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Ying Yin Tsui

Publications and source records attributed to Ying Yin Tsui.

5 recordsLinked to original sources

An Integrated DFT-FDTD Design of Plasmon-Enhanced Lead-Free $CsSn$$_x$$Ge$$_{1-x}$$I$$_3$ Perovskite LEDs

CsSn$_x$Ge$_{1-x}$I$_3$ as lead-free perovskites are promising for next generation NIR emitting perovskite LEDs due to their tunable bandgaps and stability. However, they suffer from poor light extraction efficiency, and accurate composition-specific optical data for these materials remain scarce. This study presents a DFT-FDTD framework to optimize light extraction via compositional tuning and plasmonic enhancement. First, DFT calculations were performed to obtain composition-specific complex refractive index and extinction coefficient values for $x = 0, 0.25, 0.5, 0.75$, and $1$. Results show bandgap increased from 1.331 eV for CsSnI$_3$ to 1.927 eV for CsGeI$_3$ with increasing Ge content, while refractive index ranges from 2.2 to 2.6 across compositions. These optical constants were then used as inputs for FDTD simulations of a PeLED structure with optimized Au/SiO$_2$ core-shell nanorods for plasmonic enhancement. A 12.1-fold Purcell enhancement was achieved for CsSn$_{0.25}$Ge$_{0.75}$I$_3$, while light extraction efficiency reached 25% for CsSn$_{0.5}$Ge$_{0.5}$I$_3$. LEE enhancement of 36% was obtained for CsSnI$_3$, and spectral overlap between emitter and plasmon resonance reached 96% for Sn-rich compositions. Design guidelines indicate CsSn$_{0.5}$Ge$_{0.5}$I$_3$ offers optimal balance of extraction efficiency (25%), Purcell enhancement (5.3$\times$), spectral overlap (93%), and oxidation stability for wearable and flexible optoelectronic applications, while CsSn$_{0.25}$Ge$_{0.75}$I$_3$ is recommended for applications prioritizing spontaneous emission rate.

physics.optics↗

Composition-Dependent Plasmon-Enhanced Emission in Lead-Free Cs$_3$Cu$_2$X$_5$ Halides: A DFT--FDTD Study

Lead-free Cs$_3$Cu$_2$X$_5$ (X = Cl, Br, I) halides exhibit high photoluminescence quantum yields and excellent ambient stability, yet light-emitting devices based on these materials remain limited by poor optical outcoupling. In this work, we develop an integrated density functional theory (DFT) and finite-difference time-domain (FDTD) framework to establish quantitative links between halide composition, wavelength-dependent optical constants, and plasmonic enhancement. First-principles calculations are used to obtain composition-specific refractive index (n) and extinction coefficient (k) spectra, which are directly implemented into three-dimensional FDTD simulations of a complete PeLED stack incorporating Ag/SiO$_2$ core--shell nanostructures. Among the investigated compositions, Cs$_3$Cu$_2$Cl$_5$ demonstrates the strongest plasmonic response, achieving a 4.4$\times$ Purcell enhancement and 30\% light extraction efficiency (LEE) using optimized nanorods. The superior performance originates from its lower refractive index, which reduces dielectric screening and improves near-field coupling. Cs$_3$Cu$_2$Br$_5$ exhibits the highest spectral overlap ($J_{\mathrm{cos}} = 0.955$) but yields moderate extraction (26%) due to increased optical confinement. Cs$_3$Cu$_2$I$_5$ requires a nanosphere geometry and shows limited enhancement, with LEE restricted to 10%. Distance-ependent analysis reveals composition-specific optimal emitter--plasmon separations, ranging from 8--12 nm for Cs$_3$Cu$_2$Br$_5$ to approximately 15 nm for Cs$_3$Cu$_2$Cl$_5$. These results provide composition-dependent design guidelines for plasmon-enhanced lead-free PeLEDs and highlight the critical role of accurate optical constants in predictive device optimization.

physics.optics↗

Tamm Plasmon--Enhanced Widely Tunable Near-Infrared Nanolaser with Superior Efficiency and Output Power

