arXiv subjects

Yogesh Singh

Publications and source records attributed to Yogesh Singh.

At least 19 recordsLinked to original sources

arXiv2026

Observation of linear magnetoresistance and planar Hall effect in the Dirac semimetal PdTe

PdTe is a Dirac semimetal that also exhibits superconductivity, providing an intriguing platform to explore topological superconductivity and unconventional magnetotransport phenomena. While the superconducting properties of PdTe have been extensively studied in recent years, the detailed magnetotransport phenomena have remained unexplored. Here, we present the first observation of linear magnetoresistance (LMR) and the planar Hall effect (PHE) in a high-quality single crystal of PdTe. We observe temperature-dependent unsaturated LMR in both in-plane ($B \parallel I$) and out-of-plane ($B \perp I$) configurations. The magnetoresistance (MR) shows a crossover from parabolic to linear dependence at the critical field Bc, and detailed analysis indicates that disorder-driven mobility fluctuations are the origin rather than the Abrikosov quantum-limit mechanism. Furthermore, prominent PHE has been observed by rotating the magnetic field within the plane of the sample. The detailed analysis of the field and temperature dependence of PHE-amplitude, along with the parametric plot, suggests that PHE originates predominantly from the anisotropic orbital magnetoresistance rather than the chiral anomaly. Our results demonstrate that although the Dirac point is close to the Fermi level, the observed LMR and PHE in the Dirac semimetal PdTe can be understood within a semiclassical transport framework, highlighting the importance of distinguishing between topological and conventional classical transport mechanisms in topological materials

cond-mat.mes-hall↗

arXiv2026

Role of Disorder in Governing the Magnetic Properties of Cu2IrO3

Cu$_2$IrO$_3$ is a honeycomb iridate which has been studied recently as a candidate Kitaev quantum spin liquid. Its magnetic ground state however, has been reported to be quantum disordered, spin glassy, or magnetically ordered depending on synthesis details. We have prepared a Cu$_2$IrO$_3$ sample with large antisite disorder and studied in detail its structure (global and local), charge states, and thermodynamic properties to try to quantify and characterize the disorder and its connection to the magnetic ground state. X-ray diffraction, Extended x-ray absorption fine structure(EXAFS) and X-ray pair distribution function analysis revealed a large site disorder ($\sim$25\%), while XPS and XANES reveal mixed valence of Cu and Ir following Cu$^{1+}$ + Ir$^{4+}$ $\rightarrow$ Cu$^{2+}$ + Ir$^{3+}$. This combination of site disorder and charge redistribution generates competing antiferromagnetic interactions and magnetic frustration, resulting in dynamically fluctuating AFM clusters near 80K that freeze below 29K. These results demonstrate the crucial role of synthesis dependent disorder in determining the magnetic ground state of Cu$_2$IrO$_3$.

cond-mat.str-el↗

arXiv2025

Magnetic Frustration in CuYbSe$_2$: an Yb-Based Triangular Lattice Selenide

The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect triangular lattice of Yb$^{3+}$ moments. Magnetic susceptibility and heat capacity measurements reveal no evidence of long-range magnetic ordering down to $1.8$~K in spite of a significant antiferromagnetic exchange between Yb$^{3+}$ moments, suggesting a frustrated magnetic system. Electrical resistivity measurements indicate insulating behavior, consistent with the localized nature of magnetic moments. Heat capacity reveals that CuYbSe$_2$ can be treated as an effective spin $S = 1/2$ triangular lattice antiferromagnet below $\sim 50$~K. Magnetic susceptibility measurements on single crystals reveals weak magnetic anisotropy. These properties position CuYbSe$_2$ as a promising candidate for a quantum spin liquid state and as a new platform for exploring exotic magnetic ground states in triangular lattice systems.

