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Yong-Hui Zhang

Publications and source records attributed to Yong-Hui Zhang.

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Simultaneous Determination of Multiple Nuclear Parameters of $^{229}$Th Using Highly Charged Ions

Development of a $^{229}$Th nuclear optical clock requires precise and model-insensitive nuclear-structure parameters, which presently suffer from limited accuracy and poor consistency. We propose a joint spectroscopy scheme using two highly charged $^{229}$Th ions with $J=1/2$ electronic ground states, where the lowest electronic excitation energy of each ion far exceeds the nuclear transition energy. This configuration effectively forms a three-level system comprising the electronic ground state and the nuclear ground ($g$) and isomeric ($m$) states, resulting in strongly enhanced nuclear hyperfine mixing. Within this framework, a unified analysis of precision measurements on both ions enables the simultaneous determination of five key nuclear parameters without relying on external nuclear inputs: the magnetic dipole moments $μ_g$ and $μ_m$, the bare-nucleus transition energy $ω_n$, the charge-radius difference $δ\langle r^{2}\rangle_{gm}$, and the $M1$ transition matrix element $T_{M1}$. With this approach, the uncertainties in $ω_n$ and $δ\langle r^{2}\rangle_{gm}$ are estimated to be reduced by factors of 3 and 2, respectively, relative to their current uncertainties. %compared with current values. This work could provide a useful benchmark for nuclear theory and serve as a foundation for future development of a $^{229}$Th-based nuclear optical clock.

physics.atom-ph

Ionization energies for Rydberg $^4 \mathrm{He}$ ($1snp\,^{1,3}P$) states using the correlated B-spline basis function method

We extend the correlated B-spline basis function (C-BSBF) method to high-precision calculations of the ionization energies of helium Rydberg $n^{1,3}P$ states ($n=24$--$35$). Using a unified basis set, we evaluate nonrelativistic energies, relativistic corrections of order $mα^4$ (including finite-mass recoil), QED contributions of order $mα^5$, and partial $mα^6$ terms (singlet-triplet mixing, one- and two-loop radiative corrections). The remaining higher-order contributions are estimated via $1/n^3$ scaling. The resulting ionization energies achieve kHz-level accuracy and are in excellent agreement with independent Hylleraas calculations, thereby providing cross-validation between two distinct theoretical approaches. From these data, the quantum-defect parameters are determined and used to extrapolate the ionization energies up to $n=102$. Combining our Rydberg ionization energies with high-precision experimental $2S \rightarrow nP$ transition frequencies yields the ionization energies for the metastable $2^{1}S$ and $2^{3}S$ states as \num{960332040.533(10)}$_\mathrm{stat}(20)_ \mathrm{sys}$ MHz and \num{1152842742.7274(53)}$_\mathrm{stat}(25)_ \mathrm{sys}$ MHz, respectively. The C-BSBF result for the $2 \, ^1 S$ state is consistent with the experimental ionization energy obtained from Rydberg-series extrapolation, while for the $2 \, ^3 S$ state the difference is 0.019(10) MHz.

physics.atom-ph

A spatiotemporal fused network considering electrode spatial topology and time-window transition for MDD detection

Recently, researchers have begun to experiment with deep learning-based methods for detecting major depressive disor-der (MDD) using electroencephalogram (EEG) signals in search of a more objective means of diagnosis. However, exist-ing spatiotemporal feature extraction methods only consider the functional correlation between multiple electrodes and temporal correlation of EEG signals, ignoring the spatial posi-tion connection information between electrodes and the conti-nuity between time windows, which reduces the model's fea-ture extraction capabilities. To address this issue, a Spatio-temporal fused network for MDD detection with Electrode spatial Topology and adjacent TIME-window transition in-formation (SET-TIME) is proposed in this study. SET-TIME is composed by a common feature extractor, a secondary time-correlation feature extractor, and a domain adaptation (DA) module, in which the former extractor is used to obtain the temporal and spatial features, and the latter extractor can mine the correlation between multiple time windows, and the DA module is adopted to enhance cross-subject detection ca-pability. The experimental results of 10-fold cross-validation show that the proposed SET-TIME method outperforms the state-of-the-art (SOTA) method by achieving MDD detection accuracies of 92.00% and 94.00% on the public datasets PRED+CT and MODMA, respectively. Ablation experiments demonstrate the effectiveness of the multiple modules in SET-TIME, which assist in MDD detection by exploring the intrin-sic spatiotemporal information of EEG signals.

