arXiv subjects

Yinglin Song

Publications and source records attributed to Yinglin Song.

3 recordsLinked to original sources

arXiv2024

Dual-grating single-shot pump-probe technique

A simple and effective single-shot pump-probe technique is reported for studying the ultrafast dynamic processes in various materials. Using only two commercial gratings, a large time window of ~ 95.58 ps is spatially encoded in a single probe pulse, and single-shot time-resolved measurements are implemented. This time window exceeds the maximum reported values for single-shot pump-probe techniques using the echelon or angle beam encoding strategy. The phase difference problem in the echelon encoding strategies is also eliminated and a customized echelon is not needed in this technique. The ultrafast dynamic processes of ZnSe and indolium squaraine at a wavelength of 650 nm were investigated using this technique.

physics.optics↗

arXiv2023

Single-shot pump-probe technique by the combination of an echelon and a grating with a time window of 109 ps

In this study, using only a single pulse, pump-probe measurement with a large time window of more than 100 ps is implemented. A commercial grating is used to encode a time window of ~ 56 ps in a single pulse; therefore, there is no need for machining customization. In addition, in this technique, the grating surface is accurately imaged, eliminating the image blur problem caused by phase differences in previous echelon-based techniques. Moreover, to make full use of the grating surface and obtain a larger time window, a simple reflection echelon is combined that matches the grating in the time window. This combination encoding strategy results in a total time window of ~ 109 ps and maintains accurate imaging of the grating surface. This time window is an order of magnitude greater than the maximum reported values of the echelon encoding strategy and the angle beam encoding strategy. To demonstrate this single-shot pump-probe technique, the two-photon absorption process of ZnSe and the excited-state absorption process of a symmetrical phenoxazinium bromine salt were studied. The possibility of further improving the experimental setup is also discussed.

physics.optics↗

arXiv2018

Origin of Improved Photoelectrochemical Water Splitting in Mixed Perovskite Oxides

Owing to the versatility in their chemical and physical properties, transition metal perovskite oxides have emerged as a new category of highly efficient photocatalysts for photoelectrochemical water splitting. Here, to understand the underlying mechanism for the enhanced photoelectrochemical water splitting in mixed perovskites, we explore ideal epitaxial thin films of the BiFeO3-SrTiO3 system. The electronic struture and carrier dynamics are determined from both experiment and density-functional theory calculations. The intrinsic phenomena are measured in this ideal sytem, contrasting to commonly studied polycrstalline solid solutions where extrinsic structural features obscure the intrinsic phenomena. We determined that when SrTiO3 is added to BiFeO3 the conduction band minimum position is raised and an exponential tail of trap states from hybridized Ti 3d and Fe 3d orbitals emerges near the conduction band edge. The presence of these trap states strongly suppresses the fast electron-hole recombination and improves the photocurrent density in the visible-light region, up to 16 times at 0 VRHE compared to the pure end member compositions. Our work provides a new design approach for optimising the photoelectrochemical performance in mixed perovksite oxides.

cond-mat.mtrl-sci↗