cond-mat.str-el↗

arXiv2025

Tuning electronic correlations in the Kagome metals $RT_3$B$_2$

The $RT_3$B$_2$ ($R=$Y, Lu, $T=$ Co, Os) family hosts a perfect kagome lattice of $T$ atoms, offering an interesting platform to investigate the interplay of electronic structure, superconductivity, and lattice dynamics. Here, we compare two members of this family, LuOs$_3$B$_2$ and YCo$_3$B$_2$, with similar crystallography but differing chemical composition, leading to distinct electronic correlation strengths and spin-orbit coupling effects. We confirm superconductivity in LuOs$_3$B$_2$ with $T_c = 4.75$K, while YCo$_3$B$_2$ remains non-superconducting above 1.8K. First-principles estimates of the electron-phonon coupling for LuOs$_3$B$_2$ are consistent with its observed $T_c$ and suggest a moderate coupling strength. Both materials exhibit kagome-derived electronic features, including quasi-flat bands, Dirac cones, and van Hove singularities. Fermi surface calculations reveal quasi-one-dimensional behavior along the $c$-axis in YCo$_3$B$_2$, in contrast to the more three-dimensional Fermiology of LuOs$_3$B$_2$. Phonon calculations for LuOs$_3$B$_2$ show imaginary modes, indicating potential lattice instabilities. Experimental estimates of the Wilson and Kadowaki-Woods ratios point to non-negligible electronic correlations in both compounds.

cond-mat.str-el↗

arXiv2025

Spectroscopic signature of anisotropic order parameter in Kagome lattice superconductor LaRh$_3$B$_2$

The physics of the Kagome metal LaRh$_3$B$_2$ along with its superconductivity below 2.6 K, unlike other popular Kagome metals, is not known to be significantly influenced by the electron correlations. While the indirect techniques to probe the bulk superconducting properties of LaRh$_3$B$_2$ indicate a conventional isotropic order parameter, we show that the direct spectroscopic determination of the superconducting energy gap reveals an anomalous suppression of Andreev reflection between LaRh$_3$B$_2$ and a normal metal. This observation hints to the presence of incomplete superconducting gap formation, at least along certain momentum directions, and consequent low-lying quasiparticle states. An analysis of multiple Andreev reflection spectra captured at different points on the surface of LaRh$_3$B$_2$ reveals a distribution of the superconducting energy gap which is consistent with an anisotropic superconducting order parameter.

cond-mat.supr-con↗

arXiv2024

Origin of the insulating state in the Kitaev candidate Cu$_2$IrO$_3$

Through a combination of crystal symmetry analysis and density functional theory calculations we unveil a possible microscopic origin of the unexpected insulating behavior reported in the honeycomb Kitaev material Cu$_2$IrO$_3$. Our study suggests that this material hosts an instability towards charge ordering of the Ir ions, with alternating magnetic Ir$^{4+}$ and non-magnetic Ir$^{3+}$ ions arranged on the honeycomb lattice. In this case, the next-nearest-neighbor interactions that couple magnetic Ir$^{4+}$ ions form an enlarged triangular lattice, instead of the expected honeycomb lattice. The magnetic Cu$^{2+}$ ions located at the centre of the iridium honeycomb voids also form a triangular lattice, and additionally contribute to the magnetization of the system. Together, the interpenetrated Ir$^{4+}$ and Cu$^{2+}$ triangular lattices present a novel type of honeycomb Kitaev lattice composed of two types of magnetic ions.

cond-mat.str-el↗

arXiv2024

Multigap superconductivity with non-trivial topology in a Dirac semimetal PdTe

Recently, PdTe has been identified as a Dirac semimetal with potential for unconventional superconductivity based on ARPES measurements. This study presents electrical transport and magnetization measurements conducted on high-quality single crystals of PdTe. Anisotropy in the upper critical magnetic field is observed in resistivity versus temperature data measured under various applied magnetic fields for in-plane (B II ab ) and out-of-plane (B II c) orientations. The magnetic field versus temperature (H - T) phase diagram extracted from resistivity data exhibits an upward curvature akin to several multigap superconductors. Additionally, magnetization measurements reveal de Haas-Van Alphen (dHvA) oscillations in both B II ab and B II c orientations. Fourier analysis of the quantum oscillations identifies two Fermi pockets. Moreover, the Landau fan diagram for a small Fermi pocket confirms a non-trivial Berry phase π, indicative of the Dirac nature of PdTe. Based on quantum oscillation data, a plausible band diagram is constructed.

cond-mat.supr-con↗

arXiv2023

Strong coupling of lattice and orbital excitations in quantum magnet Ca$_{10}$Cr$_7$O$_{28}$: Anomalous temperature dependence of Raman phonons

We report low-temperature Raman signatures of the Heisenberg quantum magnet Ca$_{10}$Cr$_7$O$_{28}$, showing clear anomalies in phonon mode frequencies and linewidths below $\sim$100 K. This crossover temperature lies in between the Jahn-Teller (JT) temperature scale ($>$ room temperature) and the temperature scale associated with the spin exchange interactions ($<$ 12 K). Our experimental observation is well captured by a novel secondary JT transition associated with a cooperative reorientation of the orbitals giving rise to anomalies in the temperature dependence of Raman frequencies and linewidths. Such orbital reorganisation, in turn, affects the spin-spin exchange interactions that decide the fate of the magnet at lower temperatures and hence provide important clues to understand the energetics of the possible lower temperature quantum paramagnetic phase.