cs.LG

Precise ab initio calculations of $^4$He($1snp \, ^3P_J$) fine structure of high Rydberg states

High-precision measurements of the fine-structure splittings in helium high Rydberg states have been reported, yet corresponding ab initio benchmarks for direct comparison remain unavailable. In this work, we extend the correlated B-spline basis function (C-BSBF) method to calculate the fine-structure splittings of high Rydberg states in $^4$He. The calculations include the $mα^4$- and $mα^5$-order contributions, the singlet-triplet mixing effect, and estimated spin-dependent $mα^6$-order corrections obtained using a $1/n^3$ scaling approximation. High-precision ab initio results are obtained for principal quantum numbers $n=24$-37 with kilohertz-level accuracy and further extended to $n=45$-51 by extrapolation and fitting. The theoretical results show excellent agreement with quantum-defect theory (QDT) predictions and allow direct comparison with experimental measurements. Additionally, the discrepancy observed at $n=34$ is expected to be clarified with improved experimental precision.

physics.atom-ph

Application of the correlated B-spline basis functions to the leading relativistic and QED corrections of helium

B-spline functions have been widely used in computational atomic physics. Different from the traditional B-spline basis (a simple product of two B-splines), the recently developed correlated B-spline basis functions(C-BSBF), in which the interelectronic coordinate $r_{12}$ is included explicitly, have greatly improved the computational accuracy of polarizability [S. J. Yang \textit{et al}., Phys. Rev. A \textbf{95}, 062505 (2017)] and bethe logarithm [ S. J. Yang \textit{et al}., Phys. Rev. A \textbf{100}, 042509 (2019)] for singlet states of helium. Here, we report the extension of the C-BSBF to the leading relativistic and QED correction calculations for energy levels of the $1\,^1S$, $2\,^1S$, $2\,^3S$, and $3\,^3S$ states of helium. The relativistic kinetic term $p_{1}^{4}$, contact potential $δ^{3}(r_{1})$, $δ^{3}(r_{12})$ and Araki-Sucher correction $\langle 1/r_{12}^{3} \rangle$ are calculated by using the global operator method, in which $r_{12}^n$ and $r_{12}^n\ln r_{12}$ involved are calculated with the generalization of Laplace's expansions. The obtained values for the ground state are $δE_{rel}/α^{2}=-$1.951 754 7(2) and $δE_{QED}/α^{3}=$57.288 165(2), consistent with previous results, which opens the possibility of calculating higher-order relativistic and QED effects using the C-BSBF.

physics.atom-ph

Measurement of a helium tune-out frequency: an independent test of quantum electrodynamics

Despite quantum electrodynamics (QED) being one of the most stringently tested theories underpinning modern physics, recent precision atomic spectroscopy measurements have uncovered several small discrepancies between experiment and theory. One particularly powerful experimental observable that tests QED independently of traditional energy level measurements is the `tune-out' frequency, where the dynamic polarizability vanishes and the atom does not interact with applied laser light. In this work, we measure the `tune-out' frequency for the $2^{3\!}S_1$ state of helium between transitions to the $2^{3\!}P$ and $3^{3\!}P$ manifolds and compare it to new theoretical QED calculations. The experimentally determined value of $725\,736\,700\,$$(40_{\mathrm{stat}},260_{\mathrm{syst}})$ MHz is within ${\sim} 1.7σ$ of theory ($725\,736\,252(9)$ MHz), and importantly resolves both the QED contributions (${\sim} 30 σ$) and novel retardation (${\sim} 2 σ$) corrections.

physics.atom-ph

Proposal for suppressing ac Stark shift in the He($2\,^3S_1\rightarrow 3\,^3S_1$) two-photon transition using magic wavelengths

Motivated by recent direct measurement of the forbidden $2\,^3S_1\rightarrow3\,^3S_1$ transition in helium [K. F. Thomas et al., Phys. Rev. Lett. 125, 013002(2020)], where the ac Stark shift is one of the main systematic uncertainties, we propose a dichroic two-photon transition measurement for $2\,^3S_1\rightarrow3\,^3S_1$ which could effectively suppress the ac Stark shift by utilizing magic wavelengths: one magic wavelength is used to realize state-insensitive optical trapping, the other magic wavelength is used as one of the two lasers driving the two-photon transition. Carrying out calculations based on the no-pair Dirac-Coulomb-Breit Hamiltonian with mass shift operator included, we report the magic wavelength of 1265.615 9(4) nm for $^4$He [or 1265.683 9(2) nm for $^3$He] can be used to design an optical dipole trap; the magic wavelength of 934.234 5(2) nm for $^4$He [or 934.255 4(4) nm for $^3$He] can be as one excitation laser in the two-photon process, and the ac Stark shift can be reduced to less than 100 kHz, as long as the intensity of the other excitation laser does not exceed $1\times10^4~W/cm^2$. Alternatively, by selecting detuning frequencies relative to the $2\,^3P$ state in the region of 82$\sim$103 THz, as well as adjusting the intensity ratios of the two lasers, the ac Stark shift in the $2\,^3S_1\rightarrow3\,^3S_1$ two-photon transition can be cancelled.

