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Ying Ran

Publications and source records attributed to Ying Ran.

At least 19 recordsLinked to original sources

HyperDet Wavefunction: A Phase-Agnostic Ansatz for Strongly Correlated Systems

Describing competing phases of strongly correlated systems often requires trial wave functions built from phase-specific assumptions. We propose the \emph{hyperdeterminant (HyperDet) wavefunction} as a phase-agnostic ansatz for both bosonic and fermionic quantum many-body systems exhibiting spontaneous symmetry-breaking order, fractionalization, and/or topological order with anyonic excitations. The HyperDet structure emerges naturally by fusing auxiliary fermionic parton Slater determinants into physical orbitals through a fully learnable \emph{fusion tensor} $\mathcal F$. Optimized using variational Monte Carlo, a single HyperDet architecture can achieve exceptionally high overlaps $\geq 99.9\%$ with exact-diagonalization ground states throughout the entire fractional Chern insulator phase in both bosonic and fermionic models, and across their nearby competing phases. We introduce the singular-value spectrum of the \emph{bipartite fusion matrix} as a structural diagnostic of fusion tensor, and find that its redistribution tracks many-body phase transitions without computing phase-specific observables. The optimized fusion tensor also encodes the parton-level topological data: it reproduces the parton Chern numbers expected for the bosonic and fermionic FCI states, completing their field-theory descriptions and the resulting topological order. Its intrinsic gauge structure further determines whether physical symmetries admit virtual lifts and, when faithful lifts exist, extracts their projective class; for the bosonic FCI, this recovers the expected parton translation fractionalization. We thus anticipate the HyperDet wavefunction to be a promising variational platform for both accurate ground-state searches and phase-diagram explorations across strongly correlated phases, and for providing interpretable theoretical insights from parton-level microscopics to field-theory descriptions.

cond-mat.str-el

Hyperdeterminant wavefunctions

We systematically introduce hyperdeterminant wavefunctions as a variational-wavefunction-based theoretical framework for strongly correlated quantum states of matter, together with practical numerical simulation algorithms. This framework generalizes previously known fermionic parton constructions, yields reliable microscopics with intuitive physical pictures, and allows direct access to the fractionalized degrees of freedom together with associated microscopic effective field theories. We demonstrate the applications of this framework to fractional Chern insulators and quantum spin liquids. We comment that the hyperdeterminant states belong to a more general class of variational wavefunctions: the fused Gaussian states.

cond-mat.str-el

Magnetoresistive Memory in the Paramagnetic Phase of Eu$_5$In$_2$As$_6$

Magnetoresistive materials that respond sensitively to applied fields are central to modern data storage technologies. Here we unveil a novel Magnetoresistive Memory (MRM) in Eu$_5$In$_2$As$_6$, where the electrical resistivity depends not only on the magnitude but also on the history of the applied magnetic field. Such an effect has been reported in only two classes of strongly correlated electron systems: perovskite manganites and pyrochlore iridates. In both cases, the effect has been observed in the magnetically ordered phase. It has been attributed to metastable magnetic states in manganites and conducting domain walls in iridates. Remarkably, the MRM in Eu$_5$In$_2$As$_6$ onsets at twice the antiferromagnetic transition temperature, well within the paramagnetic phase. The temperature, field, and time dependence of resistivity suggest that either a hidden order or a fluctuating phase with short-range correlations underlies this effect. Our results offer MRM as a new platform for quantum sensing and memory technologies, and encourage searching for MRM in related materials.

cond-mat.str-el

Transverse Photoresistivity from Photothermal Current Deflection in Metal Films

Quantum geometry in centrosymmetric systems has motivated the search for photocurrent responses beyond second order. In particular, electric field-induced nonlinear responses may also enable intrinsic polarization-sensitive optical detectors. Despite numerous efforts, clear methods are still needed to remove experimental artifacts, separating intrinsic from extrinsic effects, and disentangling linear responses from their higher-order counterparts. Here, we provide a systematic study of fabrication and measurement techniques to remove external artifacts in photoelectronic responses. This reveals a previously hidden photothermoelectric response in the transverse photoresistivity of symmetric thin films of simple metals. We identify its origin in thermal gradients producing current deflection and determine the device design and measurement parameters to minimize extrinsic effects that arise in photoinduced electronic responses.

