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Yilong Han

Publications and source records attributed to Yilong Han.

At least 19 recordsLinked to original sources
arXiv2025

Percolation transition in entangled granular networks

Highly nonconvex granular particles, such as staples and metal shavings, can form solid-like cohesive structures through geometric entanglement (interlocking). The network structure formed by this entanglement, however, remains largely unexplored. Here we utilize network science to investigate the entanglement networks of C-shaped granular particles under vibration through experiments and simulations. By analyzing key network properties, we demonstrate that these networks undergo a percolation transition as the number of links increases logarithmically over time; the entangled particles form a giant cluster when the number of links exceeds a critical threshold. We propose a continuum percolation model of rings that effectively describes the observed transition. Additionally, we find that particle's opening angle significantly affects mechanical bonding and, consequently, the network structure. This work highlights the potential of network-based approaches to study entangled materials, paving the way for advancements in applications ranging from mechanical metamaterials to entangled robot swarms.

cond-mat.soft↗
arXiv2024

Mechanical properties of crystalline-amorphous composites: generalisation of Hall-Petch and inverse Hall-Petch behaviours

The strength, $\sigma_{\rm y}$, of a polycrystal decreases with mean grain diameter $D$ at $D\gtrsim50$ atoms (i.e. Hall-Petch behaviour) and increases at $D\lesssim50$ (i.e. inverse Hall-Petch behaviour). Our simulations generalise $\sigma_{\rm y}(D)$ to $\sigma_{\rm y}(D,l)$, where $l$ is the mean thickness of grain boundaries. For various particle compositions, the maximum strength is reached at $(D,l)\simeq(50, 6)$ particles for single-component face-centred-cubic solids and at $(D,l)\simeq(50, 2)$ for bidispersed or body-centred-cubic solids because of the different activation stresses of dislocation motions. The results explain recent alloy experiments and provide a way to exceed the maximum strength of polycrystals. Ductility and elastic moduli are also measured in the broad $(D,l)$ space. The regimes without a strength-ductility trade-off, the maximum ductility and ductile--brittle transitions are identified. These results obtained in $(D,l)$ space are important in solid mechanics and can guide the fabrication of crystalline-amorphous composites with outstanding mechanical properties.

cond-mat.mtrl-sci↗
arXiv2024

Searching for various melting scenarios of 2D crystals

In contrast to three-dimensional (3D) crystals that melt via a first-order transition, two-dimensional (2D) crystals can exhibit various melting scenarios under different temperatures, pressures, and particle interactions, particularly when they can form partially ordered intermediate phases between crystal and liquid. The existing 2D melting theories predict some scenarios, but do not exclude other possibilities. A recent simulation observed five melting scenarios including two new types by tuning the shape of polygonal particles.

cond-mat.mtrl-sci↗
arXiv2024

Multiagent Reinforcement Learning Enhanced Decision-making of Crew Agents During Floor Construction Process

Fine-grained simulation of floor construction processes is essential for supporting lean management and the integration of information technology. However, existing research does not adequately address the on-site decision-making of constructors in selecting tasks and determining their sequence within the entire construction process. Moreover, decision-making frameworks from computer science and robotics are not directly applicable to construction scenarios. To facilitate intelligent simulation in construction, this study introduces the Construction Markov Decision Process (CMDP). The primary contribution of this CMDP framework lies in its construction knowledge in decision, observation modifications and policy design, enabling agents to perceive the construction state and follow policy guidance to evaluate and reach various range of targets for optimizing the planning of construction activities. The CMDP is developed on the Unity platform, utilizing a two-stage training approach with the multi-agent proximal policy optimization algorithm. A case study demonstrates the effectiveness of this framework: the low-level policy successfully simulates the construction process in continuous space, facilitating policy testing and training focused on reducing conflicts and blockages among crews; and the high-level policy improving the spatio-temporal planning of construction activities, generating construction patterns in distinct phases, leading to the discovery of new construction insights.

cs.CE↗
arXiv2024

Distinguishable-particle Glassy Crystal: the simplest molecular model of glass

The nature of glassy dynamics and the glass transition are long-standing problems under active debate. In the presence of a structural disorder widely believed to be an essential characteristic of structural glass, identifying and understanding key dynamical behaviors are very challenging. In this work, we demonstrate that an energetic disorder, which usually results from a structural disorder, is instead a more essential feature of glass. Specifically, we develop a distinguishable-particle glassy crystal (DPGC) in which particles are ordered in a face-centered cubic lattice and follow particle-dependent random interactions, leading to an energetic disorder in the particle configuration space. Molecular dynamics simulations in the presence of vacancy-induced particle diffusion show typical glassy behaviors. A unique feature of this molecular model is the knowledge of the complete set of inherent structures with easily calculable free energies, implying a well-understood potential energy landscape.