cond-mat.str-el↗

arXiv2022

Role of electronic correlations in the Kagome lattice superconductor LaRh$_3$B$_2$

LaRh$_3$B$_2$ crystallizes in a layered structure where Rh atoms form a perfect Kagome lattice. The material shows superconductivity at $T_c \approx 2.6$~K\@ and no signature for density wave instabilities. We report our measurements of electronic transport, magnetization, and heat capacity in the normal and superconducting state, and derive normal and superconducting parameters. From first principles calculations of the electronic band structure, we identify all features of Kagome bands predominantly formed by the Rh $d$ orbitals: a flat band, Dirac cones, and van Hove singularities. The calculation of the phonon dispersions and electron-phonon coupling suggests a strong similarity between LaRh$_3$B$_2$ and AV$_3$Sb$_5$ (A=K,Cs,Rb). For LaRh$_3$B$_2$, it matches quantitatively with the observed $T_c$, supporting a conventional phonon mediated pairing mechanism. By comparison to the $A$V$_3$Sb$_5$ family, we conjecture a reduced importance of electron correlations in LaRh$_3$B$_2$.

cond-mat.supr-con↗

arXiv2022

Pressure tuning of structure, magnetic frustration and carrier conduction in Kitaev spin liquid candidate Cu$_2$IrO$_3$: X-ray, Raman, magnetic susceptibility, resistivity and first-principles analysis

The layered honeycomb lattice iridate Cu$_2$IrO$_3$ is the closest realization of the Kitaev quantum spin liquid, primarily due to the enhanced interlayer separation and nearly ideal honeycomb lattice. We report pressure-induced structural evolution of Cu$_2$IrO$_3$ by powder x-ray diffraction (PXRD) up to $\sim$17 GPa and Raman scattering measurements up to $\sim$25 GPa. A structural phase transition (monoclinic $C2/c \: \rightarrow$ triclinic $P\bar{1}$) is observed with a broad mixed phase pressure range ($\sim$4 to 15 GPa). The triclinic phase consists of heavily distorted honeycomb lattice with Ir-Ir dimer formation and a collapsed interlayer separation. In the stability range of the low-pressure monoclinic phase, structural evolution maintains the Kitaev configuration up to 4 GPa. This is supported by the observed enhanced magnetic frustration in dc susceptibility without emergence of any magnetic ordering and an enhanced dynamic Raman susceptibility. High-pressure resistance measurements up to 25 GPa in the temperature range 1.4--300 K show resilient non-metallic $R$($T$) behaviour with significantly reduced resistivity in the high-pressure phase. The Mott 3D variable-range-hopping conduction with much reduced characteristic energy scale $T_0$ suggests that the high-pressure phase is at the boundary of localized-itinerant crossover. Using first-principles density functional theoretical (DFT) calculations, we find that at ambient pressure $\rm Cu_2IrO_3$ exists in monoclinic $P2_1/c$ phase which is energetically lower than $C2/c$ phase (both the structures are consistent with experimental XRD pattern). DFT reveals structural transition from $P2_1/c$ to $P\bar{1}$ structure at 7 GPa (involving dimerization of Ir-Ir bonds) in agreement with experimentally observed transition pressure.

cond-mat.str-el↗

arXiv2022

Unusual Magnetotransport from two dimensional Dirac Fermions in Pd$_{3}$Bi$_{2}$Se$_{2}$

Pd$_{3}$Bi$_{2}$Se$_{2}$ has been proposed to be topologically non-trivial in nature. However, evidence of its non-trivial behavior is still unexplored. We report the growth and magneto-transport study of Pd$_{3}$Bi$_{2}$Se$_{2}$ thin films, revealing for the first time the contribution of two-dimensional (2D) topological surface states. We observe exceptional non-saturated linear magnetoresistance which results from Dirac fermions inhabiting the lowest Landau level in the quantum limit. The transverse magnetoresistance changes from a semi-classical weak-field $B^{2}$ dependence to a high-field $B$ dependence at a critical field $B^{\star}$. It is found that $B^{\star} \propto T^2$, which is expected from the Landau level splitting of a linear energy dispersion. In addition, the magnetoconductivity shows signatures of 2D weak anti-localization (WAL). These novel magnetotransport signatures evince the presence of 2D Dirac fermions in Pd$_{3}$Bi$_{2}$Se$_{2}$ thin films.