cond-mat.mtrl-sci

Composite Fermion Theory of Fractional Chern Insulator Stability

We develop a mean-field theory of the stability of fractional Chern insulators based on the dipole picture of composite fermions (CFs). We construct CFs by binding vortices to Bloch electrons and derive a CF single-particle Hamiltonian that describes a Hofstadter problem in the enlarged CF Hilbert space, with the trace-condition term emerging naturally in the small-$q$ limit as part of the CF Hamiltonian. Going beyond the small-$q$ limit, we apply our theory to twisted MoTe$_2$ and calculate its CF band structures. The resulting CF phase diagram matches closely with that from exact diagonalization, and the projected many-body wavefunctions achieve exceptionally high overlaps with the latter. Our theory provides both a microscopic understanding and a computationally efficient tool for identifying fractional Chern insulators.

cond-mat.str-el

Pressure tuning of competing interactions on a honeycomb lattice

Magnetic exchange interactions are mediated via orbital overlaps across chemical bonds. Thus, modifying the bond angles by physical pressure or strain can tune the relative strength of competing interactions. Here we present a remarkable case of such tuning between the Heisenberg (J) and Kitaev (K) exchange, which respectively establish magnetically ordered and spin liquid phases on a honeycomb lattice. We observe a rapid suppression of the Neel temperature (TN) with pressure in Ag3LiRh2O6, a spin-1/2 honeycomb lattice with both J and K couplings. Using a combined analysis of x-ray data and first-principles calculations, we find that pressure modifies the bond angles in a way that increases the |K/J| ratio and thereby suppresses TN. Consistent with this picture, we observe a spontaneous onset of muon spin relaxation (muSR) oscillations below TN at low pressure, whereas in the high-pressure phase, oscillations appear only when T < TN/2. Unlike other candidate Kitaev materials, Ag3LiRh2O6 is tuned toward a quantum critical point by pressure while avoiding a structural dimerization in the relevant pressure range.

cond-mat.str-el

Hyperdeterminants and Composite fermion States in Fractional Chern Insulators

Fractional Chern insulators (FCI) were proposed theoretically about a decade ago. These exotic states of matter are fractional quantum Hall states realized when a nearly flat Chern band is partially filled, even in the absence of an external magnetic field. Recently, exciting experimental signatures of such states have been reported in twisted MoTe$_2$ bilayer systems. Motivated by these experimental and theoretical progresses, in this paper, we develop a projective construction for the composite fermion states (either the Jain's sequence or the composite Fermi liquid) in a partially filled Chern band with Chern number $C=\pm1$, which is capable of capturing the microscopics, e.g., symmetry fractionalization patterns and magnetoroton excitations. On the mean-field level, the ground states' and excitated states' composite fermion wavefunctions are found self-consistently in an enlarged Hilbert space. Beyond the mean-field, these wavefunctions can be projected back to the physical Hilbert space to construct the electronic wavefunctions, allowing direct comparison with FCI states from exact diagonalization on finite lattices. We find that the projected electronic wavefunction corresponds to the \emph{combinatorial hyperdeterminant} of a tensor. When applied to the traditional Galilean invariant Landau level context, the present construction exactly reproduces Jain's composite fermion wavefunctions. We apply this projective construction to the twisted bilayer MoTe$_2$ system. Experimentally relevant properties are computed, such as the magnetoroton band structures and quantum numbers.

