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Yongmin Liu

Publications and source records attributed to Yongmin Liu.

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The Future of Artificial Intelligence and the Mathematical and Physical Sciences (AI+MPS)

This community paper developed out of the NSF Workshop on the Future of Artificial Intelligence (AI) and the Mathematical and Physics Sciences (MPS), which was held in March 2025 with the goal of understanding how the MPS domains (Astronomy, Chemistry, Materials Research, Mathematical Sciences, and Physics) can best capitalize on, and contribute to, the future of AI. We present here a summary and snapshot of the MPS community's perspective, as of Spring/Summer 2025, in a rapidly developing field. The link between AI and MPS is becoming increasingly inextricable; now is a crucial moment to strengthen the link between AI and Science by pursuing a strategy that proactively and thoughtfully leverages the potential of AI for scientific discovery and optimizes opportunities to impact the development of AI by applying concepts from fundamental science. To achieve this, we propose activities and strategic priorities that: (1) enable AI+MPS research in both directions; (2) build up an interdisciplinary community of AI+MPS researchers; and (3) foster education and workforce development in AI for MPS researchers and students. We conclude with a summary of suggested priorities for funding agencies, educational institutions, and individual researchers to help position the MPS community to be a leader in, and take full advantage of, the transformative potential of AI+MPS.

cs.AI

Machine-Learning-Assisted Photonic Device Development: A Multiscale Approach from Theory to Characterization

Photonic device development (PDD) has achieved remarkable success in designing and implementing new devices for controlling light across various wavelengths, scales, and applications, including telecommunications, imaging, sensing, and quantum information processing. PDD is an iterative, five-step process that consists of: i) deriving device behavior from design parameters, ii) simulating device performance, iii) finding the optimal candidate designs from simulations, iv) fabricating the optimal device, and v) measuring device performance. Classically, all these steps involve Bayesian optimization, material science, control theory, and direct physics-driven numerical methods. However, many of these techniques are computationally intractable, monetarily costly, or difficult to implement at scale. In addition, PDD suffers from large optimization landscapes, uncertainties in structural or optical characterization, and difficulties in implementing robust fabrication processes. However, the advent of machine learning over the past decade has provided novel, data-driven strategies for tackling these challenges, including surrogate estimators for speeding up computations, generative modeling for noisy measurement modeling and data augmentation, reinforcement learning for fabrication, and active learning for experimental physical discovery. In this review, we present a comprehensive perspective on these methods to enable machine-learning-assisted PDD (ML-PDD) for efficient design optimization with powerful generative models, fast simulation and characterization modeling under noisy measurements, and reinforcement learning for fabrication. This review will provide researchers from diverse backgrounds with valuable insights into this emerging topic, fostering interdisciplinary efforts to accelerate the development of complex photonic devices and systems.

physics.optics

On-Demand Inverse Design for Narrowband Nanophotonic Structures Based on Generative Model and Tandem Network

Inverse design in nanophotonics remains challenging due to its ill-posed nature and sensitivity to input inaccuracies. We present a novel framework that combines a Conditional Variational Autoencoder (CVAE) with a tandem network, enabling robust and efficient on-demand inverse design of photonic structures. Unlike prior approaches that use CVAEs or tandem networks in isolation, our method integrates spectral adjustment and structural prediction in a unified architecture. Specifically, the CVAE adjusts the idealized target spectra, such as Lorentzian-shaped notches, making them more physically realizable and consistent with the training data distribution. This adjusted spectrum is then passed to the tandem network, which predicts the corresponding structural parameters. The framework effectively handles both narrowband (<50 nm) and highly complex spectra, while addressing the one-to-many mapping challenge inherent in inverse design. The model achieves high accuracy, and the designed spectra closely match full-wave simulation results, validating its practicality for advanced nanophotonic applications.