cond-mat.str-el↗

arXiv2022

Observation of Weak Anti-localization in thin films of the Topological Semimetal Candidate PdSb$_{2}$

We report results of a magneto-transport study on thin films of the topological semi-metal candidate PdSb$_{2}$ (PS). We observe a positive correction to magneto-conductivity at low temperatures, which is a signature of weak anti-localization (WAL). We analyze the WAL data within the Hikami-Larkin-Nagaoka (HLN) theory and extract the dephasing length (L$_ϕ$) whose temperature dependence reveals the various phase relaxation mechanisms. From the WAL effect, we also extract $α$ (the number of transport channels). The evolution of $α$ with temperature and film thickness reflects how the coupling between different conducting channels (Topological surface channels and bulk channels) changes. Additionally, the electron-electron interaction (EEI) effect was observed in the temperature-dependent conductivity at low temperatures. From the EEI effect, we get an alternate estimate of the number of transport channels and obtain a value similar to that obtained from the analysis of the WAL effect. This suggests that in disordered films, the EEI effect can be used to get information about the coupling of the topological surface states with each other and with bulk states.

cond-mat.str-el↗

arXiv2021

Probing signatures of fractionalization in candidate quantum spin liquid Cu2IrO3 via anomalous Raman scattering

Long-range entanglement in quantum spin liquids (QSLs) lead to novel low energy excitations with fractionalised quantum numbers and (in 2D) statistics. Experimental detection and manipulation of these excitations present a challenge particularly in view of diverse candidate magnets. A promising probe of fractionalisation is their coupling to phonons. Here we present Raman scattering results for the S = 1/2 honeycomb iridate Cu2IrO3, a candidate Kitaev QSL with fractionalised Majorana fermions and Ising flux excitations. We observe anomalous low temperature frequency shift and linewidth broadening of the Raman intensities in addition to a broad magnetic continuum both of which, we derive, are naturally attributed to the phonon decaying into itinerant Majoranas. The dynamic Raman susceptibility marks a crossover from the QSL to a thermal paramagnet at ~120 K. The phonon anomalies below this temperature demonstrate a strong phonon-Majorana coupling. These results provide for evidence of spin fractionalisation in Cu2IrO3.

cond-mat.str-el↗

arXiv2021

Rare-earth tuned magnetism and magnetocaloric effects in double perovskites $R_2$NiMnO$_6$

We present a comprehensive experimental study of magnetization and magnetocaloric effect (MCE) in double perovskite (DP) materials $R_2$NiMnO$_6$ with $R =$ Pr, Nd, Sm, Gd, Tb, and Dy. While a paramagnetic to ferromagnetic transition, with T$_{\rm C}$ in the range $\sim 100 - 200~$K, is a common feature that can be attributed to the ordering of Mn$^{4+}$ and Ni$^{2+}$ magnetic moments, qualitatively distinct behavior depending on the choice of $R$ is observed at low temperatures. These low-temperature anomalies in magnetization are also manifest in the change in magnetic entropy, $-ΔS_{M}$, whose sign depends on the choice of $R$. In order to understand these results, we present theoretical analysis based on mean-field approximation and Monte Carlo simulations on a minimal spin model. The model correctly captures the key features of the experimental observations.

cond-mat.str-el↗

arXiv2020

Weak Anti-localization in thin films of the Topological Semimetal Candidate Pd$_{3}$Bi$_{2}$S$_{2}$

We report the growth and magneto-transport studies of Pd$_{3}$Bi$_{2}$S$_{2}$ (PBS) thin films synthesized by pulsed laser deposition (PLD) technique. The magneto-transport study on pristine and post annealed films show the presence of more than one type of charge carrier with a carrier concentration in the range $0.6$ - $2.26~\times$ 10$^{21}$ cm$^{-3}$ and mobility in the range 0.96 - 1.73 $\times$ 10$^{2}$ cm$^{2}$/Vs. At low temperatures a logarithmic increase in conductivity is observed which indicates the presence of weak anti-localization (WAL). The magnetotransport data is analysed within the Hikami-Larkin-Nagaoka (HLN) theory. It is found that temperature dependence of the dephasing length can't be explained only by electron-electron scattering and that electron-phonon scattering also contributes to the phase relaxation mechanism in PBS films.

cond-mat.str-el↗

arXiv2020

Emergence of weak pyrochlore phase and signature of field induced spin ice ground state in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$; x = 0, 0.15, 0.3