cond-mat.str-el

Fractional Chern Insulator in Twisted Bilayer MoTe$_2$

A recent experiment has reported the first observation of a zero-field fractional Chern insulator (FCI) phase in twisted bilayer MoTe$_2$ moiré superlattices [Nature 622, 63-68 (2023)]. The experimental observation is at an unexpected large twist angle 3.7$^\circ$ and calls for a better understanding of the FCI in real materials. In this work, we perform large-scale density functional theory calculation for the twisted bilayer MoTe$_2$, and find that lattice reconstruction is crucial for the appearance of an isolated flat Chern band. The existence of the FCI state at $ν= -2/3$ are confirmed by exact diagonalization. We establish phase diagrams with respect to the twist angle and electron interaction, which reveal an optimal twist angle of $3.5^\circ$ for the observation of FCI. We further demonstrate that an external electric field can destroy the FCI state by changing band geometry and show evidence of the $ν=-3/5$ FCI state in this system. Our research highlights the importance of accurate single particle band structure in the quest for strong correlated electronic states and provides insights into engineering fractional Chern insulator in moiré superlattices.

cond-mat.str-el

Supercurrent-induced Anomalous Thermal Hall Effect as a New Probe to Superconducting Gap Anisotropy

Two-dimensional superconductors have been realized in various atomically thin films such as the twisted bilayer graphene, some of which are anticipated to involve unconventional pairing mechanism. Due to their low dimensionality, experimental probes of the exact nature of superconductivity in these systems have been limited. We propose, by applying a \emph{vertical} supercurrent to a bilayer superconductor where the mirror symmetry is naturally broken by the twisting, there will be anomalous thermal Hall effect induced by the supercurrent that can serve as a sharp probe for the \emph{in-plane} anisotropy of the superconducting gap function. This effect occurs in the \emph{absence} of an external magnetic field and spontaneous breaking of the time-reversal symmetry in the ground state. We derive explicit formulas for the induced thermal Hall conductivity and show them to be significant in the examples of twisted cuprates and twisted FeSe where monolayer superconductivity have already been observed. Though technical challenges still exist, we propose this to be a generic probe of the gap anisotropy in a twisted bilayer superconductor.

cond-mat.supr-con

Signatures of Fractional Quantum Anomalous Hall States in Twisted MoTe2 Bilayer

The interplay between spontaneous symmetry breaking and topology can result in exotic quantum states of matter. A celebrated example is the quantum anomalous Hall (QAH) state, which exhibits an integer quantum Hall effect at zero magnetic field thanks to its intrinsic ferromagnetism. In the presence of strong electron-electron interactions, exotic fractional-QAH (FQAH) states at zero magnetic field can emerge. These states could host fractional excitations, including non-Abelian anyons - crucial building blocks for topological quantum computation. Flat Chern bands are widely considered as a desirable venue to realize the FQAH state. For this purpose, twisted transition metal dichalcogenide homobilayers in rhombohedral stacking have recently been predicted to be a promising material platform. Here, we report experimental signatures of FQAH states in 3.7-degree twisted MoTe2 bilayer. Magnetic circular dichroism measurements reveal robust ferromagnetic states at fractionally hole filled moiré minibands. Using trion photoluminescence as a sensor, we obtain a Landau fan diagram which shows linear shifts in carrier densities corresponding to the v=-2/3 and -3/5 ferromagnetic states with applied magnetic field. These shifts match the Streda formula dispersion of FQAH states with fractionally quantized Hall conductance of -2/3$e^2/h$ and -3/5$e^2/h$, respectively. Moreover, the v=-1 state exhibits a dispersion corresponding to Chern number -1, consistent with the predicted QAH state. In comparison, several non-ferromagnetic states on the electron doping side do not disperse, i.e., are trivial correlated insulators. The observed topological states can be further electrically driven into topologically trivial states. Our findings provide clear evidence of the long-sought FQAH states, putting forward MoTe2 moiré superlattices as a fascinating platform for exploring fractional excitations.