physics.optics

Optical Propulsion and Levitation of Metajets

The quintessential hallmark distinguishing metasurfaces from traditional optical components is the engineering of subwavelength meta-atoms to manipulate light at will. Enabling this freedom, in a reverse manner, to control objects constituted by metasurfaces could expand our capability of optical manipulation to go beyond the predominant microscopic and sub-microscopic scales. Here, we introduce a driving metaphotonic force fully controllable by meta-atoms to manipulate structured objects named metajets. Upon Newton's law of motion that can apply to classical and relativistic mechanics, we develop a first-principles theory to analyze optical forces generated by refraction and reflection at an interface. We find that three-dimensional motions of metajets would be possible if one could introduce an extra wavevector component. We achieve that by creating a spatially distributed phase gradient with deliberately arranged silicon nanopillars. Our experiments and simulations reveal an in-plane propulsion and, very importantly, out-of-plane levitation of the metajets, aligning well with the theory. We also find that the metaphotonic force augments with increased light power but is not limited by the size of metajets, which could unleash new opportunities for metaphotonic control in large settings, such as interstellar light sails.

physics.optics

Electrically Tuning Quasi-Bound States in the Continuum with Hybrid Graphene-Silicon Metasurfaces

Metasurfaces have become one of the most prominent research topics in the field of optics owing to their unprecedented properties and novel applications on an ultrathin platform. By combining graphene with metasurfaces, electrical tunable functions can be achieved with fast tuning speed, large modulation depth and broad tuning range. However, the tuning efficiency of hybrid graphene metasurfaces within the short-wavelength infrared (SWIR) spectrum is typically low because of the small resonance wavelength shift in this wavelength range. In this work, through the integration of graphene and silicon metasurfaces that support quasi-bound states in the continuum (quasi-BIC), we experimentally demonstrate significant transmittance tuning even with less than 30 nm resonance wavelength shift thanks to the high quality-factor of quasi-BIC metasurfaces. The tunable transmittance spectrum was measured using Fourier Transform Infrared Spectroscopy (FTIR) with a modified reflective lens to improve the accuracy, and the electrical tuning was realized utilizing the cut-and-stick method of ion gel. At the wavelength of 3.0 um, the measured change of transmittance T_max-T_min and modulation depth (T_max-T_min)/T_max can reach 22.2% and 28.9%, respectively, under a small bias voltage ranging from -2 V to +2 V. To the best of our knowledge, this work is the first experimental demonstration of tunable graphene/quasi-BIC metasurfaces, which have potential applications in optical modulation, reconfigurable photonic devices, and optical communications.

physics.optics

Polarization-Encoded Lenticular Nano-Printing with Single-Layer Metasurfaces

Metasurface-based nano-printing has enabled ultrahigh-resolution grayscale or color image display. However, the maximum number of independent nano-printing images allowed by one single-layer metasurface is still limited despite many multiplexing methods that have been proposed to increase the design degree of freedom. In this work, we substantially push the multiplexing limit of nano-printing by transforming images at different observation angles into mapping the corresponding images to different positions in the Fourier space, and simultaneously controlling the complex electric field across multiple polarization channels. Our proposed Polarization-Encoded Lenticular Nano-Printing (Pollen), aided by a modified evolutionary algorithm, allows the display of several images based on the viewing angle, similar to traditional lenticular printing but without requiring a lenticular layer. In addition, it extends the display capability to encompass multiple polarization states. Empowered by the ability to control the complex amplitude of three polarization channels, we numerically and experimentally demonstrate the generation of 13 distinguished gray-scale Chinese ink wash painting images, 49 binary patterns, and three sets of 3D nano-printing images, totaling 25 unique visuals. These results present the largest number of recorded images with ultra-high resolution to date. Our innovative Pollen technique is expected to benefit the development of modern optical applications, including but not limited to optical encryption, optical data storage, lightweight display, and augmented reality and virtual reality.

physics.optics

Decoupled phase modulation for circularly polarized lights via chiral metasurface

Metasurfaces are believed as one of the best candidates in nano-optical devices, attributed to the key feasible modulation features of phase, polarization, and local field enhancement by structural designing. However, current methods of propagation- and geometric-phase modulation are interrelated between two eigen spin-states. This means that when the left-handed component phase of a beam is modulated by metasurfaces, its right-handed component phase will change accordingly, which limits the versatility of spin-decoupled applications. In this paper, we experimentally and numerically demonstrate a new phase modulation pathway based on chiral V-shaped holes, which enable fully decoupled one-handed phase modulation of the two eigen spin-states. Two enantiomers are proposed to realize decoupled functions for the two eign-states, e.g., the enantiomer can manipulate the left-handed component phase of a laser beam without changes of the right-handed component. This proposed method has significant meaning in metasurfaces, which can expand the methods of phase engineering.