physics.atom-ph

Probing Multiple Electric Dipole Forbidden Optical Transitions in Highly Charged Nickel Ions

Highly charged ions (HCIs) are promising candidates for the next generation of atomic clocks, owing to their tightly bound electron cloud, which significantly suppresses the common environmental disturbances to the quantum oscillator. Here we propose and pursue an experimental strategy that, while focusing on various HCIs of a single atomic element, keeps the number of candidate clock transitions as large as possible. Following this strategy, we identify four adjacent charge states of nickel HCIs that offer as many as six optical transitions. Experimentally, we demonstrated the essential capability of producing these ions in the low-energy compact Shanghai-Wuhan Electron Beam Ion Trap. We measured the wavelengths of four magnetic-dipole ($M$1) and one electric-quadrupole ($E$2) clock transitions with an accuracy of several ppm with a novel calibration method; two of these lines were observed and characterized for the first time in controlled laboratory settings. Compared to the earlier determinations, our measurements improved wavelength accuracy by an order of magnitude. Such measurements are crucial for constraining the range of laser wavelengths for finding the "needle in a haystack" narrow lines. In addition, we calculated frequencies and quality factors, evaluated sensitivity of these six transitions to the hypothetical variation of the electromagnetic fine structure constant $α$ needed for fundamental physics applications. We argue that all the six transitions in nickel HCIs offer intrinsic immunity to all common perturbations of quantum oscillators, and one of them has the projected fractional frequency uncertainty down to the remarkable level of 10$^{-19}$.

physics.atom-ph

Calculations of Bethe logarithms for Hydrogen and Helium atoms using B-splines in different gauges

The efficient and simple B-splines variational method of calculating the hydrogen atom Bethe logarithms in the acceleration gauge [Y-B Tang et.al., Phys. Rev. A $\mathbf{87}$, 022510 (2013)] is successfully applied to other gauges. The ground state Bethe logarithm of H with fourteen accurate figures is obtained in the velocity gauge, and in the length gauge the ground state value has eleven accurate figures. Present velocity- and length-gauge results for the $ns$, $np$, $nd$, and $nf$ states up to $n = 200$ of H are at the 10$^{-10}$ level of accuracy. This represents the successful variational attempt to calculate Bethe logarithms of the hydrogen atom in the velocity and length gauges. Furthermore, the B-splines variational method is successfully extended to the helium atom by the aid of configuration interaction. Bethe logarithms for $n\,^{1,3}S\,\,(n=1-8)$ states are calculated in three different gauges. The acceleration-gauge value of 4.364 036 7(2) a.u. and the velocity-acceleration gauge value of 4.364 036 4(2) a.u. for the $2\,^3S$ state are achieved, which are both at the 10$^{-7}$ level of accuracy. For other triplet states, present results in three different gauges all have five to seven accurate figures. While for the singlet states, the best convergent values are obtained in the pa-gauge, of which the numerical precision is also at the $10^{-5}$ to $10^{-7}$ level of accuracy.

physics.atom-ph

QED and relativistic nuclear recoil corrections to the 413 nm tune-out wavelength for the $2\,^3S_1$ state of helium

Comparison of high accuracy calculations with precision measurement of the 413 nm tune-out wavelength of the He($2\,^3S_1$) state provides a unique test of quantum electro-dynamic (QED). We perform large-scale relativistic-configuration-interaction (RCI) calculations of the tune-out wavelength, that include the mass-shift operator, and fully account for leading relativistic nuclear recoil terms in the Dirac-Coulomb-Breit (DCB) Hamiltonian. We obtain the QED correction to the tune-out wavelength using perturbation theory, and the effect of finite nuclear size is also evaluated. The resulting tune-out wavelengths for the $2\,^3S_1(M_J=0)$ and $2\,^3S_1(M_J=\pm 1)$ states are 413.084 26(4) nm and 413.090 15(4) nm, respectively. Compared with the only current experimental value of 413.0938(9stat)(20syst) nm for the $2\,^3S_1(M_J=\pm 1)$ state, there is 1.8$σ$ discrepancy between present theoretical work and experiment, which stimulates further theoretical and higher-precision experimental investigations on the 413 nm tune-out wavelength. In addition, we also determine the QED correction for the static dipole polarizability of the He($2\,^3S_1$) state to be 22.5 ppm, which may enable a new test of QED in the future.