cond-mat.mes-hall

Visualizing bulk and edge photocurrent flow in anisotropic Weyl semimetals

Materials that rectify light into current in their bulk are desired for optoelectronic applications. In inversion-breaking Weyl semimetals, bulk photocurrents may arise due to nonlinear optical processes that are enhanced near the Weyl nodes. However, the photoresponse of these materials is commonly studied by scanning photocurrent microscopy (SPCM), which convolves the effects of photocurrent generation and collection. Here, we directly image the photocurrent flow inside the type-II Weyl semimetals WTe2 and TaIrTe4 using high-sensitivity quantum magnetometry with nitrogen-vacancy center spins. We elucidate an unknown mechanism for bulk photocurrent generation termed the anisotropic photothermoelectric effect (APTE), where unequal thermopowers along different crystal axes drive intricate circulations of photocurrent around the photoexcitation. Using simultaneous SPCM and magnetic imaging at the sample's interior and edges, we visualize how the APTE stimulates the long-range photocurrent collected in our Weyl semimetal devices through the Shockley-Ramo theorem. Our results highlight an overlooked, but widely relevant source of current flow and inspire novel photodetectors using homogeneous materials with anisotropy.

cond-mat.mtrl-sci

Engineering chiral topological superconductivity in twisted Ising superconductors

Van der Waals materials like NbSe$_2$ or TaS$_2$ have demonstrated Ising superconductivity down to atomically thin layers. Due to the spin-orbit coupling, these superconductors have the in-plane upper critical magnetic field far beyond the Pauli limit. We theoretically demonstrate that, twisted bilayer Ising superconductors separated by a ferromagnetic buffer layer can naturally host chiral topological superconductivity with Chern numbers, which can be realized in heterostructures like $\mathrm{NbSe_2/CrCl_3/NbSe_2}$. Under appropriate experimental conditions the topological superconducting gap can reach $>0.1$ meV, leading to readily observable signatures such as the quantized thermal Hall transport at low temperatures.

cond-mat.supr-con

First demonstration of tuning between the Kitaev and Ising limits in a honeycomb lattice

Recent observations of novel spin-orbit coupled states have generated tremendous interest in $4d/5d$ transition metal systems. A prime example is the $J_{\text{eff}}=\frac{1}{2}$ state in iridate materials and $α$-RuCl$_{3}$ that drives Kitaev interactions. Here, by tuning the competition between spin-orbit interaction ($λ_{\text{SOC}}$) and trigonal crystal field splitting ($Δ_\text{T}$), we restructure the spin-orbital wave functions into a novel $μ=\frac{1}{2}$ state that drives Ising interactions. This is done via a topochemical reaction that converts Li$_{2}$RhO$_{3}$ to Ag$_{3}$LiRh$_{2}$O$_{6}$, leading to an enhanced trigonal distortion and a diminished spin-orbit coupling in the latter compound. Using perturbation theory, we present an explicit expression for the new $μ=\frac{1}{2}$ state in the limit $Δ_\text{T}\gg λ_{\text{SOC}}$ realized in Ag$_{3}$LiRh$_{2}$O$_{6}$, different from the conventional $J_\text{eff}=\frac{1}{2}$ state in the limit $λ_{\text{SOC}}\gg Δ_\text{T}$ realized in Li$_{2}$RhO$_{3}$. The change of ground state is followed by a dramatic change of magnetism from a 6 K spin-glass in Li$_{2}$RhO$_{3}$ to a 94 K antiferromagnet in Ag$_{3}$LiRh$_{2}$O$_{6}$. These results open a pathway for tuning materials between the two limits and creating a rich magnetic phase diagram.

cond-mat.mtrl-sci

Accessing new magnetic regimes by tuning the ligand spin-orbit coupling in van der Waals magnets

Van der Waals (VdW) materials have opened new directions in the study of low dimensional magnetism. A largely unexplored arena is the intrinsic tuning of VdW magnets toward new ground-states. The chromium trihalides provided the first such example with a change of inter-layer magnetic coupling emerging upon exfoliation. Here, we take a different approach to engineer new ground-states, not by exfoliation, but by tuning the spin-orbit coupling (SOC) of the non-magnetic ligand atoms (Cl,Br,I). We synthesize a three-halide series, CrCl$_{3-x-y}$Br$_{x}$I$_{y}$, and map their magnetic properties as a function of Cl, Br, and I content. The resulting triangular phase diagrams unveil a frustrated regime near CrCl$_{3}$. First-principles calculations confirm that the frustration is driven by a competition between the chromium and halide SOCs. Furthermore, we reveal a field-induced change of inter-layer coupling in the bulk of CrCl$_{3-x-y}$Br$_{x}$I$_{y}$ crystals at the same field as in the exfoliation experiments.

