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Yiting Feng

Publications and source records attributed to Yiting Feng.

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Modulation of the Nernst Thermoelectrics by Regulating the Anomalous Hall and Nernst Angles

The large anomalous Nernst effect in magnetic Weyl semimetals is one of the most intriguing transport phenomena, which draws significant attention for its potential applications in topological thermoelectrics. Despite frequent reports of substantial anomalous Nernst conductivity (ANC), methods to optimize Nernst thermoelectrics remain limited. Our research reveals that the magnitude of the ANC is directly related to the sum of the anomalous Nernst and Hall angles. While the sign of the anomalous Hall angle is relatively stable in a certain material, the sign of the anomalous Nernst angle can be intrinsically tuned. Therefore, the ANC can be effectively optimized by regulating these angles to work in concert. This finding is verified by experimental modulation from iron-doped magnetic topological material Co3Sn2S2. Additionally, we observed a robust TlnT scaling law of the ANC over the temperature range of 40 to 140 K in all studied samples, suggesting an intrinsic origin of the ANC. Considering the common opposite sign of the anomalous Nernst and Hall angles in many magnetic topological materials, our research offers an applicable scheme for optimizing the Nernst thermoelectrics.

cond-mat.mtrl-sci

Observation of hydrostatic-pressure-modulated giant caloric effect and electronic topological transition

Phase transition is a fundamental phenomenon in condensed matter physics, in which states of matter transform to each other with various critical behaviors under different conditions. The magnetic martensitic transformation features significant multi-caloric effects that benefit the solid-state cooling or heat pumping. Meanwhile, the electronic topological transition (ETT) driven by pressure has been rarely reported in martensitic systems. Here, the modulation effects of hydrostatic pressure on phase transitions in a magnetic martensitic alloy are reported. Owing to the huge volume expansion during the transition, the martensitic transition temperature is driven from 339 to 273 K by pressure within 1 GPa, resulting in highly tunable giant baro- and magneto-caloric effects (BCE and MCE) in a wide working temperature range. Interestingly, an ETT was further induced by pressure in the martensite phase, with a sudden drop of the measured saturation magnetization around 0.6 GPa. First-principles calculations reveal a sharp change in the density of states (DOS) due to the orbit shift around the Fermi level at the same pressure and reproduce the experimental observation of magnetization. Besides, the ETT is accompanied by remarkable changes in the lattice parameters and the unit-cell orthorhombicity. The study provides insight into pressure-modulated exotic phase-transition phenomena in magnetic martensitic systems.

cond-mat.mtrl-sci

Evolution of structure, magnetism, and electronic/thermal-transports of Ti(Cr)-substituted Fe2CrV all-d-metal Heusler ferromagnets

All-d-metal full-Heusler alloys possess superior mechanical properties and high spin polarization, which would play an important role in spintronic applications. Despite this, their electrical and thermal transport properties have not been comprehensively investigated till now. In this work, we present an analysis on the evolution of structural, magnetic and transport properties of Cr- and Ti-substituted Fe2CrV all-d-metal Heusler alloys by combining theoretical calculations and experiments. Both series of alloys crystallize in Hg2CuTi-type structure. With increasing Ti doping, the calculated total magnetic moments of Fe50Cr25V25-xTix decrease linearly. The experimental saturation magnetization is highly consistent with theoretical calculations and Slater-Pauling rule when x < 4, indicating the highly ordered atomic occupation. The magnetization and Curie temperature can be significantly tuned by altering spin polarizations and exchange interactions. The introduction of the foreign atom, Ti, results in a linear increase in residual resistivity, while electron-phonon scattering keeps relatively constant. The maximum values for electrical and thermal transport properties are observed in the stoichiometric Fe2CrV composition.

cond-mat.mtrl-sci