physics.optics

Probabilistic representation and inverse design of metamaterials based on a deep generative model with semi-supervised learning strategy

The research of metamaterials has achieved enormous success in the manipulation of light in an artificially prescribed manner using delicately designed sub-wavelength structures, so-called meta-atoms. Even though modern numerical methods allow to accurately calculate the optical response of complex structures, the inverse design of metamaterials is still a challenging task due to the non-intuitive and non-unique relationship between physical structures and optical responses. To better unveil this implicit relationship and thus facilitate metamaterial design, we propose to represent metamaterials and model the inverse design problem in a probabilistically generative manner. By employing an encoder-decoder configuration, our deep generative model compresses the meta-atom design and optical response into a latent space, where similar designs and similar optical responses are automatically clustered together. Therefore, by sampling in the latent space, the stochastic latent variables function as codes, from which the candidate designs are generated upon given requirements in a decoding process. With the effective latent representation of metamaterials, we can elegantly model the complex structure-performance relationship in an interpretable way, and solve the one-to-many mapping issue that is intractable in a deterministic model. Moreover, to alleviate the burden of numerical calculation in data collection, we develop a semi-supervised learning strategy that allows our model to utilize unlabeled data in addition to labeled data during training, simultaneously optimizing the generative inverse design and deterministic forward prediction in an end-to-end manner. On a data-driven basis, the proposed model can serve as a comprehensive and efficient tool that accelerates the design, characterization and even new discovery in the research domain of metamaterials and photonics in general.

physics.optics

Ultrafast fluorescent decay induced by metal-mediated dipole-dipole interaction in two-dimensional molecular aggregates

Two-dimensional molecular aggregate (2DMA), a thin sheet of strongly interacting dipole molecules self-assembled at close distance on an ordered lattice, is a fascinating fluorescent material. It is distinctively different from the single or colloidal dye molecules or quantum dots in most previous research. In this paper, we verify for the first time that when a 2DMA is placed at a nanometric distance from a metallic substrate, the strong and coherent interaction between the dipoles inside the 2DMA dominates its fluorescent decay at picosecond timescale. Our streak-camera lifetime measurement and interacting lattice-dipole calculation reveal that the metal-mediated dipole-dipole interaction shortens the fluorescent lifetime to about one half and increases the energy dissipation rate by ten times than expected from the noninteracting single-dipole picture. Our finding can enrich our understanding of nanoscale energy transfer in molecular excitonic systems and may designate a new direction for developing fast and efficient optoelectronic devices.

physics.optics

Perfect Circular Dichroic Metamirrors

In nature, the beetle Chrysina gloriosa derives its iridescence by selectively reflecting left-handed circularly polarized light only. Here, for the first time, we introduce and demonstrate the optical analogue based on an ultrathin metamaterial, which we term circular dichroic metamirror. A general method to design the circular dichroic metasmirror is presented under the framework of Jones calculus. It is analytically shown that the metamirror can be realized by two layers of anisotropic metamaterial structures, in order to satisfy the required simultaneous breakings of n-fold rotational (n>2) and mirror symmetries. We design an infrared metamirror, which shows perfect reflectance for left-handed circularly polarized light without reversing its handedness, while almost completely absorbs right-handed circularly polarized light. These findings offer new methodology to realize novel chiral optical devices for a variety of applications, including polarimetric imaging, molecular spectroscopy, as well as quantum information processing.

physics.optics

Controllable growth of Al nanorods for inexpensive and degradation-resistant surface enhanced Raman spectroscopy

Surface enhanced Raman spectroscopy (SERS) has the capacity of detecting trace amount of biological or chemical matter, even single molecules, through the use of metallic nanostructures such as nanorods. Silver (Ag) and gold (Au) nanorods have led to the impressive enhancement of Raman signals, but they are either expensive, degrade fast over time, or suffer from poor sample repeatability. In contrast, Al is much less expensive, and Al nanorods could potentially be resistant to degradation over time due to the protection from native aluminum-oxide layers. Unfortunately, the controllable growth of Al nanorods has not been reported so far. This Letter reports, for the first time, the controllable growth of Al nanorods using physical vapor deposition (PVD); through the use of oxygen (O) surfactants. The enhancement factor of the Al nanorods in SERS is as high as 1250, and shows nearly no degradation after storage in ambient for 30 days or annealing at 475 K for one day.