cond-mat.mtrl-sci

Nonreciprocal directional dichroism induced by a temperature gradient as a probe for mobile spin dynamics in quantum magnets

Novel states of matter in quantum magnets like quantum spin liquids attract considerable interest recently. Despite the existence of a plenty of candidate materials, there is no confirmed quantum spin liquid, largely due to the lack of proper experimental probes. For instance, spectrosocopy experiments like neutron scattering receive contributions from disorder-induced local modes, while thermal transport experiments receive contributions from phonons. Here we propose a thermo-optic experiment which directly probes the mobile magnetic excitations in spatial-inversion symmetric and/or time-reversal symmetric Mott insulators: the temperature-gradient-induced nonreciprocal directional dichroism (TNDD) spectroscopy. Unlike traditional probes, TNDD directly detects mobile magnetic excitations and decouples from phonons and local magnetic modes.

cond-mat.str-el

Filling-enforced constraint on the quantized Hall conductivity on a periodic lattice

We discuss quantum Hall effects in a gapped insulator on a periodic two-dimensional lattice. We derive a universal relation among the the quantized Hall conductivity, and charge and flux densities per physical unit cell. This follows from the magnetic translation symmetry and the large gauge invariance, and holds for a very general class of interacting many-body systems. It can be understood as a combination of Laughlin's gauge invariance argument and Lieb-Schultz-Mattis-type theorem. A variety of complementary arguments, based on a cut-and-glue procedure, the many-body electric polarization, and a fractionalization algebra of magnetic translation symmetry, are given. Our universal relation is applied to several examples to show nontrivial constraints. In particular, a gapped ground state at a fractional charge filling per physical unit cell must have either a nonvanishing Hall conductivity or anyon excitations, excluding a trivial Mott insulator.

cond-mat.str-el

Competing Spin Liquid Phases in the S=$\frac{1}{2}$ Heisenberg Model on the Kagome Lattice

The properties of ground state of spin-$\frac{1}{2}$ kagome antiferromagnetic Heisenberg (KAFH) model have attracted considerable interest in the past few decades, and recent numerical simulations reported a spin liquid phase. The nature of the spin liquid phase remains unclear. For instance, the interplay between symmetries and $Z_2$ topological order leads to different types of $Z_2$ spin liquid phases. In this paper, we develop a numerical simulation method based on symmetric projected entangled-pair states (PEPS), which is generally applicable to strongly correlated model systems in two spatial dimensions. We then apply this method to study the nature of the ground state of the KAFH model. Our results are consistent with that the ground state is a $U(1)$ Dirac spin liquid rather than a $Z_2$ spin liquid.

cond-mat.str-el

Bosonic SET to SPT Transition under Dyonic LSM Theorem

Employing large-scale quantum Monte Carlo simulatoins, we study the phase diagram of a quantum spin model which is subject to the recently developed dyonic Lieb-Shultz-Mattis (LSM) theorem. The theorem predicts there are symmetry enriched/protected topological (SET/SPT) phases in the phase diagram. Our numerical results reveal a first order quantum phase transition between SET and SPT phases, consistent with an anyon condensation mechanism that enforces SPT phase according to the theorem. Also there exists in the phase diagram a symmetry-breaking phase in the form of superfluid (SF). The transition between SET and SF is continuous and that between SPT and SF is first order. Interestingly, the SET, SPT and SF phases meet at a critical endpoint, whose presence can be universally explained via theory contains emergent gauge field coupled to vortex fields, and consequently reveals the exotic feature of our model even beyond the realm of dyonic LSM.

cond-mat.str-el