The pyrochlore oxides Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ are well studied spin ice systems and have shown the evidences of magnetic monopole excitations. Unlike these, Dy$_{2}$Zr$_{2}$O$_{7}$ is reported to crystallize in a distorted fluorite structure. We present here the magnetic and heat capacity studies of La substituted Dy$_{2}$Zr$_{2}$O$_{7}$. Our findings suggest the absence of spin ice state in Dy$_{2}$Zr$_{2}$O$_{7}$ but the emergence of the magnetic field induced spin freezing near T $\approx$ 10 K in ac susceptibility measurements which is similar to Dy$_{2}$Ti$_{2}$O$_{7}$. The magnetic heat capacity of Dy$_{2}$Zr$_{2}$O$_{7}$ shows a shift in the peak position from 1.2 K in zero field to higher temperatures in the magnetic field, with the corresponding decrease in the magnetic entropy. The low temperature magnetic entropy at 5 kOe field is Rln2 - (1/2)Rln(3/2) which is same as for the spin ice state. Substitution of non-magnetic, isovalent La$^{3+}$ for Dy$^{3+}$ gradually induces the structural change from highly disordered fluorite to weakly ordered pyrochlore phase. The La$^{3+}$ substituted compounds with less distorted pyrochlore phase show the spin freezing at lower field which strengthens further on the application of magnetic field. Our results suggest that the spin ice state can be stabilized in Dy$_{2}$Zr$_{2}$O$_{7}$ either by slowing down of the spin dynamics or by strengthening the pyrochlore phase by suitable substitution in the system.

cond-mat.str-el↗

arXiv2020

Robust spin liquid state against magnetic-dilution in the bi-layer Kagome material Ca$_{10}$Cr$_7$O$_{28}$

Recently, the bi-layer Kagome lattice material Ca$_{10}$Cr$_7$O$_{28}$ has been shown to be a quasi-two-dimensional quantum spin liquid (QSL) where the frustration arises from a balance between competing ferromagnetic and antiferromagnetic exchange within a bi-layer. In an attempt to understand what happens when this balance is disturbed, we present a magnetic dilution study. Specifically, we have synthesized Ca$_{10}$(Cr$_{1-x}$V$_x$)$_7$O$_{28}$ (0 $\leq$ x $\leq$ 0.5) where magnetic Cr$^{5+}$ ($S = 1/2$) is partially replaced by non-magnetic V$^{5+}$ ($S = 0$). We also synthesized the fully non-magnetic isostructural material Ca$_{10}$V$_7$O$_{27.5}$. We report a detailed structural, magnetic and heat capacity study on these materials. A monotonic increase in the unit cell parameters is found for the Ca$_{10}$(Cr$_{1-x}$V$_x$)$_7$O$_{28}$ materials with increasing $x$. An order of magnitude decrease in the Curie-Weiss temperature from $4$ to $0.5$~ K is found for the partial V substituted samples, which indicates a relative increase in antiferromagnetic exchange with increase in V content. However, despite this change in the relative balance in the exchange interactions and the large disorder introduced, no magnetic ordering or spin-glass state is observed down to $2$~K in the V substituted samples. The QSL state of the parent compound thus seems surprisingly robust against these large perturbations.

cond-mat.str-el↗

arXiv2020

Domain structure dynamics in the ferromagnetic Kagome-lattice Weyl semimetal Co$_3$Sn$_2$S$_2$

Co$_3$Sn$_2$S$_2$, a Weyl semimetal that consists of layers of Kagome lattices, transitions from a high-temperature paramagnetic phase to a low-temperature ferromagnetic phase below 177 K. The phase transition occurs through an intermediate non-trivial magnetic phase, the so-called "A"-phase just below the Curie temperature. The "A"-phase was earlier linked with a competing anti-ferromagnetic phase, a spin-glass phase and certain indirect measurements indicated the possibility of magnetic Skyrmions in this phase. We have imaged the magnetic domain structure in a single crystal of Co$_3$Sn$_2$S$_2$ at different temperatures, magnetic fields and field-angles by magnetic force microscopy. At low temperatures, we observed stripe domains indicating presence of uniaxial anisotropy. Above 130 K, the domain walls become mobile and they tend to align relatively easily when the magnetic field is increased along the $c$-axis than in the $a-b$ plane. Our detailed study of field-dependent domain dynamics reveal that the anomalous nature of the phase transition just below $T_c$ is dominantly governed by domain wall motion.

cond-mat.mtrl-sci↗