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Yin Shi

Publications and source records attributed to Yin Shi.

32 records · Page 2Linked to original sources

Universal phase dynamics in VO2 switches revealed by ultrafast operando diffraction

Strongly correlated materials that exhibit an insulator-metal transition are key candidates in the search for new computing platforms. Understanding the pathways and timescales underlying the electrically-driven insulator-metal transition is crucial for uncovering the fundamental limits of device operation. Using stroboscopic electron diffraction, we perform synchronized time-resolved measurements of atomic motions and electronic transport in operating vanadium dioxide switches. We discover an electrically-triggered, isostructural state that forms transiently on microsecond timescales, stabilized by local heterogeneities and interfacial interactions between the equilibrium phases. This metastable phase bears striking similarity to that formed under photoexcitation within picoseconds, suggesting a universal transformation pathway across eight orders of magnitude of timescale. Our results establish a new route for uncovering non-equilibrium and metastable phases in correlated materials, and open avenues for engineering novel dynamical behavior in nanoelectronics.

cond-mat.mtrl-sci↗

Landau theory of metal-insulator transition in VO$_\text{2}$ doped with metal ions

Metal-ion doping can effectively regulate the metal-insulator transition temperature in $\mathrm{VO}_2$. Experiments found that the pentavalent and hexavalent ion doping dramatically reduces the transition temperature while the trivalent ion doping increases the transition temperature and induces intermediate phases. Based on the phase-field model of the metal-insulator transition in $\mathrm{VO}_2$ we developed previously, we formulate a Landau potential of the metal-ion-doped $\mathrm{VO}_2$ taking account of the effects of doping on the electron correlation and lattice structure. The effect of metal-ion doping on the lattice structure is accounted for in a phenomenological way. Using the Landau potential, we calculate the temperature-dopant-concentration phase diagrams of $\mathrm{VO}_2$ doped with various metal ions consistent with the experiments and provide explanation to the different behaviors of different metal-ion doping. The phenomenological theory can provide estimations of phase diagrams of $\mathrm{VO}_2$ doped with other metal ions.

cond-mat.mtrl-sci↗

Transient Electronic Phase Separation During Metal-Insulator Transitions

From thermodynamic analysis we demonstrate that during metal-insulator transitions in pure matters, a nonequilibrium homogeneous state may be unstable against charge density modulations with certain wavelengths, and thus evolves to the equilibrium phase through transient electronic phase separation. This phase instability occurs as two inequalities between the first and the second derivatives of the free energy with respect to the order parameter are fulfilled. The dominant wavelength of the modulated phase is also derived. The computer simulation further confirms the theoretical derivation. Employing the pre-established phase-field model of VO$_2$, we show that this transient electronic phase separation may take place in VO$_2$ upon photoexcitation.

cond-mat.str-el↗

Isothermal current-driven insulator-to-metal transition in VO$_\text{2}$ through strong correlation effect

Electric current has been experimentally demonstrated to be able to drive the insulator-to-metal transition (IMT) in VO$_2$. The main mechanisms involved are believed to be the Joule heating effect and the strong electron-correlation effect. These effects are often entangled with each other in experiments, which complicates the understanding of the essential nature of the observations. We formulate a phase-field model to investigate theoretically in mesoscale the pure correlation effect brought by the current on the IMT in VO$_2$, i.e., the isothermal process under the current. We find that a current with a large density ($\sim 10^1$ nA/nm$^2$) induces a few-nanosecond ultrafast switch in VO$_2$, in agreement with the experiment. The temperature-current phase diagram is further calculated, which reveals that the current may induce the M2 phase at low temperatures. The current is also shown capable of driving domain walls to move. Our work may assist related experiments and provide guidance to the engineering of VO$_2$-based electric switching devices.

