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Yongho Park

Publications and source records attributed to Yongho Park.

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Electronic Orbital Angular Momentum Driven by Finite-Momentum Phonons: Beyond Chiral and Axial Phonons

We show that finite-momentum phonons generate electronic orbital angular momentum (OAM) even without phonon axiality or chirality, with the response controlled by the phonon wave vector $q$ and frequency $\omega$. We develop a general gauge-field theory in which a unitary transformation absorbs the phonon displacement into emergent vector and scalar potentials acting on the electrons, providing a perturbative classification of the OAM response in $q$ and $\omega$. We derive $q$- and $\omega$-scaling laws for AC and DC responses. Notably, AC OAM arises even for linearly polarized phonons, with its magnitude and sign tunable by $q$. Its generation is governed by the matching between the phonon geometry and the electronic orbital texture rather than solely by the phonon angular momentum. The connection of the DC response to the electronic Berry curvature further supports that phonon angular momentum is not the only degree of freedom governing electronic OAM generation. Time-dependent tight-binding simulations under acoustic-phonon driving independently confirm the core predictions. Our results extend phonon-driven OAM beyond chiral and axial phonons and establish a wave-vector-tunable route to orbitronics, accessible with surface acoustic waves.

cond-mat.mes-hall

Observation of current-induced orbital quadrupole accumulation

Spintronics and orbitronics rely on current-induced accumulations of magnetic dipoles: spin and orbital angular momentum. However, electronic orbitals inherently carry multipoles beyond the dipole, with the rank-2 orbital quadrupole as the leading term. Here we use polarization-resolved Kerr microscopy to observe current-induced orbital-quadrupole accumulation at the surfaces of Ti and Pt, metals with markedly different spin--orbit-coupling strengths. By separating the symmetric and antisymmetric components of the off-diagonal optical conductivity, we isolate the time-reversal-even quadrupolar response from the conventional time-reversal-odd magnetic-dipolar one, and find that the quadrupolar optical response exceeds the dipolar one in both metals. First-principles analysis of the measured responses indicates that the quadrupole accumulations are of the same order of magnitude in the two metals despite their widely different spin--orbit-coupling strengths, consistent with a previously unidentified channel of charge-to-orbital conversion that does not require spin--orbit coupling. Our findings establish that current-induced orbital polarization is fundamentally multipolar, expanding current-induced phenomena from the dipolar to the multipolar regime and opening a route to electrical control of orbital-ordered phases.

cond-mat.mtrl-sci