cond-mat.mtrl-sci

Plasmonic Metamaterials

Plasmonics and metamaterials have attracted considerable attention over the past decade, owing to the revolutionary impacts that they bring to both the fundamental physics and practical applications in multiple disciplines. Although the two fields initially advanced along their individual trajectories in parallel, they started to interfere with each other when metamaterials reached the optical regime. The dynamic interplay between plasmonics and metamaterials has generated a number of innovative concepts and approaches, which are impossible with either area alone. This review presents the fundamentals, recent advances and future perspectives in the emerging field of plasmonic metamaterials, aiming to open up new exciting opportunities for nanoscience and nanotechnology.

physics.optics

A Carpet Cloak Device for Visible Light

We report an invisibility carpet cloak device, which is capable of making an object undetectable by visible light. The cloak is designed using quasi conformal mapping and is fabricated in a silicon nitride waveguide on a specially developed nano-porous silicon oxide substrate with a very low refractive index. The spatial index variation is realized by etching holes of various sizes in the nitride layer at deep subwavelength scale creating a local effective medium index. The fabricated device demonstrates wideband invisibility throughout the visible spectrum with low loss. This silicon nitride on low index substrate can also be a general scheme for implementation of transformation optical devices at visible frequency.

physics.optics

Plasmonic Luneburg and Eaton Lenses

Plasmonics is an interdisciplinary field focusing on the unique properties of both localized and propagating surface plasmon polaritons (SPPs) - quasiparticles in which photons are coupled to the quasi-free electrons of metals. In particular, it allows for confining light in dimensions smaller than the wavelength of photons in free space, and makes it possible to match the different length scales associated with photonics and electronics in a single nanoscale device. Broad applications of plasmonics have been realized including biological sensing, sub-diffraction-limit imaging, focusing and lithography, and nano optical circuitry. Plasmonics-based optical elements such as waveguides, lenses, beam splitters and reflectors have been implemented by structuring metal surfaces or placing dielectric structures on metals, aiming to manipulate the two-dimensional surface plasmon waves. However, the abrupt discontinuities in the material properties or geometries of these elements lead to increased scattering of SPPs, which significantly reduces the efficiency of these components. Transformation optics provides an unprecedented approach to route light at will by spatially varying the optical properties of a material. Here, motivated by this approach, we use grey-scale lithography to adiabatically tailor the topology of a dielectric layer adjacent to a metal surface to demonstrate a plasmonic Luneburg lens that can focus SPPs. We also realize a plasmonic Eaton lens that can bend SPPs. Since the optical properties are changed gradually rather than abruptly in these lenses, losses due to scattering can be significantly reduced in comparison with previously reported plasmonic elements.

physics.optics

Transformational Plasmon Optics

Transformation optics has recently attracted extensive interest, since it provides a novel design methodology for manipulating light at will. Although transformation optics in principle embraces all forms of electromagnetic phenomena on all length scales, so far, much less efforts have been devoted to near-field optical waves, such as surface plasmon polaritons (SPPs). Due to the tight confinement and strong field enhancement, SPPs are widely used for various purposes at the subwavelength scale. Taking advantage of transformation optics, here we demonstrate that the confinement as well as propagation of SPPs can be managed in a prescribed manner by careful control of the dielectric material properties adjacent to a metal. Since the metal properties are completely unaltered, it provides a straightforward way for practical realizations. We show that our approach can assist to tightly bound SPPs over a broad wavelength band at uneven and curved surfaces, where SPPs would normally suffer significant scattering losses. In addition, a plasmonic waveguide bend and a plasmonic Luneburg lens with practical designs are proposed. It is expected that merging the unprecedented design flexibility based on transformation optics with the unique optical properties of surface modes will lead to a host of fascinating near-field optical phenomena and devices.

physics.optics