cond-mat.mtrl-sci↗

A new symmetry-based framework for discovering minimum energy pathways

Physical systems evolve from one state to another along paths of least energy barrier. Without a priori knowledge of the energy landscape, multidimensional search methods aim to find such minimum energy pathways between the initial and final states of a kinetic process. However in many cases, the user has to repeatedly provide initial guess paths, thus ensuring that the reliability of the final result is heavily user-dependent. Recently, the idea of "distortion symmetry groups" as a complete description of the symmetry of a path has been introduced. Through this, a new framework is enabled that provides a powerful means of classifying the infinite collection of possible pathways into a finite number of symmetry equivalent subsets, and then exploring each of these subsets systematically using rigorous group theoretical methods. The method is shown to lead to the discovery of new, previously hidden pathways for the case studies of bulk ferroelectric switching and domain wall motion in proper and improper ferroelectrics, as well as in multiferroic switching. This approach is applicable to a wide variety of physical phenomena ranging from structural, electronic and magnetic distortions, diffusion, and phase transitions in materials.

cond-mat.mtrl-sci↗

Generation of Gamma-ray Beam with Orbital Angular Momentum in the QED Regime

We propose a scheme to generate gamma-ray photons with an orbital angular momentum (OAM) and high energy simultaneously from laser-plasma interactions by irradiating a circularly polarized Laguerre-Gaussian laser on a thin plasma target. The spin angular momentum and OAM are first transferred to electrons from the driving laser photons, and then the OAM is transferred to the gamma-ray photons from the electrons through quantum radiation. This scheme has been demonstrated using three-dimensional quantum electrodynamics particle-in-cell simulation. The topological charge, chirality and carrier-envelope phase of the short ultra-intense vortex laser can be revealed according to the pattern feature of the energy density of radiated photons.

physics.plasm-ph↗

Generation of Ultra-intense Gamma-ray Train by QED Harmonics

When laser intensity exceeds 10^22W/cm^2, photons with energy above MeV can be generated from high-order harmonics process in the laser-plasma interaction. We find that under such laser intensity, QED effect plays a dominating role in the radiation pattern. Contrast to the gas and relativistic HHG processes, both the occurrence and energy of gamma-ray emission produced by QED harmonics are random and QED harmonics are usually not coherent, while the property of high intensity and ultra-short duration is conserved. Our simulation shows that the period of gamma-ray train is half of the laser period and the peak intensity is 1.4e22W/cm^2. This new harmonic production with QED effects are crucial to light-matter interaction in strong field and can be verified in experiments by 10PW laser facilities in the near future.

physics.plasm-ph↗

Hollow screw like drill in plasma using an intense Laguerre Gaussian laser

With the development of ultra intense laser technology, MeV ions from the laser foil interaction have been obtained by different mechanisms, such as target normal sheath acceleration, radiation pressure acceleration, collisionless shock acceleration, breakout afterburner, and a combination of different mechanisms. These energetic ion beams can be applied in fast ignition for inertial confinement fusion, medical therapy, and proton imaging. However, these ions are mainly accelerated in the laser propagation direction, and the ion acceleration in an azimuthal orientation is scarcely mentioned. Here, a doughnut Laguerre Gaussian LG laser is used for the first time to study the laser plasma interaction in the relativistic intensity regime in three dimensional particle in cell simulations. Studies have shown that a novel rotation of the plasma is produced from the hollow screw like drill of a LG mode laser. The angular momentum of the protons in the longitudinal direction produced by the LG laser is remarkably enhanced compared with that produced by the usual laser pulses, such as linearly and circularly polarized gaussian pulses. Moreover, the particles, including electrons and ions, can be trapped and uniformly compressed in the dark central minimum of the doughnut LG pulse. Such hollow structured LG laser may be used to investigate some difficult problems, such as screw like drilling in the inertial confinement fusion, laser driven particle accelerations, and pulsars in the astrophysical environment.

physics.plasm-ph↗

$(111)$ surface states of SnTe

The characterization and applications of topological insulators depend critically on their protected surface states, which, however, can be obscured by the presence of trivial dangling bond states. Our first principle calculations show that this is the case for the pristine $(111)$ surface of SnTe. Yet, the predicted surface states unfold when the dangling bond states are passivated in proper chemisorption. We further extract the anisotropic Fermi velocities, penetration lengths and anisotropic spin textures of the unfolded $\barΓ$- and $\bar M$-surface states, which are consistent with the theory in http://dx.doi.org/10.1103/PhysRevB.86.081303 Phys. Rev. B 86, 081303 (R). More importantly, this chemisorption scheme provides an external control of the relative energies of different Dirac nodes, which is particularly desirable in multi-valley transport.