cond-mat.stat-mech↗
arXiv2023

Chiral Active Particles are Sensitive Reporter to Environmental Geometry

Chiral active particles (CAPs) are self-propelling particles that break time-reversal symmetry by orbiting or spinning, leading to intriguing behaviors. Here, we examined the dynamics of CAPs moving in 2D lattices of disk obstacles through active Brownian dynamics simulations and granular experiments with grass seeds. We find that the effective diffusivity of the CAPs is sensitive to the structure of the obstacle lattice, a feature absent in achiral active particles. We further studied the transport of CAPs in obstacle arrays under an external field and found a reentrant directional locking effect, which can be used to sort CAPs with different activities. Finally, we demonstrated that the parallelogram lattice of obstacles without mirror symmetry can separate clockwise and counter-clockwise CAPs. The mechanisms of the above three novel phenomena are qualitatively explained. As such, our work provides a basis for designing chirality-based tools for single-cell diagnosis and separation, and active particle-based environmental sensors.

cond-mat.soft↗
arXiv2023

Anisotropic-Isotropic Transition of Cages at the Glass Transition

Characterizing the local structural evolution is an essential step in understanding the nature of glass transition. In this work, we probe the evolution of Voronoi cell geometry in simple glass models, and find that the individual particle cages deform anisotropically in supercooled liquid and isotropically in glass. We introduce an anisotropy parameter $k$ for each Voronoi cell, which mean value exhibits a sharp change at the mode-coupling glass transition $\phi_\mathrm{c}$. Moreover, a power law of packing fraction $\phi\propto q_1^{-d}$ is discovered in the liquid regime with $d>D$, in contrast to $d=D$ in the glass regime, where $q_1$ is the first peak position of structure factor, and $D$ is the space dimension. This power law is explained by the change of $k$. The active motions in supercooled liquid are spatially correlated with long axes rather than short axes of Voronoi cells. In addition, the dynamic slowing down approaching the glass transition can be well characterized through a modified free volume model based on $k$. These findings reveal that the nonagnostic structural parameter $k$ determines glassy dynamics and is effective in identifying the structure-dynamics correlations and the glass transition.

cond-mat.soft↗
arXiv2020

Direct evidence of void induced structural relaxations in colloidal glass formers

Particle dynamics in supercooled liquids are often dominated by string-like motions in which lines of particles perform activated hops cooperatively. The structural features triggering these motions, crucial in understanding glassy dynamics, remain highly controversial. We experimentally study microscopic particle dynamics in colloidal glass formers at high packing fractions. With a small polydispersity leading to glass-crystal coexistence, a void in the form of a vacancy in the crystal can diffuse reversibly into the glass and further induces string-like motions. In the glass, a void takes the form of a quasi-void consisting of a few neighboring free volumes and is transported by the string-like motions it induces. In fully glassy systems with a large polydispersity, similar quasi-void actions are observed. The mobile particles cluster into string-like or compact geometries, but the compact ones can further be broken down into connected sequences of strings, establishing their general importance.

cond-mat.soft↗
arXiv2017

Assembly and Phase Transitions within Colloidal Crystals

Micrometre sized colloidal particles can be viewed as large atoms with tailorable size, shape and interactions. These building blocks can assemble into extremely rich structures and phases, in which the thermal motions of particles can be directly imaged and tracked using optical microscopy. Hence, colloidal particles are excellent model systems for studying phase transitions, especially for poorly understood kinetic and nonequilibrium microscale processes. Advances in colloid fabrication, assembly and computer simulations have opened up numerous possibilities for such research. In this Review, we describe recent progress in the study of colloidal crystals composed of tunable isotropic spheres, anisotropic particles and active particles. We focus on advances in crystallization, melting and solid solid transitions, and highlight challenges and future perspectives in phase transition studies within colloidal crystals.

cond-mat.soft↗
arXiv2017

Reply to "Failure to replicate long-range tunable attractions in colloidal system"

An arxiv paper, ref. [1] by Cao et al., claimed that the tunable attraction reported in our ref. [2] could not be detected. Ref. [1] was submitted to Nature in Apr. 2016 as a Comment on our ref. [2]. Our reply in May 2016 responded to ref. [1] and was reviewed by the editor of Nature and an external referee. Ref. [1] was rejected by Nature in Aug. 2016. We provide our reply, which answers all of the criticisms in ref. [1], in Appendix I. The main text contains a brief reply to the main criticisms.

cond-mat.soft↗
arXiv2016

Surface relaxation of vapour-depositing colloidal glasses

Vapour deposition can directly produce ultrastable glasses, which are similar to conventional glasses aged over thousands of years. The highly mobile surface layer is believed to accelerate the ageing process of vapour-deposited glasses, but its microscopic kinetics has not been experimentally observed. Here we studied the deposition growth kinetics of a two-dimensional colloidal glass at the single-particle level using video microscopy. We found that newly deposited particles in the surface layer (depth $d<14$ particles) relaxed via frequent out-of-cage motions, while particles in the deeper middle layer ($14<d\lesssim100$ particles) relaxed via activation of cooperative rearrangement regions (CRRs). These CRRs were much larger, more anisotropic and occurred more frequently than CRRs in the bulk ($d\gtrsim100$ particles) or after deposition. Their centers of mass moved towards the surface, while the particles within moved towards the bulk, causing free-volume "bubbles" to move towards the surface to give a more compact bulk glass. This two-step relaxation in two surface layers is distinct from the previously assumed relaxation in one surface mobile layer