Plasmonic resonances enable strong electromagnetic field confinement and have been widely exploited in plasmonic nanolasers, particularly through surface plasmon polaritons and localized surface plasmons. However, their performance is often limited by bidirectional output coupling and multimode far-field emission, primarily due to higher-order diffraction arising from these modes. In this work, we utilize the Tamm plasmon resonance to realize lasing in the NIR region with wide tunability. The optical Tamm states are excited at the metal-DBR interface by an incident pump pulse and their emission intensity is significantly enhanced via extraordinary optical transmission through a metallic nanohole array. The subwavelength periodicity of the nanohole array restricts the emission to the zeroth order, resulting in a highly directional far-field pattern with a full width at half maximum of approximately 0.631 degrees. To further improve performance, a second DBR is incorporated beneath the pump side, which substantially suppresses backward emission around the lasing wavelength and enhances forward lasing intensity by around 1.3 X 10^4 times, thus increasing the integrated emission power. The combination of Tamm plasmon excitation and dual-DBR feedback significantly improves the cavity's optical response and overall lasing efficiency. Additionally, we have demonstrated lasing at 870 nm with a reduced pump threshold of 2.8 X 10^7 V/m (energy of 0.0031 mJ/cm^2). Moreover, a broad tunability in lasing wavelength, spanning from 850 nm to 944.5 nm, is achieved. These results demonstrate a cost-effective and versatile strategy for plasmonic nanolasers with enhanced output power, low reflection-side loss, wide tunability, and strong integration potential for on-chip photonic and quantum technologies.

physics.optics↗

Compact Plasmonic Logic Gates Enabled by Magnetoelectric Light Funneling for On-Chip Optical Computing in the Telecom Band

The realization of all-optical logic gates (AOLGs) is important for advancing photonic integrated circuit (PIC) design and optical data communication. Various photonic structures and design techniques, including two-dimensional photonic crystals, silicon waveguides, plasmonic waveguides, diffractive neural networks, and inverse design techniques, are actively being explored to achieve multifunctional, high-performance optical logic gates with fast data processing capabilities. Among these, plasmonic structure-based AOLGs often face challenges such as fabrication complexity and large device footprints when integrating multiple logic operations within a single structure. In this work, a planar and compact metal-insulator-metal (MIM) plasmonic waveguide structure is proposed for AOLG design, utilizing the light funneling effect in grooved metasurfaces. The designed device, with dimensions of 700 nm X 460 nm, successfully implements three fundamental logic gates (NOT, AND, OR) with a high contrast ratio of 18.69 dB. The device operates within the wavelength range of 1400 nm to 1450 nm, making it suitable for the telecommunications field. Its planar architecture offers fabrication feasibility and all logic gates can be controlled using a single light source incident from one specific direction, which facilitates its integration into photonic circuits with fast operational speed. This work contributes to the advancement of scalable and high-speed photonic computing platforms.

physics.optics↗

Inverse Design Optimization of MIS Nanorod Array to Enhance Wavelength-Selective Light Extraction of OLED through Guided SPCE

One of the primary causes of low light extraction efficiency (LEE) in conventional OLEDs is the trapping of light within the substrate layer. To overcome this limitation, various nanostructures have recently been investigated for integration into different OLED layers, aiming to convert the trapped loss modes into out-coupled light and thereby improve LEE. In this work, we propose a simple yet innovative nanorod array design composed of metal, insulator, and semiconductor-oxide layers, integrated on the bottom surface of the OLED structure. This configuration enhances light extraction through guided surface plasmon-coupled emission (SPCE). Using an inverse design-based optimization approach, the structural parameters of the nanorods were optimized to achieve wavelength-selective LEE enhancement. The periodic MIS nanorod array was optimized via the Particle Swarm Optimization (PSO) algorithm for different emission wavelengths, yielding improvements of 29\%, 30\%, and 51\% at 440 nm, 550 nm, and 540 nm, respectively, compared with conventional OLEDs. In addition, the optimized arrays demonstrate high spectral luminous efficiency (SLE), reduced UV transmittance, and uniform emission directionality. These enhancements have significant potential to advance OLED-based display technologies.

physics.optics↗