physics.atom-ph

Relativistic full-configuration-interaction calculations of magic wavelengths for the $2\,^3S_1\rightarrow2\,^1S_0$ transition of helium isotopes

A large-scale full-configuration-interaction calculation based on Dirac-Coulomb-Breit (DCB) Hamiltonian is performed for the $2\,^1S_0$ and $2\,^3S_1$ states of helium. The operators of the normal and specific mass shifts are directly included in the DCB framework to take the finite nuclear mass correction into account. High-accuracy energies and matrix elements involved n (the main quantum number) up to 13 are obtained from one diagonalization of Hamiltonian. The dynamic dipole polarizabilities are calculated by using the sum rule of intermediate states. And a series of magic wavelengths with QED and hyperfine effects included for the $2\,^3S_1\rightarrow2\,^1S_0$ transition of helium are identified. In addition, the high-order Ac Stark shift determined by the dynamic hyperpolarizabilities at the magic wavelengths are also evaluated. Since the most promising magic wavelength for application in experiment is 319.8 nm, the high-accuracy magic wavelength of 319.815 3(6) nm of $^4$He is in good agreement with recent measurement value of 319.815 92(15) nm [Nature Physics (2018)/arXiv:1804.06693], and present magic wavelength of 319.830 2(7) nm for $^3$He would provide theoretical support for experimental designing an optical dipole trap to precisely determine the nuclear charge radius of helium in future.

physics.atom-ph

Dynamic dipole polarizabilities for the low-lying triplet states of helium

The dynamic dipole polarizabilities for the four lowest triplet states ($2\,^3S$, $3\,^3S$, $2\,^3P$ and $3\,^3P$) of helium are calculated using the B-spline configuration interaction method. Present values of the static dipole polarizabilities in the length, velocity and acceleration gauges are in good agreement with the best Hylleraas results. Also the tune-out wavelengths in the range from 400 nm to 4.2~$μ$m for the four lowest triplet states are identified, and the magic wavelengths in the range from 460~nm to 3.5~$μ$m for the $2\,^3S \to 3\,^3S$, $2\,^3S \to 2\,^3P$, and $2\,^3S \to 3\,^3P$ transitions are determined. We show that the tune-out wavelength of $2\,^3S$ state is 413.038 28(3) nm, which corroborates the value of Mitroy and Tang (Phys. Rev. A 88, 052515 (2013)), and the magic wavelength around 1066 nm for the $2\,^3S \to 3\,^3P$ transition can be expected for precision measurement to determine the ratio of transition matrix elements $(2\,^3S \to 2\,^3P) / (3\,^3P\to 6\,^3S)$.

physics.atom-ph

Computational investigation of static multipole polarizabilities and sum rules for ground-state hydrogen-like ions

High precision multipole polarizabilities, $α_{\ell}$ for $\ell \le 4$ of the $1s$ ground state of the hydrogen isoelectronic series are obtained from the Dirac equation using the B-spline method with Notre Dame boundary conditions. Compact analytic expressions for the polarizabilities as a function of $Z$ with a relative accuracy of 10$^{-6}$ up to $Z = 100$ are determined by fitting to the calculated polarizabilities. The oscillator strengths satisfy the sum rules $\sum_i f^{(\ell)}_{0i} = 0$ for all multipoles from $\ell = 1$ to $\ell = 4$. The dispersion coefficients for the long-range H-H and H-He$^+$ interactions are given.

physics.atom-ph

Convergence of the multipole expansion of the polarization interaction

The multipole expansion of the polarization interaction between a charged particle and an electrically charged particle has long been known to be asymptotic in nature, i.e. the multiple expansion diverges at any finite distance from the atom. However, it is shown that the multipole expansion of the polarization potential of a confined hydrogen atom is absolutely convergent at a distance outside the atoms confinement radius. It is likely that the multipole expansion of the dispersion interaction of two confined atoms will also be absolutely convergent provided the internuclear separation of the two atoms is sufficiency large to exclude any overlap between the electron charge clouds of the two atoms.

physics.atom-ph