cond-mat.soft↗
arXiv2011

Glass transitions in two-dimensional suspensions of colloidal ellipsoids

We observed a two-step glass transition in monolayers of colloidal ellipsoids by video microscopy. The glass transition in the rotational degree of freedom was at a lower density than that in the translational degree of freedom. Between the two transitions, ellipsoids formed an orientational glass. Approaching the respective glass transitions, the rotational and translational fastest-moving particles in the supercooled liquid moved cooperatively and formed clusters with power-law size distributions. The mean cluster sizes diverge in power law as approaching the glass transitions. The clusters of translational and rotational fastest-moving ellipsoids formed mainly within pseudo-nematic domains, and around the domain boundaries, respectively.

cond-mat.soft↗
arXiv2010

Self-diffusion in two-dimensional hard ellipsoid suspensions

We studied the self-diffusion of colloidal ellipsoids in a monolayer near a flat wall by video microscopy. The image processing algorithm can track the positions and orientations of ellipsoids with sub-pixel resolution. The translational and rotational diffusions were measured in both the lab frame and the body frame along the long and short axes. The long-time and short-time diffusion coefficients of translational and rotational motions were measured as functions of the particle concentration. We observed sub-diffusive behavior in the intermediate time regime due to the caging of neighboring particles. Both the beginning and the ending times of the intermediate regime exhibit power-law dependence on concentration. The long-time and short-time diffusion anisotropies change non-monotonically with concentration and reach minima in the semi-dilute regime because the motions along long axes are caged at lower concentrations than the motions along short axes. The effective diffusion coefficients change with time t as a linear function of (lnt)/t for the translational and rotational diffusions at various particle densities. This indicates that their relaxation functions decay according to 1/t which provides new challenges in theory. The effects of coupling between rotational and translational Brownian motions were demonstrated and the two time scales corresponding to anisotropic particle shape and anisotropic neighboring environment were measured.

cond-mat.soft↗
arXiv2009

Phase-Space Networks of Geometrical Frustrated Systems

Geometric frustration leads to complex phases of matter with exotic properties. Antiferromagnets on triangular lattices and square ice are two simple models of geometrical frustration. We map their highly degenerated ground-state phase spaces as discrete networks such that network analysis tools can be introduced to phase-space studies. The resulting phase spaces establish a novel class of complex networks with Gaussian spectral densities. Although phase-space networks are heterogeneously connected, the systems are still ergodic except under periodic boundary conditions. We elucidate the boundary effects by mapping the two models as stacks of cubes and spheres in higher dimensions. Sphere stacking in various containers, i.e. square ice under various boundary conditions, reveals challenging combinatorial questions. This network approach can be generalized to phase spaces of some other complex systems.

cond-mat.stat-mech↗
arXiv2009

Particle dynamics in colloidal suspensions above and below the glass-liquid re-entrance transition

We study colloidal particle dynamics of a model glass system using confocal and fluorescence microscopy as the sample evolves from a hard-sphere glass to a liquid with attractive interparticle interactions. The transition from hard-sphere glass to attractive liquid is induced by short-range depletion forces. The development of liquid-like structure is indicated by particle dynamics. We identify particles which exhibit substantial motional events and characterize the transition using the properties of these motional events. As samples enter the attractive liquid region, particle speed during these motional events increases by about one order of magnitude, and the particles move more cooperatively. Interestingly, colloidal particles in the attractive liquid phase do not exhibit significantly larger displacements than particles in the hard-sphere glass.

cond-mat.soft↗
arXiv2008

Geometric Frustration in Buckled Colloidal Monolayers

Geometric frustration arises when lattice structure prevents simultaneous minimization of local interactions. It leads to highly degenerate ground states and, subsequently, complex phases of matter such as water ice, spin ice and frustrated magnetic materials. Here we report a simple geometrically frustrated system composed of closely packed colloidal spheres confined between parallel walls. Diameter-tunable microgel spheres are self-assembled into a buckled triangular lattice with either up or down displacements analogous to an antiferromagnetic Ising model on a triangular lattice. Experiment and theory reveal single-particle dynamics governed by in-plane lattice distortions that partially relieve frustration and produce ground-states with zigzagging stripes and subextensive entropy, rather than the more random configurations and extensive entropy of the antiferromagnetic Ising model. This tunable soft matter system provides an uncharted arena in which the dynamics of frustration, thermal excitations and defects can be directly visualized.

cond-mat.soft↗
arXiv2006

Colloidal Electrostatic Interactions Near a Conducting Surface

Charge-stabilized colloidal spheres dispersed in deionized water are supposed to repel each other. Instead, artifact-corrected video microscopy measurements reveal an anomalous long-ranged like-charge attraction in the interparticle pair potential when the spheres are confined to a layer by even a single charged glass surface. These attractions can be masked by electrostatic repulsions at low ionic strengths. Coating the bounding surfaces with a conducting gold layer suppresses the attraction. These observations suggest a possible mechanism for confinement-induced attractions.

cond-mat.soft↗