tool for imaging spin waves, using electronic spins associated with atomic defects in solid-state materials as sensors. However, two main limitations persist: the magnetic fields required for spin-wave control detune the sensor-spin detection frequency, and this frequency is further restricted by the color center nature. Here, we overcome these limitations by decoupling the sensor spins from the spin-wave control fields -selecting color centers with intrinsic anisotropy axes orthogonal to the film magnetization- and by using color centers in diamond and hexagonal boron nitride to operate at complementary frequencies. We demonstrate isofrequency imaging of field-controlled spin waves in a magnetic half-plane and show how intrinsic magnetic anisotropies trigger bistable spin textures that govern spin-wave transport at device edges. Our results establish color center magnetometry as a versatile tool for advancing spin-wave technologies.

cond-mat.mes-hall↗

Polarization Controlled Supercurrent in Ferroelectric Josephson Junction

Josephson junctions are essential devices in superconducting electronics and quantum computing hardware. Here we predict electrical control of the supercurrent in composite superconductor-insulator-ferroelectric-insulator-superconductor (S-I-FE-I-S) Josephson junctions. Inversion symmetry broken by unequal dielectric barrier thicknesses and/or potentials converts ferroelectric polarization reversal into a substantial change of the critical current. With a WKB tunneling model we obtain non-volatile switching of the critical current with on-off efficiency up to 0.9 for physically realistic parameters. This can be achieved by optimizing the thicknesses and potential barriers of the insulating layers, as well as the thickness and dielectric constant of the ferroelectric layer. We also derive a compact linear expression for the critical current valid for small polarizations. Our results identify ferroelectric Josephson junctions as electrically programmable superconducting current switches for cryogenic memory and logic applications.

cond-mat.supr-con↗

Dipolar-exchange spin waves in thin bilayers

We investigate the dipolar-exchange spin wave spectrum in thin ferromagnetic bilayers with inplane magnetization, incorporating interlayer exchange coupling and intra- and interlayer dipolar interactions. In the continuum approximation we analyze the nonreciprocity of propagating magnetic stray fields emitted by spin waves as a function of the relative orientation of the layer magnetizations that are observable by magnetometry of synthetic antiferromagnets or weakly coupled type-A van der Waals antiferromagnetic bilayers as a function of an applied magnetic field.

cond-mat.mes-hall↗

Magnon-magnon interaction induced by nonlinear spin wave dynamics

We experimentally and theoretically demonstrate that nonlinear spin-wave dynamics can induce an effective resonant interaction between non-resonant magnon modes in a yttrium iron garnet disk. Under strong pumping near the ferromagnetic resonance mode, we observe a spectral splitting that emerges with increasing drive amplitude. This phenomenon is well captured by a theoretical framework based on the linearization of a magnon three-wave mixing Hamiltonian, which at high power leads to parametric Suhl instabilities. The access and control of nonlinear magnon-parametric processes enables the development of experimental platforms in an unexplored parameter regime for both classical and quantum computation protocols.

cond-mat.mes-hall↗

Spin Wave Dispersion of the van der Waals Antiferromagnet NiPS$_3$

We calculate the magnon dispersion spectra of the two-dimensional zigzag van der Waals antiferromagnet NiPS$_3$ for monolayer, bilayer, and bulk systems as a function of an external magnetic field. We calculate the exchange and anisotropy constants in our spin model by first principles. We can accurately explain the transition from a collinear to a canted ground state for a magnetic field applied normal to the (in-plane) easy-axis, and a spin-flop transition when the field is parallel to it. A topologically protected Dirac nodal line is present and robust with respect to both external and anisotropy fields.

cond-mat.mes-hall↗

Spin waves in the bilayer van der Waals magnet CrSBr

We derive analytical expressions for the spin wave frequencies and precession amplitudes in monolayer and antiferromagnetically coupled bilayer CrSBr under in-plane external magnetic fields. The analysis covers the antiferromagnetic, ferromagnetic, and canted phases, demonstrating that the spin wave frequencies in all phases are tunable by the applied magnetic field. We discuss the roles of intra- and interlayer exchange interactions, triaxial anisotropy, and intralayer dynamic dipolar fields in controlling the magnetization dynamics.

cond-mat.mes-hall↗

Thermoelastic Damping Across the Phase Transition in van der Waals Magnets

A quantitative understanding of the microscopic mechanisms responsible for damping in van der Waals nanomechanical resonators remains elusive. In this work, we investigate van der Waals magnets, where the thermal expansion coefficient exhibits an anomaly at the magnetic phase transition due to magnetoelastic coupling. Thermal expansion mediates the coupling between mechanical strain and heat flow and determines the strength of thermoelastic damping (TED). Consequently, variations in the thermal expansion coefficient are reflected directly in TED, motivating our focus on this mechanism. We extend existing TED models to incorporate anisotropic thermal conduction, a critical property of van der Waals materials. By combining the thermodynamic properties of the resonator material with the anisotropic TED model, we examine dissipation as a function of temperature. Our findings reveal a pronounced impact of the phase transition on dissipation, along with transitions between distinct dissipation regimes controlled by geometry and the relative contributions of in-plane and out-of-plane thermal conductivity. These regimes are characterized by the resonant interplay between strain and in-plane or through-plane heat propagation. To validate our theory, we compare it to experimental data of the temperature-dependent mechanical resonances of FePS$_3$ resonators.

cond-mat.mes-hall↗

Roadmap on Quantum Magnetic Materials

Fundamental research on two-dimensional (2D) magnetic systems based on van der Waals materials has been gaining traction rapidly since their recent discovery. With the increase of recent knowledge, it has become clear that such materials have also a strong potential for applications in devices that combine magnetism with electronics, optics, and nanomechanics. Nonetheless, many challenges still lay ahead. Several fundamental aspects of 2D magnetic materials are still unknown or poorly understood, such as their often-complicated electronic structure, optical properties, and magnetization dynamics, and their magnon spectrum. To elucidate their properties and facilitate integration in devices, advanced characterization techniques and theoretical frameworks need to be developed or adapted. Moreover, developing synthesis methods which increase critical temperatures and achieve large-scale, high-quality homogeneous thin films is crucial before these materials can be used for real-world applications. Therefore, the field of 2D magnetic materials provides many challenges and opportunities for the discovery and exploration of new phenomena, as well as the development of new applications. This Roadmap presents the background, challenges, and potential research directions for various relevant topics in the field on the fundamentals, synthesis, characterization, and applications. We hope that this work can provide a strong starting point for young researchers in the field and provide a general overview of the key challenges for more experienced researchers.

cond-mat.mtrl-sci↗

Equivalence of pseudogap and pairing energy in a cuprate high-temperature superconductor

The pseudogap stands out in the phase diagram of the cuprate high-temperature superconductors because its origin and relationship to superconductivity remain elusive. The origin of the pseudogap has been debated, with competing hypotheses attributing it to preformed electron pairs or local order, such as charge density waves. Here, we present unambiguous evidence supporting the pairing scenario, using local shot-noise spectroscopy measurements in Bi2Sr2CaCu2O8+δ. Our data demonstrates that the pseudogap energy coincides with the onset of electron pairing, and is spatially heterogeneous with values reaching up to 70 meV. Our results exclude a pure local order origin of the pseudogap, link the pseudogap to Cooper pair formation, and show that the limiting factor for higher Tc in cuprates is phase coherence.

cond-mat.supr-con↗