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Ying Chan

Publications and source records attributed to Ying Chan.

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Collective spin excitations in trilayer nickelate La$_4$Ni$_3$O$_{10}$

Ruddlesden-Popper (RP) nickelates have recently emerged as a new family of high-temperature superconductors. In bilayer RP nickelates, magnetic excitations with large exchange couplings have been observed, supporting a spin-mediated pairing mechanism. Whether comparable spin correlations persist in trilayer nickelates, however, remains unknown. Here, we present a Ni $L$-edge resonant inelastic X-ray scattering (RIXS) study of La$_4$Ni$_3$O$_{10}$ single crystals. While the orbital excitations remain similar to those of La$_3$Ni$_2$O$_{7}$, the collective spin excitations in La$_4$Ni$_3$O$_{10}$ exhibit a comparable bandwidth of about $60$ meV but substantially suppressed spectral weight, implying a weaker electronic correlation in the trilayer compounds. Our results underscore the three-dimensional and multi-orbital electronic character in La$_4$Ni$_3$O$_{10}$, highlighting important differences from the bilayer nickelates. These findings provide crucial insights into the evolution of magnetism across the RP nickelate family and its connection to superconductivity.

cond-mat.supr-con

Impact of Electron Correlations on Infinite-Layer Cuprates and Nickelates

Optimization of unconventional superconductivity involves a balance of interaction strengths. Precise determination of correlation strength across different material families is therefore important. Here, we present a combined X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS) study of infinite-layer PrNiO$_2$ and SrCuO$_2$ that enables fair comparison of their interaction strengths. For both compounds, we study the orbital and magnetic excitations and extract their dispersions along high-symmetry directions. Using a single-band Hubbard model and including higher-order exchange interactions, we derive the correlation factor $U/t$ for both compounds. A key finding is that despite a smaller Coulomb repulsion $U$, PrNiO$_2$ exhibits a correlation strength that is 20% stronger than that of its isostructural cuprate counterpart SrCuO$_2$. This indicates that a moderation of the correlation strength may further optimize superconductivity in nickelates.

cond-mat.supr-con

Persistent paramagnons in high-temperature infinite-layer nickelate superconductors

The recent discovery of high-temperature superconductivity in hole-doped SmNiO$_2$, exhibiting the record-high transition temperature $T_c$ among infinite-layer (IL) nickelates, has opened a new avenue for exploring design principles of superconductivity. Experimentally determining the electronic structure and magnetic interactions in this new system is crucial to elucidating the mechanism behind the enhanced superconductivity. Here, we report a Ni $L$-edge resonant inelastic x-ray scattering (RIXS) study of superconducting Sm-based IL nickelate thin films Sm$_{1-x-y-z}$Eu$_x$Ca$_y$Sr$_z$NiO$_2$ (SECS). Dispersive paramagnonic excitations are observed in both optimally and overdoped SECS samples, supporting a spin-fluctuation-mediated pairing scenario. However, despite the two-fold enhancement of $T_c$ in the Sm-based nickelates compared to their Pr-based counterparts, the effective exchange coupling strength is reduced by approximately $20\%$. This behavior contrasts with hole-doped cuprates, where magnetic interactions correlate positively with $T_c$, highlighting essential differences in their superconducting mechanisms.

cond-mat.supr-con

Torus algebra and logical operators at low energy

Given a modular tensor category $\mathscr{C}$, we construct an associative algebra $\mathrm{Tor({\mathscr{C}}})$, which we call the torus algebra. We prove that the torus algebra is semisimple by explicitly constructing all the simple modules. Suppose that a topological ordered phase described by $\mathscr{C}$ is put on a torus. Physically, each simple module over $\mathrm{Tor({\mathscr{C}}})$ consists of the low energy states on the torus with one anyon excitation, or equivalently, the ground states on a punctured torus where the anyon is enclosed by the puncture. Elements in $\mathrm{Tor({\mathscr{C}}})$ can be physically interpreted as anyon hopping processes on the torus. We give the precise formula how an arbitrary logical operator on the low energy states on a torus can be realized by moving anyons on the torus. Our work thus provides a theoretical proposal that the low energy states on a torus can serve as topological qudits and one can arbitrarily manipulate them by moving anyons around.

cond-mat.str-el

Magnon interactions in a moderately correlated Mott insulator

Quantum fluctuations in low-dimensional systems and near quantum phase transitions have significant influences on material properties. Yet, it is difficult to experimentally gauge the strength and importance of quantum fluctuations. Here we provide a resonant inelastic x-ray scattering study of magnon excitations in Mott insulating cuprates. From the thin film of SrCuO$_2$, single- and bi-magnon dispersions are derived. Using an effective Heisenberg Hamiltonian generated from the Hubbard model, we show that the single-magnon dispersion is only described satisfactorily when including significant quantum corrections stemming from magnon-magnon interactions. Comparative results on La$_2$CuO$_4$ indicate that quantum fluctuations are much stronger in SrCuO$_2$ suggesting closer proximity to a magnetic quantum critical point. Monte Carlo calculations reveal that other magnetic orders may compete with the antiferromagnetic N\'eel order as the ground state. Our results indicate that SrCuO$_2$ - due to strong quantum fluctuations - is a unique starting point for the exploration of novel magnetic ground states.

cond-mat.str-el