cond-mat.mtrl-sci↗

Generation of Intense High-Order Vortex Harmonics

This paper presents the method for the first time to generate intense high-order optical vortices that carry orbital angular momentum in the extreme ultraviolet region. In three-dimensional particle-in-cell simulation, both the reflected and transmitted light beams include high-order harmonics of the Laguerre-Gaussian (LG) mode when a linearly polarized LG laser pulse impinges on a solid foil. The mode of the generated LG harmonic scales with its order, in good agreement with our theoretical analysis. The intensity of the generated high-order vortex harmonics is close to the relativistic region, and the pulse duration can be in attosecond scale. The obtained intense vortex beam possesses the combined properties of fine transversal structure due to the high-order mode and the fine longitudinal structure due to the short wavelength of the high-order harmonics. Thus, the obtained intense vortex beam may have extraordinarily promising applications for high-capacity quantum information and for high-resolution detection in both spatial and temporal scales because of the addition of a new degree of freedom.

physics.plasm-ph↗

Proton Acceleration in Underdense Plasma by Ultraintense Laguerre-Gaussian Laser Pulse

Three-dimensional particle-in-cell simulation is used to investigate the witness proton acceleration in underdense plasma with a short intense Laguerre-Gaussian (LG) laser pulse. Driven by the LG10 laser pulse, a special bubble with an electron pillar on the axis is formed, in which protons can be well-confined by the generated transversal focusing field and accelerated by the longitudinal wakefield. The risk of scattering prior to acceleration with a Gaussian laser pulse in underdense plasma is avoided, and protons are accelerated stably to much higher energy. In simulation, a proton beam has been accelerated to 7 GeV from 1 GeV in underdense tritium plasma driven by a 2.14x1022 W/cm2 LG10 laser pulse.

physics.plasm-ph↗

Light fan driven by relativistic laser pulse

When a relativistic laser pulse with high photon density interacts with a specially tailored thin foil target, a strong torque is exerted on the resulting spiral-shaped foil plasma, or light fan. Because of its structure, the latter can gain significant orbital angular momentum (OAM), and the opposite OAM is imparted to the reflected light, creating a twisted relativistic light pulse. Such an interaction scenario is demonstrated by particle-in-cell simulation as well as analytical modeling, and should be easily verifiable in the laboratory. As important characters, twisted relativistic light pulse has strong torque and ultra-high OAM density.

physics.plasm-ph↗

Positron acceleration in a hollow plasma channel up to TeV regime

We propose a plasma-based high-energy lepton accelerator, in which a weakly focusing plasma structure is formed near the beam axis. The structure preserves the emittance of the accelerated beam and produces low radiation losses. Moreover, the structure allows for a considerable decrease of the witness energy spread at the driver depletion stage.

physics.plasm-ph↗

Scheme for proton-driven plasma-wakefield acceleration of positively charged particles in a hollow plasma channel

A new scheme for accelerating positively charged particles in a plasma wakefield accelerator is proposed. If the proton drive beam propagates in a hollow plasma channel, and the beam radius is of order of the channel width, the space charge force of the driver causes charge separation at the channel wall, which helps to focus the positively charged witness bunch propagating along the beam axis. In the channel, the acceleration buckets for positively charged particles are much larger than in the blowout regime of the uniform plasma, and stable acceleration over long distances is possible. In addition, phasing of the witness with respect to the wave can be tuned by changing the radius of the channel to ensure the acceleration is optimal. Two dimensional simulations suggest that, for proton drivers likely available in future, positively charged particles can be stably accelerated over 1 km with the average acceleration gradient of 1.3 GeV/m.

physics.plasm-ph↗